arXiv subjects

N. Marginean

Publications and source records attributed to N. Marginean.

At least 19 recordsLinked to original sources

arXiv2025

The 76Cu conundrum remains unsolved

Near the doubly-magic nucleus \nuc{Ni}{78} ($Z=28$, $N=50$), there has been a decades-long debate on the existence of a long-lived isomer in \nuc{Cu}{76}. A recent mass measurement claimed to have settled the debate, by measuring the energy of the isomer and shedding light on the structure of the nucleus. In this work, we present new, more accurate, and precise values of the half-lives of the isomeric and ground states in \nuc{Cu}{76}. Our findings suggest that both states have very similar half-lives, in the 600-700 ms range, in disagreement with the literature values, implying that they cannot be differentiated by their decay curves. These results raise more questions than they answer, reopening the debate and showing that the structures in \nuc{Cu}{76} are still not fully understood.

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arXiv2024

Beta delayed neutron emission of $N=84$ $^{132}$Cd

Using the time-of-flight technique, we measured the beta-delayed neutron emission of $^{132}$Cd. From our large-scale shell model (LSSM) calculation using the N$^3$LO interaction [Z.Y. Xu et al., Phys. Rev. Lett. 131, 022501 (2023)], we suggest the decay is dominated by the transformation of a neutron in the $g_{7/2}$ orbital, deep below the Fermi surface, into a proton in the $g_{9/2}$ orbital. We compare the beta-decay half-lives and neutron branching ratios of nuclei with $Z<50$ and $N\geq82$ obtained with our LSSM with those of leading "global" models such as Finite-Range Droplet Model (FRDM). Our calculations match known half-lives and neutron branching ratios well and suggest that current leading models overestimate the yet-to-be-measured half-lives. Our model, backed by the $^{132}$Cd decay data presented here, offers robust predictive power for nuclei of astrophysical interest such as $r$-process waiting points.

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arXiv2024

Revealing the nature of yrast states in neutron-rich polonium isotopes

Polonium isotopes having two protons above the shell closure at $Z=82$ show a wide variety of low-lying high-spin isomeric states across the whole chain. The structure of neutron-deficient isotopes up to $^{210}$Po ($N=126$) is well established as they are easily produced through various methods. However, there is not much information available for the neutron-rich counterparts for which only selective techniques can be used for their production. We report on the first fast-timing measurements of yrast states up to the 8$^+$ level in $^{214,216,218}$Po isotopes produced in the $β^-$ decay of $^{214,216,218}$Bi at ISOLDE, CERN. In particular, our new half-life value of 607(14) ps for the 8$_1^+$ state in $^{214}$Po is nearly 20 times shorter than the one available in literature and comparable with the newly measured half-lives of 409(16) and 628(25) ps for the corresponding 8$_1^+$ states in $^{216,218}$Po, respectively. The measured $B(E2;8_1^+ \to 6_1^+)$ transition probability values follow an increasing trend relative to isotope mass, reaching a maximum for $^{216}$Po. The increase contradicts the previous claims of isomerism for the $8^+$ yrast states in neutron-rich $^{214}$Po and beyond. Together with the other measured yrast transitions, the $B(E2)$ values provide a crucial test of the different theoretical approaches describing the underlying configurations of the yrast band. The new experimental results are compared to shell-model calculations using the KHPE and H208 effective interactions and their pairing modified versions, showing an increase in configuration mixing when moving towards the heavier isotopes.

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arXiv2024

High-resolution spectroscopy of neutron-rich Br isotopes and signatures for a prolate-to-oblate shape transition at N=56

The first systematic experimental study of the neutron-rich Br isotopes with two complementary state-of-the-art techniques is presented. These isotopes have been populated in the fission process at two different facilities, GANIL and ILL. New spectroscopic information has been obtained for odd-even $^{87-93}$Br isotopes and the experimental results have been compared with state-of-the-art Large-Scale Shell-Model and DNO Shell-Model calculations. As a result of such theoretical approaches, a transition from prolate ($^{87,89}$Br) to oblate ($^{91,93}$Br) shapes is obtained from the subtle balance between proton and neutron quadrupole deformations, as a clear signature of pseudo-SU3 quadrupole regime.

