arXiv subjects

N. P. Armitage

Publications and source records attributed to N. P. Armitage.

At least 127 records · Page 7Linked to original sources

arXiv2012

Improved measurement of polarization state in terahertz polarization spectroscopy

A calibration scheme is presented for improved polarization state measurement of terahertz pulses. In this scheme the polarization response of a two-contact terahertz photoconductive detector is accurately measured, and is used to correct for the impact of the non-idealities of the detector. Experimental results show excellent sub-degree angular accuracy and at least 60% error reduction with this scheme.

physics.optics↗

arXiv2011

Temporal correlations of superconductivity above the transition temperature in La$_{2-x}$Sr$_x$CuO$_4$ probed by terahertz spectroscopy

The nature of the underdoped pseudogap regime of the high-temperature superconductors has been a matter of long-term debate. On quite general grounds, one expects that due to their low superfluid densities and short correlation lengths, superconducting fluctuations will be significant for transport and thermodynamic properties in this part of the phase diagram. Although there is ample experimental evidence for such correlations, there has been disagreement about how high in temperature they may persist, their role in the phenomenology of the pseudogap, and their significance for understanding high-temperature superconductivity. In this work we use THz time-domain spectroscopy (TTDS) to probe the temporal fluctuations of superconductivity above the critical temperature (T$_c$) in La$_{2-x}$Sr$_x$CuO$_4$ thin films over a doping range that spans almost the entire superconducting dome (x = 0.09 to 0.25). Signatures of the fluctuations persist in the conductivity in a comparatively narrow temperature range, at most 16 K above Tc. Our measurements show that superconducting correlations do not make an appreciable contribution to the charge transport anomalies of the pseudogap in LSCO at temperatures well above T$_c$.

cond-mat.supr-con↗

arXiv2011

On the possibility of fast vortices in the cuprates: A vortex plasma model analysis of THz conductivity and diamagnetism in La$_{2-x}$Sr$_{x}$CuO$_4$

We present measurements of the fluctuation superconductivity in an underdoped thin film of La$_{1.905}$Sr$_{0.095}$CuO$_4$ using time-domain THz spectroscopy. We compare our results with measurements of diamagnetism in a similarly doped crystal of La$_{2-x}$Sr$_x$CuO$_4$. We show through a vortex-plasma model that if the fluctuation diamagnetism solely originates in vortices, then they must necessarily exhibit an anomalously large vortex diffusion constant, which is more than two orders of magnitude larger than the Bardeen-Stephen estimate. This points to either the extremely unusual properties of vortices in the under-doped d-wave cuprates or a contribution to the diamagnetic response that is not superconducting in origin.

cond-mat.supr-con↗

arXiv2011

THz response and colossal Kerr rotation from the surface states of the topological insulator Bi$_2$Se$_3$

Ordered states of matter are typically categorized by their broken symmetries. With the ordering of spins in a ferromagnet or the freezing of a liquid into a solid, the loss of symmetry distinguishes the ordered state from the disordered one. In contrast, topological states are distinguished by specific \textit{topological} properties that are encoded in their quantum mechanical wavefunctions. Frequently, a consequence of these properties is that there are robust "topologically protected" states on the sample's boundaries. The edge states of the quantum Hall effect (QHE) are the classic example. In the last few years, it was realized that another class of such topological matter may exist in 3D band insulators with large spin-orbit interaction. These so-called topological insulators are predicted to host robust surface states, which exhibit a number of interesting properties including spin helicity, immunity to back-scattering, and weak \textit{anti}--localization. There are predictions of a number of unusual phenomena associated with these surface states, including a proximity-effect-induced exotic superconducting state with Majorana fermions bound to a vortex and an `axion' electromagnetic response, and proposals for applications, such as their use in terahertz devices. In this Letter we report the observation of an unprecedentedly large rotation of the polarization plane of linearly polarized light reflected from thin films of the topological insulator Bi$_2$Se$_3$ in magnetic fields. This Kerr rotation can be as large as 65$^\circ$ and is due almost entirely to the surface states. Our results are evidence for the intrinsic response of the topologically protected surface states and provide a benchmark for the large magneto-electric effect predicted for these materials.

