arXiv subjects

N. Ogawa

Publications and source records attributed to N. Ogawa.

15 recordsLinked to original sources

arXiv2023

Anomalous charge transport upon quantum melting of chiral spin order

A plethora of correlated and exotic metallic states have been identified on the border of itinerant magnetism, where the long-range spin texture is melted by tuning the magnetic transition temperature (T$_C$) towards zero, referred to as the quantum phase transition (QPT). So far, the study of QPT in itinerant magnets has mainly focused on low-T$_C$ materials (i.e., typically T$_C$ ~ 10 K) where the modification of electronic band structure is subtle, and only makes a small contribution to the QPT. Here we report a distinct example of a magnetic QPT accompanied by a gigantic modification of the electronic structure in FeGe, i.e., a well-studied itinerant chiral magnet hosting near-room-temperature (T$_C$ = 278 K) helical/skyrmion spin texture. The pressure-driven modification of the band structure (e.g., reduction of exchange splitting) is evidenced by magneto-transport study, suggesting a Fermi-surface reconstruction around the magnetic QPT (P ~19 GPa), in stark contrast to the case of typical metallic ferromagnets. Further application of pressure leads to a metal-to-insulator transition above P > 30 GPa, as also corroborated by our density-functional theory (DFT) calculation. Of particular interest is the occurrence of anomalous magneto-transport in the inhomogeneous short-range chiral-spin ground state (P = 20-30 GPa) above the QPT, with longitudinal fluctuations of magnetization. The unexpected observation of spontaneous anomalous Hall effect in this exotic quantum regime suggests macroscopic time-reversal symmetry (TRS) breaking, even in the absence of long-range magnetic order. Our findings mark the large body of unexplored high-T$_C$ itinerant magnets with broken inversion-symmetry as promising candidates of novel ground state formation near QPT.

cond-mat.str-el↗

arXiv2018

Impact of electrodes on the extraction of shift current from a ferroelectric semiconductor SbSI

Noncentrosymmetric bulk crystals generate photocurrent without any bias voltage. One of the dominant mechanisms, shift current, comes from a quantum interference of electron wave functions being distinct from classical current caused by electrons' drift or diffusion. The dissipation-less nature of shift current, however, has not been fully verified presumably due to the premature understanding on the role of electrodes. Here we show that the photocurrent dramatically enhances by choosing electrodes with large work function for a $p$-type ferroelectric semiconductor SbSI. An optimized device shows a nearly constant zero-bias photocurrent despite significant variation in photocarrier mobility dependent on temperature, which could be a clear hallmark for the dissipation-less nature of shift current. Distinct from conventional photovoltaic devices, the shift current generator operates as a majority carrier device. The present study provides fundamental design principles for energy-harvesting and photo-detecting devices with novel architectures optimal for the shift current photovoltaic effect.

cond-mat.mtrl-sci↗

arXiv2018

Spectral dynamics of topological shift-current in ferroelectric semiconductor SbSI

Photoexcitation in solids brings about transitions of electrons/holes between different electronic bands. If the solid lacks an inversion symmetry, these electronic transitions support spontaneous photocurrent due to the topological character of the constituting electronic bands; the Berry connection. This photocurrent, termed shift current, is expected to emerge on the time-scale of primary photoexcitation process. We observed ultrafast time evolution of the shift current in a prototypical ferroelectric semiconductor by detecting emitted terahertz electromagnetic waves. By sweeping the excitation photon energy across the band gap, ultrafast electron dynamics as a source of terahertz emission abruptly changes its nature, reflecting a contribution of Berry connection upon interband optical transition. The shift excitation carries a net charge flow, and is followed by a swing-over of the electron cloud on the sub-picosecond time-scale of electron-phonon interaction. Understanding these substantive characters of the shift current will pave the way for its application to ultrafast sensors and solar cells.

cond-mat.mtrl-sci↗

arXiv2017

Short-range test of the universality of gravitational constant $G$ at the millimeter scale using a digital image sensor

The composition dependence of gravitational constant $G$ is measured at the millimeter scale to test the weak equivalence principle, which may be violated at short range through new Yukawa interactions such as the dilaton exchange force. A torsion balance on a turning table with two identical tungsten targets surrounded by two different attractor materials (copper and aluminum) is used to measure gravitational torque by means of digital measurements of a position sensor. Values of the ratios $\tilde{G}_{Al-W}/\tilde{G}_{Cu-W} -1$ and $\tilde{G}_{Cu-W}/G_{N} -1$ were $(0.9 \pm 1.1_{\mathrm{sta}} \pm 4.8_{\mathrm{sys}}) \times 10^{-2}$ and $ (0.2 \pm 0.9_{\mathrm{sta}} \pm 2.1_{\mathrm{sys}}) \times 10^{-2}$ , respectively; these were obtained at a center to center separation of 1.7 cm and surface to surface separation of 4.5 mm between target and attractor, which is consistent with the universality of $G$. A weak equivalence principle (WEP) violation parameter of $η_{Al-Cu}(r\sim 1\: \mathrm{cm})=(0.9 \pm 1.1_{\mathrm{sta}} \pm 4.9_{\mathrm{sys}}) \times 10^{-2} $ at the shortest range of around 1 cm was also obtained.

