arXiv subjects

Natsuki Mitsuishi

Publications and source records attributed to Natsuki Mitsuishi.

7 recordsLinked to original sources

arXiv2026

Momentum-dependent charge-density-wave gap formation in ZrTe_{2.98}Se_{0.02}

We investigated the energy gap formation across the charge density wave (CDW) transition inof ZrTe_{2.98}Se_{0.02}. By employing a laser photoemission microscopy, we clearly resolved one elliptical Fermi surface (FS) around the Brillouin zone (BZ) center, and two quasi-one-dimensional FSs along the BZ boundary. We further mapped the intensity difference between the FSs below and above the CDW transition temperature. We found that the energy CDW gap formation is limited to the momentum region 0.25 Å^{-1} < ky < 0.8 Å^{-1} along \bar{B}-\bar{D} line, which coincides with the location of one of the quasi-one-dimensional FSs. Characteristic momentum dependence in the energy CDW gap suggests the importance of both FS nesting and band-dependent electron-phonon coupling for understanding the CDW state in ZrTe_{3} system.

cond-mat.other↗

arXiv2026

Fermi surface of Kagome metal CsCr$_3$Sb$_5$ observed by laser photoemission microscopy

We investigated the Fermi surface (FS) in the paramagnetic state of Kagome metal CsCr$_3$Sb$_5$ by employing a laser photoemission microscopy. We found a circular FS and two hexagonal FSs around the Brillouin zone (BZ) center. Polarization-dependent measurements further enable us to detect small FS pockets at the BZ boundary. According to the density functional theory calculations, the orbital characters of the FSs were determined from their shape and orientations. We found that the size of the FS is strongly modified for the d$_{xz}$ orbital, suggesting the orbital-dependent correlation effect. These results provide an electronic basis for exploring the interplay of antiferromagnetic/charge density wave order and possible unconventional superconductivity in this compound.

cond-mat.str-el↗

arXiv2025

Direct observation of band structure modifications from monolayer WSe2 to Janus WSSe

Janus monolayer transition metal dichalcogenides (TMDs), created by post-growth substitution of the top chalcogen layer, represent a new direction for engineering 2D crystal properties. However, their rapid ambient degradation and the difficulty of obtaining large-area monolayer samples have limited the available experimental probes, leaving their detailed electronic structure near the Fermi level largely unexplored. In this work, by performing micro-focused angle-resolved photoemission spectroscopy (μ-ARPES) on an identical sample transformed from monolayer WSe2 to Janus WSSe via a H2 plasma-assisted chalcogen-exchange method, we reveal the evolution of its electronic band structure. We observe ARPES signature consistent with the Rashba-type spin splitting due to broken horizontal mirror symmetry, and a significant upward shift of the highest valence band at the Γ-point by approximately 160 meV. These direct observations clarify the key electronic modifications that govern the material's properties and provide a pathway for band engineering in Janus TMDs.

cond-mat.mtrl-sci↗

arXiv2025

Electronic Structure of Kramers Nodal-Line Semimetal YAuGe and Anomalous Hall Effect Induced by Magnetic Rare-Earth Substitution

Nodal-line semimetals are a class of topological materials hosting one dimensional lines of band degeneracy. Kramers nodal-line (KNL) metals/semimetals have recently been theoretically recognized as a class of topological states inherent to all non-centrosymmetric achiral crystal lattices. We investigate the electronic structure of candidate KNL semimetal YAuGe by angle-resolved photoemission spectroscopy (ARPES) and quantum oscillations as well as by density functional theory (DFT) calculations. DFT has revealed that YAuGe hosts KNLs on the G-A-L-M plane of the Brillouin zone, that are protected by the time reversal and mirror-inversion symmetries. Through ARPES and quantum oscillations we identify signatures of hole bands enclosing the G point, and the observed splitting of quantum oscillation frequency with angle is attributed to spin-orbit-coupling-induced band splitting away from the KNLs. Furthermore, we show that the degeneracy of the nodal lines along the G-A line is lifted by the time-reversal-symmetry breaking when the Y is substituted by magnetic R ions (R = rare earth). This becomes a source of Berry curvature and contributes to the anomalous Hall effect in magnetic RAuGe. These findings establish RAuGe as a new class of KNL semimetals offering significant potential for engineering of anomalous magnetotransport properties via magnetic rare-earth substitution.

cond-mat.mtrl-sci↗

arXiv2024

Electronic Landscape of Group-5 Transition Metal Ditellurides $M$Te$_2$ ($M$ = V, Nb, Ta): Multiple Crystal Phases with Local Bonds and Flat Bands

Group-5 transition metal ditellurides $M$Te$_2$ ($M$ = V, Nb, Ta) are unique CdI$_2$-type layered materials that exhibit peculiar quasi-one-dimensional intralayer superstructures, known as ribbon-chains and butterfly-like clusters of $M$ atoms. In this review article, we attempt to systematically understand their electronic band structures based on our recent angle-resolved photoemission spectroscopy (ARPES) studies and first-principles calculations. We underscore the role of the localized molecular-like orbital bonds that form the anomalous flat bands in the momentum space, and demonstrate how they influence the Fermi surface anisotropy, phase stabilities of crystal structures, and nontrivial topological properties in some cases. We also elaborate the future prospects for novel quantum phenomena that can be realized in these materials.

cond-mat.mtrl-sci↗

arXiv2024

Unveiling the orbital-selective electronic band reconstruction through the structural phase transition in TaTe$_2$

Tantalum ditelluride TaTe$_2$ belongs to the family of layered transition metal dichalcogenides but exhibits a unique structural phase transition at around 170 K that accompanies the rearrangement of the Ta atomic network from a "ribbon chain" to a "butterfly-like" pattern. While multiple mechanisms including Fermi surface nesting and chemical bonding instabilities have been intensively discussed, the origin of this transition remains elusive. Here we investigate the electronic structure of single-crystalline TaTe$_2$ with a particular focus on its modifications through the phase transition, by employing core-level and angle-resolved photoemission spectroscopy combined with first-principles calculations. Temperature-dependent core-level spectroscopy demonstrates a splitting of the Ta $4f$ core-level spectra through the phase transition indicative of the Ta-dominated electronic state reconstruction. Low-energy electronic state measurements further reveal an unusual kink-like band reconstruction occurring at the Brillouin zone boundary, which cannot be explained by Fermi surface nesting or band folding effects. On the basis of the orbital-projected band calculations, this band reconstruction is mainly attributed to the modifications of specific Ta $5d$ states, namely the $d_{XY}$ orbitals (the ones elongating along the ribbon chains) at the center Ta sites of the ribbon chains. The present results highlight the strong orbital-dependent electronic state reconstruction through the phase transition in this system and provide fundamental insights towards understanding complex electron-lattice-bond coupled phenomena.

cond-mat.str-el↗

arXiv2023

Ultrafast Control of Crystal Structure in a Topological Charge-Density-Wave Material

Optical control of crystal structures is a promising route to change physical properties including topological nature of a targeting material. Time-resolved X-ray diffraction measurements using the X-ray free-electron laser are performed to study the ultrafast lattice dynamics of VTe$_2$, which shows a unique charge-density-wave (CDW) ordering coupled to the topological surface states as a first-order phase transition. A significant oscillation of the CDW amplitude mode is observed at a superlattice reflection as well as Bragg reflections. The frequency of the oscillation is independent of the fluence of the pumping laser, which is prominent to the CDW ordering of the first-order phase transition. Furthermore, the timescale of the photoinduced 1$T^{\prime\prime}$ to 1$T$ phase transition is independent of the period of the CDW amplitude mode.

cond-mat.str-el↗