arXiv subjects

Na Liu

Publications and source records attributed to Na Liu.

At least 73 records · Page 4Linked to original sources

arXiv2021

Magnesium-Based Metasurfaces for Dual-Function Switching between Dynamic Holography and Dynamic Color Display

Metasurface-based color display and holography have greatly advanced the state of the art display technologies. To further enrich the metasurface functionalities, recently a lot of research endeavors have been made to combine these two display functions within a single device. However, so far such metasurfaces have remained static and lack tunability once the devices are fabricated. In this work, we demonstrate a dynamic dual-function metasurface device at visible frequencies. It allows for switching between dynamic holography and dynamic color display, taking advantage of the reversible phase transition of magnesium through hydrogenation and dehydrogenation. Spatially arranged stepwise nanocavity pixels are employed to accurately control the amplitude and phase of light, enabling the generation of high-quality color prints and holograms. Our work represents a paradigm toward compact and multifunctional optical elements for future display technologies.

physics.optics↗

arXiv2021

Scanning Plasmonic Color Display

Control over plasmonic colors on the nanoscale is of great interest for high-resolution display, imaging, and information encryption applications. However, so far, very limited schemes have been attempted for dynamic plasmonic color generation. In this paper, we demonstrate a scanning plasmonic color generation scheme, in which subwavelength plasmonic pixels can be laterally switched on/off through directional hydrogenation/dehydrogenation of a magnesium screen. We show several dynamic plasmonic color displays with different scanning functions by varying the number and geometries of the palladium gates, where hydrogen enters the scanning screens. In particular, we employ the scanning effects to create a dynamic plasmonic quick response code. The information cannot be decrypted by varying the polarization states of light or by accessing the physical features. Rather, it can only be read out using hydrogen as a decoding key. Our work advances the established design concepts for plasmonic color printing and provides insights into the development of optical information storage and anticounterfeiting features.

physics.app-ph↗

arXiv2021

Generation of Switchable Singular Beams with Dynamic Metasurfaces

Singular beams have attracted great attention due to their optical properties and broad applications from light manipulation to optical communications. However, there has been a lack of practical schemes with which to achieve switchable singular beams with sub-wavelength resolution using ultrathin and flat optical devices. In this work, we demonstrate the generation of switchable vector and vortex beams utilizing dynamic metasurfaces at visible frequencies. The dynamic functionality of the metasurface pixels is enabled by the utilization of magnesium nanorods, which possess plasmonic reconfigurability upon hydrogenation and dehydrogenation. We show that switchable vector beams of different polarization states and switchable vortex beams of different topological charges can be implemented through simple hydrogenation and dehydrogenation of the same metasurfaces. Furthermore, we demonstrate a two-cascade metasurface scheme for holographic pattern switching, taking inspiration from orbital angular momentum-shift keying. Our work provides an additional degree of freedom to develop high-security optical elements for anti-counterfeiting applications.

physics.optics↗

arXiv2021

DNA Origami Route for Nanophotonics

The specificity and simplicity of the Watson-Crick base pair interactions make DNA one of the most versatile construction materials for creating nanoscale structures and devices. Among several DNA-based approaches, the DNA origami technique excels in programmable self-assembly of complex, arbitrary shaped structures with dimensions of hundreds of nanometers. Importantly, DNA origami can be used as templates for assembly of functional nanoscale components into three-dimensional structures with high precision and controlled stoichiometry. This is often beyond the reach of other nanofabrication techniques. In this Perspective, we highlight the capability of the DNA origami technique for realization of novel nanophotonic systems. First, we introduce the basic principles of designing and fabrication of DNA origami structures. Subsequently, we review recent advances of the DNA origami applications in nanoplasmonics, single-molecule and super-resolution fluorescent imaging, as well as hybrid photonic systems. We conclude by outlining the future prospects of the DNA origami technique for advanced nanophotonic systems with tailored functionalities.

