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Naoto Nagaosa

Publications and source records attributed to Naoto Nagaosa.

At least 19 recordsLinked to original sources

Phase-Space Quantum Geometry Beyond Adiabatic Electron Dynamics

The geometry of electronic quantum states plays an important role in the equilibrium and transport properties of solids. While the Berry curvature is known to influence electron motion, recent work has shown that the quantum metric also affects the motion of electron wave packets beyond the adiabatic approximation. To connect this nonadiabatic dynamics to many-electron observables, we derive an equivalent semiclassical formulation, valid up to second order in $\hbar$. The resulting phase-space measure and kinetic equation incorporate the quantum metric over the full phase space, including its mixed real-momentum components. We show that, in spatially inhomogeneous systems, the full phase-space quantum metric contributes to electric polarization in insulators and generates an intrinsic linear Hall response in metals. As a concrete example, we study Dirac electrons subject to a magnetic texture and a background potential that vary periodically in space. In this model, the mixed components of the phase-space metric produce a Hall contribution controlled by the relative phase between the two modulations. This phase-sensitive response can remain finite even when the conventional anomalous Hall conductivity vanishes. More broadly, our formulation enables the systematic study of equilibrium and transport responses in systems whose quantum geometry involves both position and momentum.

cond-mat.mes-hall↗

Spin nematic liquid crystal and scalar spin chirality in tetragonal lattice YbMnBi$_2$

A spin nematic order, analogous to the nematic liquid crystal, characterizes the spontaneous breaking of spin-space rotational symmetry while preserving time-reversal ($T$) symmetry. In contrast, scalar spin chirality (SSC), a composite three-spin order, breaks $T$ symmetry and is known to induce an anomalous Hall effect (AHE). Although a spin nematic phase has been suggested in frustrated magnets and the square-lattice iridate, how it might affect magnetotransport properties is unknown. Here we use polarized neutron scattering to show that tetragonal $A$MnBi$_2$ ($A$ = Ca, Yb) is a strictly $c$-axis-aligned collinear antiferromagnet (C-type), with $T_N \approx 270$ K and 290 K, respectively. On cooling from 450 K to $T_N$, low-energy spin excitations in YbMnBi$_2$ spontaneously change from isotropic to anisotropic in spin space within the tetragonal plane, forming a dynamic spin nematic phase around 400 K due to heavy Yb-induced spin-orbit coupling, before gapping out below $T_N$. Similar measurements on CaMnBi$_2$ reveal isotropic paramagnetic scattering without a spin nematic phase above $T_N$. Under an in-plane magnetic field, the Yb$^{3+}$ moments may interact with the dynamic spin nematic phase to induce nonzero SSC, giving rise to AHE and an anomalous Nernst effect (ANE) in YbMnBi$_2$ that are absent in CaMnBi$_2$ above $T_N$. A symmetry-based Ginzburg-Landau analysis shows that coupling terms between the nematic order and SSC are allowed under an external magnetic field, which could explain the rapid increase of AHE with field in YbMnBi$_2$. Our results provide compelling evidence for dynamic SSC-induced AHE and ANE in the paramagnetic phase of a compensated collinear antiferromagnet, opening a new avenue for the physics of composite spin orders and room-temperature spintronics without magnetic order.

cond-mat.str-el↗

Anomalous temperature dependence of polaron mobility in a nonlinear double-well potential: unbiased X-propagator approach

We develop an unbiased X-propagator method for calculating finite-temperature optical conductivity $σ(ω)$ and dc mobility $μ$ for arbitrary nonlinear electron-phonon interaction. We apply it to a polaron coupled to a double-well lattice potential, a minimal model for strongly anharmonic polar materials. At moderate coupling, the mobility exhibits three temperature regimes associated with confinement within one well, thermal competition with the barrier, and barrier-insensitive high-temperature dynamics. This sequence produces a concave temperature dependence of the mobility that is absent in conventional linear-coupling polaron models. At strong coupling, the mobility becomes nonmonotonic, and its temperature evolution is reflected in a characteristic redistribution of optical spectral weight. For parameters relevant to SrTiO$_3$, our results qualitatively reproduce both the anomalous concave mobility and the onset of violation of the Mott-Ioffe-Regel limit, thereby supporting nonlinear coupling to a soft anharmonic lattice mode as a microscopic mechanism for anomalous transport in dilute polar metals.

