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N. Kumada

Publications and source records attributed to N. Kumada.

At least 19 recordsLinked to original sources

Emission and Coherent Control of Levitons in Graphene

Flying qubits encode quantum information in propagating modes instead of stationary discrete states. Although photonic flying qubits are available, the weak interaction between photons limits the efficiency of conditional quantum gates. Conversely, electronic flying qubits can use Coulomb interactions, but the weaker quantum coherence in conventional semiconductors has hindered their realization. In this work, we engineered on-demand injection of a single electronic flying qubit state and its manipulation over the Bloch sphere. The flying qubit is a Leviton propagating in quantum Hall edge channels of a high-mobility graphene monolayer. Although single-shot qubit readout and two-qubit operations are still needed for a viable manipulation of flying qubits, the coherent manipulation of an itinerant electronic state at the single-electron level presents a highly promising alternative to conventional qubits.

cond-mat.mes-hall

Gate-tunable giant superconducting nonreciprocal transport in few-layer $T_{\rm d}$-MoTe$_2$

We demonstrate gate-tunable giant field-dependent nonreciprocal transport (magnetochiral anisotropy) in a noncentrosymmetric superconductor $T_{\rm d}$-MoTe$_2$ in the thin limit. Giant magnetochiral anisotropy (MCA) with a rectification coefficient $γ$ = $3.1 \times 10^6$ T$^{-1}$ A$^{-1}$, is observed at 230 mK, below the superconducting transition temperature ($T_c$). This is one of the largest values reported so far and is likely attributed to the reduced symmetry of the crystal structure. The temperature dependence of $γ$ indicates that the ratchet-like motion of magnetic vortices is the origin of the MCA, as supported by our theoretical model. For bilayer $T_{\rm d}$-MoTe$_2$, we successfully perform gate control of the MCA and realize threefold modulation of $γ$. Our experimental results provide a new route to realizing electrically controllable superconducting rectification devices in a single material.

cond-mat.mes-hall

A Monomer Mott Insulator (BEDT-TTF)Cu[N(CN)$_2$]$_2$ as a Potential Nodal Line System

We report the band structure calculations and the experimental results of resistivity and magnetic susceptibility in a spin-1/2 (BEDT-TTF)$^{\bullet +}$ monomer Mott insulator (BEDT-TTF)Cu[N(CN)$_2$]$_2$. The band calculations indicate a Dirac semimetal state with nodal lines at the Fermi level. The resistivity and the magnetic susceptibility as functions of temperature are well interpreted in terms of the monomer Mott insulating state instead of the expected semimetal state probably owing to strong electron correlation. In addition, we find that an Arrhenius-type steep reduction of the paramagnetic susceptibility appears below approximately 25 K, which indicates a spin-singlet ground state.

cond-mat.str-el

Quantum Hall valley splitters and tunable Mach-Zehnder interferometer in graphene

Graphene is a very promising test-bed for the field of electron quantum optics. However, a fully tunable and coherent electronic beam splitter is still missing. We report the demonstration of electronic beam splitters in graphene that couple quantum Hall edge channels having opposite valley polarizations. The electronic transmission of our beam splitters can be tuned from zero to near unity. By independently setting the beam splitters at the two corners of a graphene PN junction to intermediate transmissions, we realize a fully tunable electronic Mach-Zehnder interferometer. This tunability allows us to unambiguously identify the quantum interferences due to the Mach-Zehnder interferometer, and to study their dependence with the beam-splitter transmission and the interferometer bias voltage. The comparison with conventional semiconductor interferometers points towards universal processes driving the quantum decoherence in those two different 2D systems, with graphene being much more robust to their effect.

