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Naoya Tajima

Publications and source records attributed to Naoya Tajima.

7 recordsLinked to original sources

Anomalous Phase-Coherence Scaling in a Quantum-Critical Dirac Semimetal

We have investigated the weak antilocalization (WAL) in the pressurized Dirac semimetal $\alpha$-(BEDT-TTF)$_2$I$_3$ across a correlation-driven quantum phase transition to a charge-ordered insulating state and evaluated the phase coherence length $L_{\phi}$ and its temperature scaling under various pressures from the low-temperature magnetoconductivity. In the high-pressure regime, the system exhibits the conventional two-dimensional dephasing behavior ($L_{\phi} \propto T^{-p}$ with $p \approx 1/2$), characteristic of electron-electron scattering in diffusive conductors. As the pressure approaches the critical pressure ($P_c \sim 1.2$ GPa), the temperature exponent is suppressed to $p \sim 0.3$, while $L_{\phi}$ remains large ($700\text{-}800$ nm at 0.5 K). This anomalous scaling suggests nontrivial inelastic scattering associated with Dirac electrons near the quantum critical point. The persistence of WAL across the transition supports a gapless or nearly gapless quantum phase transition.

cond-mat.str-el

Evidence for three-dimensional Dirac semimetal state in strongly correlated organic quasi-two-dimensional material

The three-dimensional Dirac semimetal is distinct from its two-dimensional counterpart due to its dimensionality and symmetry. Here, we observe that molecule-based quasi-two-dimensional Dirac fermion system, $α$-(BEDT-TTF)$_2$I$_3$, exhibits chiral anomaly-induced negative magnetoresistance and planar Hall effect upon entering the coherent inter-layer tunneling regime under high pressure. Time-reversal symmetry is broken due to the strong electronic correlation effect, while the spin-orbit coupling effect is negligible. The system provides an ideal platform for investigating the chiral anomaly physics by controlling dimensionality and strong electronic correlation.

cond-mat.str-el

Coherent interlayer coupling in quasi-two-dimensional Dirac fermions in $α$-(BEDT-TTF)$_2$I$_3$

Theoretical and experimental studies have supported that the electronic structure of $α$-(BEDT-TTF)$_2$I$_3$ under pressure is described by two-dimensional Dirac fermions. When the interlayer tunneling is coherent, the electronic structure of the system becomes three-dimensional, and we expect the peak structure to appear in the interlayer resistivity under magnetic fields. We theoretically and experimentally show that the peak appears in the interlayer resistivity at low temperatures and high magnetic fields. From the experiment, we estimate that the magnitude of the interlayer tunneling is $t_1 \sim 1$ meV. Our result opens the door to investigating the three-dimensional electronic structure of $α$-(BEDT-TTF)$_2$I$_3$.

cond-mat.str-el

Pressure-induced phase switching of the Shubnikov de Haas oscillations in molecular Dirac fermion system $α-$(BETS)$_{2}$I$_{3}$

We report on the Shubnikov de Haas (SdH) oscillations in the quasi two-dimensional molecular conductor $α-$(BETS)$_{2}$I$_{3}$ [BETS: bis(ethylenedithio)tetraselenafulvalene] laminated on polyimide films at 1.7 K. From the SdH phase factor, we verified experimentally that the material is in the Dirac fermion phase under pressure. $α-$(BETS)$_{2}$I$_{3}$ is in the vicinity of the phase transition between strongly correlated insulating and Dirac fermion phases, and is a possible candidate for an ambient-pressure molecular Dirac fermion system. However, the SdH oscillations indicate that the Berry phase is zero at ambient pressure. Under pressure, a $π$ Berry phase emerges when the metal-insulator crossover is almost suppressed at $\sim$0.5 GPa. The results contrast those for the pioneering molecular Dirac fermion system $α-$(BEDT-TTF)$_{2}$I$_{3}$ [BEDT-TTF: bis(ethylenedithio)tetrathiafulvalene] in which Dirac fermions and semiconducting behavior are simultaneously observed.

cond-mat.mtrl-sci

Universal Behavior of Magnetoresistance in Organic Dirac Electron Systems

In-plane magnetoresistance for organic massless Dirac electron system (OMDES) $α$-(BEDT-TTF)$_2$I$_3$ and $θ$-(BEDT-TTF)$_2$I$_3$ in addition to possible candidates of the OMDES $α$-(BETS)$_2$I$_3$ and $α$-(BEDT-STF)$_2$I$_3$, was investigated under hydrostatic pressure. We have found the universal behavior of the in-plane magnetoresistance under a low magnetic field perpendicular to two-dimensional plane. As for $α$-(BEDT-TTF)$_2$I$_3$, the universality was examined with the parameters of temperature, magnetic field and its direction. We suggest that the universal magnetoresistance behavior is found even for the gapped state of $α$-(BEDT-TTF)$_2$I$_3$ under intermediate pressure, when the thermal energy exceeds the gap.

cond-mat.str-el

Field-induced carrier delocalization in the strain-induced Mott insulating state of an organic superconductor

We report the influence of the field effect on the dc resistance and Hall coefficient in the strain-induced Mott insulating state of an organic superconductor $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br. Conductivity obeys the formula for activated transport $σ_{\Box} = σ_{0}\exp(-W/k_{B}T)$, where $σ_{0}$ is a constant and $W$ depends on the gate voltage. The gate voltage dependence of the Hall coefficient shows that, unlike in conventional FETs, the effective mobility of dense hole carriers ($\sim1.6\times 10^{14}$ cm$^{-2}$) is enhanced by a positive gate voltage. This implies that carrier doping involves delocalization of intrinsic carriers that were initially localized due to electron correlation.

cond-mat.str-el