arXiv subjects

Naoto Tsuji

Publications and source records attributed to Naoto Tsuji.

At least 55 records · Page 3Linked to original sources

arXiv2019

SO(4) FLEX+DMFT formalism with SU(2)$\otimes$SU(2)-symmetric impurity solver for superconductivity in the repulsive Hubbard model

Here we have developed a FLEX+DMFT formalism, where the symmetry properties of the system are incorporated by constructing a SO(4) generalization of the conventional fluctuation-exchange approximation (FLEX) coupled self-consistently to the dynamical mean-field theory (DMFT). Along with this line, we emphasize that the SO(4) symmetry is the lowest group-symmetry that enables us to investigate superconductivity and antiferromagnetism on an equal footing. We have imposed this by decomposing the electron operator into auxiliary fermionic and slave-boson constituents that respect SU(2)$_{\rm spin}\otimes$SU(2)$_{η{\rm spin}}$. This is used not in a mean-field treatment as in the usual slave-boson formalisms, but instead in the DMFT impurity solver with an SU(2)$_{\rm spin}\otimes$SU(2)$_{η{\rm spin}}$ hybridization function to incorporate the FLEX-generated bath information into DMFT iterations. While there have been attempts such as the doublon-less SU(2) slave-boson formalism, the present "full-SU(2)" slave-boson formalism is expected to provide a new platform for addressing the underlying physics for various quantum orders, which compete with each other and can coexist.

cond-mat.supr-con↗

arXiv2018

Momentum-dependent relaxation dynamics of the doped repulsive Hubbard model

We study the dynamical behavior of doped electronic systems subject to a global ramp of the repulsive Hubbard interaction. We start with formulating a real-time generalization of the fluctuation-exchange approximation. Implementing this numerically, we investigate the weak-coupling regime of the Hubbard model both in the electron-doped and hole-doped regimes. The results show that both local and nonlocal (momentum-dependent) observables evolve toward a thermal state, although the temperature of the final state depends on the ramp duration and the chemical doping. We further reveal a momentum-dependent relaxation rate of the distribution function in doped systems, and trace back its physical origin to the anisotropic self-energies in the momentum space.

cond-mat.str-el↗

arXiv2018

Fluctuation theorem for quantum-state statistics

We derive the fluctuation theorem for quantum-state statistics that can be obtained when we initially measure the total energy of a quantum system at thermal equilibrium, let the system evolve unitarily, and record the quantum-state data reconstructed at the end of the process. The obtained theorem shows that the quantum-state statistics for the forward and backward processes is related to the equilibrium free-energy difference through an infinite series of independent relations, which gives the quantum work fluctuation theorem as a special case, and reproduces the out-of-time-order fluctuation-dissipation theorem near thermal equilibrium. The quantum-state statistics exhibits a system-size scaling behavior that differs between integrable and non-integrable (quantum chaotic) systems as demonstrated numerically for one-dimensional quantum lattice models.

cond-mat.stat-mech↗

arXiv2018

Out-of-time-order fluctuation-dissipation theorem

We prove a generalized fluctuation-dissipation theorem for a certain class of out-of-time-ordered correlators (OTOCs) with a modified statistical average, which we call bipartite OTOCs, for general quantum systems in thermal equilibrium. The difference between the bipartite and physical OTOCs defined by the usual statistical average is quantified by a measure of quantum fluctuations known as the Wigner-Yanase skew information. Within this difference, the theorem describes a universal relation between chaotic behavior in quantum systems and a nonlinear-response function that involves a time-reversed process. We show that the theorem can be generalized to higher-order $n$-partite OTOCs as well as in the form of generalized covariance.

cond-mat.stat-mech↗

arXiv2017

Higgs mode in the d-wave superconductor Bi2Sr2CaCu2O8+x driven by an intense terahertz pulse

We investigated the terahertz (THz)-pulse driven nonlinear response in the d-wave cuprate superconductor Bi2Sr2CaCu2O8+x (Bi2212) using a THz pump near-infrared probe scheme in the time domain. We have observed an oscillatory behavior of the optical reflectivity that follows the THz electric field squared and is strongly enhanced below Tc. The corresponding third-order nonlinear effect exhibits both A1g and B1g symmetry components, which are decomposed from polarization-resolved measurements. Comparison with a BCS calculation of the nonlinear susceptibility indicates that the A1g component is associated with the Higgs mode of the d-wave order parameter.

cond-mat.supr-con↗

arXiv2017

Nonequilibrium steady states and transient dynamics of conventional superconductors under phonon driving

