arXiv subjects

Nadya Mason

Publications and source records attributed to Nadya Mason.

At least 19 recordsLinked to original sources

arXiv2026

Domain wall motion in a polycrystalline vortex lattice

Disorder fundamentally reshapes how crystalline systems respond to external forces, yet it remains unclear whether disorder drives interacting lattices toward glassy states or instead fragments them into domains separated by mobile interfaces. Here, we investigate vortex motion in superconducting island arrays, where disorder is introduced in a controlled manner by tuning the magnetic field away from commensurate vortex fillings. By driving vortices with an applied current, we observe a two-step depinning transition at incommensurate fillings. Comparison with molecular vortex model simulations shows that this intermediate regime is consistent with domain wall motion in a polycrystalline vortex lattice. While two-step depinning has been explored theoretically in driven periodic systems, direct experimental evidence linking this behavior to interface-dominated vortex motion has been lacking. Our results demonstrate that disordered, interacting vortex systems with strong periodic pinning can favor interface physics over homogeneous glassy dynamics.

cond-mat.supr-con↗

arXiv2026

Nonplanar qubit with tunable gauge symmetry

Circuit quantum electrodynamics embeds Josephson junction qubits within superconducting cavities, and has emerged as a leading approach to quantum computing and quantum simulation. Despite the many permutations of circuit geometry that have been explored, Josephson connectivities have so far been planar, making them effectively low-dimensional. Here we show that a non-planar qubit -- a $3\times3$ crossbar Josephson array -- gives rise to flux-tunable $\mathbb{Z}_3$ combinatorial gauge symmetry (CGS), potentially enabling spin-liquid behavior when networked into a lattice. The observed excitation spectrum shows excellent agreement with predictions from a neural network trained to generate variational quantum states, demonstrating that we have predictive power over our high-dimensional quantum system. Fine-structure splittings near the CGS point are compatible with weak tunneling or symmetry breaking due to experimental imperfections. We additionally use the superconducting cavity to externally induce symmetry breaking, observing a restoration of symmetry at the CGS point where ground states differ only by a $\mathbb{Z}_3$ phase. This work initiates a general program exploring lattice gauge theories using the toolbox of circuit quantum electrodynamics. More broadly, introducing non-planar Josephson connectivities opens a vast space for experimental and theoretical exploration of structures in almost any imaginable dimensionality and geometry.

quant-ph↗

arXiv2025

Observation of a Zero-Field Josephson Diode Effect in a Helimagnet Josephson Junction

We present Josephson junctions with the metallic chiral helimagnet Cr$_{1/3}$NbS$_{2}$ as the weak link that exhibit magnetic diffraction patterns with asymmetry in both applied magnetic field and the critical (switching) current. The nonreciprocity between positive and negative critical currents (the Josephson diode effect) reaches efficiencies of $|\eta|>20\%$, where $\eta \equiv (I_{c+}-|I_{c-}|)/(I_{c+}+|I_{c-}|)$, and the effect persists even at zero applied field. As a chiral helimagnet, Cr$_{1/3}$NbS$_{2}$ lacks inversion symmetry and time reversal symmetry, providing a platform to explore the interplay of superconductivity with both symmetries broken. We propose that pinned Abrikosov vortices are a primary mechanism for the asymmetric magnetic-field response, while the nonzero spin chirality of Cr$_{1/3}$NbS$_{2}$ gives rise to the diode effect. Simulations of magnetic diffraction patterns with vortices show offsets from zero field consistent with observations, while simulations of chiral spin structures with out-of-plane canting show a diode effect.

cond-mat.supr-con↗

arXiv2025

Field-effect transistors based on charged domain walls in van der Waals ferroelectric {\alpha}-In$_2$Se$_3$