cond-mat.str-el↗

Theory of Little-Parks oscillations by vortices in two-dimensional superconductors

The Little-Parks (LP) effect is a quantum phenomenon in which the superconducting transition temperature of a superconducting cylinder (or ring) oscillates periodically as a function of the magnetic flux threading the loop. Recently, multiple experiments have observed half-quantum flux shifts in measurements of LP oscillations, where the oscillations are globally shifted by half a flux quantum compared to conventional cases, a behavior referred to as a $π$-ring. Such observations are commonly linked to unconventional pairing symmetries. In this work, we demonstrate that half-quantum flux shifts can arise in two-dimensional (2D) superconducting rings without invoking unconventional pairing symmetry, provided that vortices near the Berezinskii-Kosterlitz-Thouless (BKT) transition are taken into account. Specifically, based on the vortex-charge duality theory near the BKT transition, we map the problem onto a Coulomb gas model, in which the magnetic flux is represented as a pair of opposite boundary charges (or vortices) at the two edges. The screening of these boundary charges by thermally excited vortex-antivortex pairs is investigated through explicit Monte Carlo simulations. Importantly, we demonstrate that the oscillation of the free-vortex density as a function of magnetic flux can exhibit an anomalous half-quantum flux shift. Our work thus predicts the LP oscillations induced by vortices in 2D superconducting rings near the BKT transition, which provides a new mechanism for generating $π$-rings.

cond-mat.supr-con↗

Quantum Brownian Motion: proving that the Schmid transition belongs to the Berezinskii-Kosterlitz-Thouless universality class

We investigate the equilibrium properties of a quantum Brownian particle moving in a periodic potential, specifically addressing the nature of the dissipation-driven Schmid transition in the Ohmic regime. By employing World-Line Monte Carlo in the path-integral formalism and introducing a specific binary order parameter, we demonstrate that the transition belongs to the Berezinskii-Kosterlitz-Thouless universality class. This classification is substantiated through finite-size scaling analysis that reveals the characteristic logarithmic decay of the correlation functions associated with the order parameter at the critical point. Quantum phase transition turns out to be extremely fragile: it disappears in both over- and sub-Ohmic dissipation regimes. Crucially, we find that the presence of the periodic potential does not alter the localization properties in the sub-Ohmic and super-Ohmic regimes, where the system exhibits the same qualitative behavior as the free quantum Brownian particle. These findings highlight that the emergence of critical behavior is strictly governed by the low-frequency form of the environmental spectral function, which determines the long-range temporal decay of the dissipative kernel.

cond-mat.stat-mech↗

Visualizing Microwave-Driven Dynamics of Antiskyrmions and Surface Skyrmions

Microwaves provide coherent access to low-energy excitations and serve as effective probes of high-frequency spin dynamics in quantum and magnetic systems. For topological spin textures, microwave excitation is expected to generate rich collective responses, yet direct real-space observation of ultrafast dynamics remains limited. Here we use time-resolved Lorentz transmission electron microscopy to visualize microwave-driven dynamics in a hybrid antiskyrmion structure composed of a central antiskyrmion and surface skyrmions. We resolve the picosecond evolution of antiskyrmion area and second-harmonic signals, evidencing nonlinear responses of spin textures under microwave excitations. We track the core motions of the antiskyrmion and surface skyrmions, which follow distinct trajectories while sharing the same rotational sense. Micromagnetic simulations reproduce the key observations and associate the dynamic modes with the spatial modulation of the core profile along the thickness. These achievements establish ultrafast electron microscopy as a powerful real-space approach for probing high-frequency microwave-driven dynamics of topological magnetic solitons.