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arXiv2024

Detailed study of the decay of $^{21}$Mg

Beta-delayed proton and gamma emission in the decay of $^{21}$Mg has been measured at ISOLDE, CERN with the ISOLDE Decay Station (IDS) set-up. The existing decay scheme is updated, in particular what concerns proton transitions to excited states in $^{20}$Ne. Signatures of interference in several parts of the spectrum are used to settle spin and parity assignments to highly excited states in $^{21}$Na. The previously reported $β$p$α$ branch is confirmed. A half-life of 120.5(4) ms is extracted for $^{21}$Mg. The revised decay scheme is employed to test mirror symmetry in the decay and to extract the beta strength distribution of $^{21}$Mg that is compared with theory.

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arXiv2023

Simultaneous $γ$-ray and electron spectroscopy of $^{182,184,186}$Hg isotopes

Background: The mercury isotopes around $N=104$ are a well-known example of nuclei exhibiting shape coexistence. Mixing of configurations can be studied by measuring the monopole strength $ρ^2(E0)$, however, currently the experimental information is scarce and lacks precision, especially for the $I^π\rightarrow I^π$ ($I \neq 0$) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in $^{182,184,186}$Hg and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in $^{182,184,186}$Hg were populated in the $β$ decay of $^{182,184,186}$Tl, produced at ISOLDE and purified by laser ionization and mass separation. The $γ$-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes. Results: In total, 193, 178 and 156 transitions, including 144, 140 and 108 observed for the first time in a $β$-decay experiment, were assigned to $^{182,184,186}$Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an $E0$ component. Extracted branching ratios allowed the sign of the interference term in $^{182}$Hg as well as $ρ^2(E0;0^+_2\rightarrow 0^+_1)$ and $B(E2;0^+_2\rightarrow 2^+_1)$ in $^{184}$Hg to be determined. By means of electron-electron coincidences, the $0^+_3$ state was identified in $^{184}$Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the IBM with configuration mixing with two different parametrizations, the General Bohr Hamiltonian, the BMF model and the SCCM model. However, a quantitative description is lacking.

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arXiv2023

133In: A Rosetta Stone for decays of r-process nuclei

The $β$ decays from both the ground state and a long-lived isomer of $^{133}$In were studied at the ISOLDE Decay Station (IDS). With a hybrid detection system sensitive to $β$, $γ$, and neutron spectroscopy, the comparative partial half-lives (logft) have been measured for all their dominant $β$-decay channels for the first time, including a low-energy Gamow-Teller transition and several First-Forbidden (FF) transitions. Uniquely for such a heavy neutron-rich nucleus, their $β$ decays selectively populate only a few isolated neutron unbound states in $^{133}$Sn. Precise energy and branching-ratio measurements of those resonances allow us to benchmark $β$-decay theories at an unprecedented level in this region of the nuclear chart. The results show good agreement with the newly developed large-scale shell model (LSSM) calculations. The experimental findings establish an archetype for the $β$ decay of neutron-rich nuclei southeast of $^{132}$Sn and will serve as a guide for future theoretical development aiming to describe accurately the key $β$ decays in the rapid-neutron capture (r-) process.

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arXiv2023

Beta-delayed neutron spectroscopy of $^{133}$In

The decay properties of $^{133}$In were studied in detail at the ISOLDE Decay Station (IDS). The implementation of the Resonance Ionization Laser Ion Source (RILIS) allowed separate measurements of its $9/2^+$ ground state ($^{133g}$In) and $1/2^-$ isomer ($^{133m}$In). With the use of $β$-delayed neutron and $γ$ spectroscopy, the decay strengths above the neutron separation energy were quantified in this neutron-rich nucleus for the first time. The allowed Gamow-Teller transition $9/2^+\rightarrow7/2^+$ was located at 5.92 MeV in the $^{133g}$In decay with a logft = 4.7(1). In addition, several neutron-unbound states were populated at lower excitation energies by the First-Forbidden decays of $^{133g,m}$In. We assigned spins and parities to those neutron-unbound states based on the $β$-decay selection rules, the logft values, and systematics.

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arXiv2020

Detailed low-spin spectroscopy of 65Ni via neutron capture reaction

An extended investigation of the low-spin structure of the $^{65}$Ni nucleus was performed at the Institut Laue-Langevin, Grenoble, via the neutron capture reaction $^{64}$Ni(n,$γ$)$^{65}$Ni, using the FIPPS HPGe array. The level scheme of $^{65}$Ni was significantly expanded, with 2 new levels and 87 newly found transitions. Angular correlation analyses were also performed, allowing us to assign spins and parities for a number of states, and to determine multipolarity mixing ratios for selected $γ$ transitions. The low-energy part of the experimental level scheme (up to about 1.4 MeV) was compared with Monte Carlo Shell Model calculations, which predict spherical shapes for all states, apart from the 9/2$^+$ and the second excited 1/2$^-$ states of oblate deformation.

