arXiv subjects

N. Kanazawa

Publications and source records attributed to N. Kanazawa.

At least 19 recordsLinked to original sources

arXiv2024

A randomized benchmarking suite for mid-circuit measurements

Mid-circuit measurements are a key component in many quantum information computing protocols, including quantum error correction, fault-tolerant logical operations, and measurement based quantum computing. As such, techniques to quickly and efficiently characterize or benchmark their performance are of great interest. Beyond the measured qubit, it is also relevant to determine what, if any, impact mid-circuit measurement has on adjacent, unmeasured, spectator qubits. Here, we present a mid-circuit measurement benchmarking suite developed from the ubiquitous paradigm of randomized benchmarking. We show how our benchmarking suite can be used to both detect as well as quantify errors on both measured and spectator qubits, including measurement-induced errors on spectator qubits and entangling errors between measured and spectator qubits. We demonstrate the scalability of our suite by simultaneously characterizing mid-circuit measurement on multiple qubits from an IBM Quantum Falcon device, and support our experimental results with numerical simulations. Further, using a mid-circuit measurement tomography protocol we establish the nature of the errors identified by our benchmarking suite.

quant-ph↗

arXiv2023

Strongly pinned skyrmionic bubbles and higher-order nonlinear Hall resistances at the interface of Pt/FeSi bilayer

Engineering of magnetic heterostructures for spintronic applications has entered a new phase, driven by the recent discoveries of topological materials and exfoliated van der Waals materials. Their low-dimensional properties can be dramatically modulated in designer heterostructures via proximity effects from adjacent materials, thus enabling the realization of diverse quantum states and functionalities. Here we investigate spin-orbit coupling (SOC) proximity effects of Pt on the recently discovered quasi-two-dimensional ferromagnetic state at FeSi surface. Skyrmionic bubbles (SkBs) are formed as a result of the enhanced interfacial Dzyloshinskii-Moriya interaction. The strong pinning effects on the SkBs are evidenced from the significant dispersion in size and shape of the SkBs and are further identified as a greatly enhanced threshold current density required for depinning of the SkBs. The robust integrity of the SkB assembly leads to the emergence of higher-order nonlinear Hall effects in the high current density regime, which originate from nontrivial Hall effects due to the noncollinearity of the spin texture, as well as from the current-induced magnetization dynamics via the augmented spin-orbit torque.

cond-mat.str-el↗

arXiv2023

Anomalous charge transport upon quantum melting of chiral spin order

A plethora of correlated and exotic metallic states have been identified on the border of itinerant magnetism, where the long-range spin texture is melted by tuning the magnetic transition temperature (T$_C$) towards zero, referred to as the quantum phase transition (QPT). So far, the study of QPT in itinerant magnets has mainly focused on low-T$_C$ materials (i.e., typically T$_C$ ~ 10 K) where the modification of electronic band structure is subtle, and only makes a small contribution to the QPT. Here we report a distinct example of a magnetic QPT accompanied by a gigantic modification of the electronic structure in FeGe, i.e., a well-studied itinerant chiral magnet hosting near-room-temperature (T$_C$ = 278 K) helical/skyrmion spin texture. The pressure-driven modification of the band structure (e.g., reduction of exchange splitting) is evidenced by magneto-transport study, suggesting a Fermi-surface reconstruction around the magnetic QPT (P ~19 GPa), in stark contrast to the case of typical metallic ferromagnets. Further application of pressure leads to a metal-to-insulator transition above P > 30 GPa, as also corroborated by our density-functional theory (DFT) calculation. Of particular interest is the occurrence of anomalous magneto-transport in the inhomogeneous short-range chiral-spin ground state (P = 20-30 GPa) above the QPT, with longitudinal fluctuations of magnetization. The unexpected observation of spontaneous anomalous Hall effect in this exotic quantum regime suggests macroscopic time-reversal symmetry (TRS) breaking, even in the absence of long-range magnetic order. Our findings mark the large body of unexplored high-T$_C$ itinerant magnets with broken inversion-symmetry as promising candidates of novel ground state formation near QPT.

cond-mat.str-el↗

arXiv2023

Topological magnetic structures in MnGe: Neutron diffraction and symmetry analysis