cond-mat.mtrl-sci↗

Emergent toroidal induction in a polar Weyl ferromagnet

Spin-orbit coupling (SOC) underpins modern spintronics by enabling the electrical generation of spin torques. Its reciprocal counterpart, in which magnetization dynamics produce electromotive forces through a spin-dependent Berry phase, is known as emergent electromagnetic induction (EEMI). However, this effect has previously been observed only in magnetic textures with spatial gradients, such as domain walls, helices, and skyrmions. Here, we demonstrate that even a spatially uniform ferromagnet can host EEMI through a previously unrecognized Berry-phase mechanism inherent to noncentrosymmetric conductors. In the polar Weyl ferromagnet PrAlGe, an applied alternating current generates spin-orbit torques that drive collective magnetization dynamics. The resulting emergent toroidal moment (T = P \times M), where (P) is the crystal's polar axis and (M) is the net magnetization, acts as a gauge potential whose time derivative (dT/dt) induces a Hall voltage. This contribution appears specifically in the out-of-phase component of the AC Hall response and scales linearly with frequency, providing direct evidence for EEMI. First-principles calculations further reveal that this toroidal vector encodes the collective motion of Weyl nodes in momentum space. These findings establish "emergent toroidal induction" as a new manifestation of spin-orbit entanglement, unifying Berry phase, topology, and spin dynamics while opening a pathway toward intrinsic and energy-efficient spin-charge interconversion.

cond-mat.mtrl-sci↗

Universal Scaling of the Spin Hall Effect

We study the spin Hall (SH) effect for the Dirac electrons in terms of the spin and magnetic-moment accumulation coefficients $-Γ^{00} g_{s(m)z}^{\phantom{s(m)z} xy}$. We take short-range nonmagnetic impurities into account within the self-consistent $T$-matrix approximation. Similarly to the universal scaling for the anomalous Hall (AH) effect, we find three disctinct regimes by changing the electric conductivity $σ^{yy}$; the superclean regime with $-Γ^{00} g_{s(m)z}^{\phantom{s(m)z} xy} \propto σ^{yy}$ owing to the skew scattering, moderately dirty regime with almost constant $-Γ^{00} g_{s(m)z}^{\phantom{s(m)z} xy}$, and dirty regime with a new scaling relation $-Γ^{00} g_{s(m)z}^{\phantom{s(m)z} xy} \propto (σ^{yy})^{0.6}$ whose exponent differs from that of the AH conductivity. Our results construct a unified theory of the SH effect without any ambiguity of spin current.

cond-mat.mes-hall↗

Riemannian geometric classification and emergent phenomena of magnetic textures

We propose a new classification of magnetic textures from the viewpoint of differential geometry. Magnetic textures are conventionally classified into collinear, coplanar, and noncoplanar magnets. These classes are typically characterized by the vector spin chirality (VSC) and the scalar spin chirality (SSC), which indicate noncollinearity and noncoplanarity, respectively. However, this conventional classification is incomplete: in particular, noncoplanar textures cannot be fully characterized by the SSC alone, as exemplified by conical magnets. To refine this classification, we analyze the curves and surfaces traced by spins in real space using differential geometry and introduce two novel scalar spin chiralities that properly characterize noncoplanarity: the geodesic scalar spin chirality and the torsional scalar spin chirality. These quantities are directly connected to differential geometry: the former reflects the geodesic curvature while the latter is related to the torsion. Based on these chiralities, we identify three distinct classes of noncoplanar magnetic textures. Furthermore, analogous to the roles of the VSC and the conventional SSC in emergent electrodynamics, the geodesic SSC gives rise to novel emergent phenomena. By constructing a semiclassical theory including nonadiabatic effects and higher-order spatial gradients of magnetic textures, we demonstrate that the geodesic SSC induces an emergent band asymmetry, leading to nonreciprocal responses as a quantum geometric effect. This mechanism is a purely orbital effect, requiring no spin-orbit coupling, and the resulting discussion runs in parallel with the conventional picture of the topological Hall effect driven by the SSC. The geometric viewpoint developed here will provide broad new insights into classification, quantum geometry, emergent electrodynamics, and a wider variety of emergent phenomena.

cond-mat.mtrl-sci↗

Surface-switchable nonreciprocity protected by Fermi arcs in Weyl semimetal TaAs

Weyl semimetals host topologically protected surface states, known as Fermi arcs, which connect bulk Weyl nodes in momentum space. Both bulk Weyl nodes and Fermi arcs are anticipated to be chiral. The chirality of bulk bands has been confirmed through observations of the chiral anomaly and Weyl orbits. In contrast, despite their discovery more than a decade ago, the chiral nature of Fermi arcs has remained unresolved. Here we report Fermi-arc-induced nonlinear transport in the archetypal Weyl semimetal TaAs. Using focused ion beam techniques, we fabricated micro-scale devices that enable simultaneous transport measurements on opposing topological surfaces. While linear transport remains dominated by bulk conduction, nonlinear transport uncovers surface-specific contributions, including an exceptionally large third-order nonreciprocal response that exceeds conventional expectations and highlights the crucial role of the singular arc endpoints. Our findings unambiguously demonstrate the chiral nature of Fermi arcs and establish nonlinear transport as a direct probe of these topological surface states. By revealing a surface-switchable, room-temperature nonlinear response that is topologically protected, this work introduces a new functionality in Weyl semimetals. Given the abundance of natural materials predicted to host topological semimetal states, these results open opportunities for exploring nonlinear transport phenomena and device concepts across a broad class of systems.