gr-qc↗

arXiv2017

Critical enhancement of thermopower in a chemically tuned polar semimetal MoTe$_{\bf 2}$

Ferroelectrics with spontaneous electric polarization play an essential role in today's device engineering, such as capacitors and memories. Their physical properties are further enriched by suppressing the long-range polar order, as is exemplified by quantum paraelectrics with giant piezoelectric and dielectric responses at low temperatures. Likewise in metals, a polar lattice distortion has been theoretically predicted to give rise to various unusual physical properties. So far, however, a "ferroelectric"-like transition in metals has seldom been controlled and hence its possible impacts on transport phenomena remain unexplored. Here we report the discovery of anomalous enhancement of thermopower near the critical region between the polar and nonpolar metallic phases in 1T'-Mo$_{1-x}$Nb$_{x}$Te$_2$ with a chemically tunable polar transition. It is unveiled from the first-principles calculations and magnetotransport measurements that charge transport with strongly energy-dependent scattering rate critically evolves towards the boundary to the nonpolar phase, resulting in large cryogenic thermopower. Such a significant influence of the structural instability on transport phenomena might arise from the fluctuating or heterogeneous polar metallic states, which would pave a novel route to improving thermoelectric efficiency.

cond-mat.mtrl-sci↗

arXiv2017

A new measurement of electron transverse polarization in polarized nuclear beta decay

The Mott polarimetry for T -Violation (MTV) experiment tests time-reversal symmetry in polarized nuclear beta decay by measuring an electron's transverse polarization as a form of angular asymmetry in Mott scattering using a thin metal foil. A Mott scattering analyzer system developed using a tracking detector to measure scattering angles offers better event selectivity than conventional counter experiments. In this paper, we describe a pilot experiment conducted at KEK-TRIAC using a prototype system with a polarized 8Li beam. The experiment confirmed the sound performance of our Mott analyzer system to measure T-violating triple correlation (R correlation), and therefore recommends its use in higher-precision experiments at the TRIUMF-ISAC.

nucl-ex↗

arXiv2016

Interface-driven topological Hall effect in SrRuO$_3$-SrIrO$_3$ bilayer

Electron transport coupled with magnetism has attracted attention over the years as exemplified in anomalous Hall effect due to a Berry phase in momentum space. Another type of unconventional Hall effect -- topological Hall effect, originating from the real-space Berry phase, has recently become of great importance in the context of magnetic skyrmions. We have observed topological Hall effect in bilayers consisting of ferromagnetic SrRuO$_3$ and paramagnetic SrIrO$_3$ over a wide region of both temperature and magnetic field. The topological term rapidly decreases with the thickness of SrRuO$_3$, ending up with the complete disappearance at 7 unit cells of SrRuO$_3$. Combined with model calculation, we concluded that the topological Hall effect is driven by interface Dzyaloshinskii-Moriya interaction, which is caused by both the broken inversion symmetry and the strong spin-orbit coupling of SrIrO$_3$. Such interaction is expected to realize the Néel-type magnetic skyrmion, of which size is estimated to be $\sim$10 nm from the magnitude of topological Hall resistivity. The results established that the high-quality oxide interface enables us to tune the chirality of the system; this can be a step towards the future topological electronics.

cond-mat.str-el↗

arXiv2016

Photo-creating supercooled spiral-spin states in a multiferroic manganite

We demonstrate that dynamics of the ab-spiral-spin order in a magnetoelectric multiferroic Eu0.55Y0.45MnO3 can be unambiguously probed through optical second harmonic signals, generated via the spin-induced ferroelectric polarization. In the case of relatively weak photoexcitation,the ferroelectric and the spiral-spin order remains interlocked, both relaxing through spin-lattice relaxation in the non-equilibrium state. When the additional optical pulse illuminating sample is intense enough to induced a local phase transition thermally, the system creates a metastable state of the bc-spiral-spin order (with the electric polarization P//c) via supercooling across the first-order phase transition between ab- and bc-spiral. The supercooled state of bc-spiral spin is formed in the thermodynamical ground state of ab-spiral (P//a), displaying a prolonged lifetime with strong dependence on the magnetic field along the a-axis. The observed photo-switching between the two distinct multiferroic states sheds light on novel photoinduced phenomena in spiral-spin multiferroics.

cond-mat.str-el↗

arXiv2016

Observation of topological Faraday and Kerr rotations in quantum anomalous Hall state by terahertz magneto-optics

Electrodynamic responses from three-dimensional (3D) topological insulators (TIs) are characterized by the universal magnetoelectric $E\cdot B$ term constituent of the Lagrangian formalism. The quantized magnetoelectric coupling, which is generally referred to as topological magnetoelectric (TME) effect, has been predicted to induce exotic phenomena including the universal low-energy magneto-optical effects. Here we report the experimental demonstration of the long-sought TME effect, which is exemplified by magneto-optical Faraday and Kerr rotations in the quantum anomalous Hall (QAH) states of magnetic TI surfaces by terahertz magneto-optics. The universal relation composed of the observed Faraday and Kerr rotation angles but not of any material parameters (e.g. dielectric constant and magnetic susceptibility) well exhibits the trajectory toward the fine structure constant $α$ $(= 2πe^2/hc \sim 1/137)$ in the quantized limit. Our result will pave a way for versatile TME effects with emergent topological functions.

