arXiv subjects

N. de Séréville

Publications and source records attributed to N. de Séréville.

At least 19 recordsLinked to original sources

arXiv2026

Gamma-ray production cross sections in proton interactions with natMg, natSi and 56Fe targets: measurement over the energy range of $E_p = 66$-125 MeV, data analysis, results and discussion. Astrophysical implications

We have measured nuclear gamma-ray line production cross sections in interactions of highly accelerated proton beams with various target nuclei abundant in astrophysical sites. The experiments were carried out at the 200-MV Separated Sector Cyclotron (SSC) of iThemba LABS (near Cape Town, in South Africa) using a high-energy resolution and high efficiency detection system for registering the emitted gamma-ray photons. We report and discuss in this paper the collected experimental data sets for various gamma-ray lines produced in bombarding natMg, natSi and 56Fe targets with proton beams of incident energies of Ep = 66, 80, 95, 110 and 125 MeV. After describing the experimental set up and the data analysis method used, we report and discuss our total experimental cross section results in comparisons to previous counterparts from the literature, to a semi-empirical compilation and to the predictions of nuclear reaction theory via performed TALYS code calculations. Significantly improved agreements between theory and experiment are point out when using our modified optical model potential and Bêta (lambda) level deformation parameters instead of the default input parameters built in TALYS. Finally, we put into perspective the applications of our results in nuclear physics and astrophysics with drawing relevant conclusions. gammaKeywords: Proton-induced nuclear reactions; gamma-ray production cross sections; gamma-ray spectrometry; gamma-ray spectroscopy; Astrophysical implications

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arXiv2026

Studies of $\rm ^{144,148}Sm+α$ potential for the $p$-process nucleosynthesis

Nucleosynthesis reaction networks leading to $p$-nuclei involve a combination of different types of photodisintegration and capture reactions, as well as $β^+$ decays or electron captures. Photodisintegration reactions involving $α$ particles present a particular interest as they serve as branching points of the reaction networks. The cross sections of these reactions depend crucially on the $α$-nucleus interaction. The $α$ optical model potential (AOMP) is determined mostly by means of experimental differential elastic scattering distributions. Several previous studies have focused on the case of $\rm ^{144}Sm$, an intriguing $p$-nucleus that is semi-magic with 82 neutrons. This work presents new experimental data on $α$ elastic and inelastic scattering on $\rm ^{148}Sm$, its closest stable isotope. Isotopic effects on the description of the AOMP are studied, as well as their consequences on the prediction of $α$-induced reaction cross sections at astrophysical energies. It is shown that the isotopic ratio for $(α,γ)$ cross sections can be multiplied up to a factor of two when these effects are included.

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arXiv2026

Direct transfer to $^{46,48}$K as a survey of the $π(s_{1/2})$$-ν(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $πs_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$γ$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$γ$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $πs_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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arXiv2025

Refining the deep sub-barrier 12C+12C excitation function with STELLA

Purpose: We have investigated the cross section around the lowest direct coincident gamma-particle measurements, where previously only limits could be established with the aim of obtaining a detailed description of the excitation function. We have furthermore analysed the ratio of extreme decay branching into the first excited state of daughter nuclei with alpha or proton emission at relative kinetic energies where previous measurements are in disagreement with each other. Conclusions: Our findings in the astrophysics RoI support reaction-rate models with a lower average S-factor trend, that deviates significantly from standard extrapolations between 2.2 MeV and 2.6 MeV, for stellar carbon burning simulations of up to 25 Msol stars. Based on our data, an overall increase of the S-factor at deep subbarrier energy cannot be confirmed. The extremely low ratio of the branching into the first excited state with proton over alpha emission of ~ 2% at 3.23 MeV might indicate the presence of alpha cluster compound states in 24Mg. This highly favours α emission with fundamental consequences in possible stellar carbon burning sites.

