arXiv subjects

Natsuki Kanda

Publications and source records attributed to Natsuki Kanda.

At least 19 recordsLinked to original sources

arXiv2026

Modeling of jitter correction methods for asynchronous optical sampling

Timing jitter management is crucial in asynchronous optical sampling (ASOPS) and dual-comb spectroscopy to maintain spectral bandwidth and fidelity. However, a quantitative framework predicting jitter correction efficiency from laser phase noise has been lacking. Here, we present formulation and simulation models that evaluate jitter-suppression dynamics based on phase noise spectra. Our model quantifies the contrast between conventional triggering and software-based jitter correction. It also enables retrieval of a jitter-free spectrum by compensating for jitter-induced power degradation. This work provides a universal design framework for optimizing diverse ASOPS systems by predicting residual jitter prior to system construction.

physics.optics↗

arXiv2026

High-Field Terahertz Spin Resonance in Cr$_2$O$_3$ above the Spin-Flop Transition

We report single-shot terahertz time-domain spectroscopy of Cr$_2$O$_3$ in pulsed magnetic fields up to 30 T. Well above the spin-flop field, in the 20-30 T range, the resonance frequency exhibits a nearly linear field dependence with a slope of ~22 GHz/T, smaller than the 28 GHz/T reported from low-field measurements. This reduction is insensitive to temperature and to a 15{\deg} field tilt, suggesting an intrinsic high-field property.

cond-mat.mtrl-sci↗

arXiv2026

Broadband gain characterization of Co:MgF$_2$ for mid-infrared femtosecond pulse amplification

The broadband gain characteristics of Co:MgF$_2$ were investigated to assess its potential as a gain medium for ultrashort-pulse amplification around the 2 $\mu$m spectral region. Single-pass gain measurements performed using femtosecond seed pulses revealed broadband amplification in the 1.5-2.4 $\mu$m region. The temporal dynamics and spectra of the gain were experimentally characterized and utilized for numerical simulations to assess the feasibility of Co:MgF$_2$ as a broadband gain medium for ultrashort pulses. The results indicate its potential for broadband amplification in future short-wave infrared to mid-infrared ultrafast laser systems, particularly when combined with coherent waveform synthesis or post-compression techniques.

physics.optics↗

arXiv2026

Submicrometer focusing of isolated attosecond XUV pulses approaching 10$^{16}$ W/cm$^2$

We demonstrate submicrometer focusing of isolated attosecond pulses (IAPs) in the extreme ultraviolet (XUV) region using a custom ellipsoidal mirror. The obtained focal spot sizes were verified using knife-edge measurements with a sharp silicon edge, confirming reproducible dimensions down to 0.46 $\mu$m $\times$ 0.36 $\mu$m (FWHM), approaching the diffraction limit. Focusing a 1.1-GW tabletop IAP source yields a peak intensity of 3 $\times$ 10$^{15}$ W/cm$^2$, and a realistic pathway toward 10$^{16}$ W/cm$^2$ is obtained by optimizing the beamline throughput. These results establish a practical route toward attosecond nonlinear optics in both gas and solid phases, driven by intense XUV fields.

physics.optics↗

arXiv2025

Correction of broadband terahertz electro-optic sampling with GaSe crystals

Gallium selenide (GaSe) is an efficient nonlinear crystal for electro-optic (EO) sampling in the multi-terahertz (THz) frequency range. However, the lattice resonance at several THz frequencies hampers broadband EO sampling, resulting in distorted pulse waveforms. In this work, we experimentally evaluated the frequency-dependent response function in EO sampling, considering the effects of phonons, phase mismatch, and gate pulse waveforms. The phonon effect is described using an effective Faust-Henry coefficient, which was determined to be $-0.21 \pm 0.02$. The corrected field amplitude of multi-THz pulses aligns with additional measurements of average power and a beam diameter. The successful compensation of the frequency characteristics in GaSe will contribute to a more accurate evaluation of multi-THz transients.

physics.optics↗

arXiv2025

Robust asynchronous optical sampling terahertz spectroscopy using commercially available free-running lasers

