arXiv subjects

N. P. Ong

Publications and source records attributed to N. P. Ong.

At least 19 recordsLinked to original sources

arXiv2026

Large Thermopower with Sign-Alternating Quantum Oscillations in Insulating Monolayer WTe2

The detection of Landau-level-like energy structures near the chemical potential of an insulator is essential to the search for a class of correlated electronic matter hosting charge-neutral fermions and Fermi surfaces, a long-proposed concept that remains elusive experimentally. Here we introduce and demonstrate that the magneto-thermoelectric response of a quantum insulator can reveal critical information not available via other approaches. We report the observation of large thermopower together with quantum oscillations (QOs) in the hole-doped insulating state of monolayer tungsten ditelluride (WTe2) in magnetic fields. The measured low temperature magneto-thermopower exceeds k_B/e by more than an order of magnitude, where k_B is the Boltzmann constant and e the elementary charge. This large thermopower is a characteristic of an insulating state, consistent with high resistivity. However, as the magnetic field is swept, QOs develop in the thermopower, which remarkably undergoes sign-changes that mimic the quantum characteristic of metals due to Landau quantization. The resistivity of the sample is orders of magnitude larger than the value expected from the QOs. The sign-change in the thermoelectric response directly implies the presence of a field-induced Landau-level-like structure at the chemical potential of the insulator. Neither the large thermopower nor the sign-changes can be induced by the metallic gate nearby. Our results demonstrate a new dilemma for investigating low energy excitations in correlated materials featuring mixed quantum characteristics of metals and insulators.

cond-mat.str-el↗

arXiv2026

Crystal structure and basic properties of dirhenate quantum materials

The anhydrous divalent 3d-metal dirhenate quantum materials, M(ReO$_4$)$_2$,were synthesized using solid-state methods for M = Mn through Zn. Previously unreported Mg(ReO4)2 is also described. Their layered crystal structures, which feature an in-plane triangular lattice of M$^{2+}$, were refined using single crystal X-ray diffraction, and their optical absorption and several other physical properties were characterized. Their magnetism and heat capacity reveal long-range magnetic order at low temperatures in many of the M(ReO$_4$)$_2$ phases. Notably, many of these ordered states are sensitive to applied magnetic fields and can be readily suppressed by relatively small fields, suggesting competing magnetic interactions in a low-dimensional framework, which appear worthy of further study.

cond-mat.mtrl-sci↗

arXiv2025

High-resolution Measurements of Thermal Conductivity Matrix and Search for Thermal Hall Effect in La$_2$CuO$_4$

We investigated the longitudinal thermal conductivity $κ_{xx}$ and thermal hall conductivity $κ_{xy}$ in La$_2$CuO$_4$ at temperatures $T$ between 2 and 20 K in magnetic fields $H$ up to 10 T. Within the temperature and field intervals studied, we do not resolve any thermal Hall signal with a conservative upper bound of $|κ_{xy}/T| <1\times10^{-4}$ ${\rm Wm^{-1}K^{-2}}$. The longitudinal thermal conductivity $κ_{xx}/T$ agrees well with previous studies, in both magnitude and $T$ dependence. In both channels, we performed measurements using the field-sweep protocol. To achieve high resolution, we carefully took into account relaxation effects after each step-increase in $H$. At low $T$, we find a linear decrease in $κ/T$ vs. $H$, as well as weak hysteresis near the meta-magnetic transition of the spin degrees.

cond-mat.str-el↗

arXiv2025

Unconventional Superconducting Phase Diagram of Monolayer WTe2

The existence of a quantum critical point (QCP) and fluctuations around it are believed to be important for understanding the phase diagram in unconventional superconductors such as cuprates, iron pnictides, and heavy fermion superconductors. However, the QCP is usually buried deep within the superconducting dome and is difficult to investigate. The connection between quantum critical fluctuations and superconductivity remains an outstanding problem in condensed matter. Here combining both electrical transport and Nernst experiments, we explicitly demonstrate the onset of superconductivity at an unconventional QCP in gate-tuned monolayer tungsten ditelluride (WTe2), with features incompatible with the conventional Bardeen-Cooper-Schrieffer (BCS) scenario. The results lead to a novel superconducting phase diagram that is distinguished from other known superconductors. Two distinct gate-tuned quantum phase transitions are observed at the ends of the superconducting dome. We find that quantum fluctuations around the QCP of the underdoped regime are essential for understanding how the monolayer superconductivity is established. The unconventional phase diagram we report here illustrates a previously unknown relation between superconductivity and QCP.

