arXiv subjects

N. M. R. Peres

Publications and source records attributed to N. M. R. Peres.

At least 55 records · Page 3Linked to original sources

arXiv2020

Ionisation rate and Stark shift of a one-dimensional model of the Hydrogen molecular ion

In this paper we study the ionization rate and the Stark shift of a one-dimensional model of the H$_{2}^{+}$ ion. The finding of these two quantities is reduced to the solutions of a complex eigenvalue problem. We solve this problem both numerically and analytically. In the latter case we consider the regime of small external electrostatic fields and small internuclear distances. We find an excellent agreement between the ionization rate computed with the two approaches, even when the approximate result is pushed beyond its expected validity. The ionization rate is very sensitive to small changes of the external electrostatic field, spanning many orders of magnitude for small changes of the intensity of the external field. The dependence of the ionization on the internuclear distance is also studied, as this has a direct connection with experimental methods in molecular physics. It is shown that for large distances the ionization rate saturates, which is a direct consequence of the behavior of the energy eigenvalue with the internuclear distance. The Stark shift is computed and from it we extract the static polarizability of H$_{2}^{+}$ and compare our results with those found by other authors using more sophisticated methods.

physics.atom-ph↗

arXiv2020

Non-reciprocal magnons in a two dimensional crystal with off-plane magnetization

Non reciprocal spin waves have a chiral asymmetry so that their energy is different for two opposite wave vectors. They are found in atomically thin ferromagnetic overlayers with in plane magnetization and are linked to the anti-symmetric Dzyaloshinskii-Moriya surface exchange. We use an itinerant fermion theory based on first principles calculations to predict that non-reciprocal magnons can occur in Fe$_3$GeTe$_2$, the first stand alone metallic two dimensional crystal with off-plane magnetization. We find that both the energy and lifetime of magnons are non-reciprocal and we predict that acoustic magnons can have lifetimes up to hundreds of picoseconds, orders of magnitude larger than in other conducting magnets.

cond-mat.mes-hall↗

arXiv2020

Analytical Quantitative Semi-Classical Approach to the LoSurdo-Stark Effect and Ionization in 2D excitons

Using a semi-classical approach, we derive a fully analytical expression for the ionization rate of excitons in two-dimensional materials due to an external static electric field, which eliminates the need for complicated numerical calculations. Our formula shows quantitative agreement with more sophisticated numerical methods based on the exterior complex scaling approach, which solves a non-hermitian eigenvalue problem yielding complex energy eigenvalues, where the imaginary part describes the ionization rate. Results for excitons in hexagonal boron nitride and the $A-$exciton in transition metal dichalcogenides are given as a simple examples. The extension of the theory to include spin-orbit-split excitons in transition metal dichalcogenides is trivial.

cond-mat.mes-hall↗

arXiv2020

Magneto-optical Kerr effect in spin split two-dimensional massive Dirac materials

Two-dimensional (2D) massive Dirac electrons possess a finite Berry curvature, with Chern number $\pm 1/2$, that entails both a quantized dc Hall response and a subgap full-quarter Kerr rotation. The observation of these effects in 2D massive Dirac materials such as gapped graphene, hexagonal boron nitride or transition metal dichalcogenides (TMDs) is obscured by the fact that Dirac cones come in pairs with opposite sign Berry curvatures, leading to a vanishing Chern number. Here, we show that the presence of spin-orbit interactions, combined with an exchange spin splitting induced either by diluted magnetic impurities or by proximity to a ferromagnetic insulator, gives origin to a net magneto-optical Kerr effect in such systems. We focus on the case of TMD monolayers and study the dependence of Kerr rotation on frequency and exchange spin splitting. The role of the substrate is included in the theory and found to critically affect the results. Our calculations indicate that state-of-the-art magneto-optical Kerr spectroscopy can detect a single magnetic impurity in diluted magnetic TMDs.

