arXiv subjects

Nandini Trivedi

Publications and source records attributed to Nandini Trivedi.

At least 73 records · Page 4Linked to original sources

arXiv2018

Local spectroscopies across the superconductor-insulator transition

We explore the manifestation of quantum fluctuations across the superconductor-insulator transition (SIT) in three different local measurements: the two-particle density of states $P(\mathbf{r},ω)$, compressibility $κ(\mathbf{r})$, and diamagnetic susceptibility $χ(\mathbf{r})$. We perform Monte Carlo simulations on the 2D quantum Josephson junction array model and present local maps of these quantities as the system is tuned across the SIT. $P(\mathbf{r},ω)$, obtained using Maximum Entropy analytic continuation techniques, shows strongly diminished zero-energy spectral weight in nearly-insulating islands, that also correlate with regions of suppressed $κ(\mathbf{r})$. We investigate the signatures of quantum fluctuations in the evolution of $κ(\mathbf{r})$ and $χ(\mathbf{r})$ across the SIT, distinct from thermal fluctuations. We discuss the experimental implications of our results for scanning Josephson spectroscopy, compressibility, and scanning SQUID measurements.

cond-mat.supr-con↗

arXiv2018

Magnetotransport in Fe-intercalated \textit{T}S$_2$: the comparison between \textit{T} = Ti and Ta

Sharp magnetization switching and large magnetoresistance were previously discovered in single crystals of 2H-Fe$_x$TaS$_2$ and attributed to the Fe superstructure and its defects. We report similar sharp switching in 1T-Fe$_x$TiS$_2$ ($0.086\;{\leq}\;x\;{\leq}0.703$) and the discovery of large magnetoresistance. The switching field $H_s$ and magnetoresistance are similar to 2H-Fe$_x$TaS$_2$, with a larger than expected bowtie magnetoresistance and a sharp hysteresis loop. Despite previous reports, electron diffraction shows only the $\sqrt{3}{\times}\sqrt{3}$ superstructure in 1T-Fe$_x$TiS$_2$. The Curie and Weiss temperatures remain roughly constant below $x~\sim~1/3$ before monotonically increasing for higher x. By contrast, the switching field and magnetoresistance reach a maximum where defects in the superstructure exist, approach a minimum near perfect superstructures, and remain constant above $x~\sim~ 0.4$. Additionally, an increase in $H_s$ with annealing time is reported. Glassy behavior is shown to coexist within the ferromagnetic state in 1T-Fe$_x$TiS$_2$ for compositions between $0.1$ and $0.703$. A simple model captures the essential phenomenology and explains most similarities and differences between 1T-Fe$_x$TiS$_2$ and 2H-Fe$_x$TaS$_2$, and provides insights into other magnetically intercalated transition metal dichalcogenides.

cond-mat.str-el↗

arXiv2018

Topological magnons with nodal-line and triple-point degeneracies: Implications for thermal Hall effect in pyrochlore iridates

We analyze the magnon excitations in pyrochlore iridates with all-in-all-out (AIAO) antiferromagnetic order, focusing on their topological features. We identify the magnetic point group symmetries that protect the nodal-line band crossings and triple-point degeneracies that dominate the Berry curvature. We find three distinct regimes of magnon band topology, as a function of the ratio of Dzyaloshinskii-Moriya (DM) interaction to the antiferromagnetic exchange. We show how the thermal Hall response provides a unique probe of the topological magnon band structure in AIAO systems.

cond-mat.str-el↗

arXiv2018

Disorder induced power-law gaps in an insulator-metal Mott transition

A correlated material in the vicinity of an insulator-metal transition (IMT) exhibits rich phenomenology and variety of interesting phases. A common avenue to induce IMTs in Mott insulators is doping, which inevitably leads to disorder. While disorder is well known to create electronic inhomogeneity, recent theoretical studies have indicated that it may play an unexpected and much more profound role in controlling the properties of Mott systems. Theory predicts that disorder might play a role in driving a Mott insulator across an IMT, with the emergent metallic state hosting a power law suppression of the density of states (with exponent close to 1; V-shaped gap) centered at the Fermi energy. Such V-shaped gaps have been observed in Mott systems but their origins are as yet unknown. To investigate this, we use scanning tunneling microscopy and spectroscopy to study isovalent Ru substitutions in Sr$_3$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$ which drives the system into an antiferromagnetic, metallic state. Our experiments reveal that many core features of the IMT such as power law density of states, pinning of the Fermi energy with increasing disorder, and persistence of antiferromagnetism can be understood as universal features of a disordered Mott system near an IMT and suggest that V-shaped gaps may be an inevitable consequence of disorder in doped Mott insulators.