cond-mat.mes-hall↗

arXiv2024

Charge-Neutral Electronic Excitations in Quantum Insulators

Experiments on quantum materials have uncovered many interesting quantum phases ranging from superconductivity to a variety of topological quantum matter including the recently observed fractional quantum anomalous Hall insulators. The findings have come in parallel with the development of approaches to probe the rich excitations inherent in such systems. In contrast to observing electrically charged excitations, the detection of charge-neutral electronic excitations in condensed matter remains difficult, though they are essential to understanding a large class of strongly correlated phases. Low-energy neutral excitations are especially important in characterizing unconventional phases featuring electron fractionalization, such as quantum spin liquids, spin ices, and insulators with neutral Fermi surfaces. In this perspective, we discuss searches for neutral fermionic, bosonic, or anyonic excitations in unconventional insulators, highlighting theoretical and experimental progress in probing excitonic insulators, new quantum spin liquid candidates and emergent correlated insulators based on two-dimensional layered crystals and moiré materials. We outline the promises and challenges in probing and utilizing quantum insulators, and discuss exciting new opportunities for future advancements offered by ideas rooted in next-generation quantum materials, devices, and experimental schemes.

cond-mat.str-el↗

arXiv2024

Scaling behavior and giant field-enhancement of the thermal conductivity in the honeycomb antiferromagnet BaCo2(AsO4)2

The layered honeycomb material BaCo$_2$(AsO$_4$)$_2$ (BCAO) is of topical interest because its magnetic state is related to that of the Kitaev magnet $α$-RuCl$_3$. Using thermal transport to probe how magnetic excitations interact with phonons in the magnetically disordered regime, we have uncovered an unusually large enhancement of the thermal conductivity $κ_{xx}$ in an in-plane magnetic field ${\bf H}$. Just above the Néel temperature $T_{\rm N}$, a field of 13 T increases $κ_{xx}$ by a factor $\sim 211$, much larger than reported previously in any magnetic insulator. Interestingly, $κ_{xx}(H,T)$ exhibits a scaling behavior in the entire magnetically disordered region that surrounds the ordered zigzag state. The ratio $Δκ_{xx}(H,T)/κ_{xx}(13,T)$, measured throughout the disordered region, collapses to a one-parameter scaling function ${\rm exp}(-1/gx)$ (where $x = μ_{\rm B}B/k_{\rm B}T$ and $g$ is a constant).

cond-mat.str-el↗

arXiv2024

Anomalous Superconductivity in Twisted MoTe2 Nanojunctions

Introducing superconductivity in topological materials can lead to innovative electronic phases and device functionalities. Here, we present a new strategy for quantum engineering of superconducting junctions in moire materials through direct, on-chip, and fully encapsulated 2D crystal growth. We achieve robust and designable superconductivity in Pd-metalized twisted bilayer molybdenum ditelluride (MoTe2) and observe anomalous superconducting effects in high-quality junctions across ~ 20 moire cells. Surprisingly, the junction develops enhanced, instead of weakened, superconducting behaviors, exhibiting fluctuations to a higher critical magnetic field compared to its adjacent Pd7MoTe2 superconductor. Additionally, the critical current further exhibits a striking V-shaped minimum at zero magnetic field. These features are unexpected in conventional Josephson junctions and indeed absent in junctions of natural bilayer MoTe2 created using the same approach. We discuss implications of these observations, including the possible formation of mixed even- and odd-parity superconductivity at the moire junctions. Our results also demonstrate a pathway to engineer and investigate superconductivity in fractional Chern insulators.

cond-mat.supr-con↗

arXiv2023

The vortex-Nernst effect in a superconducting infinite-layer nickelate

We report measurements of the Nernst and Seebeck effects in Nd$_{1-x}$Sr$_x$NiO$_2$ thin films near the superconducting transition temperature, $T$ = 6.5 - 15 K. Our main result is the observation of a vortex-Nernst signal $S_{yx}(T,H)$ with a maximum at $μ_0H$ = 5 T and a tail that extends to $μ_0H$ $\approx$ 15 T, which we identify as the upper-critical field $H_{c2}$. At $T > T_{\rm c} =$ 6.1 K, $H_{c2}$ remains large (15 T), up to the highest temperature we can resolve from $S_{yx}$ (11 K). These results indicate the existence of a vortex-liquid state over a wide range of finite-resistance temperatures, as in the high-$T_{\rm c}$ cuprates.