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arXiv2025

Unbound neutron $\nu0d_{3/2}$ strength in $^{17}$C and the N=16 shell gap

Significant continuum strength has been observed to be populated in $^{17}$C produced in the d($^{16}$C,p) reaction at a beam energy of 17.2~MeV/nucleon. The strength appears at greater than $\sim$2~MeV above the single-neutron decay threshold and has been identified as arising from transfer into the neutron $0d_{3/2}$ orbital. Guided by shell model predictions the greater majority of the strength is associated with a 3/2$^+$ state at an excitation energy of 4.40$_{-0.14}^{+0.33}$ MeV and a much weaker 3/2$^+$ level at 5.60$_{-0.45}^{+1.35}$ MeV. The corresponding total widths were determined to be 3.45$_{-0.78}^{+1.82}$ and 1.6$_{-1.4}^{+4.6}$ MeV, respectively. From the backward angle proton differential cross sections and the branching ratios for neutron decay to the $^{16}$C(2$_{1}^{+}$) level, the corresponding spectroscopic factors to the ground state were deduced to be 0.47$\pm{10}$ and $<$0.09. Shell-model calculations employing the phenomenological SFO-tls interaction as well as Gamow Shell-Model calculations including continuum effects are in reasonable agreement with experiment, although the predicted strength lies at somewhat lower energy. The size of the N=16 shell gap ($\varepsilon_{ \nu0d_{3/2}}-\varepsilon _{ν1s_{1/2}}$) was estimated to be 5.08$_{-0.33}^{+0.43}$~MeV - some 1.3~MeV larger than found in the SFO-tls shell model calculation.

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arXiv2025

Low-energy neutron cross-talk between organic scintillator detectors

A series of measurements have been performed with low-energy monoenergetic neutrons to characterise cross-talk between two organic scintillator detectors. Cross-talk time-of-flight spectra and probabilities were determined for neutron energies from 1.4 to 15.5 MeV and effective scattering angles ranging from $\sim$50° to $\sim$100°. Monte-Carlo simulations incorporating both the active and inactive materials making up the detectors showed reasonable agreement with the measurements. Whilst the time-of-flight spectra were very well reproduced, the cross-talk probabilities were only in approximate agreement with the measurements, with the most significant discrepancies ($\sim$40 %) occurring at the lowest energies. The neutron interaction processes producing cross-talk at the energies explored here are discussed in the light of these results.

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arXiv2025

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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arXiv2023

N=16 magicity revealed at the proton drip-line through the study of 35Ca

The last proton bound calcium isotope $^{35}$Ca has been studied for the first time, using the $^{37}$Ca($p, t$)$^{35}$Ca two neutron transfer reaction. The radioactive $^{37}$Ca nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid hydrogen target CRYPTA, to produce tritons $t$ that were detected in the MUST2 detector array, in coincidence with the heavy residues Ca or Ar. The atomic mass of $^{35}$Ca and the energy of its first 3/2$^+$ state are reported. A large $N=16$ gap of 4.61(11) MeV is deduced from the mass measurement, which together with other measured properties, makes $^{36}$Ca a doubly-magic nucleus. The $N = 16$ shell gaps in $^{36}$Ca and $^{24}$O are of similar amplitude, at both edges of the valley of stability. This feature is discussed in terms of nuclear forces involved, within state-of-the-art shell model calculations. Even though the global agreement with data is quite convincing, the calculations underestimate the size of the $N = 16$ gap in 36Ca by 840(110) keV.

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arXiv2023

Gamma-ray emission in proton-induced nuclear reactions on natC and Mylar targets over the incident energy range of Ep = 30-200 MeV. Astrophysical implications