cond-mat.mes-hall

Unveiling excitonic properties of magnons in a quantum Hall ferromagnet

Magnons enable transferring a magnetic moment or spin over macroscopic distance. In quantum Hall ferromagnet, it has been predicted in the early 90s that spin and charges are entangled, meaning that any change of the spin texture modifies the charge distribution. As a direct consequence of this entanglement, magnons carry an electric dipole moment. Here we report the first evidence of the existence of this electric dipole moment in a graphene quantum Hall ferromagnet using a Mach-Zehnder interferometer as a quantum sensor. By propagating towards the interferometer through an insulating bulk, the magnon electric dipole moment modifies the Aharonov-Bohm flux through the interferometer, changing both its phase and its visibility. In particular, we relate the phase shift to the sign of this electric dipole moment, and the exponential loss of visibility to the flux of emitted magnons. Finally, we probe the emission energy threshold of the magnons close to filling factor v=1. Approaching v=0, we observe that the emission energy threshold diminishes towards zero, which might be linked to the existence of gapless mode in the canted-antiferromagnetic (CAF) phase at v=0. The detection and manipulation of magnons based on their electric dipole open the field for a new type of coherent magnon quantum circuits that will be electrostatically controlled.

cond-mat.mes-hall

Suppression of Gate Screening on Edge Magnetoplasmons by Highly Resistive ZnO Gate

We investigate a way to suppress high-frequency coupling between a gate and low-dimensional electron systems in the gigahertz range by measuring the velocity of edge magnetoplasmons (EMPs) in InAs quantum Hall systems.We compare the EMPvelocity in three samples with different electromagnetic environments-one has a highly resistive zinc oxide (ZnO) top gate, another has a normal metal (Ti/Au) top gate, and the other does not have a gate. The measured EMP velocity in the ZnO gate sample is one order of magnitude larger than that in the Ti/Au gate sample and almost the same as that in the ungated sample. As is well known, the smaller velocity in the Ti/Au gate sample is due to the screening of the electric field in EMPs. The suppression of the gate screening effect in the ZnO gate sample allows us to measure the velocity of unscreened EMPs while changing the electron density. It also offers a way to avoid unwanted high-frequency coupling between quantum Hall edge channels and gate electrodes.

cond-mat.mes-hall

Frustrated magnetic interactions in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12(NO3)

Inelastic neutron scattering study has been performed in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12(NO3) at ambient and high magnetic fields. Relatively broad and monotonically dispersive magnetic excitations were observed at ambient field, where no long range magnetic order exists. In the magnetic field-induced long-range ordered state at 10 T, the magnetic dispersions become slightly more intense, albeit still broad as in the disordered state, and two excitation gaps, probably originating from an easy-plane magnetic anisotropy and intrabilayer interactions, develop. Analyzing the magnetic dispersions using the linear spin-wave theory, we estimated the intraplane and intrabilayer magnetic interactions, which are almost consistent with those determined by ab initio density functional theory calculations [M. Alaei et al., Phys. Rev. B 96, 140404(R) (2017)], except the 3rd and 4th neighbor intrabilayer interactions. Most importantly, as predicted by the theory, there is no significant frustration in the honeycomb plane but frustrating intrabilayer interactions probably give rise to the disordered ground state.

cond-mat.str-el

An ab-initio study on physical properties of Pd2+ incorporated double perovskites CaPd3B4O12 (B = Ti, V)

Numerous physical properties of CaPd3Ti4O12 (CPTO) and CaPd3V4O12 (CPVO) double perovskites have been explored based on density functional theory (DFT). The calculated structural parameters fairly agree with the experimental data to confirm their stability. The mechanical stability of these two compounds was clearly observed by the Born stability criteria. To rationalize the mechanical behavior, we investigate elastic constants, bulk, shear and Young's modulus, Pugh's ratio, Poisson's ratio and elastic anisotropy index. The ductility index confirms that both materials are ductile in nature. The electronic band structure of CPTO and CPVO reveals the direct band gap semiconducting in nature and metallic characteristics, respectively. The calculated partial density of states indicates the strong hybridization between Pd 4d and O 2p orbital electrons for CPTO and Pd 4d and V 3d O 2p for CPVO. The study of electronic charge density map confirms the coexistence of covalent, ionic and metallic bonding for both compounds. Fermi surface calculation of CPVO ensures both electron and hole like surfaces indicating the multiple band nature. In the midst of optical properties, photoconductivity and absorption coefficient of both compounds reveal well qualitative compliance with consequences of band structure computations. Among the thermodynamic properties, the Debye temperature has been calculated to correlate its topical features including thermoelectric behavior. The studied thermoelectric transport properties of CPTO yielded the Seebeck coefficient (186 microVK-1), power factor (11.9 microWcm-1K-2) and figure of merit (ZT) value of about 0.8 at 800 K indicate that this material could be a promising candidate for thermoelectric device application.

