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N. Sinclair

Publications and source records attributed to N. Sinclair.

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Diamond Mirrors for High-Power Lasers

High-power lasers have numerous scientific and industrial applications. Some key areas include laser cutting and welding in manufacturing, directed energy in fusion reactors or defense applications, laser surgery in medicine, and advanced photolithography in the semiconductor industry. These applications require optical components, in particular mirrors, that withstand high optical powers for directing light from the laser to the target. Ordinarily, mirrors are comprised of multilayer coatings of different refractive index and thickness. At high powers, imperfections in these layers lead to absorption of light, resulting in thermal stress and permanent damage to the mirror. Here we design, simulate, fabricate, and demonstrate monolithic and highly reflective dielectric mirrors which operate under high laser powers without damage. The mirrors are realized by etching nanostructures into the surface of single-crystal diamond, a material with exceptional optical and thermal properties. We measure reflectivities of greater than 98% and demonstrate damage-free operation using 10 kW of continuous-wave laser light at 1070 nm, with intensities up to 4.6 MW/cm2. In contrast, at these laser powers, we observe damage to a standard dielectric mirror based on optical coatings. Our results initiate a new category of broadband optics that operate in extreme conditions.

physics.optics

Quantum repeaters with individual rare-earth ions at telecommunication wavelengths

We present a quantum repeater scheme that is based on individual erbium and europium ions. Erbium ions are attractive because they emit photons at telecommunication wavelength, while europium ions offer exceptional spin coherence for long-term storage. Entanglement between distant erbium ions is created by photon detection. The photon emission rate of each erbium ion is enhanced by a microcavity with high Purcell factor, as has recently been demonstrated. Entanglement is then transferred to nearby europium ions for storage. Gate operations between nearby ions are performed using dynamically controlled electric-dipole coupling. These gate operations allow entanglement swapping to be employed in order to extend the distance over which entanglement is distributed. The deterministic character of the gate operations allows improved entanglement distribution rates in comparison to atomic ensemble-based protocols. We also propose an approach that utilizes multiplexing in order to enhance the entanglement distribution rate.

quant-ph

Entanglement between more than two hundred macroscopic atomic ensembles in a solid

We create a multi-partite entangled state by storing a single photon in a crystal that contains many large atomic ensembles with distinct resonance frequencies. The photon is re-emitted at a well-defined time due to an interference effect analogous to multi-slit diffraction. We derive a lower bound for the number of entangled ensembles based on the contrast of the interference and the single-photon character of the input, and we experimentally demonstrate entanglement between over two hundred ensembles, each containing a billion atoms. In addition, we illustrate the fact that each individual ensemble contains further entanglement. Our results are the first demonstration of entanglement between many macroscopic systems in a solid and open the door to creating even more complex entangled states.

quant-ph

Spectroscopic investigations of a Ti:Tm:LiNbO3 waveguide for photon-echo quantum memory

We report the fabrication and characterization of a Ti$^{4+}$:Tm$^{3+}$:LiNbO$_3$ optical waveguide in view of photon-echo quantum memory applications. In particular, we investigated room- and cryogenic-temperature properties via absorption, spectral hole burning, photon echo, and Stark spectroscopy. We found radiative lifetimes of 82 $\mu$s and 2.4 ms for the $^3$H$_4$ and $^3$F$_4$ levels, respectively, and a 44% branching ratio from the $^3$H$_{4}$ to the $^3$F$_4$ level. We also measured an optical coherence time of 1.6 $\mu$s for the $^3$H$_6\leftrightarrow{}^3$H$_4$, 795 nm wavelength transition, and investigated the limitation of spectral diffusion to spectral hole burning. Upon application of magnetic fields of a few hundred Gauss, we observed persistent spectral holes with lifetimes up to seconds. Furthermore, we measured a linear Stark shift of 25 kHz$\cdot$cm/V. Our results are promising for integrated, electro-optical, waveguide quantum memory for photons.

quant-ph

Tripartite entanglement versus tripartite nonlocality in 3-qubit GHZ-class states

We analyze the relationship between tripartite entanglement and genuine tripartite nonlocality for 3-qubit pure states in the GHZ class. We consider a family of states known as the generalized GHZ states and derive an analytical expression relating the 3-tangle, which quantifies tripartite entanglement, to the Svetlichny inequality, which is a Bell-type inequality that is violated only when all three qubits are nonlocally correlated. We show that states with 3-tangle less than 1/2 do not violate the Svetlichny inequality. On the other hand, a set of states known as the maximal slice states do violate the Svetlichny inequality, and exactly analogous to the two-qubit case, the amount of violation is directly related to the degree of tripartite entanglement. We discuss further interesting properties of the generalized GHZ and maximal slice states.

quant-ph