cond-mat.str-el↗

arXiv2010

Fluctuations, dissipation, and nonuniversal superfluid jumps in two-dimensional superconductors

We report a comprehensive study of the complex AC conductivity of thin effectively 2D amorphous superconducting InO_x films at zero applied field. Below a temperature scale T_c0 where the superconducting order parameter amplitude becomes well defined, there is a temperature where both the generalized superfluid stiffness acquires a frequency dependence and the DC mangetoresistance becomes linear in field. We associate this with a transition of the Kosterlitz-Thouless-Berezinskii (KTB) type. At our measurement frequencies the superfluid stiffness at T_KTB is found to be larger than the universal value. Although this may be understood with a vortex dielectric constant of epsilon_v ~ 1.9 within the usual KTB theory, this is a relatively large value and indicates that such a system may be out of the domain of applicability of the low-fugacity (low vortex density) KTB treatment. This opens up the possibility that at least some of the discrepancy from a non-universal magnitude is intrinsic. Our finite frequency measurements allow us access to a number of other phenomena concerning the charge dynamics in superconducting thin films, including an enhanced conductivity near the amplitude fluctuation temperature T_c0 and a finite dissipation at low temperature which appears to be a universal aspect of highly disordered superconducting films.

cond-mat.supr-con↗

arXiv2010

Survival of superconducting correlations across the 2D superconductor-insulator transition: A finite frequency study

The complex ac conductivity of thin highly disordered InOx films was studied as a function of magnetic field through the nominal two-dimensional superconductor-insulator transition. We have resolved a significant finite-frequency superfluid stiffness well into the insulating regime, giving direct evidence for quantum superconducting fluctuations around an insulating ground state and a state of matter with localized Cooper pairs. A phase diagram is established that includes the superconducting state, a transition to a "Bose" insulator, and an eventual crossover to a "Fermi" insulating state at high fields. We speculate on the consequences of these observations, their impact on our understanding of the insulating state, and its relevance as a prototype for other insulating states of matter that derive from superconductors.

cond-mat.supr-con↗

arXiv2010

Infrared Conductivity of Elemental Bismuth under Pressure: Evidence for an Avoided Lifshitz-Type Semimetal-Semiconductor Transition

The application of pressure to elemental bismuth reduces its conduction-valence band overlap, and results in a semimetal-semiconductor (SMSC) transition around 25 kbar. This transition is nominally of the topological "Lifshitz" Fermi surface variety, but there are open questions about the role of interactions at low charge densities. Using a novel pressure cell with optical access, we have performed an extensive study of bismuth's infrared conductivity under pressure. In contrast to the expected pure band behavior we find signatures of enhanced interaction effects, including strongly coupled charge-plasmon (plasmaron) features and a plasma frequency that remains finite up to the transition. These effect are inconsistent with a pure Lifshitz bandlike transition. We postulate that interactions play a central role in driving the transition.

cond-mat.str-el↗

arXiv2010

Ultrafast (but Many-Body) Relaxation in a Low-Density Electron Glass

We present a study of the relaxation dynamics of the photoexcited conductivity of the impurity states in the low-density electronic glass, phosphorous-doped silicon Si:P. Using optical pump-terahertz probe spectroscopy we find strongly temperature and fluence dependent glassy power-law relaxation occurring over sub-ns time scales. Such behavior is in contrast to the much longer time scales found in higher electron density glassy systems. We also find evidence for both multi-particle relaxation mechanisms and/or coupling to electronic collective modes and a low temperature quantum relaxational regime.

cond-mat.dis-nn↗

arXiv2010

Observation of a coherence peak and pair-breaking effects in THz conductivity of BaFe$_{2-2x}$Co$_{2x}$As$_2$

We report a study of high quality pnictide superconductor BaFe$_{1.84}$Co$_{0.16}$As$_2$ thin films using time-domain THz spectroscopy. Near T$_c$ we find evidence for a coherence peak and qualitative agreement with the weak-coupling Mattis-Bardeen form of the conductivity. At low temperature, we find that the real part of the THz conductivity is not fully suppressed and $σ_2$ is significantly smaller than the Matthis-Bardeen expectation. The temperature dependence of the penetration depth $λ$ follows a power law with an unusually high exponent of 3.1. We interpret these results as consistent with impurity scattering induced pair-breaking. Taken together our results are strong evidence for an extended s$\pm$ symmetry order parameter.

