arXiv subjects

N. L. Wang

Publications and source records attributed to N. L. Wang.

At least 55 records · Page 3Linked to original sources

arXiv2016

Revealing a Triangular Lattice Ising Antiferromagnet in a Single-Crystal CeCd$_3$As$_3$

We report the single-crystal growth and the fundamental magnetic and thermodynamic properties of a rare-earth triangular lattice antiferromagnet CeCd$_3$As$_3$. In this rare-earth antiferromagnet, the Ce local moments form a perfect triangular lattice. Due to the spin-orbital-entangled nature of the Ce local moments, the compound exhibits extremely anisotropic antiferromagnetic couplings along the c direction and in the ab plane respectively. We show that CeCd$_3$As$_3$ represents a {\it rare} experimental realization of an antiferromagnetic Ising model on a two dimensional triangular lattice and thus provides a prototype example for geometrical frustration. We further discuss the quantum effect of the perturbative interactions on the top of the predominant Ising interaction.

cond-mat.str-el↗

arXiv2016

Dramatic change of photoexcited quasiparticle relaxation dynamics across Yb valence state transition in YbInCu$_4$

YbInCu$_4$ undergoes a first order structural phase transition near $T_v$=40 K associated with an abrupt change of Yb valence state. We perform ultrafast pump-probe measurement on YbInCu$_4$ and find that the expected heavy fermion properties arising from the \emph{c-f} hybridization exist only in a limited temperature range above $T_v$. Below $T_v$, the compound behaves like a normal metal though a prominent hybridization energy gap is still present in infrared measurement. We elaborate that those seemingly controversial phenomena could be well explained by assuming that the Fermi level suddenly shifts up and becomes far away from the flat \emph{f}-electron band as well as the indirect hybridization energy gap in the mixed valence state below $T_v$.

cond-mat.str-el↗

arXiv2016

Revealing extremely low energy amplitude modes in the charge-density-wave compound LaAgSb$_2$

The layered lanthanum silver antimonide LaAgSb$_2$ was known to experience two charge density (CDW) phase transitions, which were proposed recently to be closely related to the newly identified Dirac cone. We present optical spectroscopy and ultrafast pump-probe measurement on the compound. The development of energy gaps were clearly observed below the phase transition temperatures in optical conductivity, which removes most part of the free carrier spectral weight. Time resolved measurement demonstrated the emergence of strong oscillations upon entering the CDW states, which were illuminated to come from the amplitude mode of CDW collective excitations. The frequencies of them are surprisingly low: only 0.12 THz for the CDW order with higher transition temperature and 0.34 THz for the lower one, which shall be caused by their small modulation wave vectors. Furthermore, the amplitude and relaxation time of photoinduced reflectivity stayed unchanged across the two phase transitions, which might be connected to the extremely low energy scales of amplitude modes.

cond-mat.str-el↗

arXiv2016

Angle-resolved spectroscopy study of Ni-based superconductor SrNi$_2$As$_2$

We performed an angle-resolved photoemission spectroscopy study of the Ni-based superconductor SrNi$_2$As$_2$. Electron and hole Fermi surface pockets are observed, but their different shapes and sizes lead to very poor nesting conditions. The experimental electronic band structure of SrNi$_2$As$_2$ is in good agreement with first-principles calculations after a slight renormalization (by a factor 1.1), confirming the picture of Hund's exchange-dominated electronic correlations decreasing with increasing filling of the $3d$ shell in the Fe-, Co- and Ni-based compounds. These findings emphasize the importance of Hund's coupling and $3d$-orbital filling as key tuning parameters of electronic correlations in transition metal pnictides.

cond-mat.supr-con↗

arXiv2016

Anisotropic transport and optical spectroscopy study on antiferromagentic triangular lattice EuCd_2As_2: an interplay between magnetism and charge transport properties