We perform a systematic analysis of the influence of phonon driving on the superconducting Holstein model coupled to heat baths by studying both the transient dynamics and the nonequilibrium steady state (NESS) in the weak and strong electron-phonon coupling regimes. Our study is based on the nonequilibrium dynamical mean-field theory, and for the NESS we present a Floquet formulation adapted to electron-phonon systems. The analysis of the phonon propagator suggests that the effective attractive interaction can be strongly enhanced in a parametric resonant regime because of the Floquet side bands of phonons. While this may be expected to enhance the superconductivity (SC), our fully self-consistent calculations, which include the effects of heating and nonthermal distributions, show that the parametric phonon driving generically results in a suppression or complete melting of the SC order. In the strong coupling regime, the NESS always shows a suppression of the SC gap, the SC order parameter and the superfluid density as a result of the driving, and this tendency is most prominent at the parametric resonance. Using the real-time nonequilibrium DMFT formalism, we also study the dynamics towards the NESS, which shows that the heating effect dominates the transient dynamics, and SC is weakened by the external modulations, in particular at the parametric resonance. In the weak coupling regime, we find that the SC fluctuations above the transition temperature are generally weakened under the driving. The strongest suppression occurs again around the parametric resonances because of the efficient energy absorption.

cond-mat.supr-con↗

arXiv2017

Bound on the exponential growth rate of out-of-time-ordered correlators

It has been conjectured by Maldacena, Shenker, and Stanford [J. High Energy Phys.~08 (2016) 106] that the exponential growth rate of the out-of-time-ordered correlator (OTOC) $F(t)$ has a universal upper bound $2πk_B T/\hbar$. Here we introduce a one-parameter family of out-of-time-ordered correlators $F_γ(t)$ ($0\leqγ\leq 1$), which has as good properties as $F(t)$ as a regularization of the out-of-time-ordered part of the squared commutator $\langle [A(t), B(0)]^2\rangle$ that diagnoses quantum many-body chaos, and coincides with $F(t)$ at $γ=1/2$. We rigorously prove that if $F_γ(t)$ shows a transient exponential growth for all $γ$ in $0\leqγ\leq 1$, that is, if the OTOC shows an exponential growth regardless of the choice of the regularization, then the growth rate $λ$ does not depend on the regularization parameter $γ$, and satisfies the inequality $λ\leq 2πk_B T/\hbar$.

cond-mat.stat-mech↗

arXiv2017

Multiple amplitude modes in strongly-coupled phonon-mediated superconductors

We study collective amplitude modes of the superconducting order parameter in strongly-coupled electron-phonon systems described by the Holstein model using the nonequilibrium dynamical mean-field theory with the self-consistent Migdal approximation as an impurity solver. The frequency of the Higgs amplitude mode is found to coincide with the superconducting gap even in the strongly-coupled (beyond BCS) regime. Besides the Higgs mode, we unravel another collective mode involving the dynamics of both the phonons and the superconducting order parameter. The frequency of this mode, higher than twice the renormalized phonon frequency in the superconducting phase, is shown to reflect a strong electron-mediated phonon-phonon interaction. Both types of collective excitations contribute to time-resolved photoemission spectra after a strong laser pump as vertex corrections to produce resonance peaks, which allows one to distinguish them from quasiparticle excitations.

cond-mat.supr-con↗

arXiv2017

Polarization-resolved terahertz third-harmonic generation in a superconductor NbN: dominance of Higgs mode beyond the BCS approximation

Recent advances in time-domain terahertz (THz) spectroscopy have unveiled that resonantly-enhanced strong THz third-harmonic generation (THG) mediated by the collective Higgs amplitude mode occurs in s-wave superconductors, where charge-density fluctuations (CDF) have also been shown to contribute to the nonlinear third-order susceptibility. It has been theoretically proposed that the nonlinear responses of Higgs and CDF exhibit essentially different polarization dependences. Here we experimentally discriminate the two contributions by polarization-resolved intense THz transmission spectroscopy for a single-crystal NbN film. The result shows that the resonant THG in the transmitted light always appears in the polarization parallel to that of the incident light with no appreciable crystal axis dependence. When we compare this with the theoretical calculation here with the BCS approximation and the dynamical mean-field theory for a model of NbN constructed from first principles, the experimental result strongly indicates that the Higgs mode rather than the CDF dominates the THG resonance in NbN. A possible mechanism for this is discussed such as the retardation effect in the phonon-mediated pairing interaction beyond BCS.

cond-mat.supr-con↗

arXiv2017

Interplay of Pomeranchuk instability and superconductivity in the two-dimensional repulsive Hubbard model