Charged domain walls (CDW) in ferroelectrics are emerging as functional interfaces with potential applications in nonvolatile memory, logic, and neuromorphic computing. However, CDWs in conventional ferroelectrics are vertical, buried, or electrically inaccessible interfaces that prevent their use in functional devices. Here, we overcome these challenges by stacking two opposite polar domains of van der Waals ferroelectric $\alpha$-In$_2$Se$_3$ to generate artificial head-head (H-H) CDWs and use edge contact to fabricate charged domain wall-based field-effect transistors (CDW-FET). We relate the atomic structure to the temperature-dependent electrical and magneto-transport of the CDW-FET. CDW-FETs exhibit a metal-to-insulator transition with decreasing temperature and enhanced conductance and field-effect mobility compared to single domain $\alpha$-In$_2$Se$_3$. We identify two regimes of transport: variable range hopping due to disorder in the band edge below 70 K and thermally activated interfacial trap-assisted transport above 70 K. The CDW-FETs show room-temperature resistance down to 3.1 k$\Omega$ which is 2-9 orders of magnitude smaller than the single CDW in thin-film ferroelectrics. These results resolve longstanding challenges with high CDW resistance and their device integration, opening opportunities for gigahertz memory and neuromorphic computing.

cond-mat.mtrl-sci↗

arXiv2024

Spin-polarized antiferromagnetic metals

Spin-polarized antiferromagnets have recently gained significant interest because they combine the advantages of both ferromagnets (spin polarization) and antiferromagnets (absence of net magnetization) for spintronics applications. In particular, spin-polarized antiferromagnetic metals can be useful as active spintronics materials because of their high electrical and thermal conductivities and their ability to host strong interactions between charge transport and magnetic spin textures. We review spin and charge transport phenomena in spin-polarized antiferromagnetic metals, in which the interplay of metallic conductivity and spin-split bands offers novel practical applications and new fundamental insights into antiferromagnetism. We focus on three types of antiferromagnets: canted antiferromagnets, noncollinear antiferromagnets, and collinear altermagnets. We also discuss how the investigation of spin-polarized antiferromagnetic metals can open doors to future research directions.

cond-mat.mtrl-sci↗

arXiv2023

Evidence of Pseudogravitational Distortions of the Fermi Surface Geometry in the Antiferromagnetic Metal FeRh

The confluence between high-energy physics and condensed matter has produced groundbreaking results via unexpected connections between the two traditionally disparate areas. In this work, we elucidate additional connectivity between high-energy and condensed matter physics by examining the interplay between spin-orbit interactions and local symmetry-breaking magnetic order in the magnetotransport of thin-film magnetic semimetal FeRh. We show that the change in sign of the normalized longitudinal magnetoresistance observed as a function of increasing in-plane magnetic field results from changes in the Fermi surface morphology. We demonstrate that the geometric distortions in the Fermi surface morphology are more clearly understood via the presence of pseudogravitational fields in the low-energy theory. The pseudogravitational connection provides additional insights into the origins of a ubiquitous phenomenon observed in many common magnetic materials and points to an alternative methodology for understanding phenomena in locally-ordered materials with strong spin-orbit interactions.

cond-mat.mes-hall↗

arXiv2022

A new quasi-one-dimensional transition metal chalcogenide semiconductor (Nb$_4$Se$_{15}$I$_2$)I$_2$

The discovery of new low-dimensional transition metal chalcogenides is contributing to the already prosperous family of these materials. In this study, needle-shaped single crystals of a new quasi-one-dimensional material (Nb$_4$Se$_{15}$I$_2$)I$_2$ were grown by chemical vapor transport, and the structure was solved by single crystal X-ray diffraction (XRD). The new structure has one-dimensional (Nb$_4$Se$_{15}$I$_2$)$_n$ chains along the [101] direction, with two I$^-$ ions per formula unit directly bonded to Nb$^{5+}$. The other two I$^-$ ions are loosely coordinated and intercalate between the chains. Individual chains are chiral, and stack along the $b$ axis in opposing directions, giving space group $P2_1/c$. The phase purity and crystal structure was verified by powder XRD. Density functional theory calculations show (Nb$_4$Se$_{15}$I$_2$)I$_2$ to be a semiconductor with a direct band gap of around 0.6 eV. Resistivity measurements of bulk crystals and micro-patterned devices demonstrate that (Nb$_4$Se$_{15}$I$_2$)I$_2$ has an activation energy of around 0.1 eV, and no anomaly or transition was seen upon cooling. (Nb$_4$Se$_{15}$I$_2$)I$_2$ does not undergo structural phase transformation from room temperature down to 8.2 K, based on cryogenic temperature single crystal XRD. This compound represents a well-characterized and valence-precise member of a diverse family of anisotropic transition metal chalcogenides.