From new neutron powder diffraction experiments on the chiral cubic ($P2{_1}3$) magnet manganese germanide MnGe, we analyse all of the possible crystal symmetry-allowed magnetic superstructures that are determined successfully from the data. The incommensurate propagation vectors $k$ of the magnetic structure are found to be aligned with the [100] cubic axes, and correspond to a magnetic periodicity of about 30 $Å$ at 1.8 K. Several maximal crystallographic symmetry magnetic structures are found to fit the data equally well and are presented. These include topologically non-trivial magnetic hedgehog and "skyrmion'' structures in multi-$k$ cubic or orthorhombic 3+3 and orthorhombic 3+2 dimensional magnetic superspace groups respectively, with either potentially responsible for topological Hall effect. The presence of orthorhombic distortions in the space group $P2_12_12_1$ caused by the transition to the magnetically ordered state does not favour the cubic magnetic hedgehog structure, and leave both orthorhombic hedgehog and "skyrmion'' models as equal candidates for the magnetic structures. We also report on a new combined mechanochemical and solid-state chemical route to synthesise MnGe at ambient pressures and moderate temperatures, and compare with samples obtained by the traditional high pressure synthesis.

cond-mat.str-el↗

arXiv2021

Dislocation-driven relaxation processes at the conical to helical phase transition in FeGe

The formation of topological spin textures at the nanoscale has a significant impact on the long-range order and dynamical response of magnetic materials. We study the relaxation mechanisms at the conical-to-helical phase transition in the chiral magnet FeGe. By combining ac susceptibility, magnetic force microscopy measurements and micromagnetic simulations, we demonstrate how the motion of magnetic topological defects, here edge dislocations, impacts the local formation of a stable helimagnetic spin structure. Although the simulations show that the edge dislocations move with a velocity of about 100 m/s through the helimagnetic background, their dynamics are observed to disturb the magnetic order on the timescale of minutes due to pinning by randomly distributed structural defects. The results corroborate the substantial impact of dislocation motions on the nanoscale spin structure in chiral magnets, revealing previously hidden effects on the formation of helimagnetic domains and domain walls.

cond-mat.mtrl-sci↗

arXiv2020

Topological Kagome magnet Co3Sn2S2 thin flakes with high electron mobility and large anomalous Hall effect

Magnetic Weyl semimetals attract considerable interest not only for their topological quantum phenomena but also as an emerging materials class for realizing quantum anomalous Hall effect in the two-dimensional limit. A shandite compound Co3Sn2S2 with layered Kagome-lattices is one such material, where vigorous efforts have been devoted to synthesize the two-dimensional crystal. Here we report a synthesis of Co3Sn2S2 thin flakes with a thickness of 250 nm by chemical vapor transport method. We find that this facile bottom-up approach allows the formation of large-sized Co3Sn2S2 thin flakes of high-quality, where we identify the largest electron mobility (~2,600 cm2V-1s-1) among magnetic topological semimetals, as well as the large anomalous Hall conductivity (~1,400 Ω-1cm-1) and anomalous Hall angle (~32 %) arising from the Berry curvature. Our study provides a viable platform for studying high-quality thin flakes of magnetic Weyl semimetal and stimulate further research on unexplored topological phenomena in the two-dimensional limit.

cond-mat.mtrl-sci↗

arXiv2020

Topological Magnetic Phase in the Candidate Weyl Semimetal CeAlGe

We report the discovery of topological magnetism in the candidate magnetic Weyl semimetal CeAlGe. Using neutron scattering we find this system to host several incommensurate, square-coordinated multi-$\vec{k}$ magnetic phases below $T_{\rm{N}}$. The topological properties of a phase stable at intermediate magnetic fields parallel to the $c$-axis are suggested by observation of a topological Hall effect. Our findings highlight CeAlGe as an exceptional system for exploiting the interplay between the nontrivial topologies of the magnetization in real space and Weyl nodes in momentum space.

cond-mat.str-el↗

arXiv2018

Emergent topological spin structures in a centrosymmetric cubic perovskite

The skyrmion crystal (SkX) characterized by a multiple-q helical spin modulation has been reported as a unique topological state that competes with the single-q helimagnetic order in non-centrosymmetric materials. Here we report the discovery of a rich variety of multiple-q helimagnetic spin structures in the centrosymmetric cubic perovskite SrFeO3. On the basis of neutron diffraction measurements, we have identified two types of robust multiple-q topological spin structures that appear in the absence of external magnetic fields: an anisotropic double-q spin spiral and an isotropic quadruple-q spiral hosting a three-dimensional lattice of hedgehog singularities. The present system not only diversifies the family of SkX host materials, but furthermore provides an experimental missing link between centrosymmetric lattices and topological helimagnetic order. It also offers perspectives for integration of SkXs into oxide electronic devices.

cond-mat.str-el↗

arXiv2017

Spin-wave spectroscopy on Dzyaloshinskii-Moriya interaction in room-temperature chiral magnets hosting skyrmions

