arXiv subjects

N. T. Brewer

Publications and source records attributed to N. T. Brewer.

11 recordsLinked to original sources

arXiv2025

Impact of newly measured $β$\nobreakdash-delayed neutron emitters around \myisoSimp{78}{Ni} on light element nucleosynthesis in the neutrino-wind following a neutron star merger

Neutron emission probabilities and half-lives of 37 beta-delayed neutron emitters from 75Ni to 92Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and 6 half-lives measured for the first time, which supersede theoretical estimates. These nuclei lie in the path of the weak r-process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars, synthesizing elements in the A~80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and has been identified in the AT2017gfo event, associated with the gravitational wave detection GW170817. Abundance calculations based on over 17000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50-70 percent in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal-poor stars and is therefore significant in the comparison with other possible astrophysical processes contributing to light-element production. These results underline the importance of including experimental decay data for very neutron-rich beta-delayed neutron emitters into r-process models.

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arXiv2024

YSO implantation detector for beta-delayed neutron spectroscopy

A segmented-scintillator-based implantation detector was developed to study the energy distribution of beta-delayed neutrons emitted from exotic isotopes. The detector comprises a 34 $\times$ 34 YSO scintillator coupled to an 8 $\times$ 8 Position-Sensitive Photo-Multiplier Tube (PSPMT) via a tapered light guide. The detector was used at RIBF, RIKEN, for time-of-flight-based neutron spectroscopy measurement in the $^{78}$Ni region. The detector provides the position and timing resolution necessary for ion-beta correlations and ToF measurements. The detector provides a high $\sim$ 80 $\%$ beta-detection efficiency and a sub-nanosecond timing resolution. This contribution discusses the details of the design, operation, implementation, and analysis developed to obtain neutron time-of-flight spectrum and the analysis methods in the context of neutron-rich nuclei in the $^{78}$Ni region.

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arXiv2023

Rare $^{40}$K decay with implications for fundamental physics and geochronology

Potassium-40 is a widespread, naturally occurring isotope whose radioactivity impacts subatomic rare-event searches, nuclear structure theory, and estimated geological ages. A predicted electron-capture decay directly to the ground state of argon-40 has never been observed. The KDK (potassium decay) collaboration reports strong evidence of this rare decay mode. A blinded analysis reveals a non-zero ratio of intensities of ground-state electron-captures ($I_{\text{EC}^0}$) over excited-state ones ($I_\text{EC*}$) of $ I_{\text{EC}^0} / I_\text{EC*} = 0.0095 \stackrel{\text{stat}}{\pm} 0.0022 \stackrel{\text{sys}}{\pm} 0.0010 $ (68% C.L.), with the null hypothesis rejected at 4$σ$. In terms of branching ratio, this signal yields $I_{\text{EC}^0} = 0.098\% \stackrel{\text{stat}}{\pm} 0.023\% \stackrel{\text{sys}}{\pm} 0.010\% $, roughly half of the commonly used prediction, with consequences for various fields [L. Hariasz et al., companion paper, DOI: 10.1103/PhysRevC.108.014327].

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arXiv2023

Precision measurement of $^{65}$Zn electron-capture decays with the KDK coincidence setup

$^{65}$Zn is a common calibration source, moreover used as a radioactive tracer in medical and biological studies. In many cases, $γ$-spectroscopy is a preferred method of $^{65}$Zn standardization, which relies directly on the branching ratio of $J π(^{65}\text{Zn} ) = 5/2^- \rightarrow J π(^{65}\text{Cu}) = 5/2^- $ via electron capture (EC*). We measure the relative intensity of this branch to that proceeding directly to the ground state (EC$^0$) using a novel coincidence technique, finding $I_{\text{EC}^0}/I_{\text{EC*}} = 0.9684 \pm 0.0018$. Re-evaluating the decay scheme of $^{65}$Zn by adopting the commonly evaluated branching ratio of $I_{β^+}= 1.4271(7)\%$ we obtain $I_{\text{EC*}} = (50.08 \pm 0.06)\%$, and $I_\text{EC^0} = (48.50 \pm 0.06) \%$. The associated 1115 keV gamma intensity agrees with the previously reported NNDC value, and is now accessible with a factor of ~2 increase in precision. Our re-evaluation removes reliance on the deduction of this gamma intensity from numerous measurements, some of which disagree and depend directly on total activity determination. The KDK experimental technique provides a new avenue for verification or updates to the decay scheme of $^{65}$Zn, and is applicable to other isotopes.