physics.optics↗

arXiv2021

Watching a Single Fluorophore Molecule Walk into a Plasmonic Hotspot

Plasmonic nanoantennas allow for enhancing the spontaneous emission, altering the emission polarization, and shaping the radiation pattern of quantum emitters. A critical challenge for the experimental realizations is positioning a single emitter into the hotspot of a plasmonic antenna with nanoscale accuracy. We demonstrate a dynamic light-matter interaction nanosystem enabled by the DNA origami technique. A single fluorophore molecule can autonomously and unidirectionally walk into the hotspot of a plasmonic nanoantenna along a designated origami track. Successive fluorescence intensity increase and lifetime reduction are in situ monitored using single-molecule fluorescence spectroscopy, while the fluorophore walker gradually approaches and eventually enters the plasmonic hotspot. Our scheme offers a dynamic platform, which can be used to develop functional materials, investigate intriguing light-matter interaction phenomena, and serve as prototype system for examining theoretical models.

physics.optics↗

arXiv2021

Gold nanocrystal-mediated sliding of doublet DNA origami filaments

Sliding is one of the fundamental mechanical movements in machinery. In macroscopic systems, double-rack pinion machines employ gears to slide two linear tracks along opposite directions. In microscopic systems, kinesin-5 proteins crosslink and slide apart antiparallel microtubules, promoting spindle bipolarity and elongation during mitosis. Here we demonstrate an artificial nanoscopic analog, in which gold nanocrystals can mediate coordinated sliding of two antiparallel DNA origami filaments powered by DNA fuels. Stepwise and reversible sliding along opposite directions is in situ monitored and confirmed using fluorescence spectroscopy. A theoretical model including different energy transfer mechanisms is developed to understand the observed fluorescence dynamics. We further show that such sliding can also take place in the presence of multiple DNA sidelocks that are introduced to inhibit the relative movements. Our work enriches the toolbox of DNA-based nanomachinery, taking one step further toward the vision of molecular nanofactories.

physics.bio-ph↗

arXiv2021

DNA origami

Biological materials are self-assembled with near-atomic precision in living cells, whereas synthetic 3D structures generally lack such precision and controllability. Recently, DNA nanotechnology, especially DNA origami technology, has been useful in the bottom-up fabrication of well-defined nanostructures ranging from tens of nanometres to sub-micrometres. In this Primer, we summarize the methodologies of DNA origami technology, including origami design, synthesis, functionalization and characterization. We highlight applications of origami structures in nanofabrication, nanophotonics and nanoelectronics, catalysis, computation, molecular machines, bioimaging, drug delivery and biophysics. We identify challenges for the field, including size limits, stability issues and the scale of production, and discuss their possible solutions. We further provide an outlook on next-generation DNA origami techniques that will allow in vivo synthesis and multiscale manufacturing.

physics.bio-ph↗

arXiv2021

Self-recording and manipulation of fast long-range hydrogen diffusion in quasifree magnesium

Understanding diffusion of large solutes such as hydrogen and lithium in solids is of paramount importance for energy storage in metal hydrides and advanced batteries. Due to its high gravimetric and volumetric densities, magnesium is a material of great potential for solid-state hydrogen storage. However, the slow hydrogen diffusion kinetics and the deleterious blocking effect in magnesium have hampered its practical applications. Here, we demonstrate fast lateral hydrogen diffusion in quasifree magnesium films without the blocking effect. Massive concomitant lattice expansion leads to the formation of remarkable self-organized finger patterns extending over tens of micrometers. Detailed visualization of diffusion fronts reveals that the fingers in these patterns follow locally the direction of hydrogen diffusion. Thus, the streamlines of the diffusion process are self-recorded by means of the finger pattern. By inclusion of fast hydrogen diffusion objects or local gaps, the resulting streamlines exhibit a clear analogy to optical rays in geometric optics. The possibility to spatially manipulate hydrogen diffusion opens an avenue to build advanced hydrogen storage systems, cloaking and active plasmonic devices, as well as prototype systems for computational models.