cond-mat.mtrl-sci↗

arXiv2022

Evidence for a robust sign-changing s-wave order parameter in monolayer films of superconducting Fe (Se,Te)/Bi2Te3

The Fe-based superconductor Fe (Se,Te) combines non-trivial topology with unconventional superconductivity and may be an ideal platform to realize exotic states such as high-order topological corner modes and Majorana modes. Thin films of Fe (Se,Te) are important for device fabrication, phase sensitive transport measurements and for realizing proposals to engineer higher-order modes. However, while bulk Fe (Se,Te) has been extensively studied with a variety of techniques, the nature of the superconducting order parameter in the monolayer limit has not yet been explored. In this work, we study monolayer films of Fe (Se,Te) on Bi2Te3 with scanning tunneling spectroscopy and Bogoliubov quasiparticle interference (BQPI). We discover that the monolayer Fe (Se,Te)/Bi2Te3 heterostructures host a robust, multigap superconducting state that strongly resembles the bulk. BQPI maps at the gap energies show a strong spatial modulation, oriented 45 degrees to the Fe-Se bond direction. Analysis of the phase-referenced quasiparticle interference signal reveals a sign-changing s-wave order parameter similar to the bulk. Moreover, we observe a unique pattern of sign changes in the BQPI signal which have not been observed in the bulk. Our work establishes monolayer Fe (Se,Te)/Bi2Te3 as a robust multi-band unconventional superconductor and sets the stage for explorations of non-trivial topology in this highly-tunable system.

cond-mat.supr-con↗

arXiv2022

Local imaging of diamagnetism in proximity coupled niobium nano-island arrays on gold thin films

In this work we study the effect of engineered disorder on the local magnetic response of proximity coupled superconducting island arrays by comparing scanning Superconducting Quantum Interference Device (SQUID) susceptibility measurements to a model in which we treat the system as a network of one-dimensional (1D) superconductor-normal metal-superconductor (SNS) Josephson junctions, each with a Josephson coupling energy $E_J$ determined by the junction length or distance between islands. We find that the disordered arrays exhibit a spatially inhomogeneous diamagnetic response which, for low local applied magnetic fields, is well described by this junction network model, and we discuss these results as they relate to inhomogeneous two-dimensional (2D) superconductors. Our model of the static magnetic response of the arrays does not fully capture the onset of nonlinearity and dissipation with increasing applied field, as these effects are associated with vortex motion due to the dynamic nature of the scanning SQUID susceptometry measurement. This work demonstrates a model 2D superconducting system with engineered disorder and highlights the impact of dissipation on the local magnetic properties of 2D superconductors and Josephson junction arrays.

cond-mat.supr-con↗

arXiv2022

Unidirectional Magnetoresistance in Antiferromagnet/Heavy-metal bilayers

The interplay between electronic transport and antiferromagnetic order has attracted a surge of interest as recent studies have shown that a moderate change in the spin orientation of a collinear antiferromagnet may have a significant effect on the electronic band structure. Among numerous electrical probes to read out such magnetic order, unidirectional magnetoresistance (UMR), where the resistance changes under the reversal of the current direction, can provide rich insights into the transport properties of spin-orbit coupled systems. However, UMR has never been observed in antiferromagnets before, given the absence of intrinsic spin-dependent scattering. Here, we report a UMR in the antiferromagnetic phase of a FeRh$|$Pt bilayer, which undergoes a sign change and then increases strongly with an increasing external magnetic field, in contrast to UMRs in ferromagnetic and nonmagnetic systems. We show that Rashba spin-orbit coupling alone cannot explain the sizable UMR in the antiferromagnetic bilayer and that field-induced spin canting distorts the Fermi contours to greatly enhance the UMR by two orders of magnitude. Our results can motivate the growing field of antiferromagnetic spintronics, and suggest a route to the development of tunable antiferromagnet-based spintronics devices.