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arXiv2023

Evidence for ground-state electron capture of $^{40}$K

Potassium-40 is a widespread isotope whose radioactivity impacts estimated geological ages spanning billions of years, nuclear structure theory, and subatomic rare-event searches - including those for dark matter and neutrinoless double-beta decay. The decays of this long-lived isotope must be precisely known for its use as a geochronometer, and to account for its presence in low-background experiments. There are several known decay modes for $^{40}$K, but a predicted electron-capture decay directly to the ground state of argon-40 has never been observed, while theoretical predictions span an order of magnitude. The KDK Collaboration reports on the first observation of this rare decay, obtained using a novel combination of a low-threshold X-ray detector surrounded by a tonne-scale, high-efficiency $γ$-ray tagger at Oak Ridge National Laboratory. A blinded analysis reveals a distinctly nonzero ratio of intensities of ground-state electron-captures ($I_{\text{EC}^0}$) over excited-state ones ($I_{\text{EC}^*}$) of $I_{\text{EC}^0} / I_{\text{EC}^*}=0.0095\stackrel{\text{stat}}{\pm}0.0022\stackrel{\text{sys}}{\pm}0.0010$ (68% CL), with the null hypothesis rejected at 4$σ$ [Stukel et al., DOI:10.1103/PhysRevLett.131.052503]. This unambiguous signal yields a branching ratio of $I_{\text{EC}^0}=0.098\%\stackrel{\text{stat}}{\pm}0.023\%\stackrel{\text{sys}}{\pm}0.010$, roughly half of the commonly used prediction. This first observation of a third-forbidden unique electron capture improves understanding of low-energy backgrounds in dark-matter searches and has implications for nuclear-structure calculations. A shell-model based theoretical estimate for the $0νββ$ decay half-life of calcium-48 is increased by a factor of $7^{+3}_{-2}$. Our nonzero measurement shifts geochronological ages by up to a percent; implications are illustrated for Earth and solar system chronologies.

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arXiv2021

A novel experimental system for the KDK measurement of the $^{40}$K decay scheme relevant for rare event searches

Potassium-40 ($^{40}$K) is a long-lived, naturally occurring radioactive isotope. The decay products are prominent backgrounds for many rare event searches, including those involving NaI-based scintillators. $^{40}$K also plays a role in geochronological dating techniques. The branching ratio of the electron capture directly to the ground state of argon-40 has never been measured, which can cause difficulty in interpreting certain results or can lead to lack of precision depending on the field and analysis technique. The KDK (Potassium (K) Decay (DK)) collaboration is measuring this decay. A composite method has a silicon drift detector with an enriched, thermally deposited $^{40}$K source inside the Modular Total Absorption Spectrometer. This setup has been characterized in terms of energy calibration, gamma tagging efficiency, live time and false negatives and positives. A complementary, homogeneous, method is also discussed; it employs a KSr$_2$I$_5$:Eu scintillator as source and detector.

