arXiv subjects

N. E. Hussey

Publications and source records attributed to N. E. Hussey.

71 records · Page 4Linked to original sources

arXiv2007

Angle dependent magnetoresistance measurements in Tl$_2$Ba$_2$CuO$_{6+δ}$ and the need for anisotropic scattering

The angle-dependent interlayer magnetoresistance of overdoped Tl$_2$Ba$_2$CuO$_{6+δ}$ has been measured in high magnetic fields up to 45 Tesla. A conventional Boltzmann transport analysis with no basal-plane anisotropy in the cyclotron frequency $ω_c$ or transport lifetime $τ$ is shown to be inadequate for explaining the data. We describe in detail how the analysis can be modified to incorporate in-plane anisotropy in these two key quantities and extract the degree of anisotropy for each by assuming a simple four-fold symmetry. While anisotropy in $ω_c$ and other Fermi surface parameters may improve the fit, we demonstrate that the most important anisotropy is that in the transport lifetime, thus confirming its role in the physics of overdoped superconducting cuprates.

cond-mat.supr-con↗

arXiv2007

Violation of the isotropic-$\ell$ approximation in overdoped La_{2-x}Sr_xCuO_4

Magnetotransport measurements on the overdoped cuprate La_{1.7}Sr_{0.3}CuO_4 are fitted using the Ong construction and band parameters inferred from angle-resolved photoemission. Within a band picture, the low temperature Hall data can only be fitted satisfactorily by invoking strong basal-plane anisotropy in the mean-free-path $\ell$. This violation of the isotropic-$\ell$ approximation supports a picture of dominant small-angle elastic scattering in cuprates due to out-of-plane substitutional disorder. We show that both band anisotropy and anisotropy in the elastic scattering channel strongly renormalize the Hall coefficient in overdoped La_{2-x}Sr_xCuO_4 over a wide doping and temperature range.

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arXiv2006

Optical response of high-$T_c$ cuprates: possible role of scattering rate saturation and in-plane anisotropy

We present a generalized Drude analysis of the in-plane optical conductivity $σ_{ab}$($T$,$ω$) in cuprates taking into account the effects of in-plane anisotropy. A simple ansatz for the scattering rate $Γ$($T$,$ω$), that includes anisotropy, a quadratic frequency dependence and saturation at the Mott-Ioffe-Regel limit, is able to reproduce recent normal state data on an optimally doped cuprate over a wide frequency range. We highlight the potential importance of including anisotropy in the full expression for $σ_{ab}$($T$,$ω$) and challenge previous determinations of $Γ$($ω$) in which anisotropy was neglected and $Γ$($ω$) was indicated to be strictly linear in frequency over a wide frequency range. Possible implications of our findings for understanding thermodynamic properties and self-energy effects in high-$T_c$ cuprates will also be discussed.

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arXiv2006

Anisotropic Scattering and Anomalous Transport in a High Temperature Superconductor

The metallic state of high temperature cuprate superconductors is markedly different from that of textbook metals. The origin of this unconventional state, characterized by unusual and distinct temperature dependences in the transport properties, remains unresolved despite intense theoretical efforts. Our understanding is impaired by our inability to determine experimentally the temperature and momentum dependence of the transport scattering rate. Here we use a novel magnetotransport probe to show that the unusual temperature dependences of the resistivity and the Hall coefficient in highly doped Tl$_2$Ba$_2$CuO$_{6+δ}$ originate from two distinct inelastic scattering channels. One channel is due to conventional electron-electron scattering whilst the other is highly anisotropic, has the same symmetry as the superconducting gap and a magnitude that grows approximately linearly with temperature. The observed form and anisotropy put tight constraints on theories of the metallic state. Moreover, in heavily doped non-superconducting cuprates, this anisotropic scattering term appears to be absent, suggesting an intimate connection between the origin of this scattering and superconductivity itself.

cond-mat.supr-con↗

arXiv2006

Shubnikov de Haas effect in the metallic state of Na$_{0.3}$CoO$_2$

Shubnikov de Haas oscillations for two well defined frequencies, corresponding respectively to areas of 0.8 and 1.36% of the first Brillouin zone (FBZ), were observed in single crystals of Na$_{0.3}$CoO$_2$. The existence of Na superstructures in Na$_{0.3}$CoO$_2$, coupled with this observation, suggests the possibility that the periods are due to the reconstruction of the large Fermi surface around the $Γ$ point. An alternative interpretation in terms of the long sought-after $ε_g^\prime$ pockets is also considered but found to be incompatible with existing specific heat data.

