arXiv subjects

Nathan Beaulieu

Publications and source records attributed to Nathan Beaulieu.

13 recordsLinked to original sources

arXiv2026

Nonlinear mode interactions under parametric excitation in a YIG microdisk

A pair of quantized spin-wave modes is driven by two-tone parallel pumping in a YIG microdisk. The nonlinear dynamics is experimentally investigated by probing the resulting steady state, which is found to critically depend on the chosen pair of modes, the detuning between the pump frequencies and the modes parametric resonance, as well as the temporal sequence of the two rf tones. A general theory of parametric excitation in confined structures based on magnetization normal modes is developed and quantitatively accounts for the observed dependence and non-commutative behaviors, which emerge from the interplay between the self and mutual nonlinear frequency shifts of the spin-wave modes. Owing to its high degree of external controllability and scalability to larger sets of modes, this dynamical system provides a model platform for exploring nonlinear phenomena and a promising route toward rf driven state mapping relevant to neuromorphic and unconventional computing.

cond-mat.mes-hall↗

arXiv2025

Low-temperature-compatible iron garnet films grown by liquid phase epitaxy

Single-crystalline yttrium iron garnet (YIG) thin films (< 100 nm) form the backbone of magnonics, owing to the record-low losses affecting their magnetization dynamics. However, thin epitaxial YIG has mostly been investigated under ambient temperatures, limited by the paramagnetic losses occurring at low temperatures due to the gadolinium gallium garnet (GGG) substrates required for epitaxial growth. Driven by a growing interest in magnonic devices that can operate in cryogenic conditions and address quantum information applications, there is a strong need for iron garnet epitaxial films grown on diamagnetic substrates that can maintain low losses at low temperatures. In this work, we use liquid phase epitaxy (LPE) to grow ultrathin films of strained YIG on a commercial diamagnetic substrate, yttrium scandium gallium garnet (YSGG). We investigate their magnetization dynamics in the 3-300 K temperature range, and compare them to equivalent films grown on paramagnetic GGG. We demonstrate for LPE YIG on YSGG substrates a ferromagnetic resonance linewidth below 1 mT at 3 K, together with a very weak temperature and frequency dependence of the losses. The growth of YIG/YSGG by LPE provides a straightforward approach to producing iron garnet thin films for use in low-temperature investigations.

cond-mat.mtrl-sci↗

arXiv2023

Degenerate and non-degenerate parametric excitation in YIG nanostructures

We study experimentally the processes of parametric excitation in microscopic magnetically saturated disks of nanometer-thick Yttrium Iron Garnet. We show that, depending on the relative orientation between the parametric pumping field and the static magnetization, excitation of either degenerate or non-degenerate magnon pairs is possible. In the latter case, which is particularly important for applications associated with the realization of computation in the reciprocal space, a single-frequency pumping can generate pairs of magnons whose frequencies correspond to different eigenmodes of the disk. We show that, depending on the size of the disk and the modes involved, the frequency difference in a pair can vary in the range 0.1-0.8 GHz. We demonstrate that in this system, one can easily realize a practically important situation where several magnon pairs share the same mode. We also observe the simultaneous generation of up to six different modes using a fixed-frequency monochromatic pumping. Our experimental findings are supported by numerical calculations that allow us to unambiguously identify the excited modes. Our results open new possibilities for the implementation of reciprocal-space computing making use of low damping magnetic insulators.

cond-mat.mes-hall↗

arXiv2023

Complete identification of spin-wave eigenmodes excited by parametric pumping in YIG microdisks

We present the parametric excitation of spin-wave modes in YIG micro-disks via parallel pumping. Their spectroscopy is performed using magnetic resonance force microscopy (MRFM), while their spatial profiles are determined by micro-focus Brillouin light scattering (BLS). We observe that almost all the fundamental eigenmodes of an in-plane magnetized YIG micro-disk, calculated using a micromagnetic eigenmode solver, can be excited using the parallel pumping scheme, as opposed to the transverse one. The comparison between the MRFM and BLS data on one side, and the simulations on the other side, provides the complete spectroscopic labeling of over 40 parametrically excited modes. Our findings could be promising for spin-wave-based computation schemes, in which the amplitudes of a large number of spin-wave modes have to be controlled.

physics.app-ph↗

arXiv2022

Non-local magnon transconductance in extended magnetic insulating films.\\ Part I: spin diode effect