cond-mat.mes-hall↗

Quantum Information Geometry of Multicomponent Superconducting Fluctuation Transport

Quantum geometry underlies many electronic responses, but its transport signatures have so far been established mainly for pure single-particle Bloch states. Whether collective many-body fluctuations possess a measurable quantum geometry remains largely unexplored. Here we show that superconducting fluctuation transport provides a direct probe of quantum information geometry in collective many-body matter. Starting from a multicomponent time-dependent Ginzburg-Landau theory in the Gaussian fluctuation regime, we identify the equilibrium density matrix of fluctuating Cooper pairs as the static pair propagator, which defines a positive mixed-state manifold in momentum space. The geometry of this manifold is directly measurable through paraconductivity: the longitudinal paraconductivity is governed by the quantum Fisher information of superconducting fluctuation modes, while the fluctuational anomalous Hall effect is governed by the mean Uhlmann curvature, the mixed-state counterpart of Berry curvature. This correspondence further yields geometric bounds between these two transport components, with no direct analogue in normal electronic transport. Applied to chiral superconducting fluctuations in quarter-metal systems motivated by rhombohedral multilayer graphene, a symmetry-allowed Lifshitz invariant generates finite mean Uhlmann curvature and logarithmically enhances the anomalous Hall conductivity above the critical temperature. Our results establish collective superconducting fluctuations as an experimentally accessible transport probe of mixed-state quantum information geometry.

cond-mat.mes-hall↗

Emergent Quantum-Geometric Equivalence of Injection and Shift Currents

Injection and shift currents are generally regarded as distinct nonlinear optical responses with separate microscopic origins. Here, we uncover a general hidden connection between them through interband Berry-curvature and quantum-metric dipoles. In systems with approximately linear electronic dispersion near the Fermi level and at low photon energies, this relation sharpens into an emergent equivalence, with injection and shift currents governed by the same interband quantum-geometric dipole. This regime is naturally realized in Dirac and Weyl semimetals, as well as in strained graphene, where measurements of injection and shift currents probe a unified geometric property of the electronic wavefunctions rather than distinct dynamical processes. Our results establish a new framework for interpreting nonlinear optical experiments and suggest that quantum geometry may provide a broader organizing principle linking seemingly distinct nonlinear optical responses in solids.

cond-mat.mes-hall↗

Berry curvature and field-induced intrinsic anomalous Hall effect in an antiferromagnet FeTe

Berry curvature is ubiquitous in condensed matter physics and materials science. Its main consequence is the intrinsic anomalous Hall effect (AHE) in magnetic materials and plays a pivotal role in spintronic applications and quantum technologies. Here, we present a theoretical study of the intrinsic AHE in tetragonal FeTe, a semimetallic van der Waals antiferromagnet with compensated magnetic ordering at low temperatures. Using a realistic spin-fermion model, we demonstrate that FeTe exhibits a large Berry-curvature-driven AHE under an applied magnetic field. Our calculations reveal that the Hall conductivity of this compound is extremely sensitive to temperature and field strength and even exhibits sign reversal, highlighting FeTe as a prototypical platform where magnetism and topology combine to produce robust intrinsic Hall responses. This work establishes FeTe as a promising candidate for exploring quantum transport in low-dimensional correlated systems. We also discuss the implications for recent experimental results of the AHE and ordinary Hall effect reported for FeTe.

cond-mat.mtrl-sci↗

Nonmonotonic Scaling of the Anomalous Hall Effect in a Bicollinear Antiferromagnet

