arXiv subjects

N. Trivedi

Publications and source records attributed to N. Trivedi.

At least 19 recordsLinked to original sources

arXiv2023

Temperature dependence and limiting mechanisms of the upper critical field of FeSe thin films

We use magnetoresistance measurements at high magnetic field (B \leq 65 T) and low temperature (T \geq 500 mK) to gain fresh insights into the behavior of the upper critical field, Hc2, in superconducting ultrathin FeSe films of varying degrees of disorder, grown by molecular beam epitaxy on SrTiO3. Measurements of Hc2 across samples with a widely varying superconducting critical temperature (1.2 K \leq Tc \leq 21 K) generically show similar qualitative temperature dependence. We analyze the temperature dependence of Hc2 in the context of Werthamer-Helfand-Hohenberg (WHH) theory. The analysis yields parameters that indicate a strong Pauli paramagnetic pair-breaking mechanism which is also reflected by pseudo-isotropic superconductivity in the limit of zero temperature. In the lower Tc samples, we observe a spin-orbit scattering driven enhancement of Hc2 above the strongly-coupled Pauli paramagnetic limit. We also observe clear deviations from WHH theory at low temperature, regardless of Tc. We attribute this to the multi-band superconductivity of FeSe and possibly to the emergence of a low temperature, high field superconducting phase.

cond-mat.supr-con↗

arXiv2022

Ring-Exchange Interaction Effects on Magnons in Dirac Magnet CoTiO$_3$

The magnetic interactions that determine magnetic order and magnon energies typically involve only two spins. While rare, multi-spin interactions can also appear in quantum magnets and be the driving force in the ground state selection and in the nature of its excitations. By performing time-domain terahertz and magneto-Raman spectroscopy measurements combined with theoretical modeling, we determine the origin of the magnon excitation gap in Dirac antiferromagnet CoTiO$_3$. By adding a ring-exchange interaction in a hexagonal plaquette of the honeycomb lattice to both an XXZ spin model and to a low energy spin-orbital flavor wave model, a gap is generated in the magnon spectrum at the Brillouin zone center. With this addition, the flavor wave model reproduces a large swath of experimental results including terahertz, Raman, inelastic neutron scattering, and magnetization experiments.

cond-mat.str-el↗

arXiv2018

A machine learning approach to the Berezinskii-Kosterlitz-Thouless transition in classical and quantum models

The Berezinskii-Kosterlitz-Thouless transition is a very specific phase transition where all thermodynamic quantities are smooth. Therefore, it is difficult to determine the critical temperature in a precise way. In this paper we demonstrate how neural networks can be used to perform this task. In particular, we study how the accuracy of the transition identification depends on the way the neural networks are trained. We apply our approach to three different systems: (i) the classical XY model, (ii) the phase-fermion model, where classical and quantum degrees of freedom are coupled and (iii) the quantum XY model.

cond-mat.stat-mech↗

arXiv2018

Spectroscopic fingerprints of many-body renormalizations in$1T$-TiSe$_2$

We have employed high resolution angle resolved photoemission spectroscopy (ARPES) measurements to investigate many-body renormalizations of the single-particle excitations in $1T$-TiSe$_2$. The energy distribution curves of the ARPES data reveal intrinsic peak-dip-hump feature, while the electronic dispersion derived from the momentum distribution curves of the data highlights, for the first time, multiple kink structures. These are canonical signatures of a coupling between the electronic degrees of freedom and some Bosonic mode in the system. We demonstrate this using a model calculation of the single-particle spectral function at the presence of an electron-Boson coupling. From the self-energy analysis of our ARPES data, we discern some of the critical energy scales of the involved Bosonic mode, which are $\sim$15 and 26 meV. Based on a comparison between these energies and the characteristic energy scales of our Raman scattering data, we identify these Bosonic modes as Raman active breathing (${\text{A}}_\text{1g}$) and shear (${\text{E}}_\text{g}$) modes, respectively. Direct observation of the band-renormalization due to electron-phonon coupling increases the possibility that electron-phonon interactions are central to the collective quantum states such as charge density wave (CDW) and superconductivity in the compounds based on $1T$-TiSe$_2$.

cond-mat.str-el↗

arXiv2017

Particle-hole character of the Higgs and Goldstone modes in strongly-interacting lattice bosons

We study the low-energy excitations of the Bose-Hubbard model in the strongly-interacting superfluid phase using a Gutzwiller approach and extract the single-particle and single-hole excitation amplitudes for each mode. We report emergent mode-dependent particle-hole symmetry on specific arc-shaped lines in the phase diagram connecting the well-known Lorentz-invariant limits of the Bose-Hubbard model. By tracking the in-phase particle-hole symmetric oscillations of the order parameter, we provide an answer to the long-standing question about the fate of the pure amplitude Higgs mode away from the integer-density critical point. Furthermore, we point out that out-of-phase oscillations are responsible for a full suppression of the condensate density oscillations of the gapless Goldstone mode. Possible detection protocols are also discussed.