This review provides a comprehensive study of the nonlinear transport properties of magnons, which are electrically emitted or absorbed inside extended YIG films by spin transfer effects via a YIG$\vert$Pt interface. Our purpose is to experimentally elucidate the pertinent picture behind the asymmetric electrical variation of the magnon transconductance analogous to an electric diode. The feature is rooted in the variation of the density of low-lying spin excitations via an electrical shift of the magnon chemical potential. As the intensity of the spin transfer increases in the forward direction (regime of magnon emission), the transport properties of low-energy magnon go through 3 distinct regimes: \textit{i)} at low currents, where the spin current is a linear function of the electrical current, the spin transport is ballistic and set by the film thickness; \textit{ii)} for amplitudes of the order of the damping compensation threshold, it switches to a highly correlated regime limited by magnon-magnon relaxation process and marked by a saturation of the magnon transconductance. Here the main bias, that controls the magnon density, are thermal fluctuations beneath the emitter. \textit{iii)} As the temperature under the emitter approaches the Curie temperature, scattering with high-energy magnons dominates, leading to diffusive transport. We note that such sequence of transport regimes bears analogy with electron hydrodynamic transport in ultra-pure media predicted by Radii Gurzhi. This study restricted to low energy part of the magnon manifold complements part II of this review\cite{kohno_2F}, which concentrates instead on the whole spectrum of propagating magnons.

cond-mat.mes-hall↗

arXiv2022

Non-local magnon transconductance in extended magnetic insulating films.\\Part II: two-fluid behavior

This review presents a comprehensive study of the spatial dispersion of propagating magnons electrically emitted in extended yttrium-iron garnet (YIG) films by the spin transfer effects across a YIG$\vert$Pt interface. Our goal is to provide a generic framework to describe the magnon transconductance inside magnetic films. We experimentally elucidate the relevant spectral contributions by studying the lateral decay of the magnon signal. While most of the injected magnons do not reach the collector, the propagating magnons can be split into two-fluids: \textit{i)} a large fraction of high-energy magnons carrying energy of about $k_B T_0$, where $T_0$ is the lattice temperature, with a characteristic decay length in the sub-micrometer range, and \textit{ii)} a small fraction of low-energy magnons, which are particles carrying energy of about $\hbar \omega_K$, where $\omega_K/(2 \pi)$ is the Kittel frequency, with a characteristic decay length in the micrometer range. Taking advantage of their different physical properties, the low-energy magnons can become the dominant fluid \textit{i)} at large spin transfer rates for the bias causing the emission of magnons, \textit{ii)} at large distance from the emitter, \textit{iii)} at small film thickness, or \textit{iv)} for reduced band mismatch between the YIG below the emitter and the bulk due to variation of the magnon concentration. This broader picture complements part I \cite{kohno_SD}, which focuses solely on the nonlinear transport properties of low-energy magnons.

cond-mat.mes-hall↗

arXiv2020

Enhancement of YIG$|$Pt spin conductance by local Joule annealing

We report that Joule heating can be used to enhance the interfacial spin conductivity between a metal and an oxide. We observe that local annealing of the interface at about 550\,K by injecting large current densities ($>10^{12}\text{A/m}^{2}$) into a pristine 7\,nm thick Pt nanostrip evaporated on top of yttrium iron garnet (YIG), can improve the spin transmission up to a factor 3: a result of particular interest for interfacing ultra thin garnet films where strong chemical etching of the surface has to be avoided. The effect is confirmed by different methods: spin Hall magnetoresistance, spin pumping and non-local spin transport. We use it to study the influence of the YIG$|$Pt coupling on the non-linear spin transport properties. We find that the cross-over current from a linear to a non-linear spin transport regime is independent of this coupling, suggesting that the behavior of pure spin currents circulating in the dielectric are mostly governed by the physical properties of the bare YIG film beside the Pt nanostrip.

cond-mat.mtrl-sci↗

arXiv2020

Short-range Thermal Magnon Diffusion in Magnetic Garnet

Using the spin Seebeck effect (SSE), we study the propagation distance of thermal spin currents inside a magnetic insulator thin film in the short-range regime. We disambiguate spin currents driven by temperature and chemical potential gradients by comparing the SSE signal before and after adding a thermalization capping layer on the same device. We report that the measured spin decay behavior near the heat source is well accounted for by a diffusion model where the magnon diffusion length is in submicron range, \textit{i.e.} two orders of magnitude smaller than previous estimates inferred from the long-range behavior. Our results highlight the caveat in applying a diffusive theory to describe thermal magnon transport, where a single decay length may not capture the behavior on all length scales.

cond-mat.mtrl-sci↗

arXiv2020

Coherent long-range transfer of angular momentum between magnon Kittel modes by phonons

We report ferromagnetic resonance in the normal configuration of an electrically insulating magnetic bilayer consisting of two yttrium iron garnet (YIG) films epitaxially grown on both sides of a 0.5-mm-thick nonmagnetic gadolinium gallium garnet (GGG) slab. An interference pattern is observed and it is explained as the strong coupling of the magnetization dynamics of the two YIG layers either in phase or out of phase by the standing transverse sound waves, which are excited through a magnetoelastic interaction. This coherent mediation of angular momentum by circularly polarized phonons through a nonmagnetic material over macroscopic distances can be useful for future information technologies.