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arXiv2020

Decay studies of the long-lived states in $^{186}$Tl

Decay spectroscopy of the long-lived states in $^{186}$Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The $α$ decay from the low-spin $(2^-)$ state in $^{186}$Tl was observed for the first time and a half-life of $3.4^{+0.5}_{-0.4}$ s was determined. Based on the $α$-decay energy, the relative positions of the long-lived states were fixed, with the $(2^-)$ state as the ground state, the $7^{(+)}$ state at 77(56)~keV and the $10^{(-)}$ state at 451(56) keV. The level scheme of the internal decay of the $^{186}$Tl($10^{(-)}$) state ($T_{1/2} = 3.40(9)$ s), which was known to decay solely through emission of 374 keV $γ$-ray transition, was extended and a lower-limit for the $β$-decay branching $b_β> 5.9(3)\%$ was determined. The extracted retardation factors for the $γ$ decay of the $10^{(-)}$ state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the $πd_{3/2}$ shell in the isomeric decay and significant structure differences between $^{184}$Tl and $^{186}$Tl.

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arXiv2020

Detailed spectroscopy of doubly magic $^{132}$Sn

The structure of the doubly magic $^{132}_{50}$Sn$_{82}$ has been investigated at the ISOLDE facility at CERN, populated both by the $β^-$decay of $^{132}$In and $β^-$-delayed neutron emission of $^{133}$In. The level scheme of $^{132}$Sn is greatly expanded with the addition of 68 $γ$-transitions and 17 levels observed for the first time in the $β$ decay. The information on the excited structure is completed by new $γ$-transitions and states populated in the $β$-n decay of $^{133}$In. Improved delayed neutron emission probabilities are obtained both for $^{132}$In and $^{133}$In. Level lifetimes are measured via the Advanced Time-Delayed $βγγ$(t) fast-timing method. An interpretation of the level structure is given based on the experimental findings and the particle-hole configurations arising from core excitations both from the \textit{N} = 82 and \textit{Z} = 50 shells, leading to positive and negative parity particle-hole multiplets. The experimental information provides new data to challenge the theoretical description of $^{132}$Sn.

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arXiv2020

Experimental study of the 2n-transfer reaction $^{138}$Ba($^{18}$O,$^{16}$O)$^{140}$Ba in the projectile energy range 61-67 MeV

Two-neutron transfer reactions serve as an important tool for nuclear structure studies in the neutron rich part of the nuclear chart. In this article, we report on the first experimental attempt to populate the excited states of $^{140}$Ba employing the 2n-neutron transfer reaction $^{138}$Ba($^{18}$O,$^{16}$O)$^{140}$Ba. $^{140}$Ba is highly important, as it is placed on the onset of octupole correlations and the lifetimes of its excited states are completely unknown, with the sole exception of the first 2$^+$ state. The experiment was carried out at the Horia Hulubei National Institute for Physics and Nuclear Engineering (IFIN-HH) in Magurele, Romania. Lower limits on the lifetimes of ground state band up to the 8$^+$ state are reported. Furthermore, relative cross sections regarding the 2n-transfer reaction with respect to the fusion and the total inelastic reaction channels have been deduced. Further investigation directions of the nuclear structure of $^{140}$Ba are also discussed.

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arXiv2019

Normal and intruder configurations in $^{34}$Si populated in the $β^-$ decay of $^{34}$Mg and $^{34}$Al

The structure of $^{34}$Si was studied through $γ$ spectroscopy separately in the $β^-$ decays of $^{34}$Mg and $^{34}$Al at the ISOLDE facility of CERN. Different configurations in $^{34}$Si were populated independently from the two recently identified $β$-decaying states in $^{34}$Al having spin-parity assignments $J^π= 4^-$ dominated by the normal configuration $π(d_{5/2})^{-1} \otimes ν(f_{7/2})$ and $J^π= 1^+$ by the intruder configuration $π(d_{5/2})^{-1} \otimes ν(d_{3/2})^{-1}(f_{7/2})^{2}$. The paper reports on spectroscopic properties of $^{34}$Si such as an extended level scheme, spin and parity assignments based on log($ft$) values and $γ$-ray branching ratios, absolute $β$ feeding intensities and neutron emission probabilities. A total of 11 newly identified levels and 26 transitions were added to the previously known level scheme of $^{34}$Si. Large scale shell-model calculations using the {\sc sdpf-u-mix} interaction, able to treat higher order intruder configurations, are compared with the new results and conclusions are drawn concerning the predictive power of {\sc sdpf-u-mix}, the $N=20$ shell gap, the level of mixing between normal and intruder configurations for the 0$_1^+$, 0$_2^+$ and 2$_1^+$ states and the absence of triaxial deformation in $^{34}$Si.