physics.app-ph↗

arXiv2021

Selective control of reconfigurable chiral plasmonic metamolecules

Selective configuration control of plasmonic nanostructures using either top-down or bottom-up approaches has remained challenging in the field of active plasmonics. We demonstrate the realization of DNA-assembled reconfigurable plasmonic metamolecules, which can respond to a wide range of pH changes in a programmable manner. This programmability allows for selective reconfiguration of different plasmonic metamolecule species coexisting in solution through simple pH tuning. This approach enables discrimination of chiral plasmonic quasi-enantiomers and arbitrary tuning of chiroptical effects with unprecedented degrees of freedom. Our work outlines a new blueprint for implementation of advanced active plasmonic systems, in which individual structural species can be programmed to perform multiple tasks and functions in response to independent external stimuli.

physics.optics↗

arXiv2021

Addressable metasurfaces for dynamic holography and optical information encryption

Metasurfaces enable manipulation of light propagation at an unprecedented level, benefitting from a number of merits unavailable to conventional optical elements, such as ultracompactness, precise phase and polarization control at deep subwavelength scale, and multifunctionalities. Recent progress in this field has witnessed a plethora of functional metasurfaces, ranging from lenses and vortex beam generation to holography. However, research endeavors have been mainly devoted to static devices, exploiting only a glimpse of opportunities that metasurfaces can offer. We demonstrate a dynamic metasurface platform, which allows independent manipulation of addressable subwavelength pixels at visible frequencies through controlled chemical reactions. In particular, we create dynamic metasurface holograms for advanced optical information processing and encryption. Plasmonic nanorods tailored to exhibit hierarchical reaction kinetics upon hydrogenation/dehydrogenation constitute addressable pixels in multiplexed metasurfaces. The helicity of light, hydrogen, oxygen, and reaction duration serve as multiple keys to encrypt the metasurfaces. One single metasurface can be deciphered into manifold messages with customized keys, featuring a compact data storage scheme as well as a high level of information security. Our work suggests a novel route to protect and transmit classified data, where highly restricted access of information is imposed.

physics.optics↗

arXiv2021

DNA-assembled nanoarchitectures with multiple components in regulated and coordinated motion

Coordinating functional parts to operate in concert is essential for machinery. In gear trains, meshed gears are compactly interlocked, working together to impose rotation or translation. In photosynthetic systems, a variety of biological entities in the thylakoid membrane interact with each other, converting light energy into chemical energy. However, coordinating individual parts to carry out regulated and coordinated motion within an artificial nanoarchitecture poses challenges, owing to the requisite control on the nanoscale. Here, we demonstrate DNA-directed nanosystems, which comprise hierarchically-assembled DNA origami filaments, fluorophores, and gold nanocrystals. These individual building blocks can execute independent, synchronous, or joint motion upon external inputs. These are optically monitored in situ using fluorescence spectroscopy, taking advantage of the sensitive distance-dependent interactions between the gold nanocrystals and fluorophores positioned on the DNA origami. Our work leverages the complexity of DNA-based artificial nanosystems with tailored dynamic functionality, representing a viable route towards technomimetic nanomachinery.

physics.bio-ph↗

arXiv2021

Chiral Plasmonic Nanostructures Enabled by Bottom-Up Approaches

We present a comprehensive review of recent developments in the field of chiral plasmonics. Significant advances have been made recently in understanding the working principles of chiral plasmonic structures. With advances in micro- and nanofabrication techniques, a variety of chiral plasmonic nanostructures have been experimentally realized; these tailored chiroptical properties vastly outperform those of their molecular counterparts. We focus on chiral plasmonic nanostructures created using bottom-up approaches, which not only allow for rational design and fabrication but most intriguingly in many cases also enable dynamic manipulation and tuning of chiroptical responses. We first discuss plasmon-induced chirality, resulting from the interaction of chiral molecules with plasmonic excitations. Subsequently, we discuss intrinsically chiral colloids, which give rise to optical chirality owing to their chiral shapes. Finally, we discuss plasmonic chirality, achieved by arranging achiral plasmonic particles into handed configurations on static or active templates. Chiral plasmonic nanostructures are very promising candidates for real-life applications owing to their significantly larger optical chirality than natural molecules. In addition, chiral plasmonic nanostructures offer engineerable and dynamic chiroptical responses, which are formidable to achieve in molecular systems. We thus anticipate that the field of chiral plasmonics will attract further widespread attention in applications ranging from enantioselective analysis to chiral sensing, structural determination, and in situ ultrasensitive detection of multiple disease biomarkers, as well as optical monitoring of transmembrane transport and intracellular metabolism.