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arXiv2021

Pseudo spin doublet bands and Gallagher Moszkowski doublet bands in $^{100}$Y

New transitions in neutron rich $^{100}$Y have been identified in a $^9$Be+$^{238}$U experiment with mass- and Z- gates to provide full fragment identification. These transitions and high spin levels of $^{100}$Y have been investigated by analyzing the high statistics $γ$-$γ$-$γ$ and $γ$-$γ$-$γ$-$γ$ coincidence data from the spontaneous fission of $^{252}$Cf at the Gammasphere detector array. Two new bands, 14 new levels and 23 new transitions have been identified. The $K^π=4^+$ new band decaying to an 1s isomeric state is assigned to be the high-$K$ Gallagher-Moszkowski (GM) partner of the known $K^π=1^+$ band, with the $π5/2[522] \otimes ν3/2[411]$ configuration. This 4$^+$ band is also proposed to be the pseudo spin partner of the new $K^π=5^+$ band with a 5$^{+}$ $π5/2[422] \otimes ν5/2[413]$ configuration, to form a $π5/2[422] \otimes ν[312$ $5/2,3/2]$ neutron pseudospin doublet. Constrained triaxial covariant density functional theory and quantal particle rotor model calculations have been applied to interpret the band structure and available electromagnetic transition probabilities and are found in good agreement with experimental values.

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arXiv2019

Segmented YSO scintillation detectors as a new ${\rm β}$-implant detection tool for decay spectroscopy in fragmentation facilities

A newly developed segmented YSO scintillator detector was implemented for the first time at the RI-beam Factory at RIKEN Nishina Center as an implantation-decay counter. The results from the experiment demonstrate that the detector is a viable alternative to conventional silicon-strip detectors with its good timing resolution and high detection efficiency for ${\rm β}$ particles. A Position-Sensitive Photo-Multiplier Tube (PSPMT) is coupled with a $48\times48$ segmented YSO crystal. To demonstrate its capabilities, a known short-lived isomer in $^{76}$Ni and the ${\rm β}$ decay of $^{74}$Co were measured by implanting those ions into the YSO detector. The half-lives and ${\rm γ}$-rays observed in this work are consistent with the known values. The ${\rm β}$-ray detection efficiency is more than 80~\% for the decay of $^{74}$Co.

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arXiv2018

Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

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arXiv2018

The ORNL Analysis Technique for Extracting $β$-Delayed Multi-Neutron Branching Ratios with BRIKEN

Many choices are available in order to evaluate large radioactive decay networks. %multi-particle decay data. There are many parameters that influence the calculated $β$-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on $β$-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining $β$-delayed multi-neutron branching ratios in $β$-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and $β$ trigger. The technique allows one to extract $β$-delayed multi-neutron decay branching ratios measured with the hybrid \textsuperscript{3}He BRIKEN neutron counter. As an example, two analyses of the $β$-neutron emitter \textsuperscript{77}Cu based on different {\it a priori} assumptions are presented along with comparisons to literature values.

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arXiv2015

Identification of new transitions and mass assignments of levels in $^{143-153}$Pr

The previously reported levels assigned to 151,152,153Pr have recently been called into question regarding their mass assignment. The above questioned level assignments are clarified by measuring g-transitions tagged with A and Z in an in-beam experiment in addition to the measurements from 252Cf spontaneous fission (SF) and establish new spectroscopic information from $N=84$ to $N=94$ in the Pr isotopic chain. The isotopic chain 143-153Pr has been studied from the spontaneous fission of 252Cf by using Gammasphere and also from the measurement of the prompt g-rays in coincidence with isotopically-identified fission fragments using VAMOS++ and EXOGAM at GANIL. The latter were produced using 238U beams on a 9Be target at energies around the Coulomb barrier. The g-g-g-g data from 252Cf (SF) and those from the GANIL in-beam A- and Z-gated spectra were combined to unambiguously assign the various transitions and levels in 151,152,153Pr and other isotopes. New transitions and bands in 145,147,148,149,150Pr were identified by using g-g-g and g-g-g-g coincidences and A and Z gated g-g spectra. The transitions and levels previously assigned to 151,153Pr have been confirmed by the (A,Z) gated spectra. The transitions previously assigned to 152Pr are now assigned to 151Pr on the basis of the (A,Z) gated spectra. Two new bands with 20 new transitions in 152Pr and one new band with 7 new transitions in 153Pr are identified from the g-g-g-g coincidence spectra and the (A,Z) gated spectrum. In addition, new g-rays are also reported in 143-146Pr. New levels of 145,147-153Pr have been established, reliable mass assignments of the levels in 151,152,153Pr have been reported and new transitions have been identified in 143-146Pr showing the new avenues that are opened by combining the two experimental approaches.

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