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Natsuki Okada

Publications and source records attributed to Natsuki Okada.

4 recordsLinked to original sources

Superconductivity-enhanced phonon angular momentum

We theoretically investigate the properties of phonon angular momentum in the superconducting state, using fulleride compounds in an external magnetic field as a model system. The electron orbital angular momentum injected by an external field is transferred to the phonon subsystem via electron--phonon coupling. We show that this field-induced phonon angular momentum is significantly enhanced and undergoes a sign reversal upon entering the superconducting state. In the normal state, the dominant energy scale governing the response function is the electronic bandwidth $D$. In the superconducting state, the phonon energy scale $\omega_1$ enters the denominator, leading to an enhancement of order $D/\omega_1$. The observed sign change in the response can be explained by the competition between Fermi surface and Fermi volume contributions.

cond-mat.supr-con

Symmetry-breaking perturbations in the Jahn-Teller-Hubbard model

We study the effect of symmetry-breaking perturbations in the multiorbital Hubbard model coupled to anisotropic Jahn-Teller phonons, which is relevant for the description of fulleride superconductors. This system is often approximated by a model with static antiferromagnetic (AFM) Hund's coupling, in which the coupling to the Jahn-Teller phonon is effectively described, but the retardation effect associated with phonon propagation is neglected. We compare the properties of the models with static AFM Hund's coupling and dynamical Jahn-Teller electron-phonon interaction by means of the Eliashberg theory. Considering the susceptibilities for the spin, magnetic orbital, electric orbital, and superconductivity, we reveal a qualitatively different behavior between the two models in the case of the magnetic orbital susceptibility. We further study the effect of a magnetic field on the $s$-wave spin-singlet superconducting state. In the presence of the field, the magnetic orbital susceptibility becomes nonzero due to a combination of multiorbital and retardation effects, while the spin susceptibility remains zero at low temperatures. By analyzing this phenomenon both numerically and analytically, we clarify that odd-frequency pairs induced by the magnetic field play a crucial role in the spin and orbital magnetic susceptibilities. Thus, the magnetic degrees of freedom produce interesting behaviors in the presence of retardation effects associated with electron-phonon coupling.

cond-mat.supr-con

Weak coupling approach to magnetic and orbital susceptibilities for superconducting states in multiorbital electron-phonon coupled model

Alkali-doped fullerides are molecular-based superconductors with multiple active orbitals. In this paper, using the Eliashberg theory with the retardation effect of Jahn-Teller phonons, we study the response of the spin-singlet superconducting state relevant to fulleride materials. The spin Zeeman field is not active for the singlet pairing state, and the magnetic orbital field, which physically generates a circular electron motion inside the fullerene molecule, is also shown to be inactive. On the other hand, the electric orbital (or quadrupolar) field, which corresponds to a uniaxial distortion, remains active across the superconducting phase transition. This is understood by the orbital-symmetric structure of the Cooper pair, which is susceptible to the electric orbital field, while it is not the case for the magnetic orbital field which tends to create an antisymmetric part.

cond-mat.supr-con

Low-rank quantics tensor train representations of Feynman diagrams for multiorbital electron-phonon models

Feynman diagrams are an essential tool for simulating strongly correlated electron systems. However, stochastic quantum Monte Carlo sampling suffers from the sign problem, particularly when solving a multiorbital quantum impurity model. Recently, two approaches have been proposed for efficient numerical treatment of Feynman diagrams: Tensor Cross Interpolation (TCI) to replace stochastic sampling and the Quantics Tensor Train (QTT) representation for compressing space-time dependence. One of the remaining challenges is the nontrivial task of identifying low-rank structures in weak-coupling Feynman diagrams for multiorbital electron-phonon systems. In particular, the traditional TCI algorithm faces an ergodicity problem, which prevents it from fully exploring the multiorbital space. To address this, we incorporate a new algorithm called global search, which resolves this issue. By combining this approach with QTT, we uncover low-rank structures and achieve efficient numerical integration with exponential resolution in time and faster-than-power-law convergence of error relative to computational cost. Additionally, our approach does not require the division of discontinuous regions necessary in non-quantics TCI.

cond-mat.str-el