Propagation character of spin wave was investigated for chiral magnets FeGe and Co-Zn-Mn alloys, which can host magnetic skyrmions near room temperature. On the basis of the frequency shift between counter-propagating spin waves, the magnitude and sign of Dzyaloshinskii-Moriya (DM) interaction were directly evaluated. The obtained magnetic parameters quantitatively account for the size and helicity of skyrmions as well as their materials variation, proving that the DM interaction plays a decisive role in the skyrmion formation in this class of room-temperature chiral magnets. The propagating spin-wave spectroscopy can thus be an efficient tool to study DM interaction in bulk single-phase compounds. Our results also demonstrate a function of spin-wave diode based on chiral crystal structures at room temperature.

cond-mat.mtrl-sci↗

arXiv2017

Topological domain walls in helimagnets

A magnetic helix arises in chiral magnets with a wavelength set by the spin-orbit coupling. We show that the helimagnetic order is a nanoscale analog to liquid crystals, exhibiting topological structures and domain walls that are distinctly different from classical magnets. Using magnetic force microscopy and micromagnetic simulations, we demonstrate that - similar to cholesteric liquid crystals - three fundamental types of domain walls are realized in the helimagnet FeGe. We reveal the micromagnetic wall structure and show that they can carry a finite skyrmion charge, permitting coupling to spin currents and contributions to a topological Hall effect. Our study establishes a new class of magnetic nano-objects with non-trivial topology, opening the door to innovative device concepts based on helimagnetic domain walls.

cond-mat.str-el↗

arXiv2017

Electrical magnetochiral effect induced by chiral spin fluctuations

Chirality of matter can produce unique responses in optics, electricity and magnetism. In particular, magnetic crystals transmit their handedness to the magnetism via antisymmetric exchange interaction of relativistic origin, producing helical spin orders as well as their fluctuations. Here we report for a chiral magnet MnSi that chiral spin fluctuations manifest themselves in the electrical magnetochiral effect (eMChE), i.e. the nonreciprocal and nonlinear response characterized by the electrical conductance depending on inner product of electric and magnetic fields $\boldsymbol{E} \cdot \boldsymbol{B}$. Prominent eMChE signals emerge at specific temperature-magnetic field-pressure regions: in the paramagnetic phase just above the helical ordering temperature and in the partially-ordered topological spin state at low temperatures and high pressures, where thermal and quantum spin fluctuations are conspicuous in proximity of classical and quantum phase transitions, respectively. The finding of the asymmetric electron scattering by chiral spin fluctuations may explore new electromagnetic functionality in chiral magnets.

cond-mat.str-el↗

arXiv2016

Local dynamics of topological magnetic defects in the itinerant helimagnet FeGe

Chiral magnetic interactions induce complex spin textures including helical and conical spin waves, as well as particle-like objects such as magnetic skyrmions and merons. These spin textures are the basis for innovative device paradigms and give rise to exotic topological phenomena, thus being of interest for both applied and fundamental sciences. Present key questions address the dynamics of the spin system and emergent topological defects. Here we analyze the micromagnetic dynamics in the helimagnetic phase of FeGe. By combining magnetic force microscopy, single-spin magnetometry, and Landau-Lifschitz-Gilbert simulations we show that the nanoscale dynamics are governed by the depinning and subsequent motion of magnetic edge dislocations. The motion of these topologically stable objects triggers perturbations that can propagate over mesoscopic length scales. The observation of stochastic instabilities in the micromagnetic structure provides new insight to the spatio-temporal dynamics of itinerant helimagnets and topological defects, and discloses novel challenges regarding their technological usage.

cond-mat.mtrl-sci↗

arXiv2016

Temperature and magnetic field dependence of the internal and lattice structures of skyrmions by off-axis electron holography

The internal and lattice structures of magnetic skyrmions in B20-type FeGe are investigated using off-axis electron holography. The temperature, magnetic field and angular dependence of the magnetic moments of individual skyrmions are analyzed. Whereas the internal skyrmion shape is found to vary with magnetic field, the inter-skyrmion distance remains almost unchanged in the lattice phase. The amplitude of the local magnetic moment is found to depend on temperature, while the skyrmion shape does not. Deviations from a circular to a hexagonal skyrmion structure are observed in the lattice phase.

cond-mat.mes-hall↗

arXiv2015

Topological stability versus thermal agitation in a metastable magnetic skyrmion lattice