cond-mat.mtrl-sci

Quantum Hall effect in epitaxial graphene with permanent magnets

We have observed the well-kown quantum Hall effect (QHE) in epitaxial graphene grown on silicon carbide (SiC) by using, for the first time, only commercial NdFeB permanent magnets at low temperature. The relatively large and homogeneous magnetic field generated by the magnets, together with the high quality of the epitaxial graphene films, enables the formation of well-developed quantum Hall states at Landau level filling factors $ν=\pm 2$, commonly observed with superconducting electro-magnets. Furthermore, the chirality of the QHE edge channels can be changed by a top gate. These results demonstrate that basic QHE physics are experimentally accessible in graphene for a fraction of the price of conventional setups using superconducting magnets, which greatly increases the potential of the QHE in graphene for research and applications.

cond-mat.mes-hall

Compositional and temperature evolution of crystal structure of new thermoelectric compound LaOBiS2-xSex

We examined the crystal structure of the new thermoelectric material LaOBiS2-xSex, whose thermoelectric performance is enhanced by Se substitution, by using powder synchrotron X-ray diffraction and Rietveld refinement. The emergence of metallic conductivity and enhancement of the thermoelectric power factor of LaOBiS2-xSex can be explained with the higher in-plane chemical pressure caused by the increase of Se concentration at the in-plane Ch1 site (Ch = S, Se). High-temperature X-ray diffraction measurements for optimally substituted LaOBiSSe revealed anomalously large atomic displacement parameters (Uiso) for Bi and Ch atoms in the BiCh2 conduction layers. The anisotropic analysis of the atomic displacement parameters (U11 and U33) for the in-plane Bi and Ch1 sites suggested that Bi atoms exhibit large atomic displacement along the c-axis direction above 300 K, which could be the origin of the low thermal conductivity in LaOBiSSe. The large Bi vibration along the c-axis direction could be related to in-plane rattling, which is a new strategy for attaining low thermal conductivity and phonon-glass-electron-crystal states.

cond-mat.mtrl-sci

Shot noise generated by graphene p-n junctions in the quantum Hall effect regime

Owing to a linear and gapless band structure and a tunability of the charge carrier type, graphene offers a unique system to investigate transport of Dirac Fermions at p-n junctions (PNJs). In a magnetic field, combination of quantum Hall physics and the characteristic transport across PNJs leads to a fractionally quantized conductance associated with the mixing of electron-like and hole-like modes and their subsequent partitioning. The mixing and partitioning suggest that a PNJ could be used as an electronic beam-splitter. Here we report the shot noise study of the mode mixing process and demonstrate the crucial role of the PNJ length. For short PNJs, the amplitude of the noise is consistent with an electronic beam-splitter behavior, whereas, for longer PNJs, it is reduced by the energy relaxation. Remarkably, the relaxation length is much larger than typical size of mesoscopic devices, encouraging using graphene for electron quantum optics and quantum information processing.

cond-mat.mes-hall

Intrinsic and extrinsic decay of edge magnetoplasmons in graphene

We investigate intrinsic and extrinsic decay of edge magnetoplasmons (EMPs) in graphene quantum Hall (QH) systems by high-frequency electronic measurements. From EMP resonances in disk shaped graphene, we show that the dispersion relation of EMPs is nonlinear due to interactions, giving rise to intrinsic decay of EMP wavepacket. We also identify extrinsic dissipation mechanisms due to interaction with localized states in bulk graphene from the decay time of EMP wavepackets. We indicate that, owing to the unique linear and gapless band structure, EMP dissipation in graphene can be lower than that in GaAs systems.

cond-mat.mes-hall

Spatial distribution of dynamically polarized nuclear spins in electron spin domains in the $ν= 2/3$ fractional quantum Hall state studied by nuclear electric resonance