Interplay of Pomeranchuk instability (spontaneous symmetry breaking of the Fermi surface) and d-wave superconductivity is studied for the repulsive Hubbard model on the square lattice with the dynamical mean field theory combined with the fluctuation exchange approximation (FLEX+DMFT). We show that the four-fold symmetric Fermi surface becomes unstable against a spontaneous distortion into two-fold near the van Hove filling, where the symmetry of superconductivity coexisting with the Pomeranchuk distorted Fermi surface is modified from the d-wave pairing to (d+s)-wave. By systematically shifting the position of van Hove filling with varied second- and third-neighbor hoppings, we find that the transition temperature $T_{\rm c}^{\rm PI}$ of Pomeranchuk instability is more sensitively affected by the position of van Hove filling than the superconducting $T_{\rm c}^{\rm SC}$. This implies that the filling region for strong Pomeranchuk instability and that for strong superconducting fluctuations can be separated, and Pomeranchuk instability can appear even if the peak of $T_c^{\rm PI}$ is lower than the peak of $T_c^{\rm SC}$. An interesting observation is that the Fermi surface distortion can enhance the superconducting $T_{\rm c}^{\rm SC}$ in the overdoped regime, which is explained with a perturbation picture for small distortions.

cond-mat.supr-con↗

arXiv2016

Theory of light-induced resonances with collective Higgs and Leggett modes in multiband superconductors

We theoretically investigate coherent optical excitations of collective modes in two-band BCS superconductors, which accommodate two Higgs modes and one Leggett mode corresponding, respectively, to the amplitude and relative-phase oscillations of the superconducting order parameters associated with the two bands. We find, based on a mean-field analysis, that each collective mode can be resonantly excited through a nonlinear light-matter coupling when the doubled frequency of the driving field coincides with the frequency of the corresponding mode. Among the two Higgs modes, the higher-energy one exhibits a sharp resonance with light, while the lower-energy mode has a broadened resonance width. The Leggett mode is found to be resonantly induced by a homogeneous ac electric field because the leading nonlinear effect generates a potential offset between the two bands that couples to the relative phase of the order parameters. The resonance for the Leggett mode becomes sharper with increasing temperature. All of these light-induced collective modes along with density fluctuations contribute to the third-harmonic generation. We also predict an experimental possibility of optical detection of the Leggett mode.

cond-mat.supr-con↗

arXiv2016

Nonlinear light-Higgs coupling in superconductors beyond BCS: Effects of the retarded phonon-mediated interaction

We study the contribution of the Higgs amplitude mode on the nonlinear optical response of superconductors beyond the BCS approximation by taking into account the retardation effect in the phonon-mediated attractive interaction. To evaluate the vertex correction in nonlinear optical susceptibilities that contains the effect of collective modes, we propose an efficient scheme which we call the "dotted DMFT" based on the nonequilibrium dynamical mean-field theory (nonequilibrium DMFT) to go around the difficulty of solving the Bethe-Salpeter equation and analytical continuation. The vertex correction is represented by the derivative of the self-energy with respect to the external driving field, which is self-consistently determined by the differentiated ("dotted") DMFT equations. We apply the method to the Holstein model, a prototypical electron-phonon-coupled system, to calculate the susceptibility for the third-harmonic generation including the vertex correction. The results show that, in sharp contrast to the BCS theory, the Higgs mode can contribute to the third-harmonic generation for general polarization of the laser field with an order of magnitude comparable to the contribution from the pair breaking or charge density fluctuations. The physical origin is traced back to the nonlinear resonant light-Higgs coupling, which has been absent in the BCS approximation.

cond-mat.supr-con↗

arXiv2016

Exact out-of-time-ordered correlation functions for an interacting lattice fermion model

Exact solutions for local equilibrium and nonequilibrium out-of-time-ordered correlation (OTOC) functions are obtained for a lattice fermion model with on-site interactions, namely the Falicov-Kimball (FK) model, in the large dimensional and thermodynamic limit. Our approach is based on the nonequilibrium dynamical mean-field theory generalized to an extended Kadanoff-Baym contour. We find that the density-density OTOC is most enhanced at intermediate coupling around the metal-insulator phase transition. In the high-temperature limit, the OTOC remains nontrivially finite and interaction-dependent, even though dynamical charge correlations probed by an ordinary response function are completely suppressed. We propose an experiment to measure OTOCs of fermionic lattice systems including the FK and Hubbard models in ultracold atomic systems.

cond-mat.quant-gas↗

arXiv2016

Nonequilibrium Dynamical Cluster Approximation study of the Falicov-Kimball Model

We use a nonequilibrium implementation of the dynamical cluster approximation (DCA) to study the effect of short-range correlations on the dynamics of the two-dimensional Falicov-Kimball model after an interaction quench. As in the case of single-site dynamical mean field theory, thermalization is absent in DCA simulations, and for quenches across the metal-insulator boundary, nearest-neighbor charge correlations in the nonthermal steady state are found to be larger than in the thermal state with identical energy. We investigate to what extent it is possible to define an effective temperature of the trapped state after a quench. Based on the ratio between the lesser and retarded Green's function we conclude that a roughly thermal distribution is reached within the energy intervals corresponding to the momentum-patch dependent subbands of the spectral function. The effectively different chemical potentials of these distributions however lead to a very hot, or even negative, effective temperature in the energy intervals between these subbands.