cond-mat.mtrl-sci↗

arXiv2021

Large Exotic Spin Torques in Antiferromagnetic Iron Rhodium

Spin torque is a promising tool for driving magnetization dynamics for novel computing technologies. These torques can be easily produced by spin-orbit effects, but for most conventional spin source materials, a high degree of crystal symmetry limits the geometry of the spin torques produced. Magnetic ordering is one way to reduce the symmetry of a material and allow exotic torques, and antiferromagnets are particularly promising because they are robust against external fields. We present spin torque ferromagnetic resonance measurements and second harmonic Hall measurements characterizing the spin torques in antiferromagnetic iron rhodium alloy. We report extremely large, strongly temperature-dependent exotic spin torques with a geometry apparently defined by the magnetic ordering direction. We find the spin torque efficiency of iron rhodium to be (330$\pm$150) % at 170 K and (91$\pm$32) % at room temperature. We support our conclusions with theoretical calculations showing how the antiferromagnetic ordering in iron rhodium gives rise to such exotic torques.

cond-mat.mtrl-sci↗

arXiv2021

Imaging and controlling vortex dynamics in mesoscopic superconductor-normal-metal-superconductor arrays

Harnessing the properties of vortices in superconductors is crucial for fundamental science and technological applications; thus, it has been an ongoing goal to locally probe and control vortices. Here, we use a scanning probe technique that enables studies of vortex dynamics in superconducting systems by leveraging the resonant behavior of a raster-scanned, magnetic-tipped cantilever. This experimental setup allows us to image and control vortices, as well as extract key energy scales of the vortex interactions. Applying this technique to lattices of superconductor island arrays on a metal, we obtain a variety of striking spatial patterns that encode information about the energy landscape for vortices in the system. We interpret these patterns in terms of local vortex dynamics and extract the relative strengths of the characteristic energy scales in the system, such as the vortex-magnetic field and vortex-vortex interaction strengths, as well as the vortex chemical potential. We also demonstrate that the relative strengths of the interactions can be tuned and show how these interactions shift with an applied bias. The high degree of tunability and local nature of such vortex imaging and control not only enable new understanding of vortex interactions, but also have potential applications in more complex systems such as those relevant to quantum computing.

cond-mat.supr-con↗

arXiv2020

Perspective on Metallic Antiferromagnets

Antiferromagnet materials have recently gained renewed interest due to their possible use in spintronics technologies, where spin transport is the foundation of their functionalities. In that respect metallic antiferromagnets are of particular interest, since they enable complex interplays between electronic charge transport, spin, optical, and magnetization dynamics. Here we review phenomena where the metallic conductivity provides unique perspectives for the practical use and fundamental properties of antiferromagnetic materials.

cond-mat.str-el↗

arXiv2020

Observation of an antiferromagnetic quantum critical point in high-purity LaNiO$_3$

Amongst the rare-earth perovskite nickelates, LaNiO$_3$ (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic instability. Our work suggests that LNO is a quantum critical metal, close to an antiferromagnetic quantum critical point (QCP). The QCP behavior in LNO is manifested in epitaxial thin films with unprecedented high purities. We find that the temperature and magnetic field dependences of the resistivity of LNO at low temperatures are consistent with scatterings of charge carriers from weak disorder and quantum fluctuations of an antiferromagnetic nature. Furthermore, we find that the introduction of a small concentration of magnetic impurities qualitatively changes the magnetotransport properties of LNO, resembling that found in some heavy-fermion Kondo lattice systems in the vicinity of an antiferromagnetic QCP.

