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N. I. Zheludev

Publications and source records attributed to N. I. Zheludev.

At least 19 recordsLinked to original sources
arXiv2021

Observation of Toroidal Pulses of Light

The transverse electromagnetic waves are major information and energy carriers. In 1996, Hellwarth and Nouchi theoretically identified a radically different, non-transverse type of electromagnetic pulses of toroidal topology. These pulses, which are propagating counterparts of localized toroidal dipole excitations in matter and exhibit unique electromagnetic wave properties, have never been observed before. Here, we report the generation and characterization of such optical and terahertz Toroidal Light Pulses (TLPs), launched from tailored nanostructured metasurfaces comprising toroidal emitters. This achievement paves the way for experimental studies of energy and information transfer with TLPs, their space-time "entanglement", and their light-matter interactions involving anapoles, localized space-time entangled excitations, skyrmions, and toroidal qubits that are of growing interest for the fundamental science of light and applications.

physics.optics↗
arXiv2019

Infrared dielectric metamaterials from high refractive index chalcogenides

High-index dielectric materials are in great demand for nanophotonic devices and applications, from ultrathin optical elements to metal-free sub-diffraction light confinement and waveguiding. Here we show that chalcogenide topological insulators are particularly apt candidates for dielectric nanophotonic architectures in the infrared spectral range by reporting metamaterial resonances in chalcogenide crystals sustained well inside the mid-infrared, choosing Bi$_2$Te$_3$ as case study within this family of materials. Strong resonant modulation of the incident electromagnetic field is achieved thanks to the exceptionally high refractive index ranging between 7 and 8 throughout the 2-10 $μ$m region. Analysis of the complex mode structure in the metamaterial allude to the excitation of poloidal surface currents which could open pathways for enhanced light-matter interaction and low-loss plasmonic configurations by coupling to the spin-polarized topological surface carriers, thereby providing new opportunities to combine dielectric, plasmonic and magnetic metamaterials in a single platform.

physics.optics↗
arXiv2019

Unlabelled Far-field Deeply Subwavelength Superoscillatory Imaging (DSSI)

Recently it was reported that deeply subwavelength features of free space superoscillatory electromagnetic fields can be observed experimentally and used in optical metrology with nanoscale resolution [Science 364, 771 (2019)]. Here we introduce a new type of imaging, termed Deeply Subwavelength Superoscillatory Imaging (DSSI), that reveals the fine structure of a physical object through its far-field scattering pattern under superoscillatory illumination. The object is reconstructed from intensity profiles of scattered light recorded for different positions of the object in the superoscillatory field. The reconstruction is performed with a convolutional neural network trained on a large number of scattering events. We show that DSSI offers resolution far beyond the conventional 'diffraction limit'. In modelling experiments, a dimer comprising two subwavelength opaque particles is imaged with a resolution exceeding $λ/200$.

physics.optics↗
arXiv2017

Generation of Flying Electromagnetic Donuts

Transverse electromagnetic plane waves are fundamental solutions of Maxwell's equations. It is less known that a radically different type of solutions has been described theoretically, but has never been realized experimentally, that exist only in the form of short burst of electromagnetic energy propagating in free-space at the speed of light. They are distinguished from transverse waves by a donut-like configuration of electric and magnetic fields with a strong field component along the propagation direction. Here, we report that such 'Flying Donuts' can be generated from conventional pulses using a singular metamaterial converter designed to manipulate both the spatial and spectral structure of the input pulse. The ability to generate Flying Donuts is of fundamental interest, as they shall interact with matter in unique ways, including non-trivial field transformations upon reflection from interfaces and the excitation of toroidal response and anapole modes in matter, thus offering new opportunities for telecommunications, sensing, and spectroscopy.