physics.optics↗

arXiv2021

Reconfigurable Multistate Optical Systems Enabled by VO2 Phase Transitions

Reconfigurable optical systems are the object of continuing, intensive research activities, as they hold great promise for realizing a new generation of compact, miniaturized, and flexible optical devices. However, current reconfigurable systems often tune only a single state variable triggered by an external stimulus, thus, leaving out many potential applications. Here we demonstrate a reconfigurable multistate optical system enabled by phase transitions in vanadium dioxide (VO2). By controlling the phase-transition characteristics of VO2 with simultaneous stimuli, the responses of the optical system can be reconfigured among multiple states. In particular, we show a quadruple-state dynamic plasmonic display that responds to both temperature tuning and hydrogen-doping. Furthermore, we introduce an electron-doping scheme to locally control the phase-transition behavior of VO2, enabling an optical encryption device encoded by multiple keys. Our work points the way toward advanced multistate reconfigurable optical systems, which substantially outperform current optical devices in both breadth of capabilities and functionalities.

physics.app-ph↗

arXiv2019

Doubly Enhanced Third Harmonic Generation in Metal-Based Silicon Nanodisks

Doubly enhanced third harmonic generation (THG) is realized by the electric dipole resonance (EDR) in silicon nanodisks placed onto a metallic film at near-infrared. By introducing the metal substrate, the perfect electric conductor (PEC) surface effect can be formed to not only enhance the electric field in silicon, but also improve the near-field distribution. Meanwhile, in consideration of the periodic nanostructure, the silicon nanodisk, acting as a high-refractive-index dielectric grating, can generate a propagating surface plasmon resonance (PSPR) on the metal surface. By flexibly manipulating the array period, PSPR can effectively couple with EDR, which produces further enhancement and novel properties for EDR. On account of the dual enhancements from these two effects, it is demonstrated that the total THG conversion efficiency of the proposed nanostructure is raised by more than eight orders of magnitude as compared with that of the all-dielectric nanostructure. In addition, the influence of silicon Kerr effect on the coupling and THG is investigated as well, manifesting an unprecedent THG efficiency around 10^-2 with input internsity 2 GW/cm^2. This work will pave a new way for improving the multipolar mode in metal-dielectric nanosturctures and facilitate its engineered applications in nonlinear optics, e.g. frequency conversion, spectroscopic and biochemical sensing.

physics.optics↗

arXiv2019

Fine-Grained Age Estimation in the wild with Attention LSTM Networks

Age estimation from a single face image has been an essential task in the field of human-computer interaction and computer vision, which has a wide range of practical application values. Accuracy of age estimation of face images in the wild is relatively low for existing methods, because they only take into account the global features, while neglecting the fine-grained features of age-sensitive areas. We propose a novel method based on our attention long short-term memory (AL) network for fine-grained age estimation in the wild, inspired by the fine-grained categories and the visual attention mechanism. This method combines the residual networks (ResNets) or the residual network of residual network (RoR) models with LSTM units to construct AL-ResNets or AL-RoR networks to extract local features of age-sensitive regions, which effectively improves the age estimation accuracy. First, a ResNets or a RoR model pretrained on ImageNet dataset is selected as the basic model, which is then fine-tuned on the IMDB-WIKI-101 dataset for age estimation. Then, we fine-tune the ResNets or the RoR on the target age datasets to extract the global features of face images. To extract the local features of age-sensitive regions, the LSTM unit is then presented to obtain the coordinates of the agesensitive region automatically. Finally, the age group classification is conducted directly on the Adience dataset, and age-regression experiments are performed by the Deep EXpectation algorithm (DEX) on MORPH Album 2, FG-NET and 15/16LAP datasets. By combining the global and the local features, we obtain our final prediction results. Experimental results illustrate the effectiveness and robustness of the proposed AL-ResNets or AL-RoR for age estimation in the wild, where it achieves better state-of-the-art performance than all other convolutional neural network.