cond-mat.str-el↗

arXiv2018

Electronic transport in a two-dimensional superlattice engineered via self-assembled nanostructures

Nanoscience offers a unique opportunity to design modern materials from the bottom up, via low-cost, solution processed assembly of nanoscale building blocks. These systems promise electronic band structure engineering using not only the nanoscale structural modulation, but also the mesoscale spatial patterning, although experimental realization of the latter has been challenging. Here we design and fabricate a new type of artificial solid by stacking graphene on a self-assembled, nearly periodic array of nanospheres, and experimentally observe superlattice miniband effects. We find conductance dips at commensurate fillings of charge carriers per superlattice unit cell, which are key features of minibands that are induced by the quasi-periodic deformation of the graphene lattice. These dips become stronger when the lattice strain is larger. Using a tight-binding model, we simulate the effect of lattice deformation as a parameter affecting the inter-atomic hopping integral, and confirm the superlattice transport behavior. This 2D material-nanoparticle heterostructure enables facile band structure engineering via self-assembly, promising for large area electronics and optoelectronics applications.

cond-mat.mes-hall↗

arXiv2018

Strain Modulation of Graphene by Nanoscale Substrate Curvatures: A Molecular View

Spatially nonuniform strain is important for engineering the pseudomagnetic field and band structure of graphene. Despite the wide interest in strain engineering, there is still a lack of control on device-compatible strain patterns due to the limited understanding of the structure-strain relationship. Here, we study the effect of substrate corrugation and curvature on the strain profiles of graphene via combined experimental and theoretical studies of a model system: graphene on closely packed SiO2 nanospheres with different diameters (20-200 nm). Experimentally, via quantitative Raman analysis, we observe partial adhesion and wrinkle features and find that smaller nanospheres induce larger tensile strain in graphene, theoretically, molecular dynamics simulations confirm the same microscopic structure and size dependence of strain and reveal that a larger strain is caused by a stronger, inhomogeneous interaction force between smaller nanospheres and graphene. This molecular-level understanding of the strain mechanism is important for strain engineering of graphene and other two-dimensional materials.

cond-mat.mes-hall↗

arXiv2018

Finite momentum Cooper pairing in 3D topological insulator Josephson junctions

Unconventional superconductivity arising from the interplay between strong spin-orbit coupling and magnetism is an intensive area of research. One form of unconventional superconductivity arises when Cooper pairs subjected to a magnetic exchange coupling acquire a finite momentum. Here, we report on a signature of finite momentum Cooper pairing in the 3D topological insulator Bi2Se3. We apply in-plane and out-of-plane magnetic fields to proximity-coupled Bi2Se3 and find that the in-plane field creates a spatially oscillating superconducting order parameter in the junction as evidenced by the emergence of an anomalous Fraunhofer pattern. We describe how the anomalous Fraunhofer patterns evolve for different device parameters, and we use this to understand the microscopic origin of the oscillating order parameter. The agreement between the experimental data and simulations shows that the finite momentum pairing originates from the coexistence of the Zeeman effect and Aharonov-Bohm flux.

cond-mat.mes-hall↗

arXiv2017

Graphene Transport Mediated by Micropatterned Substrates

Engineered substrates offer a promising avenue towards graphene devices having tunable properties. In particular, topographically patterned substrates can expose unique behavior due to their ability to induce local variations in strain and electrostatic doping. However, to explore the range of possible science and applications, it is important to create topographic substrates which both have tunable features and are suitable for transport measurements. In this Letter we describe the fabrication of tunable, topographically patterned substrates suitable for transport measurements. We report both optical and transport measurements of graphene devices fabricated on these substrates, and demonstrate characteristic strain and local doping behavior induced by the topographic features.

cond-mat.mes-hall↗