We have measured the gamma-ray line production cross sections in proton-induced nuclear reactions on various target nuclei abundant in astrophysical sites over the incident energy range of Ep = 30 - 200 MeV. We carried out experimental campaigns in joint collaboration at the K = 200 cyclotron of iThemba LABS using a high-energy resolution, high-efficiency detection array composed of 8 Compton-suppressed clover detectors comprising 32 HP-Ge crystals for recording the gamma-ray spectra. In the current paper, we focus on de-excitation lines produced in proton irradiations of natC and Mylar targets. In particular, on the prominent 4.439 and 6.129 MeV lines of $^{12}$C and $^{16}$O which are among the strongest lines emitted in solar flares and in interactions of low-energy cosmic rays with the gas and dust of the inner galaxy. We report new gamma-ray production experimental cross section data for ten nuclear lines that we compare to previous low-energy data sets from the literature, to the predictions of the TALYS code of modern nuclear reactions and to a semi-empirical compilation. In first approach, performing calculations with default input parameters of TALYS we observed substantial deviations between the predicted cross sections and experimental data. Then, using modified optical model potential and nuclear level deformation parameters as input data we generated theoretical excitation functions for the above two main lines fully consistent with experimental data. In contrast, the experimental data sets for the other eight analyzed lines from the two proton-irradiated targets exhibit significant deviations with the predicted cross section values. We also report line-shape experimental data for the line complex observed at $E_g$ = 4.44 MeV in irradiations of the two targets. Finally, we emphasize the astrophysical implications of our results.

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arXiv2023

Cross-shell states in $^{15}$C: a test for p-sd interactions

The low-lying structure of $^{15}$C has been investigated via the neutron-removal $^{16}$C$(d,t)$ reaction. Along with bound neutron sd-shell hole states, unbound p-shell hole states have been firmly confirmed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the $[(p)^{-1}(sd)^{2}]$ neutron configurations in $^{15}$C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for $^{15}$C. However, a modification of the $p$-$sd$ and $sd$-$sd$ monopole terms was applied in order to reproduce the $N=9$ isotone $^{17}$O. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of $^{15}$C with the $ab~ initio$ self-consistent Green's function method employing the NNLO$_{sat}$ interaction. The results show the sensitivity to the size of the $N=8$ shell gap and highlight the need of going beyond the current truncation scheme in the theory.

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arXiv2022

The structure of $^{36}$Ca under the Coulomb magnifying glass

Detailed spectroscopy of the neutron-deficient nucleus $^{36}$Ca was obtained up to 9 MeV using the $^{37}$Ca($p$,$d$)$^{36}$Ca and the $^{38}$Ca($p$,$t$)$^{36}$Ca transfer reactions. The radioactive nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid Hydrogen target CRYPTA, to produce light ejectiles (the deuteron $d$ or triton $t$) that were detected in the MUST2 detector array, in coincidence with the heavy residues %identified by a zero degree detection system. %States have been measured up to 9 MeV. Our main findings are: i) a similar shift in energy for the 1$^+_1$ and 2$^+_1$ states by about -250 keV, as compared to the mirror nucleus $^{36}$S, ii) the discovery of an intruder 0$^+_2$ state at 2.83(13) MeV, which appears below the first 2$^+$ state, in contradiction with the situation in $^{36}$S, and iii) a tentative 0$^+_3$ state at 4.83(17) MeV, proposed to exhibit a bubble structure with two neutron vacancies in the 2s$_{1/2}$ orbit. The inversion between the 0$^+_2$ and 2$^+_1$ states is due to the large mirror energy difference (MED) of -516(130) keV for the former. This feature is reproduced by Shell Model (SM) calculations, using the $sd$-$pf$ valence space, predicting an almost pure intruder nature for the 0$^+_2$ state, with two protons (neutrons) being excited across the $Z$=20 magic closure in $^{36}$Ca ($^{36}$S). This mirror system has the largest MEDs ever observed, if one excludes the few cases induced by the effect of the continuum.

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arXiv2022

Experimental study of the $^{30}$Si($^{3}$He,$d$)$^{31}$P reaction and thermonuclear reaction rate of $^{30}$Si($p$,$γ$)$^{31}$P