cond-mat.str-el↗

arXiv2018

Nernst Thermopower of Time-Reversal Breaking Type-II Weyl Semimetals

Weyl semimetals host linear energy dispersions around Weyl nodes, as well as monopoles of Berry curvature in momentum space around these points. These features give rise to unique transport signatures in a Weyl semimetal, such as transverse transport without an applied magnetic field, known as anomalous transport. The type-II Weyl semimetal, recently experimentally demonstrated in several materials, is classified by a tilting of the Weyl nodes. This paper provides a theoretical study on thermoelectric transport in time-reversal breaking type-II Weyl semimetals. Our results examine the balance between anomalous and non-anomalous contributions to the Nernst effect when subject to an external magnetic field. We also show how increasing scattering times have on enhancing effect on thermoelectric transport in these materials. Since a temperature-dependent chemical potential has been theoretically shown to be paramount when considering anomalous transport, we also study how similar considerations impact the Nernst thermopower in the non-anomalous case.

cond-mat.mes-hall↗

arXiv2018

Two-particle spectral function for disordered s-wave superconductors: local maps and collective modes

We make the first testable predictions for the local two-particle spectral function of a disordered s-wave superconductor, probed by scanning Josephson spectroscopy (sjs), providing complementary information to scanning tunneling spectroscopy (sts). We show that sjs provides a direct map of the local superconducting order parameter that is found to be anticorrelated with the gap map obtained by sts. Furthermore, this anticorrelation increases with disorder. For the momentum resolved spectral function, we find the Higgs mode shows a non-dispersive subgap feature at low momenta, spectrally separated from phase modes, for all disorder strengths. The amplitude-phase mixing remains small at low momenta even when disorder is large. Remarkably, even for large disorder and high momenta, the amplitude-phase mixing oscillates rapidly in frequency and hence do not affect significantly the purity of the Higgs and phase dominated response functions.

cond-mat.str-el↗

arXiv2017

Localized-itinerant dichotomy and unconventional magnetism in SrRu$_2$O$_6$

Electron correlations tend to generate local magnetic moments that usually order if the lattices are not too frustrated. The hexagonal compound SrRu$_2$O$_6$ has a relatively high Neel temperature but small local moments, which seem to be at odds with the nominal valence of Ru$^{5+}$ in the $t_{2g}^3$ configuration. Here, we investigate the electronic property of SrRu$_2$O$_6$ using density functional theory (DFT) combined with dynamical-mean-field theory (DMFT). We find that the strong hybridization between Ru $d$ and O $p$ states results in a Ru valence that is closer to $+4$, leading to the small ordered moment $\sim1.2μ_B$. While this is consistent with a DFT prediction, correlation effects are found to play a significant role. The local moment per Ru site remains finite $\sim2.3μ_B$ in the whole temperature range investigated. Due to the lower symmetry, the $t_{2g}$ manifold is split and the quasiparticle weight is renormalized significantly in the $a_{1g}$ state, while the renormalization in $e_g'$ states is about a factor of 2--3 weaker. Our theoretical Neel temperature $\sim700$~K is in reasonable agreement with experimental observations. SrRu$_2$O$_6$ is a unique system in which localized and itinerant electrons coexist with the proximity to an orbitally-selective Mott transition within the $t_{2g}$ sector.

cond-mat.str-el↗

arXiv2017

The semiclassical theory of anomalous transport in type-II topological Weyl semimetals

