Charge radii of Cl isotopes from x-ray spectroscopy of muonic atoms
Nuclear charge radii are vital for nuclear and atomic physics, the determination of fundamental constants, and searches for new physics. Muonic atoms, where a single negative muon orbits a nucleus, are sensitive tools for determining nuclear radii due to the large wavefunction overlap of the muon and nucleus. Here we report on a new measurement of the $2, 3, 4p\to1s$ x-ray energies in muonic $^{35,37}$Cl with uncertainties reaching 18 ppm. By employing a large-scale germanium detector array, it was possible to extract these energies from a high statistics dataset using highly enriched samples of only a few tens of milligrams. Combining these results with state-of-the-art atomic and nuclear theory input, the charge radii of the stable chlorine isotopes were determined to be $R(^{35}\text{Cl}) = 3.3333(23)~fm$ and $R(^{37}\text{Cl}) = 3.3444(23)~fm$. This is an order of magnitude more precise and significantly different from previously tabulated values. Our new values solve a discrepancy observed for the charge radius difference in mirror nuclei, agreeing with the overall global trend. The charge radius difference $δ\langle r^2 \rangle (^{37}\text{Cl} - {^{35}\text{Cl}}) = -0.0776(64)~fm^2$ we extract is 25 times more precise than the previous values. This precision is crucial for establishing reference values for future laser spectroscopy measurements of radioactive isotopes.