cond-mat.mes-hall↗

arXiv2018

Temperature Dependence of Magnetic Properties of an 18-nm-thick YIG Film Grown by Liquid Phase Epitaxy: Effect of a Pt Overlayer

Liquid phase epitaxy of an 18 nm thick Yttrium Iron garnet (YIG) film is achieved. Its magnetic properties are investigated in the 100 -- 400 K temperature range, as well as the influence of a 3 nm thick Pt overlayer on them. The saturation magnetization and the magnetocrystalline cubic anisotropy of the bare YIG film behave similarly to bulk YIG. A damping parameter of only a few $10^{-4}$ is measured, together with a low inhomogeneous contribution to the ferromagnetic resonance linewidth. The magnetic relaxation increases upon decreasing temperature, which can be partly ascribed to impurity relaxation mechanisms. While it does not change its cubic anisotropy, the Pt capping strongly affects the uniaxial perpendicular anisotropy of the YIG film, in particular at low temperatures. The interfacial coupling in the YIG/Pt heterostructure is also revealed by an increase of the linewidth, which substantially grows by lowering the temperature.

cond-mat.mtrl-sci↗

arXiv2018

Ultra-low damping insulating magnetic thin films get perpendicular

A magnetic material combining low losses and large Perpendicular Magnetic Anisotropy (PMA) is still a missing brick in the magnonic and spintronic fields. We report here on the growth of ultrathin Bismuth doped Y$_{3}$Fe$_{5}$O$_{12}$ (BiYIG) films on Gd$_{3}$Ga$_{5}$O$_{12}$ (GGG) and substituted GGG (sGGG) (111) oriented substrates. A fine tuning of the PMA is obtained using both epitaxial strain and growth induced anisotropies. Both spontaneously in-plane and out-of-plane magnetized thin films can be elaborated. Ferromagnetic Resonance (FMR) measurements demonstrate the high dynamic quality of these BiYIG ultrathin films, PMA films with Gilbert damping values as low as 3 10$^{-4}$ and FMR linewidth of 0.3 mT at 8 GHz are achieved even for films that do not exceed 30 nm in thickness. Moreover, we measure Inverse Spin Hall Effect (ISHE) on Pt/BiYIG stacks showing that the magnetic insulator$'$s surface is transparent to spin current making it appealing for spintronic applications.

cond-mat.mes-hall↗

arXiv2017

Spin conductance of YIG thin films driven from thermal to subthermal magnons regime by large spin-orbit torque

We report a study on spin conductance in ultra-thin films of Yttrium Iron Garnet (YIG), where spin transport is provided by propagating spin waves, that are generated and detected by direct and inverse spin Hall effects in two Pt wires deposited on top. While at low current the spin conductance is dominated by transport of thermal magnons, at high current, the spin conductance is dominated by low-damping non-equilibrium magnons thermalized near the spectral bottom by magnon-magnon interaction, with consequent a sensitivity to the applied magnetic field and a longer decay length. This picture is supported by microfocus Brillouin Light Scattering spectroscopy.

cond-mat.mtrl-sci↗

arXiv2016

Giant Rashba effect at the topological surface of PrGe revealing antiferromagnetic spintronics

Rashba spin-orbit splitting in the magnetic materials opens up a new perspective in the field of spintronics. Here, we report a giant Rashba-type spin-orbit effect on PrGe [010] surface in the paramagnetic phase with Rashba coefficient α_R=5 eVÅ. Significant changes in the electronic band structure has been observed across the phase transitions from paramagnetic to antiferromagnetic (44 K) and from antiferromagnetic to the ferromagnetic ground state (41.5 K). We find that Pr 4f states in PrGe is strongly hybridized with the Pr 5d and Ge 4s-4p states near the Fermi level. The behavior of Rashba effect is found to be different in the k_x and the k_y directions showing electron-like and the hole-like bands, respectively. The possible origin of Rashba effect in the paramagnetic phase is related to the anti-parallel spin polarization present in this system. First-principles density functional calculations of Pr terminated surface with the anti-parallel spins shows a fair agreement with the experimental results. We find that the anti-parallel spins are strongly coupled to the lattice such that the PrGe system behaves like weak ferromagnetic system. Analysis of the energy dispersion curves at different magnetic phases showed that there is a competition between the Dzyaloshinsky-Moriya interaction and the exchange interaction which gives rise to the magnetic ordering in PrGe. Supporting evidences of the presence of Dzyaloshinsky-Moriya interaction are observed as anisotropic magnetoresistance with respect to field direction and first-order type hysteresis in the X-ray diffraction measurements. A giant negative magnetoresistance of 43% in the antiferromagnetic phase and tunable Rashba parameter with temperature across the magnetic transitions makes this material a suitable candidate for technological application in the antiferromagnetic spintronic devices.

cond-mat.mtrl-sci↗