Weyl semimetals possess low energy excitations which act as monopoles of Berry curvature in momentum space. These emergent monopoles are at the heart of the extensive novel transport properties that Weyl semimetals exhibit. The singular nature of the Berry curvature around the nodal points in Weyl semimetals allows for the possibility of large anomalous transport coefficients in zero applied magnetic field. Recently a new class, termed type-II Weyl semimetals, has been demonstrated in a variety of materials, where the Weyl nodes are tilted. We present here a study of anomalous transport in this new class of Weyl semimetals. We find that the parameter governing the tilt of these type-II Weyl points is intimately related to the zero field transverse transport properties. We also find that the temperature dependence of the chemical potential plays an important role in determining how the transport coefficients can effectively probe the Berry curvature of the type-II Weyl points. We also discuss the experimental implications of our work for time-reversal breaking type-II Weyl semimetals.

cond-mat.mes-hall↗

arXiv2017

Dirac dispersion generates large Nernst effect in Weyl semimetals

Weyl semimetals expand research on topologically protected transport by adding bulk Berry monopoles with linearly dispersing electronic states and topologically robust, gapless surface Fermi arcs terminating on bulk node projections. Here, we show how the Nernst effect, combining entropy with charge transport, gives a unique signature for the presence of Dirac bands. The Nernst thermopower of NbP (maximum of 800 microV K-1 at 9 T, 109 K) exceeds its conventional thermopower by a hundredfold and is significantly larger than the thermopower of traditional thermoelectric materials. The Nernst effect has a pronounced maximum near T_M=90 +/- 20 K=mu_0/kB (mu_0 is chemical potential at T=0 K). A self-consistent theory without adjustable parameters shows that this results from electrochemical potential pinning to the Weyl point energy at T>=TM, driven by charge neutrality and Dirac band symmetry. Temperature and field dependences of the Nernst effect, an even function of the charge polarity, result from the intrinsically bipolar nature of the Weyl fermions. Through this study, we offer an understanding of the temperature dependence of the position of the electrochemical potential vis-a-vis the Weyl point, and we show a direct connection between topology and the Nernst effect, a potentially robust experimental tool for investigating topological states and the chiral anomaly.

cond-mat.mes-hall↗

arXiv2017

Temperature-driven BCS-BEC crossover in a coupled boson-fermion system

We propose a simple bose-fermi model in two dimensions, with a coupling that converts pairs of opposite spin fermions into localized bosons and vice versa. We show that tracing out one of the degrees, either the bosons or fermions, generates temperature-dependent long range effective interactions between bosons as well as effective attractive interactions between fermions. Using Monte Carlo techniques we obtain the thermodynamic properties and phase stiffness as a function of temperature, dominated by vortex-antivortex unbinding of the bosons. Remarkably in the fermion sector we observe a temperature-induced BCS-BEC crossover signaled by a distinct change of their spectral properties: the minimum gap locus moves from the Fermi wave vector to the $Γ$ point. Such a model is relevant for describing aspects of high $T_c$ superconductivity in cuprates and pnictides, superconducting islands on graphene, and bose-fermi mixtures in cold atomic systems.

cond-mat.supr-con↗

arXiv2017

Fermi arc mediated entropy transport in topological semimetals

In topological Weyl semimetals, the low energy excitations are comprised of linearly dispersing Weyl fermions, which act as monopoles of Berry curvature in momentum space and result in topologically protected Fermi arcs on the surfaces. We propose that these Fermi arcs in Weyl semimetals lead to an anisotropic magnetothermal conductivity, strongly dependent on externally applied magnetic field and resulting from entropy transport driven by circulating electronic currents. The circulating currents result in no net charge transport, but they do result in a net entropy transport. This translates into a magnetothermal conductivity that should be a unique experimental signature for the existence of the arcs. We analytically calculate the Fermi arc-mediated magnetothermal conductivity in the low-field semiclassical limit as well as in the high-field ultra-quantum limit, where only the chiral Landau levels are involved. By numerically including the effects of higher Landau levels, we show how the two limits are linked at intermediate magnetic fields. This work provides the first proposed signature of Fermi arc-mediated thermal transport and sets the stage for utilizing and manipulating the topological Fermi arcs in experimental thermal applications.