cond-mat.mes-hall↗

arXiv2020

Topological magnons in CrI$_3$ monolayers: an itinerant fermion description

Magnons dominate the magnetic response of the recently discovered insulating ferromagnetic two dimensional crystals such as CrI$_3$. Because of the arrangement of the Cr spins in a honeycomb lattice, magnons in CrI$_3$ bear a strong resemblance with electronic quasiparticles in graphene. Neutron scattering experiments carried out in bulk CrI$_3$ show the existence of a gap at the Dirac points, that has been conjectured to have a topological nature. Here we propose a theory for magnons in ferromagnetic CrI$_3$ monolayers based on an itinerant fermion picture, with a Hamiltonian derived from first principles. We obtain the magnon dispersion for 2D CrI$_3$ with a gap at the Dirac points with the same Berry curvature in both valleys. For CrI$_3$ ribbons, we find chiral in-gap edge states. Analysis of the magnon wave functions in momentum space further confirms their topological nature. Importantly, our approach does not require to define a spin Hamiltonian, and can be applied to both insulating and conducting 2D materials with any type of magnetic order.

cond-mat.mes-hall↗

arXiv2020

Topological Photonic Tamm-States and the Su-Schrieffer-Heeger Model

In this paper we study the formation of topological Tamm states at the interface between a semi-infinite one-dimensional photonic-crystal and a metal. We show that when the system is topologically non-trivial there is a single Tamm state in each of the band-gaps, whereas if it is topologically trivial the band-gaps host no Tamm states. We connect the disappearance of the Tamm states with a topological transition from a topologically non-trivial system to a topologically trivial one. This topological transition is driven by the modification of the dielectric functions in the unit cell. Our interpretation is further supported by an exact mapping between the solutions of Maxwell's equations and the existence of a tight-binding representation of those solutions. We show that the tight-binding representation of the 1D photonic crystal, based on Maxwell's equations, corresponds to a Su-Schrieffer-Heeger-type model (SSH-model) for each set of pairs of bands. Expanding this representation near the band edge we show that the system can be described by a Dirac-like Hamiltonian. It allows one to characterize the topology associated with the solution of Maxwell's equations via the winding number. In addition, for the infinite system, we provide an analytical expression for the photonic bands from which the band-gaps can be computed.

cond-mat.mes-hall↗

arXiv2020

Excitonic Magneto-Optical Kerr Effect in 2D Transition Metal Dichalcogenides Induced by Spin Proximity

In this paper we develop the excitonic theory of Kerr rotation angle in a two-dimensional (2D) transition metal dichalcogenide at zero magnetic field. The finite Kerr angle is induced by the interplay between spin-orbit splitting and proximity exchange coupling due to the presence of a ferromagnet. We compare the excitonic effect with the single particle theory approach. We show that the excitonic properties of the 2D material lead to a dramatic change in the frequency dependence of the optical response function. We also find that the excitonic corrections enhance the optical response by a factor of two in the case of MoS2 in proximity to a Cobalt thin film.

cond-mat.mes-hall↗

arXiv2019

Excitons in Phosphorene: A Semi-Analytical Perturbative Approach

In this paper we develop a semi-analytical perturbation-theory approach to the calculation of the energy levels (binding energies) and wave functions of excitons in phosphorene. Our method gives both the exciton wave function in real and reciprocal spaces with the same ease. This latter aspect is important for the calculation of the nonlinear optical properties of phosphorene. We find that our results are in agreement with calculations based both on the Bethe-Salpeter equation and on Monte Carlo simulations, which are computationally much more demanding. Our approach thus introduces a simple, viable, and accurate method to address the problem of excitons in anisotropic two-dimensional materials.

cond-mat.mes-hall↗

arXiv2019

The magnetic Purcell effect: the case of an emitter near an antiferromagnet

In this paper we discuss the magnetic Purcell effect of a magnetic dipole near a semi-infinite antiferromagnet. Contrary to the electric Purcell effect, the magnetic one is not so well studied in the literature. We derive the dispersion relation of the surface wave existing at an antiferromagnetic-dielectric interface from the calculation of the reflection coefficient of the structure. After characterizing the surface wave we quantize the electromagnetic vector potential of the surface wave. This allow us to discuss the magnetic Purcell effect via Fermi golden rule.