[Background] Abundance anomalies in some globular clusters, such as the enhancement of potassium and the depletion of magnesium, can be explained in terms of an earlier generation of stars polluting the presently observed ones. It was shown that the potential range of temperatures and densities of the polluting sites depends on the strength of a few number of critical reaction rates. The reaction has been identified as one of these important reactions. [Purpose] The key ingredient for evaluating the thermonuclear reaction rate is the strength of the resonances which, at low energy, are proportional to their proton width. Therefore the goal of this work is to determine the proton widths of unbound 31P states. [Method] States in 31P were studied at the Maier-Leibnitz-Laboratorium using the one-proton transfer reaction. Deuterons were detected with the Q3D magnetic spectrometer. Angular distribution and spectroscopic factors were extracted for 27 states, and proton widths and resonance strengths were calculated for the unbound states. [Results] Several unbound states have been observed for the first time in a one-proton transfer reaction. Above 20 MK, the reaction rate is now entirely estimated from the observed properties of states. The reaction rate uncertainty from all resonances other than the resonance has been reduced down to less than a factor of two above that temperature. The unknown spin and parity of the resonance dominates the uncertainty in the rate in the relevant temperature range. [Conclusion] The remaining source of uncertainty on the reaction rate comes from the unknown spin and parity of the resonance which can change the reaction rate by a factor of ten in the temperature range of interest.

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arXiv2021

Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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arXiv2021

Pulse shape discrimination for GRIT: beam test of a new integrated charge and current preamplifier coupled with high granularity Silicon detectors

The GRIT (Granularity, Resolution, Identification, Transparency) Silicon array is intended to measure direct reactions. Its design is based on several layers (three layers in the forward direction, two backward) of custom-made trapezoidal and square detectors. The first stage is 500 μm thick and features 128x128 orthogonal strips. Pulse shape analysis for particle identification is implemented for this first layer. Given the compacity of this array and the large number of channels involved (>7,500), an integrated preamplifier, iPACI, that gives charge and current information has been developed in the AMS 0.35 μm BiCMOS technology. The design specifications and results of the test bench are presented. Considering an energy range of 50 MeV and an energy resolution (FWHM) of 12 keV (FWHM) for the preamplifier, the energy resolution for one strip obtained from alpha source measurement in real conditions is 35 keV. The current output bandwidth is measured at 130 MHz for small signals and the power consumption reaches 40 mW per detector channel. A first beam test was performed coupling a nTD trapezoidal double-sided stripped Silicon detector of GRIT with the iPACI preamplifier and a 64-channel digitizer. Z=1 particles are discriminated with pulse shape analysis technique down to 2 MeV for protons, 2.5 MeV for deuterons and 3 MeV for tritons. The effect of the strip length due to the trapezoidal shape of the detector is investigated on both the N- and the P-side, showing no significant impact.

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arXiv2021

Evaluation of the $^{35}$K($p$,$γ$)$^{36}$Ca reaction rate using the $^{37}$Ca($p$,$d$)$^{36}$Ca transfer reaction

A recent sensitivity study has shown that the $^{35}$K$(p,γ)^{36}$Ca reaction is one of the ten $(p,γ)$ reaction rates that could significantly impact the shape of the calculated X-ray burst light curve. In this work, we propose to reinvestigate the $^{35}$K$(p,γ)^{36}$Ca reaction rate, as well as related uncertainties, by determining the energies and decay branching ratios of $^{36}$Ca levels, within the Gamow window, in the 0.5 to 2 GK X-ray burst temperature range. These properties were studied using the one neutron pick-up transfer reaction $^{37}$Ca$(p,d)^{36}$Ca in inverse kinematics using a radioactive beam of $^{37}$Ca at 48 MeV nucleon$^{-1}$. The experiment performed at GANIL, used the liquid Hydrogen target CRYPTA, the MUST2 detector array for the detection of the light charged particles and a zero degree detection system for the outgoing heavy ions. The atomic mass of $^{36}$Ca is confirmed and new resonances have been proposed together with their proton decay branching ratios. This spectroscopic information, used in combination with recent theoretical predictions for the $γ$-width, were used to calculate the $^{35}$K$(p,γ)^{36}$Ca reaction rate. The recommended rate of the present work was obtain within a uncertainty factor of 2 at 1 sigma. This is consistent, with the previous estimate in the X-ray burst temperature range. A large increase of the reaction rate was found at higher temperatures due to two newly discovered resonances. The $^{35}$K$(p,γ)^{36}$Ca thermonuclear reaction rate is now well constrained by the present work in a broad range of temperatures. Our results show that the $^{35}$K$(p,γ)^{36}$Ca reaction does not affect the shape of the X-ray burst light curve, and that it can be removed from the list of the few influential proton radiative captures reactions having a strong impact on the light curve.