cond-mat.mes-hall↗

arXiv2017

Orbital and spin order in spin-orbit coupled $d^1$ and $d^2$ double perovskites

We consider strongly spin-orbit coupled double perovskites A$_2$BB'O$_6$ with B' magnetic ions in either $d^1$ or $d^2$ electronic configuration and non-magnetic B ions. We provide insights into several experimental puzzles, such as the predominance of ferromagnetism in $d^1$ versus antiferromagnetism in $d^2$ systems, the appearance of negative Curie-Weiss temperatures for ferromagnetic materials, and the size of effective magnetic moments. We develop and solve a microscopic model with both spin and orbital degrees of freedom within the Mott insulating regime at finite temperature using mean field theory. The interplay between anisotropic orbital degrees of freedom and spin-orbit coupling results in complex ground states in both $d^1$ and $d^2$ systems. We show that the ordering of orbital degrees of freedom in $d^1$ systems results in coplanar canted ferromagnetic and 4-sublattice antiferromagnetic structures. In $d^2$ systems we find additional colinear antiferromagnetic and ferromagnetic phases not appearing in $d^1$ systems. At finite temperatures, we find that orbital ordering driven by both superexchange and Coulomb interactions may occur at much higher temperatures compared to magnetic order and leads to distinct deviations from Curie-Weiss law.

cond-mat.str-el↗

arXiv2016

Observation of canted antiferromagnetism with ultracold fermions in an optical lattice

Understanding the magnetic response of the normal state of the cuprates is considered a key piece in solving the puzzle of their high-temperature superconductivity. The essential physics of these materials is believed to be captured by the Fermi-Hubbard model, a minimal model that has been realized with cold atoms in optical lattices. Here we report on site-resolved measurements of the Fermi-Hubbard model in a spin-imbalanced atomic gas, allowing us to explore the response of the system to large effective magnetic fields. We observe short-range canted antiferromagnetism at half-filling with stronger spin correlations in the direction orthogonal to the magnetization, in contrast with the spin-balanced case where identical correlations are measured for any projection of the pseudospin. The rotational anisotropy of the spin correlators is found to increase with polarization and with distance between the spins. Away from half-filling, the polarization of the gas exhibits non-monotonic behavior with doping for strong interactions, resembling the behavior of the magnetic susceptibility in the cuprates. We compare our measurements to predictions from Determinantal Quantum Monte Carlo (DQMC) and Numerical Linked Cluster Expansion (NLCE) algorithms and find good agreement. Calculations on the doped system are near the limits of these techniques, illustrating the value of cold atom quantum simulations for studying strongly-correlated materials.

cond-mat.quant-gas↗

arXiv2016

Entanglement and corner Hamiltonian spectra of integrable open spin chains

Entanglement spectra (ES) for the critical SU(N) (2 <= N <= 4) spin chains and other integrable models of finite length are studied with the density matrix renormalization group method. For all models under investigation, the level spacings and the degeneracy structure of the ES are in excellent agreement with the spectra of the corner Hamiltonian, defined as the generator of the associated corner transfer matrix. The correspondence holds between the ES (n) at the n-th cut position from the edge of the spin model, and the corner Hamiltonian of length n, for all small values of n. The cut position dependence of the ES shows a period-N oscillatory behavior for a given SU(N) chain, reminiscent of the oscillatory part of the entanglement entropy observed in the past for the same models. Oscillations of the ES do not die out in the bulk of the chain, in contrast to the asymptotically vanishing oscillation of the entanglement entropy. Heuristic argument based on Young tableaux consideration can explain the period-N structure of the ES qualitatively.