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arXiv2018

First Accurate Normalization of the $β$-delayed $α$ Decay of $^{16}$N and Implications for the $^{12}$C$(α,γ)^{16}$O Astrophysical Reaction Rate

The $^{12}\text{C}(α,γ){}^{16}\text{O}$ reaction plays a central role in astrophysics, but its cross section at energies relevant for astrophysical applications is only poorly constrained by laboratory data. The reduced $α$ width, $γ_{11}$, of the bound $1^-$ level in $^{16}$O is particularly important to determine the cross section. The magnitude of $γ_{11}$ is determined via sub-Coulomb $α$-transfer reactions or the $β$-delayed $α$ decay of $^{16}$N, but the latter approach is presently hampered by the lack of sufficiently precise data on the $β$-decay branching ratios. Here we report improved branching ratios for the bound $1^-$ level [$b_{β,11} = (5.02\pm 0.10)\times 10^{-2}$] and for $β$-delayed $α$ emission [$b_{βα} = (1.59\pm 0.06)\times 10^{-5}$]. Our value for $b_{βα}$ is 33% larger than previously held, leading to a substantial increase in $γ_{11}$. Our revised value for $γ_{11}$ is in good agreement with the value obtained in $α$-transfer studies and the weighted average of the two gives a robust and precise determination of $γ_{11}$, which provides significantly improved constraints on the $^{12}$C$(α,γ)$ cross section in the energy range relevant to hydrostatic He burning.

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arXiv2016

The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus 133Sb

The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

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arXiv2012

Nuclear photonics at ultra-high counting rates and higher multipole excitations

Next-generation gamma beams beams from laser Compton-backscattering facilities like ELI-NP (Bucharest)] or MEGa-Ray (Livermore) will drastically exceed the photon flux presently available at existing facilities, reaching or even exceeding 10^13 gamma/sec. The beam structure as presently foreseen for MEGa-Ray and ELI-NP builds upon a structure of macro-pulses (~120 Hz) for the electron beam, accelerated with X-band technology at 11.5 GHz, resulting in a micro structure of 87 ps distance between the electron pulses acting as mirrors for a counterpropagating intense laser. In total each 8.3 ms a gamma pulse series with a duration of about 100 ns will impinge on the target, resulting in an instantaneous photon flux of about 10^18 gamma/s, thus introducing major challenges in view of pile-up. Novel gamma optics will be applied to monochromatize the gamma beam to ultimately Delta E/E~10^-6. Thus level-selective spectroscopy of higher multipole excitations will become accessible with good contrast for the first time. Fast responding gamma detectors, e.g. based on advanced scintillator technology (e.g. LaBr3(Ce)) allow for measurements with count rates as high as 10^6-10^7 gamma/s without significant drop of performance. Data handling adapted to the beam conditions could be performed by fast digitizing electronics, able to sample data traces during the micro-pulse duration, while the subsequent macro-pulse gap of ca. 8 ms leaves ample time for data readout. A ball of LaBr3 detectors with digital readout appears to best suited for this novel type of nuclear photonics at ultra-high counting rates.

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arXiv2012

Fast-timing measurements in 95,96Mo

Half-lives of the 19/2+ and 21/2+ states in 95Mo and of the 8+ and 10+ states in 96Mo were measured. Matrix elements for yrast transitions in 95Mo and 96Mo are discussed.

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arXiv2011

In-beam fast-timing measurements in 103,105,107Cd

Fast-timing measurements were performed recently in the region of the medium-mass 103,105,107Cd isotopes, produced in fusion evaporation reactions. Emitted gamma-rays were detected by eight HPGe and five LaBr3:Ce detectors working in coincidence. Results on new and re-evaluated half-lives are discussed within a systematic of transition rates. The $7/2_1^+$ states in 103,105,107Cd are interpreted as arising from a single-particle excitation. The half-life analysis of the $11/2_1^-$ states in 103,105,107Cd shows no change in the single-particle transition strength as a function of the neutron number.

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