physics.optics↗
arXiv2016

Spontaneous natural optical activity in disordered media

We demonstrate natural optical activity in disordered ensembles of non-chiral plasmonic resonators. We show that the statistical distributions of rotatory power and spatial dichroism are strongly dependent on the scattering mean free path in diffusive random media. This result is explained in terms of the intrinsic geometric chirality of disordered media, as they lack mirror symmetry. We argue that chirality and natural optical activity of disordered systems can be quantified by the standard deviation of both rotatory power and spatial dichroism. Our results are based on microscopic electromagnetic wave transport theory coupled to vectorial Green's matrix method for pointlike scatterers, and are independently confirmed by full-wave simulations.

physics.optics↗
arXiv2015

Focused electromagnetic doughnut pulses and their interaction with interfaces and nanostructures

We study the propagation properties and light-matter interactions of the focused doughnut pulses, broadband, single-cycle electromagnetic perturbations of toroidal topology first described by Hellwarth and Nouchi in 1996. We show how focused doughnuts are reflected and refracted at planar metallic and vacuum-dielectric interfaces leading to complex distortions of the field structure. We also identify the conditions under which these toroidal pulses excite dominant dynamic toroidal dipoles in spherical dielectric particles.

physics.optics↗
arXiv2015

Toroidal optical activity

Optical activity is ubiquitous across natural and artificial media and is conventionally understood in terms of scattering from electric and magnetic moments. Here we demonstrate experimentally and confirm numerically a type of optical activity that cannot be attributed to electric and magnetic multipoles. We show that our observations can only be accounted for by the inclusion of the toroidal dipole moment, the first term of the recently established peculiar family of toroidal multipoles.

physics.optics↗
arXiv2015

Dirac Phase interferometer in a plasmonic waveguide

By viewing plasmon waves in metallic waveguides as propagating electric and magnetic dipoles we show that according to laws of quantum mechanics they will acquire additional phase when propagating through space with static magnetic field. The new effect is physically different from conventional magneto-plasmonic phenomena and is sufficiently strong to observe it under routinely accessible experimental conditions.

physics.optics↗
arXiv2014

A Random Access Reconfigurable Metamaterial and a Tunable Flat Lens

The ability to control resonant properties of individual metamolecule in a metamaterial structure will offer an ultimate freedom for dynamically shaping wavefronts of electromagnetic radiation for applications such as variable aberration corrected planar lenses, dynamic holograms and spatial intensity and phase modulators. Here we report the first demonstration of a metamaterial where resonant properties of every individual metamolecule can be continuously controlled at will thus offering an ultimate freedom in achieving a dynamic control of electromagnetic wavefront of microwave radiation. We call this a Random Access Reconfigurable Metamaterial (RARM). To achieve a RARM we created an array of cavities that were filled with liquid metal in a precise fashion using microfluidic technology. The developed RARM was used provide the first demonstration of a tunable flat lens.

physics.optics↗
arXiv2013

Macroscopic electromagnetic response of metamaterials with toroidal resonances

Toroidal dipole, first described by Ia. B. Zeldovich [Sov. Phys. JETP 33, 1184 (1957)], is a distinct electromagnetic excitation that differs both from the electric and the magnetic dipoles. It has a number of intriguing properties: static toroidal nuclear dipole is responsible for parity violation in atomic spectra; interactions between static toroidal dipole and oscillating magnetic dipole are claimed to violate Newton's Third Law while non-stationary charge-current configurations involving toroidal multipoles have been predicted to produce vector potential in the absence of electromagnetic fields. Existence of the toroidal response in metamaterials was recently demonstrated and is now a growing field of research. However, no direct analytical link has yet been established between the transmission and reflection of macroscopic electromagnetic media and toroidal dipole excitations. To address this essential gap in electromagnetic theory we have developed an analytical approach linking microscopic and macroscopic electromagnetic response of a metamaterial and showed, using a case study, the key role of the toroidal dipole in shaping the electromagnetic properties of the metamaterial.

physics.optics↗
arXiv2013

Controlling Intensity and Phase of Terahertz Radiation with an Optically Thin Liquid Crystal-Loaded Metamaterial