cond-mat.quant-gas↗

arXiv2017

Magnetism out of disorder in a J=0 compound Ba2YIrO6

We systematically investigate the magnetic properties and local structure of Ba2YIrO6 to demonstrate that Y and Ir lattice defects in the form of antiphase boundary or clusters of antisite disorder affect the magnetism observed in this $d^4$ compound. We compare the magnetic properties and atomic imaging of (1) a slow cooled crystal, (2) a crystal quenched from 900\degree C after growth, and (3) a crystal grown using a faster cooling rate than the slow cooled one. Atomic imaging by scanning transmission electron microscopy (STEM) shows that quenching from 900oC introduces antiphase boundary to the crystals, and a faster cooling rate during crystal growth leads to clusters of Y and Ir antisite disorder. STEM study suggests the antiphase boundary region is Ir-rich with a composition of Ba2YIrO6. The magnetic measurements show that Ba2YIrO6 crystals with clusters of antisite defects have a larger effective moment and a larger saturation moment than the slow-cooled crystals. Quenched crystals with Ir-rich antiphase boundary shows a slightly suppressed saturation moment than the slow cooled crystals, and this seems to suggest that antiphase boundary is detrimental to the moment formation. Our DFT calculations suggest magnetic condensation is unlikely as the energy to be gained from superexchange is small compared to the spin-orbit gap. However, once Y is replaced by Ir in the antisite disordered region, the picture of local non-magnetic singlets breaks down and magnetism can be induced. This is because of (a) enhanced interactions due to increased overlap of orbitals between sites, and, (b) increased number of orbitals mediating the interactions. Our work highlights the importance of lattice defects in understanding the experimentally observed magnetism in Ba2YIrO6 and other J=0 systems.

cond-mat.mtrl-sci↗

arXiv2016

Fragile singlet ground state magnetism in pyrochlore osmates R2Os2O7 (R=Y and Ho)

The singlet ground state magnetism in pyrochlore osmates Y$_2$Os$_2$O$_7$ and Ho$_2$Os$_2$O$_7$ is studied by DC and AC susceptibility, specific heat, and neutron powder diffraction measurements. Despite the expected non-magnetic singlet in the strong spin-orbit coupling (SOC) limit for Os$^{4+}$ ($5d^4$), Y$_2$Os$_2$O$_7$ exhibits a spin-glass (SG) ground state below 4 K with weak magnetism, suggesting possible proximity to a quantum phase transition between the non-magnetic state in the strong SOC limit and the magnetic state in the strong superexchange limit. Ho$_2$Os$_2$O$_7$ has the same structural distortion as occurs in Y$_2$Os$_2$O$_7$. However, the Os sublattice in Ho$_2$Os$_2$O$_7$ shows long-range magnetic ordering below 36\,K. The sharp difference of the magnetic ground state between Y$_2$Os$_2$O$_7$ and Ho$_2$Os$_2$O$_7$ signals the singlet ground state magnetism in $R_2$Os$_2$O$_7$ is fragile and can be disturbed by the weak $4f-5d$ interactions.

cond-mat.str-el↗

arXiv2015

Emergence of coherence in the charge-density wave state of 2H-NbSe$_2$

A charge-density wave (CDW) state has a broken symmetry described by a complex order parameter with an amplitude and a phase. The conventional view, based on clean, weak-coupling systems, is that a finite amplitude and long-range phase coherence set in simultaneously at the CDW transition temperature T$_{cdw}$. Here we investigate, using photoemission, X-ray scattering and scanning tunneling microscopy, the canonical CDW compound 2H-NbSe$_2$ intercalated with Mn and Co, and show that the conventional view is untenable. We find that, either at high temperature or at large intercalation, CDW order becomes short-ranged with a well-defined amplitude that impacts the electronic dispersion, giving rise to an energy gap. The phase transition at T$_{cdw}$ marks the onset of long-range order with global phase coherence, leading to sharp electronic excitations. Our observations emphasize the importance of phase fluctuations in strongly coupled CDW systems and provide insights into the significance of phase incoherence in `pseudogap' states.

cond-mat.str-el↗

arXiv2015

High antiferromagnetic transition temperature of a honeycomb compound SrRu$_2$O$_6$