We present anisotropic transport and optical spectroscopy studies on EuCd_2As_2. The measurements reveal that EuCd_2As_2 is a low carrier density semimetal with moderate anisotropic resistivity ratio. The charge carriers experience very strong scattering from Eu magnetic moments, resulting in a Kondo-like increase of resistivity at low temperature. Below the antiferromagnetic transition temperature at $T_N$= 9.5 K, the resistivity drops sharply due to the reduced scattering from the ordered Eu moments. Nevertheless, the anisotropic ratio of $ρ_c/ρ_{ab}$ keeps increasing, suggesting that the antiferromagnetic coupling is along the c-axis. The optical spectroscopy measurement further reveals, besides an overdamped reflectance plasma edge at low energy, a strong coupling between phonon and electronic continuum. Our study suggests that EuCd_2As_2 is a promising candidate displaying intriguing interplay among charge, magnetism and the underlying crystal lattice.

cond-mat.str-el↗

arXiv2016

Infrared properties of heavy-fermions: evolution from weak to strong hybridizations

In this article, we review the charge excitations of heavy fermion compounds probed by infrared spectroscopy. The article is not meant to be a comprehensive survey of experimental investigations. Rather it focuses on the dependence of charge excitations on the hybridization strength. In this context, the infrared properties of the Ce$_m$M$_n$In$_{3m+2n}$ family are discussed in detail since the hybridization strengths differ dramatically in different members despite their similar lattice structures. Investigations on some mixed valent compounds are also presented aiming to elucidate the generic trend on the evolution. In particular, we address the scaling between hybridization energy gap $Δ_{dir}$ and the hybridization strength $\tilde{V}$($\propto\sqrt{WT_K}$) in a wide range of heavy fermions compounds which demonstrates that the periodic Anderson model can generally and quantitatively describe the low-energy charge excitations.

cond-mat.str-el↗

arXiv2016

Optical spectroscopy and ultrafast pump-probe studies on the heavy fermion compound CePt$_2$In$_7$

We report optical spectroscopy and ultrafast pump-probe measurements on the antiferromagnetic heavy fermion compound CePt$_2$In$_7$, a member showing stronger two dimensionality than other compounds in CeIn$_3$-derived heavy-fermion family. We identify clear and typical hybridization spectral structures at low temperature from the two different spectroscopy probes. However, the strength and related energy scale of the hybridization are much weaker and smaller than that in the superconducting compounds CeCoIn$_5$ and CeIrIn$_5$. The features are more similar to observations on the antiferromagnetic compounds CeIn$_3$ and CeRhIn$_5$ in the same family. The results clearly indicate that the Kondo interaction and hybridizations exist in the antiferromagnetic compounds but with weaker strength.

cond-mat.str-el↗

arXiv2015

Optical properties of TlNi2Se2: Observation of pseudogap formation

The quasi-two-dimensional nickel chalcogenides $TlNi_2Se_2$ is a newly discovered superconductor. We have performed optical spectroscopy study on $TlNi_2Se_2$ single crystals over a broad frequency range at various temperatures. The overall optical reflectance spectra are similar to those observed in its isostructure $BaNi_2As_2$. Both the suppression in $R(ω)$ and the peaklike feature in $σ_1(ω)$ suggest the progressive formation of a pseudogap feature in the midinfrared range with decreasing temperatures, which might be originated from the dynamic local fluctuation of charge-density-wave (CDW) instability. We propose that the CDW instability in $TlNi_2Se_2$ is driven by the saddle points mechanism, due to the existence of van Hove singularity very close to the Fermi energy.

cond-mat.supr-con↗

arXiv2015

Magneto-infrared spectroscopy of Landau levels and Zeeman splitting of three-dimensional massless Dirac Fermions in ZrTe$_5$

We present a magneto-infrared spectroscopy study on a newly identified three-dimensional (3D) Dirac semimetal ZrTe$_5$. We observe clear transitions between Landau levels and their further splitting under magnetic field. Both the sequence of transitions and their field dependence follow quantitatively the relation expected for 3D \emph{massless} Dirac fermions. The measurement also reveals an exceptionally low magnetic field needed to drive the compound into its quantum limit, demonstrating that ZrTe$_5$ is an extremely clean system and ideal platform for studying 3D Dirac fermions. The splitting of the Landau levels provides a direct and bulk spectroscopic evidence that a relatively weak magnetic field can produce a sizeable Zeeman effect on the 3D Dirac fermions, which lifts the spin degeneracy of Landau levels. Our analysis indicates that the compound evolves from a Dirac semimetal into a topological line-node semimetal under current magnetic field configuration.