An anomalous Hall effect (AHE) in antiferromagnetic (AF) systems with no net magnetization is of considerable interest for both fundamental physics and spintronic applications. Of particular interest is the two-dimensional van der Waals antiferromagnet FeTe that has an unusual fully magnetically compensated bicollinear AF structure and exhibits pronounced Kondo interaction leading to strong band renormalization. Here, we investigate the AHE in epitaxial FeTe thin films grown by molecular beam epitaxy. A large anomalous Hall conductivity is exhibited below the Neel temperature (T_N ~ 60 K) and, strikingly, becomes nonlinear at high fields within a narrow temperature window around 49 K, deviating from conventional AHE scaling behavior versus its longitudinal conductivity. Linear fits reveal a pronounced negative peak in the intercept, accompanied by a field-induced canted magnetic moment. The AHE responses are related to the Berry curvature derived from FeTe's topological band structure, highlighting the intricate interplay between topology, magnetism, and electronic transport.

cond-mat.mtrl-sci↗

Quantum Fisher information in many-photon states from shift current shot noise

Quantum Fisher information (QFI) sets the ultimate precision of optical phase measurements and reveals multiphoton entanglement, but it is not accessible with conventional photodetection. We theoretically predict that a photodetector utilizing the shot noise of the quantum-geometric shift current of exciton polaritons can directly measure the QFI of nonclassical light. By solving the Lindblad equation, we obtain the time-dependent nonlinear photocurrent for an arbitrary initial photon state. It turns out that, regardless of the quantum state of the incident light, the integrated current depends only on the mean photon number. In stark contrast, the shot noise retains the quantum information: its Fano factor is proportional to the photon number variance and therefore encodes the QFI. Numerical calculations confirm these relations for illumination with optical Schrödinger cat and squeezed vacuum states. Quantum correlations in nonclassical light, usually hidden from direct detection, become observable in the form of shift current shot noise

cond-mat.mes-hall↗

Topological pumping of bimerons in spiral magnets

Precise positioning of topological defects is essential for racetrack memories, where their positions along a magnetic nanotrack encode information. Traditional methods achieve nanometric precision by engineering pinning landscapes that enforce discrete steps in defect motion. However, accessing each bit requires overcoming a depinning threshold, which increases power consumption. Here, we demonstrate that spiral magnets provide a natural ruler, enabling precise positioning of bimerons (topological spin textures analogous to skyrmions) without relying on engineered pinning sites. A rotating magnetic field couples directly to the bimeron position, displacing it by exactly one spiral period per full rotation of the field. Such quantized transport of skyrmionic textures, reminiscent of Thouless pumping, is topologically protected and remains robust against perturbations, positioning spiral magnets as a natural skyrmion racetrack. The findings establish a paradigm for topologically protected transport of spin textures.

cond-mat.str-el↗

Role of Ward-Takahashi identity in an electron-phonon coupled system -- Revisiting phonon shift current

We study bulk photovoltaic effects in electron-phonon coupled systems. The conservation of current or gauge invariance, manifested as the Ward-Takahashi identity, plays an essential role in the analysis of the Feynman diagrams, and the leading order contribution to the phonon shift current is identified accordingly. The leading order contribution essentially arises from the electric polarization carried by optically excited phonons, where the shift current is generated due to a change of electric polarization in the steady state under the optical excitation of phonons.

cond-mat.str-el↗

Wavefunction-Free Approach for Predicting Nonlinear Responses in Weyl Semimetals

By sidestepping the intractable calculations of many-body wavefunctions, density functional theory (DFT) has revolutionized the prediction of ground states of materials. However, predicting nonlinear responses--critical for next-generation quantum devices--still relies heavily on explicit wavefunctions, limiting computational efficiency. In this letter, using the circular photogalvanic effect (CPGE) in Weyl semimetals as a representative example, we realize a 1000-fold computational speedup by eliminating the explicit dependence on wavefunctions. Our approach leverages the one-to-one correspondence between free parameters of Weyl fermions and the associated responses to obtain precise wavefunction-free formulations. Applying our methodology, we systematically investigated known Weyl semimetals and revealed that Ta$_3$S$_2$ exhibits photocurrents an order of magnitude greater than those observed in TaAs, with potential for an additional order-of-magnitude enhancement under strain. To further demonstrate the generality of our approach, we obtained a wavefunction-free formula for the Berry-curvature dipole in Weyl semimetals. Our work paves the way for substantially more efficient screening and optimization of nonlinear electromagnetic properties in topological quantum materials.

cond-mat.mtrl-sci↗