cond-mat.str-el↗

arXiv2004

Magnetic-field-induced Fermi surface reconstruction in Na$_{0.5}$CoO$_2$

We have performed electrical transport measurements at low temperatures and high magnetic fields in Na$_{0.5}$CoO$_2$ single crystals. Shubnikov de Haas oscillations were observed for two frequencies F_1 150 and F_2 40 T corresponding respectively to 1 and .25% of the area of the orthorhombic Brillouin zone. These small Fermi surface (FS) pockets indicate that most of the original FS vanishes at the charge ordering (CO) transition. Furthermore, in-plane magnetic fields strongly suppress the CO state. For fields rotating within the conducting planes we observe angular magnetoresistance oscillations (AMRO), whose periodicity changes from two- to six-fold at the transition, suggesting that a reconstructed hexagonal FS emerges at a field of about 40 T.

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arXiv2004

Non-generality of the Kadowaki-Woods ratio in correlated oxides

An explicit expression for the Kadowaki-Woods ratio in correlated metals is derived by invoking saturation of the (high-frequency) Fermi-liquid scattering rate at the Mott-Ioffe-Regel limit. Significant deviations observed in a number of oxides are quantitatively explained due to variations in carrier density, dimensionality, unit cell volume and the number of individual sheets in the Brillouin zone. A generic re-scaling of the original Kadowaki-Woods plot is also presented.

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arXiv2004

Universality of the Mott-Ioffe-Regel limit in metals

The absence of resistivity saturation in many strongly correlated metals, including the high-temperature superconductors, is critically examined from the viewpoint of optical conductivity measurements. Coherent quasiparticle conductivity, in the form of a Drude peak centred at zero frequency, is found to disappear as the mean free path (at $ω$ = 0) becomes comparable to the interatomic spacing. This basic loss of coherence at the so-called Mott-Ioffe-Regel (MIR) limit suggests that the universality of the MIR criterion is preserved even in the presence of strong electron correlations. We argue that the shedding of spectral weight at low frequencies, induced by strong correlation effects, is the primary origin of the extended positive slope of the resistivity to high temperatures observed in all so-called "bad metals". Moreover, in common with those metals which exhibit resistivity saturation at high temperatures, the scattering rate itself, as extracted from optical spectra, saturates at a value consistent with the MIR limit. We consider possible implications that this ceiling in the scattering rate may have for our understanding of transport within a wide variety of bad metals and suggest a better method for analysing their optical response.

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arXiv2003

Field-Induced Thermal Metal-to-Insulator Transition in Underdoped LSCO

The transport of heat and charge in cuprates was measured in single crystals of La_{2-x}Sr_xCuO_{4+δ} (LSCO) across the doping phase diagram at low temperatures. In underdoped LSCO, the thermal conductivity is found to decrease with increasing magnetic field in the T goes to 0 limit, in striking contrast to the increase observed in all superconductors, including cuprates at higher doping. In heavily underdoped LSCO, where superconductivity can be entirely suppressed with an applied field, we show that a novel thermal metal-to-insulator transition takes place upon going from the superconducting state to the field-induced normal state.

cond-mat.supr-con↗

arXiv2003

Determination of the Fermi Surface of MgB$_2$ by the de Haas-van Alphen effect

We report measurements of the de Haas-van Alphen effect for single crystals of MgB$_2$, in magnetic fields up to 32 Tesla. In contrast to our earlier work, dHvA orbits from all four sheets of the Fermi surface were detected. Our results are in good overall agreement with calculations of the electronic structure and the electron-phonon mass enhancements of the various orbits, but there are some small quantitative discrepancies. In particular, systematic differences in the relative volumes of the Fermi surface sheets and the magnitudes of the electron-phonon coupling constants could be large enough to affect detailed calculations of T$_{c}$ and other superconducting properties.

cond-mat.supr-con↗

arXiv2003

Thermal Conductivity across the Phase Diagram of Cuprates: Low-Energy Quasiparticles and Doping Dependence of the Superconducting Gap

Heat transport in the cuprate superconductors YBa$_2$Cu$_3$O$_{y}$ and La$_{2-x}$Sr$_x$CuO$_4$ was measured at low temperatures as a function of doping. A residual linear term kappa_{0}/T is observed throughout the superconducting region and it decreases steadily as the Mott insulator is approached from the overdoped regime. The low-energy quasiparticle gap extracted from kappa_{0}/T is seen to scale closely with the pseudogap. The ubiquitous presence of nodes and the tracking of the pseudogap shows that the overall gap remains of the pure d-wave form throughout the phase diagram, which excludes the possibility of a complex component (ix) appearing at a putative quantum phase transition and argues against a non-superconducting origin to the pseudogap. A comparison with superfluid density measurements reveals that the quasiparticle effective charge is weakly dependent on doping and close to unity.