This study presents asynchronous optical sampling (ASOPS) terahertz spectroscopy using commercially available Ti:Sapphire lasers without stabilizing repetition frequency. Our postprocessing algorithm using the multiplied repetition frequency difference as the calibration signal successfully corrected the jitter, thereby allowing broadband (2.5 THz) spectroscopy with a high spectral resolution (82 MHz). The robustness of the jitter correction based on the free-running laser setup and broadband electric circuits was rigorously examined under varying temperatures, thereby demonstrating reliable long-term operations over 60 h. This study expands the applicability of the ASOPS terahertz time-domain spectroscopy.

physics.optics↗

arXiv2024

Valley polarization dynamics of photoinjected carriers at the band edge in room-temperature silicon studied by terahertz polarimetry

Sixfold-degenerate valleys in Si have attracted considerable attention for valleytronics application. Using optical pump-terahertz (THz) probe spectroscopy, we study the dynamics of valley polarization in bulk Si(001) at room temperature. Linearly polarized pump pulses excite electrons and holes with asymmetric distributions in momentum space, leading to in-plane anisotropic conductivity. By varying the polarization directions of the pump light relative to the in-plane crystalline axes, the valley polarization of electrons and the momentum asymmetry of holes are separately probed through observing the polarization rotation of THz pulses. We demonstrate that the valley relaxation time of electrons near the conduction band minimum exceeds 1.5 ps at room temperature, in good agreement with theoretically calculated intervalley phonon scattering with f process. This work paves the way for Si-based room-temperature valleytronics.

cond-mat.mtrl-sci↗

arXiv2024

Light-induced inverse spin Hall effect and field-induced circular photogalvanic effect in GaAs revealed by two-dimensional terahertz Fourier analysis

The electromotive force transverse to a bias field under irradiation of circularly polarized light, namely the photovoltaic Hall response or light-induced anomalous Hall effect, has attracted considerable attention to investigate the topologically nontrivial states in Floquet engineering and the inverse spin Hall effect of spin-polarized carriers in spintronics. However, taking into account inversion symmetry breaking by the bias field, the circularly polarized light can excite photocarriers with asymmetric momentum distribution, which generates injection current transverse to the bias field. Therefore, the field-induced circular photogalvanic effect (FI-CPGE) should also emerge in the very same experimental configuration for light-induced anomalous Hall effect but has been overlooked in literature. In this work, using terahertz pulses as a bias field for a semiconductor GaAs, we conduct two-dimensional Fourier analysis and demonstrate that FI-CPGE can play a major role in the photovoltaic Hall response. Counterintuitively, FI-CPGE is significantly enhanced when the photocarriers are excited near the bandgap with small density of states and low group velocity, which can be explained by a three-level resonant nonlinear interaction near the band degeneracy point. We also clarified that FI-CPGE would be further largely detected in the contact-type measurement using electrodes because of the absence of a filtering effect inherent to terahertz pulses. This work provides a comprehensive, generalized view of the photovoltaic Hall response in biased materials, paving a new avenue for detecting topological monopoles in momentum space hidden in equilibrium using third-order nonlinear responses.

cond-mat.mtrl-sci↗

arXiv2023

Programmable generation of counterrotating bicircular light pulses in the multi-terahertz frequency range

The manipulation of solid states using intense infrared or terahertz light fields is a pivotal area in contemporary ultrafast photonics research. While conventional circular polarization has been well explored, the potential of counterrotating bicircular light remains widely underexplored, despite growing interest in theory. In the mid-infrared or multi-terahertz region, experimental challenges lie in difficulties in stabilizing the relative phase between two-color lights and the lack of available polarization elements. Here, we successfully generated phase-stable counterrotating bicircular light pulses in the 10-40 THz frequency range circumventing the above problems. Employing spectral broadening, polarization pulse shaping with a spatial light modulator, and intra-pulse difference frequency generation leveraging a distinctive angular-momentum selection rule within the nonlinear crystal, we achieved direct conversion from near-infrared pulses into the designed counterrotating bicircular multi-terahertz pulses. Use of the spatial light modulator enables programmable control over the shape, orientation, rotational symmetry, and helicity of the bicircular light field trajectory. This advancement provides a novel pathway for the programmable manipulation of light fields, and marks a significant step toward understanding and harnessing the impact of tailored light fields on matter, particularly in the context of topological semimetals.