cond-mat.str-el↗

arXiv2016

First-Principles Design of a Half-Filled Flat Band of the Kagome Lattice in Two-Dimensional Metal-Organic Frameworks

We design from first principles a new type of two-dimensional metal-organic frameworks (MOFs) using phenalenyl-based ligands to exhibit a half-filled flat band of the kagome lattice, which is one of the lattice family that shows Lieb-Mielke-Tasaki's flat-band ferromagnetism. Among various MOFs, we find that $\textit{trans}$-Au-THTAP(trihydroxytriaminophenalenyl) has such an ideal band structure, where the Fermi energy is adjusted right at the flat band due to unpaired electrons of radical phenalenyl. The spin-orbit coupling opens a band gap giving a non-zero Chern number to the nearly flat band, as confirmed by the presence of the edge states in first-principles calculations and by fitting to the tight-binding model. This is a novel and realistic example of a system in which a nearly flat band is both ferromagnetic $\textit{and}$ topologically non-trivial.

cond-mat.str-el↗

arXiv2016

Brillouin-Wigner theory for high-frequency expansion in periodically driven systems: Application to Floquet topological insulators

We construct a systematic high-frequency expansion for periodically driven quantum systems based on the Brillouin-Wigner (BW) perturbation theory, which generates an effective Hamiltonian on the projected zero-photon subspace in the Floquet theory, reproducing the quasienergies and eigenstates of the original Floquet Hamiltonian up to desired order in $1/ω$, with $ω$ being the frequency of the drive. The advantage of the BW method is that it is not only efficient in deriving higher-order terms, but even enables us to write down the whole infinite series expansion, as compared to the van Vleck degenerate perturbation theory. The expansion is also free from a spurious dependence on the driving phase, which has been an obstacle in the Floquet-Magnus expansion. We apply the BW expansion to various models of noninteracting electrons driven by circularly polarized light. As the amplitude of the light is increased, the system undergoes a series of Floquet topological-to-topological phase transitions, whose phase boundary in the high-frequency regime is well explained by the BW expansion. As the frequency is lowered, the high-frequency expansion breaks down at some point due to band touching with nonzero-photon sectors, where we find numerically even more intricate and richer Floquet topological phases spring out. We have then analyzed, with the Floquet dynamical mean-field theory, the effects of electron-electron interaction and energy dissipation. We have specifically revealed that phase transitions from Floquet-topological to Mott insulators emerge, where the phase boundaries can again be captured with the high-frequency expansion.

cond-mat.mes-hall↗

arXiv2015

Electronic structure of helicoidal graphene: massless Dirac particles on a curved surface with a screw symmetry

Massless Dirac particles on the helicoid are theoretically investigated. With its possible application being helical graphene, we explore how the peculiarities of Dirac particles appear on the curved, screw-symmetric surface. The zweibein is used to derive the massless Dirac equation on the helicoid, as well as general curved surfaces. Bound states of massless Dirac electrons are shown to be absent on the helicoid, and then the scattering probabilities and the phase shifts on the surface are obtained from numerically calculated wave functions. We find the local density of states and the phase shifts idiosyncratic especially around the axis of the helicoid. Bound states of massive Dirac electrons on the surface are also shown to be absent as an extension of the above result on massless Dirac electrons.

cond-mat.mes-hall↗

arXiv2015

FLEX+DMFT approach to the $d$-wave superconducting phase diagram of the two-dimensional Hubbard model

The dynamical mean-field theory (DMFT) combined with the fluctuation exchange (FLEX) method, namely FLEX+DMFT, is an approach for correlated electron systems to incorporate both local and non-local long-range correlations in a self-consistent manner. We formulate FLEX+DMFT in a systematic way starting from a Luttinger-Ward functional, and apply it to study the $d$-wave superconductivity in the two-dimensional repulsive Hubbard model. The critical temperature ($T_c$) curve obtained in the FLEX+DMFT exhibits a dome structure as a function of the filling, which has not been clearly observed in the FLEX approach alone. We trace back the origin of the dome to the local vertex correction from DMFT that renders a filling dependence in the FLEX self-energy. We compare the results with those of GW+DMFT, where the $T_c$-dome structure is qualitatively reproduced due to the same vertex correction effect, but a crucial difference from FLEX+DMFT is that $T_c$ is always estimated below the Néel temperature in GW+DMFT. The single-particle spectral function obtained with FLEX+DMFT exhibits a double-peak structure as a precursor of the Hubbard bands at temperature above $T_c$.

cond-mat.supr-con↗