cond-mat.supr-con↗

arXiv2002

The ground state of heavily-overdoped non-superconducting La$_{2-x}$Sr$_x$CuO$_4$

We report detailed thermodynamic and transport measurements for non-superconducting La$_{1.7}$Sr$_{0.3}$CuO$_4$. Collectively, these data reveal that a highly-correlated Fermi-liquid ground state exists in La$_{2-x}$Sr$_x$CuO$_4$ beyond the superconducting dome, and confirm that charge transport in the cuprates is dominated at finite temperatures by intense electron-electron scattering.

cond-mat.str-el↗

arXiv2002

The normal state scattering rate in high-Tc cuprates

I present a new phenomenological model for the normal state transport properties of high-Tc cuprates. In particular, I identify a form of scattering rate that may account, qualitatively and quantitatively, for the normal state (magneto)-transport properties of Tl2Ba2CuO6+δand Bi2Sr2CaCu2O8+δfrom optimal doping through to the overdoped side of the phase diagram. The form of the scattering rate is also consistent with features seen in photoemission spectroscopy in Bi2Sr2CaCu2O8+δand offers a new intuitive way to understand the evolution of the temperature dependence of the inverse Hall angle with disorder and with carrier concentration.

cond-mat.supr-con↗

arXiv2002

de Haas-van Alphen effect in single crystal MgB_2

We report observations of quantum oscillations in single crystals of the high temperature superconductor MgB_2. Three de Haas-van Alphen frequencies are clearly resolved. Comparison with band structure calculations strongly suggests that two of these come from a single warped Fermi surface tube along the c direction, and that the third arises from cylindrical sections of an in-plane honeycomb network. The measured values of the effective mass range from 0.44-0.68 m_e. By comparing these with band masses calculated recently by three groups, we find that the electron-phonon coupling strength lambda, is a factor \~3 larger for the c-axis tube orbits than for the in-plane network orbit, in accord with recent microscopic calculations.

cond-mat.supr-con↗

arXiv2002

Exponential Temperature Dependence of Penetration Depth in Single Crystal MgB_2

The temperature dependence of the London penetration depth,lambda(T), was measured in both single crystal and polycrystalline MgB_2 samples by a high-resolution, radio frequency technique. A clear exponential temperature dependence of lambda(T) was observed at low temperature, indicating s-wave pairing. A BCS fit to the lowest temperature data gives an in-plane energy gap Delta of 2.6\pm0.2 meV (2Δ/T_c=1.5\pm0.1), which is significantly smaller than the standard BCS weak coupling value of 3.5. We find that the data are best described by a two-gap model.

cond-mat.supr-con↗

arXiv2000

Absence of residual quasiparticle conductivity in the underdoped cuprate YBa2Cu4O8

We report here measurements of the in-plane thermal conductivity K(T) of the underdoped cuprate YBa2Cu4O8 (Y124) below 1K. K(T) is shown to follow a simple, phononic T^3 dependence at the lowest temperatures for both current directions, with a negligible linear, quasiparticle contribution. This observation is in marked contrast with behavior reported in optimally doped cuprates, and implies that extended zero-energy (or low energy) low-energy quasiparticles are absent in YBa2Cu4O8 at low temperatures.

cond-mat.supr-con↗

arXiv1998

Band-width control in a perovskite-type 3d^1 correlated metal Ca_{1-x}Sr_xVO_3. I. Evolution of the electronic properties and effective mass

Single crystals of the perovskite-type $3d^{1}$ metallic alloy system Ca$_{1-x}$Sr$_x$VO$_3$ were synthesized in order to investigate metallic properties near the Mott transition. The substitution of a Ca$^{2+}$ ion for a Sr$^{2+}$ ion reduces the band width $W$ due to a buckling of the V-O-V bond angle from $\sim180^\circ$ for SrVO$_3$ to $\sim160^\circ$ for CaVO$_3$. Thus, the value of $W$ can be systematically controlled without changing the number of electrons making Ca$_{1-x}$Sr$_x$VO$_3$: one of the most ideal systems for studying band-width effects. The Sommerfeld-Wilson's ratio ($\simeq2$), the Kadowaki-Woods ratio (in the same region as heavy Fermion systems), and a large $T^{2}$ term in the electric resistivity, even at 300 K, substantiate a large electron correlation in this system, though the effective mass, obtained by thermodynamic and magnetic measurements, shows only a systematic but moderate increase in going from SrVO$_3$ to CaVO$_3$, in contrast to the critical enhancement expected from the Brinkmann-Rice picture. It is proposed that the metallic properties observed in this system near the Mott transition can be explained by considering the effect of a non-local electron correlation.

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