cond-mat.supr-con↗

arXiv2010

Progress and perspectives on the electron-doped cuprates

Although the vast majority of high-$T_c$ cuprate superconductors are hole-doped, a small family of electron-doped compounds exists. Under investigated until recently, there has been tremendous recent progress in their characterization. A consistent view is being reached on a number of formerly contentious issues, such as their order parameter symmetry, phase diagram, and normal state electronic structure. Many other aspects have been revealed exhibiting both their similarities and differences with the hole-doped compounds. This review summarizes the current experimental status of these materials, with a goal to providing a snapshot of our current understanding of electron-doped cuprates. When possible we put our results in the context of the hole-doped compounds. We attempt to synthesize this information into a consistent view on a number of topics important to both this material class as well as the overall cuprate phenomenology including the phase diagram, the superconducting order parameter symmetry, phase separation, pseudogap effects, the role of competing orders, the spin-density wave mean-field description of the normal state, and electron-phonon coupling.

cond-mat.supr-con↗

arXiv2008

Optical spectra of the heavy fermion uniaxial ferromagnet UGe$_2$

We report a detailed study of UGe$_{2}$ single crystals using infrared reflectivity and spectroscopic ellipsometry. The optical conductivity suggests the presence of a low frequency interband transition and a narrow free-carrier response with strong frequency dependence of the scattering rate and effective mass. We observe sharp changes in the low frequency mass and scattering rate below the upper ferromagnetic transition $T_C = 53 K$. The characteristic changes are exhibited most strongly at an energy scale of around 12 meV (100 cm$^{-1}$). They recover their unrenormalized value above $T_C$ and for $ω>$ 40 meV. In contrast no sign of an anomaly is seen at the lower transition temperature of unknown nature $T_x \sim$ 30 K, observed in transport and thermodynamic experiments. In the ferromagnetic state we find signatures of a strong coupling to the longitudinal magnetic excitations that have been proposed to mediate unconventional superconductivity in this compound.

cond-mat.str-el↗

arXiv2007

Electron-phonon interaction and charge carrier mass enhancement in SrTiO3

We report a comprehensive THz, infrared and optical study of Nb doped SrTiO3 as well as DC conductivity and Hall effect measurements. Our THz spectra at 7K show the presence of a very narrow (<2 meV) Drude peak, the spectral weight of which shows approximately a factor of three enhancement of the band mass for all carrier concentrations. The missing spectral weight is regained in a broad 'mid-infrared' band which originates from electron-phonon coupling. We find no evidence of a particularly large electron-phonon coupling that would result in small polaron formation. Analysis of the results yields an electron-phonon coupling parameter of an intermediate strength, $α\approx 4$.

cond-mat.str-el↗

arXiv2007

Direct observation of quantum superconducting fluctuations in an insulating groundstate

We review our recent measurements of the complex AC conductivity of thin InO_x films studied as a function of magnetic field through the nominal 2D superconductor-insulator transition. These measurements - the first of their type to probe nonzero frequency - reveals a significant finite frequency superfluid stiffness well into the insulating regime. Unlike conventional fluctuation superconductivity in which thermal fluctuations give a superconducting response in regions of parameter space that don't exhibit long range order, these fluctuations are temperature independent as T --> 0 and are exhibited in samples where the resistance is large (greater than 10^6 Ohms/Square) and strongly diverging. We interpret this as the direct observation of quantum superconducting fluctuations around an insulating ground state. This system serves as a prototype for other insulating states of matter that derive from superconductors.

cond-mat.supr-con↗

arXiv2007

Charge carrier interaction with a purely electronic collective mode: Plasmarons and the infrared response of elemental bismuth