Nuclear electric resonance (NER) is based on nuclear magnetic resonance mediated by spatial oscillations of electron spin domains excited by a radio frequency (RF) electric field, and it allows us to investigate the spatial distribution of the nuclear spin polarization around domain walls (DWs). Here, NER measurements were made of the dynamic nuclear spin polarization (DNP) at the spin phase transition of the fractional quantum Hall state at a Landau level filling factor of $ν=2/3$. From the RF pulse power and pulse duration dependence of the NER spectrum, we show that the DNP occurs only within $\sim 100$ nm around DWs, and that it does not occur in DWs. We also show that DWs are pinned by the hyperfine field from polarized nuclear spins.

cond-mat.mes-hall

Plasmon transport in graphene investigated by time-resolved measurement

Plasmons, which are collective charge oscillations, offer the potential to use optical signals in nano-scale electric circuits. Recently, plasmonics using graphene have attracted interest, particularly because of the tunable plasmon frequency through the carrier density $n$. However, the $n$ dependence of the plasmon velocity is weak ($\propto n^{1/4}$) and it is difficult to tune the frequency over orders of magnitude. Here, we demonstrate that the velocity of plasmons in graphene can be changed over two orders of magnitude by applying a magnetic field $B$ and by the presence/absence of a gate; at high $B$, edge magnetoplasmons (EMPs), which are plasmons localized at the sample edge, are formed and their velocity depends on $B$ and the gate screening effect. The wide range tunability of the velocity and the observed low-loss plasmon transport encourage designing graphene nanostructures for plasmonics applications.

cond-mat.mes-hall

Disordered Ground State and Magnetic Field-Induced Long-Range Order in an S=3/2 Antiferromagnetic Honeycomb Lattice Compound Bi3Mn4O12(NO3)

Bi3Mn4O12(NO3), in which the Mn4+ ions carry S=3/2, is the first honeycomb lattice system that shows no long-range magnetic order. Using neutron scattering, we have determined that short-range antiferromagnetic correlations develop at low temperatures. Applied magnetic fields induce a magnetic transition, in which the short-range order abruptly expands into a long-range order.

cond-mat.str-el

Anisotropy of Magnetoresistance Hysteresis around the $ν=2/3$ Quantum Hall State in Tilted Magnetic Field

We present an anisotropy of the hysteretic transport around the spin transition point at Landau level filling factor $ν=2/3$ in tilted magnetic field. When the direction of the in-plane component of the magnetic field $B_{\parallel}$ is normal to the probe current $I$, a strong hysteretic transport due to the current-induced nuclear spin polarization occurs. When $B_{\parallel}$ is parallel to $I$, on the other hand, the hysteresis almost disappears. We also demonstrate that the nuclear spin-lattice relaxation rate $T_{1}^{-1}$ at the transition point increases with decreasing angle between the directions of $B_{\parallel}$ and $I$. These results suggest that the morphology of electron spin domains around $ν=2/3$ is affected by the current direction.

cond-mat.str-el

Intrinsic gap and exciton condensation in the nu_T=1 bilayer system

We investigate the quasiparticle excitation of the bilayer quantum Hall (QH) system at total filling factor $ν_{\mathrm{T}} = 1$ in the limit of negligible interlayer tunneling under tilted magnetic field. We show that the intrinsic quasiparticle excitation is of purely pseudospin origin and solely governed by the inter- and intra-layer electron interactions. A model based on exciton formation successfully explains the quantitative behavior of the quasiparticle excitation gap, demonstrating the existence of a link between the excitonic QH state and the composite fermion liquid. Our results provide a new insight into the nature of the phase transition between the two states.

cond-mat.str-el

Electric-Field-Induced Nuclear Spin Resonance Mediated by Oscillating Electron Spin Domains in GaAs-Based Semiconductors

We demonstrate an alternative nuclear spin resonance using radio frequency (RF) electric field (nuclear electric resonance: NER) instead of magnetic field. The NER is based on the electronic control of electron spins forming a domain structure. The RF electric field applied to a gate excites spatial oscillations of the domain walls and thus temporal oscillations of the hyperfine field to nuclear spins. The RF power and burst duration dependence of the NER spectrum provides insight into the interplay between nuclear spins and the oscillating domain walls.

cond-mat.mes-hall