Topologically stable matters can have a long lifetime, even if thermodynamically costly, when the thermal agitation is sufficiently low. A magnetic skyrmion lattice (SkL) represents a unique form of long-range magnetic order that is topologically stable, and therefore, a long-lived, metastable SkL can form. Experimental observations of the SkL in bulk crystals, however, have mostly been limited to a finite and narrow temperature region in which the SkL is thermodynamically stable; thus, the benefits of the topological stability remain unclear. Here, we report a metastable SkL created by quenching a thermodynamically stable SkL. Hall-resistivity measurements of MnSi reveal that, although the metastable SkL is short-lived at high temperatures, the lifetime becomes prolonged (>> 1 week) at low temperatures. The manipulation of a delicate balance between thermal agitation and the topological stability enables a deterministic creation/annihilation of the metastable SkL by exploiting electric heating and subsequent rapid cooling, thus establishing a facile method to control the formation of a SkL.

cond-mat.mtrl-sci↗

arXiv2015

Formation of In-plane Skyrmions in Epitaxial MnSi Thin Films as Revealed by Planar Hall Effect

We investigate skyrmion formation in both a single crystalline bulk and epitaxial thin films of MnSi by measurements of planar Hall effect. A prominent stepwise field profile of planar Hall effect is observed in the well-established skyrmion phase region in the bulk sample, which is assigned to anisotropic magnetoresistance effect with respect to the magnetic modulation direction. We also detect the characteristic planar Hall anomalies in the thin films under the in-plane magnetic field at low temperatures, which indicates the formation of skyrmion strings lying in the film plane. Uniaxial magnetic anisotropy plays an important role in stabilizing the in-plane skyrmions in the MnSi thin film.

cond-mat.str-el↗

arXiv2015

Thermally Driven Ratchet Motion of Skyrmion Microcrystal and Topological Magnon Hall Effect

Spontaneously emergent chirality is an issue of fundamental importance across the natural sciences. It has been argued that a unidirectional (chiral) rotation of a mechanical ratchet is forbidden in thermal equilibrium, but becomes possible in systems out of equilibrium. Here we report our finding that a topologically nontrivial spin texture known as a skyrmion - a particle-like object in which spins point in all directions to wrap a sphere - constitutes such a ratchet. By means of Lorentz transmission electron microscopy we show that micron-sized crystals of skyrmions in thin films of Cu2OSeO3 and MnSi display a unidirectional rotation motion. Our numerical simulations based on a stochastic Landau-Lifshitz-Gilbert equation suggest that this rotation is driven solely by thermal fluctuations in the presence of a temperature gradient, whereas in thermal equilibrium it is forbidden by the Bohr-van Leeuwen theorem. We show that the rotational flow of magnons driven by the effective magnetic field of skyrmions gives rise to the skyrmion rotation, therefore suggesting that magnons can be used to control the motion of these spin textures.

cond-mat.str-el↗

arXiv2015

Discretized Topological Hall Effect Emerging from Skyrmions in Constricted Geometry

We investigate the skyrmion formation process in nano-structured FeGe Hall-bar devices by measurements of topological Hall effect, which extracts the winding number of a spin texture as an emergent magnetic field. Step-wise profiles of topological Hall resistivity are observed in the course of varying the applied magnetic field, which arise from instantaneous changes in the magnetic nano-structure such as creation, annihilation, and jittering motion of skyrmions. The discrete changes in topological Hall resistivity demonstrate the quantized nature of emergent magnetic flux inherent in each skyrmion, which had been indistinguishable in many-skyrmion systems on a macroscopic scale.

cond-mat.str-el↗

arXiv2013

Skyrmions with varying size and helicity in composition-spread helimagnetic alloys

The chirality, i.e. left or right handedness, is an important notion in a broad range of science. In condensed matter, this occurs not only in molecular or crystal forms but also in magnetic structures. A magnetic skyrmion, a topologically-stable spin vortex structure, as observed in chiral-lattice helimagnets is one such example; the spin swirling direction (skyrmion helicity) should be closely related to the underlying lattice chirality via the relativistic spin-orbit coupling (SOC). Here, we report on the correlation between skyrmion helicity and crystal chirality as observed by Lorentz transmission electron microscopy (TEM) and convergent-beam electron diffraction (CBED) on the composition-spread alloys of helimagnets Mn1-xFexGe over a broad range (x = 0.3 - 1.0) of the composition. The skyrmion lattice constant or the skyrmion size shows non-monotonous variation with the composition x, accompanying a divergent behavior around x = 0.8, where the correlation between magnetic helicity and crystal chirality is reversed. The underlying mechanism is a continuous x-variation of the SOC strength accompanying sign reversal in the metallic alloys. This may offer a promising way to tune the skyrmion size and helicity.

cond-mat.mtrl-sci↗