physics.optics↗

arXiv2023

Emergence of high-mobility carriers in topological kagome bad metal Mn$_3$Sn by intense photoexcitation

Kagome-lattice materials offer novel playgrounds of exploring topologically nontrivial states of electrons under influence of many-body interactions. A noncollinear kagome antiferromagnet Mn$_3$Sn has attracted particular interest for application in spintronics owing to the large anomalous Hall effect related to the Weyl dispersion near the Fermi energy. In addition, strong electronic correlation suggesting the Kondo physics has also been implied. However, the effect of correlation on the band topology and their interplay remains elusive. Here, we investigate nonequilibrium Hall transport in a photoexcited Mn$_3$Sn using time-resolved terahertz Faraday rotation spectroscopy. In equilibrium, Mn$_3$Sn is a bad metal close to the Mott-Ioffe-Regal limit with low carrier mobility, and thus only the anomalous Hall effect is discerned. By contrast, intense photoexcitation beyond an approximate threshold gives rise to a clear cyclotron resonance, namely the normal Hall effect, indicating the emergence of unusual carriers with 50 times lighter effective mass and 40 times less scattering. The lifetime of high-mobility carriers as long as a few tens of picoseconds and a threshold-like behavior for the pump fluence are hardly explained by contribution of photoexcited hot carriers. Instead, the emergence of unusual carriers may be accounted for by dielectric screening of the on-site Coulomb interaction by high-density delocalized photocarriers. A possible role of electronic correlation in equilibrium transport in Mn$_3$Sn beyond the single-particle picture is discussed.

cond-mat.str-el↗

arXiv2023

Anomalous Hall transport by optically injected isospin degree of freedom in Dirac semimetal thin film

Chirality of massless fermions emergent in condensed matter is a key to understand their characteristic behavior as well as to exploit their functionality. However, chiral nature of massless fermions in Dirac semimetals has remained elusive, due to equivalent occupation of carriers with the opposite chirality in thermal equilibrium. Here, we show that the isospin degree of freedom, which labels the chirality of massless carriers from a crystallographic point of view, can be injected by circularly polarized light. Terahertz Faraday rotation spectroscopy successfully detects the anomalous Hall conductivity by a light-induced isospin polarization in a three-dimensional Dirac semimetal, Cd$_3$As$_2$. Spectral analysis of the Hall conductivity reveals a long scattering time and a long decay time, which are characteristic of the isospin. The long-lived, robust, and reversible character of the isospin promises potential application of Dirac semimetals in future information technology.

cond-mat.mes-hall↗

arXiv2023

Time-domain characterization of electric field vector in multi-terahertz pulses using polarization-modulated electro-optic sampling

We demonstrated characterizing the electric field waveform of multi-terahertz pulses (10-50 THz) as vector quantities in the time domain by applying the polarization modulated electro-optic sampling (POMEOS) method. The problem of an ultrabroadband gate pulse was solved by modifying the fitting function in POMEOS and its validity was confirmed through numerical simulations. High accuracy and precision of approximately 1 mrad with 3 s accumulation were demonstrated. Our method can be applied not only to multi-terahertz polarization measurements for linear response but also to the evaluation of the driving field of intense pulses for nonlinear response or material control.

physics.optics↗

arXiv2023

Observation of Terahertz Spin Hall Conductivity Spectrum in GaAs with Optical Spin Injection

We report the first observation of the spin Hall conductivity spectrum in GaAs at room temperature. Our terahertz polarimetry with a precision of several $\mu$rads resolves the Faraday rotation of terahertz pulses arising from the inverse spin Hall effect of optically injected spin-polarized electrons. The obtained spin Hall conductivity spectrum exhibits an excellent quantitative agreement with theory, demonstrating a crossover in the dominant origin from impurity scattering in the DC regime to the intrinsic Berry-curvature mechanism in the terahertz regime. Our spectroscopic technique opens a new pathway to analyze anomalous transports related to spin, valley, or orbital degrees of freedom.