cond-mat.supr-con↗

arXiv2023

Developing high-impedance superconducting resonators and on-chip filters for semiconductor quantum dot circuit quantum electrodynamics

Spin-photon coupling presents an enticing opportunity for the long-range coupling of spin qubits. The spin-photon coupling rate $g_{s}$ is proportional to the charge-photon coupling rate $g_{c}$. To move deeper into the strong coupling regime, $g_{c}$ can be enhanced by fabricating high-impedance cavities using high kinetic inductance films. Here we report dc transport and microwave response investigations of niobium nitride (NbN) films of different thicknesses. The kinetic inductance increases rapidly as the film thickness is reduced below 50 nm and for 15 nm NbN films we measure a sheet kinetic inductance $L_{k,S}$ = 41.2 pH/$\Box$. As an application of the high kinetic inductance films, we fabricate compact LC filters that are commonly used to reduce microwave leakage in circuit quantum electrodynamics (cQED) devices. These filters feature up to 60 dB of attenuation near typical cavity resonance frequencies $f_c$ = 8 GHz.

cond-mat.mes-hall↗

arXiv2023

Eavesdropping on competing condensates by the edge supercurrent in a Weyl superconductor

In a topological insulator the metallic surface states are easily distinguished from the insulating bulk states (FuKane07). By contrast, in a topological superconductor (FuKane08,Qi,FuBerg,Oppen), much less is known about the relationship between an edge supercurrent and the bulk pair condensate. Can we force their pairing symmetries to be incompatible? In the superconducting state of the Weyl semimetal MoTe$_2$, an edge supercurrent is observed as oscillations in the current-voltage (\emph{I-V}) curves induced by fluxoid quantization (Wang). We have found that the $s$-wave pairing potential of supercurrent injected from niobium contacts is incompatible with the intrinsic pair condensate in MoTe$_2$. The incompatibility leads to strong stochasticity in the switching current $I_c$ as well as other anomalous properties such as an unusual antihysteretic behavior of the ``wrong'' sign. Under supercurrent injection, the fluxoid-induced edge oscillations survive to much higher magnetic fields \emph{H}. Interestingly, the oscillations are either very noisy or noise-free depending on the pair potential that ends up dictating the edge pairing. Using the phase noise as a sensitive probe that eavesdrops on the competiting bulk states, we uncover an underlying blockade mechanism whereby the intrinsic condensate can pre-emptively block proximitization by the Nb pair potential depending on the history.

cond-mat.supr-con↗

arXiv2023

Unconventional Superconducting Quantum Criticality in Monolayer WTe2

The superconductor to insulator or metal transition in two dimensions (2D) provides a valuable platform for studying continuous quantum phase transitions (QPTs) and critical phenomena. Distinct theoretical models, including both fermionic and bosonic localization scenarios, have been developed, but many questions remain unsettled despite decades of research. Extending Nernst experiments down to millikelvin temperatures, we uncover anomalous quantum fluctuations and identify an unconventional superconducting quantum critical point (QCP) in a gate-tuned excitonic quantum spin Hall insulator (QSHI), the monolayer tungsten ditelluride (WTe2). The observed vortex Nernst effect reveals singular superconducting fluctuations in the resistive normal state induced by magnetic fields or temperature, even well above the transition. Near the doping-induced QCP, the Nernst signal driven by quantum fluctuations is exceptionally large in the millikelvin regime, with a coefficient of ~ 4,100 uV/KT at zero magnetic field, an indication of the proliferation of vortices. Surprisingly, the Nernst signal abruptly disappears when the doping falls below the critical value, in striking conflict with conventional expectations. This series of phenomena, which have no prior analogue, call for careful examinations of the mechanism of the QCP, including the possibility of a continuous QPT between two distinct ordered phases in the monolayer. Our experiments open a new avenue for studying unconventional QPTs and quantum critical matter.