We present a detailed optical study of single crystal bismuth using infrared reflectivity and ellipsometry. Colossal changes in the plasmon frequency are observed as a function of temperature due to charge transfer between hole and electron Fermi pockets. In the optical conductivity, an anomalous temperature dependent mid-infrared absorption feature is observed. An extended Drude model analysis reveals that it can be connected to a sharp upturn in the scattering rate, the frequency of which exactly tracks the temperature dependent plasmon frequency. We interpret this absorption and increased scattering as the first direct optical evidence for a charge carrier interaction with a collective mode of purely electronic origin; here electron-plasmon scattering. The observation of a \emph{plasmaron} as such is made possible only by the unique coincidence of various energy scales and exceptional properties of semi-metal bismuth.

cond-mat.str-el↗

arXiv2006

Electronic Structure of Electron-doped Sm1.86Ce0.14CuO4: Strong `Pseudo-Gap' Effects, Nodeless Gap and Signatures of Short Range Order

Angle resolved photoemission (ARPES) data from the electron doped cuprate superconductor Sm$_{1.86}$Ce$_{0.14}$CuO$_4$ shows a much stronger pseudo-gap or "hot-spot" effect than that observed in other optimally doped $n$-type cuprates. Importantly, these effects are strong enough to drive the zone-diagonal states below the chemical potential, implying that d-wave superconductivity in this compound would be of a novel "nodeless" gap variety. The gross features of the Fermi surface topology and low energy electronic structure are found to be well described by reconstruction of bands by a $\sqrt{2}\times\sqrt{2}$ order. Comparison of the ARPES and optical data from the $same$ sample shows that the pseudo-gap energy observed in optical data is consistent with the inter-band transition energy of the model, allowing us to have a unified picture of pseudo-gap effects. However, the high energy electronic structure is found to be inconsistent with such a scenario. We show that a number of these model inconsistencies can be resolved by considering a short range ordering or inhomogeneous state.

cond-mat.supr-con↗

arXiv2006

Anomalous high energy dispersion in photoemission spectra from insulating cuprates

Angle resolved photoelectron spectroscopic measurements have been performed on an insulating cuprate Ca_2CuO_2Cl_2. High resolution data taken along the Γto (pi,pi) cut show an additional dispersive feature that merges with the known dispersion of the lowest binding energy feature, which follows the usual strongly renormalized dispersion of ~0.35 eV. This higher energy part reveals a dispersion that is very close to the unrenormalized band predicted by band theory. A transfer of spectral weight from the low energy feature to the high energy feature is observed as the Γpoint is approached. By comparing with theoretical calculations the high energy feature observed here demonstrates that the incoherent portion of the spectral function has significant structure in momentum space due to the presence of various energy scales.

cond-mat.str-el↗

arXiv2004

Missing Quasiparticles and the Chemical Potential Puzzle in the Doping Evolution of the Cuprate Superconductors

The evolution of Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_{2}$ from Mott insulator to superconductor was studied using angle-resolved photoemission spectroscopy. By measuring both the excitations near the Fermi energy as well as non-bonding states, we tracked the doping dependence of the electronic structure and the chemical potential with unprecedented precision. Our work reveals failures in the conventional quasiparticle theory, including the broad lineshapes of the insulator and the apparently paradoxical shift of the chemical potential within the Mott gap. To resolve this, we develop a model where the quasiparticle is vanishingly small at half filling and grows upon doping, allowing us to unify properties such as the dispersion and Fermi wavevector with the behavior of the chemical potential.

cond-mat.supr-con↗

arXiv2003

Fully Gapped Single-Particle Excitations in the Lightly Doped Cuprates

The low-energy excitations of the lightly doped cuprates were studied by angle-resolved photoemission spectroscopy. A finite gap was measured over the entire Brillouin zone, including along the d_{x^2 - y^2} nodal line. This effect was observed to be generic to the normal states of numerous cuprates, including hole-doped La_{2-x}Sr_{x}CuO_{4} and Ca_{2-x}Na_{x}CuO_{2}Cl_{2} and electron-doped Nd_{2-x}Ce_{x}CuO_{4}. In all compounds, the gap appears to close with increasing carrier doping. We consider various scenarios to explain our results, including the possible effects of chemical disorder, electronic inhomogeneity, and a competing phase.

cond-mat.supr-con↗