cond-mat.mtrl-sci↗

arXiv2023

Jitter correction for asynchronous optical sampling terahertz spectroscopy using free-running pulsed lasers

We demonstrate a jitter correction method for asynchronous optical sampling (ASOPS) terahertz (THz) time-domain spectroscopy using two free-running oscillators. This method simultaneously records the THz waveform and a harmonic of the laser repetition rate difference, to monitor the jitter information for software jitter correction. By suppressing the residual jitter below 0.1 ps, the accumulation of the THz waveform is achieved without losing the measurement bandwidth. Our measurement of water vapor successfully resolves the absorption linewidths below 1 GHz, demonstrating a robust ASOPS with a flexible, simple, and compact setup without any feedback control or additional continuous-wave THz source.

physics.optics↗

arXiv2022

Disentangling the Competing Mechanisms of Light-Induced Anomalous Hall Conductivity in Three-Dimensional Dirac Semimetal

We experimentally elucidate the origin of the anomalous Hall conductivity in a three-dimensional Dirac semimetal, Cd$_3$As$_2$, driven by circularly polarized light. Using time-resolved terahertz Faraday rotation spectroscopy, we determine the transient Hall conductivity spectrum with special attention to its sign. Our results clearly show the dominance of direct photocurrent generation assisted by the terahertz electric field. The contribution from the Floquet-Weyl nodes is found to be minor when the driving light is in resonance with interband transitions. We develop a generally applicable classification of microscopic mechanisms of light-induced anomalous Hall conductivity.

cond-mat.mtrl-sci↗

arXiv2022

Ultrafast Dynamics of Intrinsic Anomalous Hall Effect in the Topological Antiferromagnet Mn3Sn

We investigate ultrafast dynamics of the anomalous Hall effect (AHE) in the topological antiferromagnet Mn3Sn with sub-100 fs time resolution. Optical pulse excitations largely elevate the electron temperature up to 700 K, and terahertz probe pulses clearly resolves ultrafast suppression of the AHE before demagnetization. The result is well reproduced by microscopic calculation of the intrinsic Berry-curvature mechanism while the extrinsic contribution is clearly excluded. Our work opens a new avenue for the study of nonequilibrium AHE to identify the microscopic origin by drastic control of the electron temperature by light.

cond-mat.mtrl-sci↗

arXiv2021

Stimulated Rayleigh Scattering Enhanced by a Longitudinal Plasma Mode in a Periodically Driven Dirac Semimetal Cd$_3$As$_2$

Using broadband (12-45 THz) multi-terahertz spectroscopy, we show that stimulated Rayleigh scattering dominates the transient optical conductivity of cadmium arsenide, a Dirac semimetal, under an optical driving field at 30 THz. The characteristic dispersive lineshape with net optical gain is accounted for by optical transitions between light-induced Floquet subbands, strikingly enhanced by the longitudinal plasma mode. Stimulated Rayleigh scattering with an unprecedentedly large refractive index change may pave the way for slow light generation in conductive solids at room temperature.

cond-mat.mtrl-sci↗

arXiv2021

Tracking ultrafast change of multiterahertz broadband response functions in a photoexcited Dirac semimetal Cd$_3$As$_2$ thin film

The electromagnetic response of Dirac semimetals in the infrared and terahertz frequency ranges is attracting growing interest for potential applications in optoelectronics and nonlinear optics. The interplay between the free-carrier response and interband transitions in the gapless, linear dispersion relation plays a key role in enabling novel functionalities. Here we investigate ultrafast dynamics in thin films of a photoexcited Dirac semimetal Cd$_3$As$_2$ by probing the broadband response functions as complex quantities in the multiterahertz region (10-45 THz, 40-180 meV, or 7-30 $\mu$m), which covers the crossover between the inter and intraband response. We resolve dynamics of the photoexcited nonthermal electrons which merge with originally existing carriers to form a single thermalized electron gas and how it is facilitated by high-density excitation. We also demonstrate that a large reduction of the refractive index by 80% dominates the nonequilibrium infrared response, which can be utilized for designing ultrafast switches in active optoelectronics.

cond-mat.mtrl-sci↗