cond-mat.mes-hall↗

arXiv2022

Anisotropic resistance with a 90-degree twist in a ferromagnetic Weyl semimetal, Co2MnGa

Co$_2$MnGa is a ferromagnetic semimetal with Weyl nodal lines identified by ARPES. We studied electrical transport in thin Co$_2$MnGa lamellae (10 $\times$ 10 $\times$ 0.4-5 microns) cut from single-crystals using a focused ion beam. These crystals exhibit an unexpected and highly unusual planar resistance anisotropy ($\sim$10 times) with principal axes that rotate by 90 degrees between the upper and lower faces. Using symmetry arguments and simulations, we find that the observed resistance anisotropy resembles that of an isotropic conductor with anisotropic surface states that are impeded from hybridization with bulk states. The origin of these states awaits further experiments that can correlate the surface bands with the observed 90$^\circ$-twist geometry.

cond-mat.mes-hall↗

arXiv2022

The planar thermal Hall conductivity in the Kitaev magnet α-RuCl3

We report detailed measurements of the Onsager-like planar thermal Hall conductivity $κ_{xy}$ in $α$-RuCl$_3$, a spin-liquid candidate of topical interest. With the thermal current ${\bf J}_{\rm Q}$ and magnetic field $\bf B\parallel a$ (zigzag axis), the observed $κ_{xy}/T$ varies strongly with temperature $T$ (1-10 K). The results are well-described by bosonic edge excitations which evolve to topological magnons at large $B$. Fits to $κ_{xy}/T$ yield a Chern number $\sim 1$ and a band energy $ω_1\sim$1 meV, in agreement with sharp modes seen in electron spin-resonance experiments. The bosonic character is incompatible with half-quantization of $κ_{xy}/T$.

cond-mat.str-el↗

arXiv2021

Phase tuning of multiple Andreev reflections of Dirac fermions and the Josephson supercurrent in Al-MoTe2-Al junctions

When a normal metal $N$ is sandwiched between two superconductors, the energy gaps in the latter act as walls that confine electrons in $N$ in a square-well potential. If the voltage $V$ across $N$ is finite, an electron injected into the well undergoes multiple Andreev reflections (MAR) until it gains enough energy to overcome the energy barrier. Because each reflection converts an electron to a hole (or vice versa), while creating (or destroying) a Cooper pair, the MAR process shuttles a stream of pairs across the junction. An interesting question is, given a finite $V$, what percentage of the shuttled pairs end up as a Josephson supercurrent? This fraction does not seem to have been measured. Here we show that, in high-transparency junctions based on the type II Dirac semimetal MoTe$_2$, the MAR leads to a stair-case profile in the current-voltage ($I$-$V$) response, corresponding to pairs shuttled incoherently by the $n^{th}$-order process. By varying the phase $φ$ across the junction, we demonstrate that a Josephson supercurrent ${\bf J}_{\rm s}\sim \sinφ$ co-exists with the MAR steps, even at large $V$. The observed linear increase in the amplitude of ${\bf J}_{\rm s}$ with $n$ (for small $n$) implies that ${\bf J}_{\rm s}$ originates from the population of pairs that are coherently shuttled. We infer that the MAR steps and the supercurrent are complementary aspects of the Andreev process. The experiment yields the percentage of shuttled pairs that form the supercurrent. At large $V$, the coherent fraction is initially linear in $n$. However, as $V\to 0$ ($n\gg 1$), almost all the pairs end up as the observed Josephson supercurrent.

cond-mat.supr-con↗

arXiv2021

Singular angular magnetoresistance and sharp resonant features in a high-mobility metal with open orbits, ReO3

We report high-resolution angular magnetoresistance (AMR) experiments performed on crystals of ReO$_3$ with high mobility (90,000 cm$^2$/Vs at 2 K) and extremely low residual resistivity (5-8 n$Ω$cm). The Fermi surface, comprised of intersecting cylinders, supports open orbits. The resistivity $ρ_{xx}$ in a magnetic field $B$ = 9 T displays a singular pattern of behavior. With $\bf E\parallel \hat{x}$ and $\bf B$ initially $\parallel\bf\hat{z}$, tilting $\bf B$ in the longitudinal $k_z$-$k_x$ plane leads to a steep decrease in $ρ_{xx}$ by a factor of 40. However, if $\bf B$ is tilted in the transverse $k_y$-$k_z$ plane, $ρ_{xx}$ increases steeply by a factor of 8. Using the Shockley tube integral approach, we show that, in ReO$_3$, the singular behavior results from the rapid conversion of closed to open orbits, resulting in opposite signs for AMR in orthogonal planes. The floor values of $ρ_{xx}$ in both AMR scans are identified with specific sets of open and closed orbits. Also, the "completion angle" $γ_c$ detected in the AMR is shown to be an intrinsic geometric feature that provides a new way to measure the Fermi radius $k_F$. However, additional sharp resonant features which appear at very small tilt angles in the longitudinal AMR scans are not explained by the tube integral approach.