cond-mat.mes-hall↗

arXiv2015

Optical spectroscopy study of three dimensional Dirac semimetal ZrTe$_5$

Three dimensional (3D) topological Dirac materials are under intensive study recently. The layered compound ZrTe$_5$ has been suggested to be one of them by transport and ARPES experiments. Here, we perform infrared reflectivity measurement to investigate the underlying physics of this material. The derived optical conductivity exhibits linear increasing with frequency below normal interband transitions, which provides the first optical spectroscopic proof of a 3D Dirac semimetal. Apart from that, the plasma edge shifts dramatically to lower energy upon temperature cooling, which might be associated with the consequence of lattice parameter shrinking. In addition, an extremely sharp peak shows up in the frequency dependent optical conductivity, indicating the presence of a Van Hove singularity in the joint density of state.

cond-mat.mtrl-sci↗

arXiv2015

Optical study of phase transitions in single-crystalline RuP

RuP single crystals of MnP-type orthorhombic structure were synthesized by the Sn flux method. Temperature-dependent x-ray diffraction measurements reveal that the compound experiences two structural phase transitions, which are further confirmed by enormous anomalies shown in temperature-dependent resistivity and magnetic susceptibility. Particularly, the resistivity drops monotonically upon temperature cooling below the second transition, indicating that the material shows metallic behavior, in sharp contrast with the insulating ground state of polycrystalline samples. Optical conductivity measurements were also performed in order to unravel the mechanism of these two transitions. The measurement revealed a sudden reconstruction of band structure over a broad energy scale and a significant removal of conducting carriers below the first phase transition, while a charge-density-wave-like energy gap opens below the second phase transition.

cond-mat.str-el↗

arXiv2014

Kondo effect in a novel 5d quasi-skutterudite Yb3Os4Ge13

We report the crystal growth of a new compound, Yb3Os4Ge13, by using a Bi-flux method. X-ray diffraction measurement shows that it crystallizes in the quasi-skutterudite-type caged structure with a cubic space group of Pm-3n (No. 223). Magnetic measurements reveal almost fully localized Yb f-moments above 120 K. The resistivity exhibits a crossover from metallic to insulating behavior with a logarithmic increase below ~ 40 K. The specific heat coefficient shows a rapid upturn below ~5 K and exceeds 2 J mol-1 K-2 at 2 K. Our experimental analysis and electronic band structure calculations demonstrate that Yb3Os4Ge13 exhibits the Kondo effect due to strong hybridization of the localized Yb f-moments with the p-electrons of the surrounding Ge-cages.

cond-mat.str-el↗

arXiv2014

Coexistence of superconductivity and density wave in $\mathrm{Ba_2Ti_2Fe_2As_4O}$: an optical spectroscopy study

We performed an optical spectroscopy measurement on single crystals of $\mathrm{Ba_2Ti_2Fe_2As_4O}$, which is a newly discovered superconductor showing a coexistence of superconductivity and density wave order. The study reveals a spectral change related to the formation density wave energy gap below $T_{DW}\approx$125 K, leading to the removal of about half of the multiple Fermi surface sheets. The ratio of 2$Δ_{DW}$/$k_B T_{DW}\approx$ 11.9 is considerably larger than the mean-field value based on the weak-coupling BCS theory. At the lowest temperature in the superconducting state, we observed opening of superconducting energy gaps $Δ_1(0) =3.4$ meV and $Δ_2(0)=7.9$ meV. The properties of superconducting state in $\mathrm{Ba_2Ti_2Fe_2As_4O}$ are similar to that in $\mathrm{BaFe_{1.85}Co_{0.15}As_2}$.

cond-mat.supr-con↗

arXiv2014

Optical spectroscopy study of the collapsed tetragonal phase of CaFe$_2$(As$_{0.935}$P$_{0.065}$)$_2$ single crystals