The high temperature magnetic order in SrRu$_2$O$_6$ was studied by measuring magnetization and neutron powder diffraction with both polarized and unpolarized neutrons. SrRu$_2$O$_6$ crystallizes into the hexagonal lead antimonate (PbSb$_2$O$_6$, space group \textit{P}$\overline{3}$1\textit{m}) structure with layers of edge-sharing RuO$_6$ octahedra separated by Sr$^{2+}$ ions. SrRu$_2$O$_6$ orders at $T_N$=565\,K with Ru moments coupled antiferromagnetically both in-plane and out-of-plane. The magnetic moment is 1.30(2) $μ_\mathrm{B}$/Ru at room temperature and is along the crystallographic \textit{c}-axis in the G-type magnetic structure. We performed density functional calculations with constrained RPA to obtain the electronic structure and effective intra- and inter-orbital interaction parameters. The projected density of states show strong hybridization between Ru 4$d$ and O 2$p$. By downfolding to the target $t_{2g}$ bands we extracted the effective magnetic Hamiltonian. We performed Monte Carlo simulations to determine the transition temperature as a function of inter- and intra-plane couplings and find weak inter plane coupling, 3\% of the intra-plane coupling, permits three dimensional magnetic order at $T_N$. As suggested by the magnetic susceptibility, two-dimensional correlations persist above $T_N$ due to the strong intra-plane coupling.

cond-mat.str-el↗

arXiv2012

Gapless inhomogeneous superfluid phase with spin-dependent disorder

We show that the presence of a spin-dependent random potential in a superconductor or a superfluid atomic gas leads to distinct transitions at which the energy gap and average order parameter vanish, generating an intermediate gapless superfluid phase, in marked contrast to the case of spin-symmetric randomness where no such gapless superfluid phase is seen. By allowing the pairing amplitude to become inhomogeneous, the gapless superconducting phase persists to considerably higher disorder compared with the prediction of Abrikosov-Gorkov. The low-lying excited states are located predominantly in regions where the pairing amplitude vanishes and coexist with the superfluid regions with a finite pairing. Our results are based on inhomogeneous Bogoliubov-de Gennes mean field theory for a two dimensional attractive Hubbard model with spin-dependent disorder.

cond-mat.dis-nn↗

arXiv2011

Probing Phases and Quantum Criticality using Deviations from the Local Fluctuation-Dissipation Theorem

Introduction Cold atomic gases in optical lattices are emerging as excellent laboratories for testing models of strongly interacting particles in condensed matter physics. Currently, one of the major open questions is how to obtain the finite temperature phase diagram of a given quantum Hamiltonian directly from experiments. Previous work in this direction required quantum Monte Carlo simulations to directly model the experimental situation in order to extract quantitative information, clearly defeating the purpose of an optical lattice emulator. Here we propose a new method that utilizes deviations from a local fluctuation dissipation theorem to construct a finite temperature phase diagram, for the first time, from local observables accessible by in situ experimental observations. Our approach extends the utility of the fluctuation-dissipation theorem from thermometry to the identification of quantum phases, associated energy scales and the quantum critical region. We test our ideas using state-of-the-art large-scale quantum Monte Carlo simulations of the two-dimensional Bose Hubbard model.

cond-mat.quant-gas↗

arXiv2011

Mystery of Excess Low Energy States in a Disordered Superconductor in a Zeeman Field

Tunneling density of states measurements of disordered superconducting (SC) Al films in high Zeeman fields reveal a significant population of subgap states which cannot be explained by standard BCS theory. We provide a natural explanation of these excess states in terms of a novel disordered Larkin-Ovchinnikov (dLO) phase that occurs near the spin-paramagnetic transition at the Chandrasekhar-Clogston critical field. The dLO superconductor is characterized by a pairing amplitude that changes sign at domain walls. These domain walls carry magnetization and support Andreev bound states, which lead to distinct spectral signatures at low energy.

cond-mat.supr-con↗

arXiv2011

Repulsive Fermions in Optical Lattices: Phase separation versus Coexistence of Antiferromagnetism and d-Superfluidity

We investigate a system of fermions on a two-dimensional optical square lattice in the strongly repulsive coupling regime. In this case, the interactions can be controlled by laser intensity as well as by Feshbach resonance. We compare the energetics of states with resonating valence bond d-wave superfluidity, antiferromagnetic long range order and a homogeneous state with coexistence of superfluidity and antiferromagnetism. We show that the energy density of a hole $e_{hole}(x)$ has a minimum at doping $x=x_c$ that signals phase separation between the antiferromagnetic and d-wave paired superfluid phases. The energy of the phase-separated ground state is however found to be very close to that of a homogeneous state with coexisting antiferromagnetic and superfluid orders. We explore the dependence of the energy on the interaction strength and on the three-site hopping terms and compare with the nearest neighbor hopping {\it t-J} model.