cond-mat.str-el↗

arXiv2016

Effective magnetic interactions in spin-orbit coupled $d^4$ Mott insulators

Transition metal compounds with the $(t_{2g})^4$ electronic configuration are expected to be nonmagnetic atomic singlets both in the weakly interacting regime due to spin-orbit coupling, as well as in the Coulomb dominated regime with oppositely aligned $L=1$ and $S=1$ angular momenta. However, starting with the full multi-orbital electronic Hamiltonian, we show the low energy effective magnetic Hamiltonian contains isotropic superexchange spin interactions but anisotropic orbital interactions. By tuning the ratio of superexchange to spin-orbit coupling $J_\mathrm{SE}/λ$, we obtain a phase transition from nonmagnetic atomic singlets to novel magnetic phases depending on the strength of Hund's coupling, the crystal structure and the number of active orbitals. Spin-orbit coupling plays a non-trivial role in generating a triplon condensate of weakly interacting excitations at antiferromagnetic ordering vector $\vec k=\vec π$, regardless of whether the local spin interactions are ferromagnetic or antiferromagnetic. In the large $J_\mathrm{SE} / λ$ regime, the localized spin and orbital moments produce anisotropic orbital interactions that are frustrated or constrained even in the absence of geometric frustration. Orbital frustration leads to frustration in the spin channel opening up the possibility of spin-orbital liquids with both spin and orbital entanglement.

cond-mat.str-el↗

arXiv2016

Observation of Spatial Charge and Spin Correlations in the 2D Fermi-Hubbard Model

Strong electron correlations lie at the origin of transformative phenomena such as colossal magneto-resistance and high-temperature superconductivity. Already near room temperature, doped copper oxide materials display remarkable features such as a pseudo-gap and a "strange metal" phase with unusual transport properties. The essence of this physics is believed to be captured by the Fermi-Hubbard model of repulsively interacting, itinerant fermions on a lattice. Here we report on the site-resolved observation of charge and spin correlations in the two-dimensional (2D) Fermi-Hubbard model realized with ultracold atoms. Antiferromagnetic spin correlations are maximal at half-filling and weaken monotonically upon doping. Correlations between singly charged sites are negative at large doping, revealing the Pauli and correlation hole\textemdash a suppressed probability of finding two fermions near each other. However, as the doping is reduced below a critical value, correlations between such local magnetic moments become positive, signaling strong bunching of doublons and holes. Excellent agreement with numerical linked-cluster expansion (NLCE) and determinantal quantum Monte Carlo (DQMC) calculations is found. Positive non-local moment correlations directly imply potential energy fluctuations due to doublon-hole pairs, which should play an important role for transport in the Fermi-Hubbard model.

cond-mat.quant-gas↗

arXiv2016

Strain-induced topological transition in SrRu$_2$O$_6$ and CaOs$_2$O$_6$

The topological property of SrRu$_2$O$_6$ and isostructural CaOs$_2$O$_6$ under various strain conditions is investigated using density functional theory. Based on an analysis of parity eigenvalues, we anticipate that a three-dimensional strong topological insulating state should be realized when band inversion is induced at the A point in the hexagonal Brillouin zone. For SrRu$_2$O$_6$, such a transition requires rather unrealistic tuning, where only the $c$ axis is reduced while other structural parameters are unchanged. However, given the larger spin-orbit coupling and smaller lattice constants in CaOs$_2$O$_6$, the desired topological transition does occur under uniform compressive strain. Our study paves a way to realize a topological insulating state in a complex oxide, which has not been experimentally demonstrated so far.

cond-mat.str-el↗

arXiv2016

Minimal models for topological Weyl semimetals

Topological Weyl semimetals (TWS) can be classified as type-I TWS, in which the density of states vanishes at the Weyl nodes, and type-II TWS where an electron and a hole pocket meet with finite density of states at the nodal energy. The dispersions of type-II Weyl nodes are tilted and break Lorentz invariance, allowing for physical properties distinct from those in a type-I TWS. We present minimal lattice models for both time-reversal-breaking and inversion-breaking type-II Weyl semimetals, and investigate their bulk properties and topological surface states. These lattice models capture the extended Fermi pockets and the connectivities of Fermi arcs. In addition to the Fermi arcs, which are topologically protected, we identify surface "track states" that arise out of the topological Fermi arc states at the transition from type-I to type-II with multiple Weyl nodes, and persist in the type-II TWS.

cond-mat.mes-hall↗