cond-mat.mes-hall↗

arXiv2019

Propagation of surface plasmons on plasmonic Bragg gratings

We use coupled-mode theory to describe the scattering of a surface-plasmon polariton (SPP) from a square wave grating (Bragg grating) of finite extension written on the surface of either a metal-dielectric interface or a dielectric-dielectric interface covered with a patterned graphene sheet. We find analytical solutions for the reflectance and transmittance of SPP's when only two modes (forward- and back-scattered) are considered. We show that in both cases the reflectance spectrum presents stop-bands where the SPP is completely back-scattered, if the grating is not too shallow. In addition, the reflectance coefficient shows Fabry-Pérot oscillations when the frequency of the SPP is out of the stop-band region. For a single dielectric well, we show that there are frequencies of transmission equal to 1. We also provide simple analytical expression for the different quantities in the electrostatic limit.

cond-mat.mes-hall↗

arXiv2019

Twisted bilayer graphene: low-energy physics, electronic and optical properties

Van der Waals (vdW) heterostructures ---formed by stacking or growing two-dimensional (2D) crystals on top of each other--- have emerged as a new promising route to tailor and engineer the properties of 2D materials. Twisted bilayer graphene (tBLG), a simple vdW structure where the interference between two misaligned graphene lattices leads to the formation of a moiré pattern, is a test bed to study the effects of the interaction and misalignment between layers, key players for determining the electronic properties of these stackings. In this chapter, we present in a pedagogical way the general theory used to describe lattice mismatched and misaligned vdW structures. We apply it to the study of tBLG in the limit of small rotations and see how the coupling between the two layers leads both to an angle dependent renormalization of graphene's Fermi velocity and appearance of low-energy van Hove singularities. The optical response of this system is then addressed by computing the optical conductivity and the dispersion relation of tBLG surface plasmon-polaritons.

cond-mat.mes-hall↗

arXiv2019

Absorption of single-layer hexagonal boron nitride in the ultraviolet

In this paper we theoretically describe the absorption of hexagonal boron nitride (hBN) single layer. We develop the necessary formalism and present an efficient method for solving the Wannier equation for excitons. We give predictions for the absorption of hBN on quartz and on graphite. We compare our predictions with recently published results [Elias {\it et al.}, Nat. Comm. {\bf 10}, 2639 (2019)] for a monolayer of hBN on graphite. The spontaneous radiative lifetime of excitons in hBN is also computed. We argue that the optical properties of hBN in the ultraviolet are very useful for the study of peptides and other biomolecules.

cond-mat.mes-hall↗

arXiv2019

Excitation of SPP's in graphene by a waveguide mode

We present a semi-analytical model that predicts the excitation of surface-plasmon polaritons (SPP) on a graphene sheet located in front of a sub-wavelength slit drilled in thick metal screen. We identify the signature of the SPP in the transmission, reflection, and absorption curves. Following previous literature on noble-metal plasmonics, we characterize the efficiency of excitation of SPP's in graphene computing a spatial probability density. This quantity shows the presence of plasmonics resonances dispersing with the Fermi energy, $E_F$, as $\sqrt{E_F}$ an unambiguous signature of graphene plasmons.