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arXiv2021

Neutron occupancies and single-particle energies across the stable tin isotopes

The occupancies and vacancies of the valence neutron orbitals across the stable tin isotopic chain from $112\leq A\leq 124$ have been determined. These were inferred from the cross sections of neutron-adding and -removing reactions. In each case, the reactions were chosen to have good angular-momentum matching for transfer to the low- and high-$\ell$ orbitals present in this valence space. These new data are compared to older systematic studies. The effective single-neutron energies are determined by combining information from energy centroids determined from the adding and removing reactions. Two of the five orbitals are nearly degenerate, below $N=64$, and approximately two MeV more bound than the other three, which are also degenerate.

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arXiv2021

Charged-particle branching ratios above the neutron threshold in $^{19}$F: constraining $^{15}$N production in core-collapse supernovae

Spatially-correlated overabundances of $^{15}$N and $^{18}$O observed in some low-density graphite meteoritic grains have been connected to nucleosynthesis taking place in the helium-burning shell during core-collapse supernovae. Two of the reactions which have been identified as important to the final abundances of $^{15}$N and $^{18}$O are $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O. The relative strengths of the $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O reactions depend on the relative $α_0$ and $p_0$ decays from states above the neutron threshold in $^{19}$F in addition to other properties. Experimental data on the charged-particle decays from these highly excited states are lacking or inconsistent. Two experiments were performed using proton inelastic scattering from LiF targets and magnetic spectrographs. The first experiment used the high-resolution Q3D spectrograph at Munich to constrain properties of levels in $^{19}$F. A second experiment using the Orsay Split-Pole spectrograph and an array of silicon detectors was performed in order to measure the charged-particle decays of neutron-unbound levels in $^{19}$F. A number of levels in $^{19}$F have been identified along with their corresponding charged-particle decays. The first state above the neutron threshold which has an observed proton-decay branch to the ground state of $^{18}$O lies 68 keV above the neutron threshold while the $α$-particle decays from the neutron-unbound levels are generally observed to be much stronger than the proton decays. Neutron-unbound levels in $^{19}$F are observed to decay predominantly by $α$-particle emission, supporting the role of $^{18}$F($n,α$)$^{15}$N in the production of $^{15}$N in the helium-burning shell of supernovae. Improved resonant-scattering reaction data are required in order to be able to determine the reaction rates accurately.

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arXiv2020

Sub-threshold states in $^{19}$Ne relevant to $^{18}$F(p,$α$)$^{15}$O

Classical novae result from thermonuclear explosions producing several $γ$-ray emitters which are prime targets for satellites observing in the MeV range. The early 511 keV gamma-ray emission depends critically on the $^{18}$F(p,$α$)$^{15}$O reaction rate which, despite many experimental and theoretical efforts, still remains uncertain. One of the main uncertainties in the $^{18}$F(p,$α$)$^{15}$O reaction rate is the contribution in the Gamow window of interference between sub-threshold $^{19}$Ne states and known broad states at higher energies. Therefore the goal of this work is to clarify the existence and the nature of these sub-threshold states. States in the $^{19}$Ne compound nucleus were studied at the Tandem-ALTO facility using the $^{19}$F($^3$He,t)$^{19}$Ne charge exchange reaction. Tritons were detected with an Enge Split-pole spectrometer while decaying protons or $α$-particles from unbound $^{19}$Ne states were collected, in coincidence, with a double-sided silicon strip detector array. Angular correlations were extracted and constraints on the spin and parity of decaying states established. The coincidence yield at $E_x$ = 6.29 MeV was observed to be high spin, supporting the conclusion that it is indeed a doublet consisting of high spin and low spin components. Evidence for a broad, low spin state was observed around 6 MeV. Branching ratios were extracted for several states above the proton threshold and were found to be consistent with the literature. R-matrix calculations show the relative contribution of sub-threshold states to the astrophysically important energy region above the proton threshold. The levels schemes of $^{19}$Ne and $^{19}$F are still not sufficiently well known and further studies of the analogue assignments are needed. The tentative broad state at 6 MeV may only play a role if the reduced proton width is large.

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