cond-mat.mes-hall↗

arXiv2016

Enhanced photogalvanic current in topological insulators via Fermi energy tuning

We achieve the enhancement of circular photogalvanic effect arising from the photo-injection of spins in topological insulator thin films by tuning the Fermi level ($E_{\rm F}$). A series of (Bi$_{1-x}$Sb$_x$)$_2$Te$_3$ thin films were tailored so that the Fermi energy ranges above 0.34 eV to below 0.29 eV of the Dirac point, i.e., from the bulk conduction band bottom to the valence band top through the bulk in-gap surface-Dirac cone. The circular photogalvanic current, indicating a flow of spin-polarized surface-Dirac electrons, shows a pronounced peak when the $E_{\rm F}$ is set near the Dirac point and is also correlated with the carrier mobility. Our observation reveals that there are substantial scatterings between the surface-Dirac and bulkstate electrons in the generation process of spin-polarized photocurrent, which can be avoided by designing the electronic structure in topological insulators.

cond-mat.mtrl-sci↗

arXiv2015

Phase-change memory function of correlated electrons in organic conductors

Phase-change memory (PCM), a promising candidate for next-generation non-volatile memories, exploits quenched glassy and thermodynamically stable crystalline states as reversibly switchable state variables. We demonstrate PCM functions emerging from a charge-configuration degree of freedom in strongly correlated electron systems. Non-volatile reversible switching between a high-resistivity charge-crystalline (or charge-ordered) state and a low-resistivity quenched state, charge glass, is achieved experimentally via heat pulses supplied by optical or electrical means in organic conductors $θ$-(BEDT-TTF)$_2$$X$. Switching that is one order of magnitude faster is observed in another isostructural material that requires faster cooling to kinetically avoid charge crystallization, indicating that the material's critical cooling rate can be useful guidelines for pursuing a faster correlated-electron PCM function.

cond-mat.str-el↗

arXiv2009

Nonlinear Optical Response of SrTiO3/LaAlO3 Superlattices

The electronic symmetry of the SrTiO3/LaAlO3 interface was investigated by optical second harmonic generation, using superlattices with varying periodicity to study the evolution of the electronic reconstruction while avoiding substrate contributions. The superlattices show large perpendicular optical nonlinearity, which abruptly increases when the sublattice thickness goes above 3 unit cells, revealing substantial effects of the polar-nonpolar interface. The nonlinear 'active' area is primarily in SrTiO3, develops with increasing thickness, and extends up to 8 unit cells from the interface.

cond-mat.str-el↗

arXiv2004

Relative contributions of lattice distortion and orbital ordering to resonant x-ray scattering in manganites

We investigated the origin of the energy splitting observed in the resonant x-ray scattering (RXS) in manganites. Using thin film samples with controlled lattice parameters and orbital states at a fixed orbital filling, we estimated that the contribution of the interatomic Coulomb interaction relative to the Jahn-Teller mechanism is insignificant and at most 0.27. This indicates that RXS probes mainly Jahn-Teller distortion in manganites.

cond-mat.str-el↗

arXiv1997

Geometrically Induced Gauge Structure on Manifolds Embedded in a Higher Dimensional Space

We explain in a context different from that of Maraner the formalism for describing motion of a particle, under the influence of a confining potential, in a neighbourhood of an n-dimensional curved manifold M^n embedded in a p-dimensional Euclidean space R^p with p >= n+2. The effective Hamiltonian on M^n has a (generally non-Abelian) gauge structure determined by geometry of M^n. Such a gauge term is defined in terms of the vectors normal to M^n, and its connection is called the N-connection. In order to see the global effect of this type of connections, the case of M^1 embedded in R^3 is examined, where the relation of an integral of the gauge potential of the N-connection (i.e., the torsion) along a path in M^1 to the Berry's phase is given through Gauss mapping of the vector tangent to M^1. Through the same mapping in the case of M^1 embedded in R^p, where the normal and the tangent quantities are exchanged, the relation of the N-connection to the induced gauge potential on the (p-1)-dimensional sphere S^{p-1} (p >= 3) found by Ohnuki and Kitakado is concretely established. Further, this latter which has the monopole-like structure is also proved to be gauge-equivalent to the spin-connection of S^{p-1}. Finally, by extending formally the fundamental equations for M^n to infinite dimensional case, the present formalism is applied to the field theory that admits a soliton solution. The resultant expression is in some respects different from that of Gervais and Jevicki.

hep-th↗

arXiv1997

Equivalence between Schwinger and Dirac schemes of quantization

This paper introduces the modified version of Schwinger's quantization method, in which the information on constraints and the choice of gauge conditions are included implicitly in the choice of variations used in quantization scheme. A proof of equivalence between Schwinger- and Dirac-methods for constraint systems is given.

hep-th↗