cond-mat.quant-gas↗

arXiv2011

Finite temperature study of bosons in a two dimensional optical lattice

We use quantum Monte Carlo (QMC) simulations to study the combined effects of harmonic confinement and temperature for bosons in a two dimensional optical lattice. The scale invariant, finite temperature, state diagram is presented for the Bose-Hubbard model in terms of experimental parameters -- the particle number, confining potential and interaction strength. To distinguish the nature of the spatially separated superfluid, Mott Insulator and normal Bose liquid phases, we examine the local density, compressibility, superfluid density and Green's function. In the annular superfluid rings, as the width of the ring decreases, the long range superfluid correlations start to deviate from an equivalent homogeneous 2D system. At zero temperature, the correlation decay is intermediate between 1D and 2D, while at finite temperature, the decay is similar to that in 1D at a much lower temperature. The calculations reveal shortcomings of the local density approximation (LDA) in describing superfluid properties of trapped bosons. We also present the finite temperature phase diagram for the homogeneous two dimensional Bose-Hubbard model. We compare our state diagram with the results of a recent experiment at NIST on a harmonically trapped 2D lattice [Phys. Rev. Lett. 105, 110401 (2010)], and identify a finite temperature effect in the experiment.

cond-mat.quant-gas↗

arXiv2010

Weak Mott insulators on the triangular lattice: possibility of a gapless nematic quantum spin liquid

We study the energetics of Gutzwiller projected BCS states of various symmetries for the triangular lattice antiferromagnet with a four particle ring exchange using variational Monte Carlo methods. In a range of parameters the energetically favored state is found to be a projected $d_{x^2-y^2}$ paired state which breaks lattice rotational symmetry. We show that the properties of this nematic or orientationally ordered paired spin liquid state as a function of temperature and pressure can account for many of the experiments on organic materials. We also study the ring-exchange model with ferromagnetic Heisenberg exchange and find that amongst the studied ansätze, a projected $f-$wave state is the most favorable.

cond-mat.str-el↗

arXiv2010

Ferromagnetism in repulsive Fermi gases: upper branch of Feshbach resonance versus hard spheres

We use quantum Monte Carlo, including backflow corrections, to investigate a two-component Fermi gas on the upper branch of a Feshbach resonance and contrast it with the hard sphere gas. We find that, in both cases, the Fermi liquid becomes unstable to ferromagnetism at a $k_F a$ smaller than the mean field result, where $k_F$ is the Fermi wavevector and $a$ the scattering length. Even though the total energies $E(k_F a)$ are similar in the two cases, their pair correlations and kinetic energies are completely different, reflecting the underlying potentials. We discuss the extent to which our calculations shed light on recent experiments.

cond-mat.quant-gas↗

arXiv2009

Large Range of Stability of Larkin-Ovchinnikov States for Imbalanced Fermi Gases in Optical Lattices

We show that Larkin-Ovchinnikov (LO) states with modulated superfluid order parameters have a considerably larger range of stability in a lattice than in the continuum. We obtain the phase diagram for the 3D cubic attractive Hubbard model with an unequal population of up and down fermions using the Bogoliubov-de Gennes fully self-consistent method. We find a strong modulation of the local polarization that should provide a distinct signature for detection of the LO phase. The shell structure in the presence of a trap generates singularities in the density at the phase boundaries and provide additional evidence for the LO phase. Depending on specific parameters, the LO ground state occurs over a large range of population imbalance, involving 80% of the atoms in the trap, and can exist up to an entropy s ~ 0.5 k_B per fermion.

cond-mat.quant-gas↗

arXiv2004

The Physics Behind High-Temperature Superconducting Cuprates: The "Plain Vanilla" Version Of RVB

One of the first theoretical proposals for understanding high temperature superconductivity in the cuprates was Anderson's RVB theory using a Gutzwiller projected BCS wave function as an approximate ground state. Recent work by Paramekanti, Randeria and Trivedi has shown that this variational approach gives a semi-quantitative understanding of the doping dependences of a variety of experimental observables in the superconducting state of the cuprates. In this paper we revisit these issues using the ``renormalized mean field theory'' of Zhang, Gros, Rice and Shiba based on the Gutzwiller approximation in which the kinetic and superexchange energies are renormalized by different doping-dependent factors $g_{t}$ and $g_{S}$ respectively. We point out a number of consequences of this early mean field theory for experimental measurements which were not available when it was first explored, and observe that it is able to explain the existence of the pseudogap, properties of nodal quasiparticles and approximate spin-charge separation, the latter leading to large renormalizations of the Drude weight and superfluid density. We use the Lee-Wen theory of the phase transition as caused by thermal excitation of nodal quasiparticles, and also obtain a number of further experimental confirmations. Finally, we remark that superexchange, and not phonons, are responsible for d-wave superconductivity in the cuprates.

cond-mat.str-el↗