cond-mat.mtrl-sci↗

arXiv2021

Quantum matter in ultrahigh magnetic fields

In writing this report we had two goals in mind. The first is to provide a survey of a subset of discoveries from recent experiments performed on quantum matter in high magnetic fields, and to anticipate the scientific opportunities to be realized in even higher fields. Hopefully, the survey will convey a sense of the excitement and pace of high-magnetic-field research in the quantum-matter community to a broader audience (undergraduates, especially). The second goal is to discuss the comparative merits of two options: a pulsed-field facility for attaining a magnetic field of 150 Tesla (of duration 1-10 msec) or a DC field facility that attains 60 Tesla. A workshop involving leading scientists involved with quantum phenomena in high magnetic fields was held at NSF, Alexandria Sep. 21,22 (2017) to address these issues.

cond-mat.str-el↗

arXiv2021

Oscillations of the thermal conductivity observed in the spin-liquid state of $α$-RuCl$_3$

In the class of materials called spin liquids, a magnetically ordered state cannot be attained even at milliKelvin temperatures because of conflicting constraints on each spin (for e.g. from geometric or exchange frustration). The resulting quantum spin-liquid (QSL) state is currently of intense interest because it exhibits novel excitations as well as wave-function entanglement. The layered insulator $α$-RuCl$_3$ orders as a zigzag antiferromagnet below $\sim$7 K in zero magnetic field. The zigzag order is destroyed when a magnetic field $\bf H$ is applied parallel to the zigzag axis a. Within the field interval (7.3, 11) Tesla, there is growing evidence that a QSL state exists. Here we report the observation of oscillations in its thermal conductivity below 4 K. The oscillation amplitude is very large within the interval (7.3, 11) T and strongly suppressed on either side. Paradoxically, the oscillations are periodic in 1/\emph{H}, analogous to quantum oscillations in metals, even though $α$-RuCl$_3$ is an excellent insulator with a gap of 1.9 eV. By tilting $\bf H$ out of the plane, we find that the oscillation period is determined by the in-plane component $H_a$. As the temperature is raised above 0.5 K, the oscillation amplitude decreases exponentially. The decrease anticorrelates with the emergence above $\sim$2 K of an anomalous planar thermal Hall conductivity measured with $\bf H\parallel a$. To exclude extrinsic artifacts, we carried out several tests. The implications of the oscillations are discussed.

cond-mat.str-el↗

arXiv2020

Review of experiments on the chiral anomaly in Dirac-Weyl semimetals

We provide a review of recent experimental results on the chiral anomaly in Dirac/Weyl semimetals. After a brief introduction, we trace the steps leading to the prediction of materials that feature protected 3D bulk Dirac nodes. The chiral anomaly is presented in terms of charge pumping between the chiral Landau levels of Weyl fermions in parallel electric and magnetic fields. The related chiral magnetic effect and chiral zero sound are described. Current jetting effects, which present major complications in experiments on the longitudinal magnetoresistance, are carefully analyzed. We describe a recent test that is capable of distinguishing these semiclassical artifacts from intrinsic quantum effects. Turning to experiments, we review critically the longitudinal magnetoresistance experiments in the Dirac/Weyl semimetals Na3Bi, GdPtBi, ZrTe5 and TaAs. Alternate approaches to the chiral anomaly, including experiments on non-local transport, thermopower, thermal conductivity and optical pump-probe response are reviewed. In the Supplement, we provide a brief discussion of the chiral anomaly in the broader context of high energy physics and relativistic quantum field theory, as well the anomaly's starring role at the nexus of quantum physics and differential geometry.

cond-mat.str-el↗