cond-mat.mes-hall↗

arXiv2019

Quantization of graphene plasmons

In this article we perform the quantization of graphene plasmons using both a macroscopic approach based on the classical average electromagnetic energy and a quantum hydrodynamic model, in which graphene charge carriers are modeled as a charged fluid. Both models allow to take into account the dispersion of graphenes optical response, with the hydrodynamic model also allowing for the inclusion of non-local effects. Using both methods, the electromagnetic field mode-functions, and the respective frequencies, are determined for two different graphene structures. we show how to quantize graphene plasmons, considering that graphene is a dispersive medium, and taking into account both local and nonlocal descriptions. It is found that the dispersion of graphene's optical response leads to a non-trivial normalization condition for the mode-functions. The obtained mode-functions are then used to calculate the decay of an emitter, represented by a dipole, via the excitation of graphene surface plasmon-polaritons. The obtained results are compared with the total spontaneous decay rate of the emitter and a near perfect match is found in the relevant spectral range. It is found that non-local effects in graphene's conductivity, become relevant for the emission rate for small Fermi energies and small distances between the dipole and the graphene sheet.

cond-mat.mes-hall↗

arXiv2019

Excitonic magneto-optics in monolayer transition metal dichalcogenides: From nanoribbons to two-dimensional response

The magneto-optical response of monolayer transition metal dichalcogenides (TMDs), including excitonic effects, is studied using a nanoribbon geometry. We compute the diagonal optical conductivity and the Hall conductivity. Comparing the excitonic optical Hall conductivity to results obtained in the independent particle approximation, we find an increase in the amplitude corresponding to one order of magnitude when excitonic effects are included. The Hall conductivities are used to calculate Faraday rotation spectra for MoS2 and WSe2. Finally, we have also calculated the diamagnetic shift of the exciton states of WSe2 in different dielectric environments. Comparing the calculated diamagnetic shift to recent experimental measurements, we find a very good agreement between the two.

cond-mat.mes-hall↗

arXiv2019

Optical orientation with linearly polarized light in transition metal dichalcogenides

We study the optical properties of semiconducting transition metal dichalcogenide monolayers under the influence of strong out-of-plane magnetic fields, using the effective massive Dirac model. We pay attention to the role of spin-orbit coupling effects, doping level and electron-electron interactions, treated at the Hartree-Fock level. We find that optically-induced valley and spin imbalance, commonly attained with circularly polarized light, can also be obtained with linearly polarized light in the doped regime. Additionally, we explore an exchange-driven mechanism to enhance the spin-orbit splitting of the conduction band, in n-doped systems, controlling both the carrier density and the intensity of the applied magnetic field.

cond-mat.mes-hall↗

arXiv2019

Hybrid plasmon-magnon polaritons in graphene-antiferromagnet heterostructures

We consider a hybrid structure formed by graphene and an insulating antiferromagnet, separated by a dielectric of thickness up to $d\simeq 500 \,nm$. When uncoupled, both graphene and the antiferromagnetic surface host their own polariton modes coupling the electromagnetic field with plasmons in the case of graphene, and with magnons in the case of the antiferromagnet. We show that the hybrid structure can host two new types of hybrid polariton modes. First, a surface magnon-plasmon polariton whose dispersion is radically changed by the carrier density of the graphene layer, including a change of sign in the group velocity. Second, a surface plasmon-magnon polariton formed as a linear superposition of graphene surface plasmon and the antiferromagnetic bare magnon. This polariton has a dispersion with two branches, formed by the anticrossing between the dispersive surface plasmon and the magnon. We discuss the potential these new modes have for combining photons, magnons, and plasmons to reach new functionalities.

cond-mat.mes-hall↗

arXiv2018

Two-dimensional materials in the presence of nonplanar interfaces

We consider a planar two-dimensional system between two media with different dielectric constants and in the presence of a third dielectric medium separated by a nonplanar interface. Extending a perturbative method for solving Poisson's equation, developed by Clinton, Esrick, and Sacks [Phys. Rev. B, 31, 7540 (1985)], in the presence of nonplanar conducting boundaries to the situation proposed here, we obtain, up to the first order in terms of the function which defines the nonplanar interface, the effective potential, the effective electrostatic field, the effective dielectric constant for the planar 2D system, and the effective external field acting in-plane in the 2D system. Implications of the results to properties of 2D systems are discussed. In the limit of planar surfaces, vacuum-dielectric or vacuum-conducting media, our results are in agreement with those found in the literature.

cond-mat.mes-hall↗