cs.CV↗

arXiv2019

Spectral Numerical Mode Matching Method for 3D Layered Multi-Region Structures

The spectral numerical mode-matching (SNMM) method is developed to simulate the 3D layered multi-region structures. The SNMM method is a semi-analytical solver having the properties of dimensionality reduction to reduce computational costs; it is especially useful for microwave and optical integrated circuits where fabrication is often done in a layered structure. Furthermore, at some layer interfaces, very thin surfaces such as good conductor surfaces and metasurfaces can be deposited to achieve desired properties such as high absorbance and/or anomalous reflection/refraction. In this work, the 3D SNMM method is further extended from a single interface to multiple layers so that the electromagnetic propagation and scattering in the longitudinal direction is treated analytically through reflection and transmission matrices by using the eigenmode expansions in the transverse directions. Therefore, it effectively reduces the original 3D problem into a series of 2D eigenvalue problems for periodic structures. We apply this method to characterize metasurfaces and lithography models, and show that the SNMM method is especially efficient when the longitudinal layer thicknesses are large compared with wavelength. Numerical experiments indicate that the SNMM method is highly efficient and accurate for the metasurfaces and the lithography models.

physics.optics↗

arXiv2019

Single photon emission in $WSe_2$ up 160 K by quantum yield control

Two dimensional semiconductors hosting strain-induced quantum emitters offer unique abilities to achieve scalable architectures for deterministic coupling to nanocavities and waveguides that are required to enable chip-based quantum information processing technologies. A severe drawback remains that exciton emission from quantum emitters in $WSe_2$ quenches beyond 30 K, which requires cryogenic cooling. Here we demonstrate an approach to increase the temperature survival of exciton quantum emitters in $WSe_2$ that is based on maximizing the emitter quantum yield. Utilizing optimized material growth that leads to reduced density of nonradiative defects as well as coupling of the exciton emission to plasmonic nanocavities modes, we achieve average quantum yields up to 44%, thermal activation energies up to 92 meV, and single photon emission signatures up to temperatures of 160 K. At these values non-cryogenic cooling with thermo-electric chips becomes already feasible, while quantitative analysis shows that room temperature operation is within reach through active strain engineering.

cond-mat.mtrl-sci↗

arXiv2018

A pore-scale model for permeable biofilm: numerical simulations and laboratory experiments

In this paper we derive a pore-scale model for permeable biofilm formation in a two-dimensional pore. The pore is divided in two phases: water and biofilm. The biofilm is assumed to consist of four components: water, extracellular polymeric substances (EPS), active bacteria, and dead bacteria. The flow of water is modeled by the Stokes equation whereas a diffusion-convection equation is involved for the transport of nutrients. At the water/biofilm interface, nutrient transport and shear forces due to the water flux are considered. In the biofilm, the Brinkman equation for the water flow, transport of nutrients due to diffusion and convection, displacement of the biofilm components due to reproduction/dead of bacteria, and production of EPS are considered. A segregated finite element algorithm is used to solve the mathematical equations. Numerical simulations are performed based on experimentally determined parameters. The stress coefficient is fitted to the experimental data. To identify the critical model parameters, a sensitivity analysis is performed. The Sobol sensitivity indices of the input parameters are computed based on uniform perturbation by $\pm 10 \%$ of the nominal parameter values. The sensitivity analysis confirms that the variability or uncertainty in none of the parameters should be neglected.

physics.flu-dyn↗