We experimentally demonstrate intensity and phase modulation of terahertz radiation using actively controlled large-area planar metamaterial (metafilm) hybridized with a 12 um thick layer of a liquid crystal. Active control was introduced through in-plane electrical switching of the liquid crystal, which enabled us to achieve a reversible single-pass absolute transmission change of 20 % and a phase change of 40 deg at only 20 V.

physics.optics↗
arXiv2012

Non-Trivial Non-Radiating Excitation as a Mechanism of Resonant Transparency in Toroidal Metamaterials

We demonstrate theoretically and confirm experimentally a new mechanism of resonant electromagnetic transparency, which yields extremely narrow isolated symmetric Lorentzian lines of full transmission in metamaterials. It exploits the long sought non-trivial non-radiating charge-current excitation based on toroidal dipole moment, predicted to generate waves of gauge-irreducible vector potential in the complete absence of scattered electromagnetic fields.

physics.optics↗
arXiv2012

Metamaterial 'Gecko Toe': Optically-Controlled Adhesion to Any Surface

On the mesoscopic scale, electromagnetic forces are of fundamental importance to an enormously diverse range of systems, from optical tweezers to the adhesion of gecko toes. Here we show that a strong light-driven force may be generated when a plasmonic metamaterial is illuminated in close proximity to a dielectric or metal surface. This near-field force can exceed radiation pressure and Casimir forces to provide an optically controlled adhesion mechanism mimicking the gecko toe: at illumination intensities of just a few tens of nW/um^2 it is sufficient to overcome the Earth's gravitational pull.

physics.optics↗
arXiv2010

Coherent control of nanoscale light localization in metamaterial: creating and positioning a sub-wavelength energy hot-spot

Precise control and manipulation of optical fields on a nanoscale is one of the most important and challenging problems in "nanophotonics". Since optical wavelength is on a much larger microscale, it is impossible to employ conventional focusing for that purpose. We show the strong optically-induced interactions between discrete meta-molecules in a metamaterial system and coherent monochromatic continuous light beam with a spatially-tailored phase profile can be used to prepare a sub-wavelength scale energy localization. Well isolated energy hot-spots as small as $λ/10$ can be created and positioned at will on the metamaterial landscape offering new opportunities for data storage and imaging applications.

physics.optics↗
arXiv2010

A combinatorial approach to metamaterials discovery

We report a high through-put combinatorial approach to photonic metamaterial optimization. The new approach is based on parallel synthesis and consecutive optical characterization of large numbers of spatially addressable nano-fabricated metamaterial samples (libraries) with quasi-continuous variation of design parameters under real manufacturing conditions. We illustrate this method for Fano-resonance plasmonic nanostructures arriving at explicit recipes for high quality factors needed for switching and sensing applications.

physics.optics↗
arXiv2010

Multi-fold Enhancement of Quantum Dot Luminescence in a Plasmonic Metamaterial

We report that hybridizing semiconductor quantum dots with plasmonic metamaterial leads to a multi-fold intensity increase and narrowing of their photoluminescence spectrum. The luminescence enhancement is a clear manifestation of the cavity quantum electrodynamics Purcell effect that can be controlled by the metamaterial's design. This observation is an essential step towards understanding loss compensation in metamaterials with gain media and for developing metamaterial-enhanced gain media.

physics.optics↗
arXiv2010

Asymmetric transmission: a generic property of lossy periodic interfaces

Asymmetric transmission of circularly polarized waves is a well-established property of lossy, anisotropic, two-dimensionally chiral patterns. Here we show that asymmetric transmission can be observed for oblique incidence onto any lossy periodically structured plane. Our results greatly expand the range of natural and artificial materials in which directionally asymmetric transmission can be expected making it a cornerstone electromagnetic effect rather than a curiosity of planar chiral metamaterials. Prime candidates for asymmetric transmission at oblique incidence are rectangular arrays of plasmonic spheres or semiconductor quantum dots, lossy double-periodic gratings and planar metamaterial structures.

physics.optics↗