We present an optical spectroscopy study on P-doped CaFe$_2$As$_2$ which experiences a structural phase transition from tetragonal to collapsed tetragonal (cT) phase near 75 K. The measurement reveals a sudden reduction of low frequency spectral weight and emergence of a new feature near 3200 \cm (0.4 eV) in optical conductivity across the transition, indicating an abrupt reconstruction of band structure. The appearance of new feature is related to the interband transition arising from the sinking of hole bands near $Γ$ point below Fermi level in the cT phase, as expected from the density function theory calculations in combination with the dynamical mean field theory. However, the reduction of Drude spectral weight is at variance with those calculations. The measurement also indicates an absence of the abnormal spectral weight transfer at high energy (near 0.5-0.7 eV) in the cT phase, suggesting a suppression of electron correlation effect.

cond-mat.supr-con↗

arXiv2014

Raman scattering investigation of the electron-phonon coupling in superconducting Nd(O,F)BiS$_2$

We have performed polarized Raman scattering measurements on the newly discovered superconductor Nd(O,F)BiS$_2$ ($T_c = 4$ K). We observe 2 Raman active modes, with frequencies in accordance with first-principles calculations. One A$_{1g}$ phonon mode at 112.4 cm$^{-1}$ exhibits a Fano line shape due to electron-phonon coupling. We find a resonance for this mode at 2.45 eV excitation energy. We estimate a 0.68 contribution of this mode to the electron-phonon coupling constant $λ$. Our Raman results suggest that the BiS$_2$-based superconductors are possibly phonon-mediated BCS superconductors.

cond-mat.supr-con↗

arXiv2014

Coexistence and competition of multiple charge-density-wave orders in rare-earth tri-telluride RTe3

The occurrences of collective quantum states, such as superconductivity (SC) and charge- or spin-densitywaves (CDWs or SDWs), are among the most fascinating phenomena in solids. To date much effort has been made to explore the interplay between different orders, yet little is known about the relationship of multiple orders of the same type. Here we report optical spectroscopy study on CDWs in the rare-earth tri-telluride compounds RTe3 (R = rare earth elements). Besides the prior reported two CDW orders, the study reveals unexpectedly the presence of a third CDW order in the series which evolves systematically with the size of R element. With increased chemical pressure, the first and third CDW orders are both substantially suppressed and compete with the second one by depleting the low energy spectral weight. A complete phase diagram for the multiple CDW orders in this series is established.

cond-mat.str-el↗

arXiv2014

Unconventional charge-density wave in Sr3Ir4Sn13 cubic superconductor revealed by optical spectroscopy study

Sr3Ir4Sn13 is an interesting compound showing a coexistence of structural phase transition and superconductivity. The structural phase transition at 147 K leads to the formation of a superlattice. We performed optical spectroscopy measurements across the structural phase transition on single crystal sample of Sr3Ir4Sn13. The optical spectroscopy study reveals an unusual temperature induced spectral weight transfer over broad energy scale, yielding evidence for the presence of electron correlation effect. Below the structural phase transition temperature an energy gap-like suppression in optical conductivity was observed, leading to the removal of partial itinerant carriers near Fermi level. Unexpectedly, the suppression appears at much higher energy scale than that expected for a usual charge density wave phase transition.

cond-mat.supr-con↗

arXiv2014

Optical spectroscopy study of Nd(O,F)BiS2 single crystals

We present an optical spectroscopy study on F-substituted NdOBiS$_2$ superconducting single crystals grown using KCl/LiCl flux method. The measurement reveals a simple metallic response with a relatively low screened plasma edge near 5000 \cm. The plasma frequency is estimated to be 2.1 eV, which is much smaller than the value expected from the first-principles calculations for an electron doping level of x=0.5, but very close to the value based on a doping level of 7$\%$ of itinerant electrons per Bi site as determined by ARPES experiment. The energy scales of the interband transitions are also well reproduced by the first-principles calculations. The results suggest an absence of correlation effect in the compound, which essentially rules out the exotic pairing mechanism for superconductivity or scenario based on the strong electronic correlation effect. The study also reveals that the system is far from a CDW instability as being widely discussed for a doping level of x=0.5.

cond-mat.supr-con↗