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Nazanin Hoghooghi

Publications and source records attributed to Nazanin Hoghooghi.

At least 19 recordsLinked to original sources

Redefining the limits of real-time noise cancellation in optical fiber links

A broad and growing array of applications rely on the faithful transmission of ultrastable optical signals over noisy paths, requiring cancellation of environmentally induced noise. A generally accepted limit constrains how well the path length noise can be suppressed in real time. Here, we show that this standard limit is not fundamental and can be improved upon. By considering the temporal correlations between the round-trip and one-way signals, we develop a new framework for optimizing the noise cancellation feedback signal for any spatial distribution of noise along the signal path. We use this framework to surpass the standard limit in two sets of experiments. First, we demonstrate noise cancellation in a deployed urban optical fiber, where we achieve noise suppression approximately 6 dB beyond the standard limit. Then, in a reconfigurable lab-based fiber-optic testbed, we show that, for certain spatial distributions of noise, suppression of well over 10 dB beyond the standard limit is readily achievable. With the use of digital signal processing to generate the correction signal, our new technique requires no new electro-optic hardware relative to the field-standard noise cancellation scheme. This will allow for widespread adoption of these improved limits in existing systems, with applications in optical clock distribution, optical clock comparisons for fundamental physics and geodesy, and quantum networking.

physics.optics↗

Fiber Link Stabilization with a Multicore Fiber Amplifier

We study the use of separate cores of a multicore erbium-doped fiber amplifier (MC-EDFA) in a noise-canceled link for ultrastable optical frequency transfer. We demonstrate fractional frequency instability of $5\times10^{-19}$ at 1000 s averaging time for the stabilized MC-EDFA alone and $1.4\times10^{-18}$ at 1000 s averaging time when integrated with a 40 km-long 7-core spooled fiber. This study further establishes multicore fiber (MCF) networks as a promising platform for ultrastable frequency transfer, serving as an important step toward incorporating precision time and frequency distribution into future MCF communication infrastructures.

physics.optics↗

Visible dual-comb spectroscopy across more than 100 THz with lithium niobate nanophotonic waveguides

Broadband and high-resolution spectroscopy in the visible and ultraviolet is central to advances in multiple fields, including fundamental quantum physics, biology, atmospheric science and astronomy. Traditionally, these measurements are performed with grating or Fourier-transform spectrometers using incoherent light sources. Leveraging coherent light enables powerful frequency-comb-based techniques, but is limited by the technical complexity of efficiently generating broad spectral bandwidths from relatively narrowband and spectrally distant laser sources. Current visible dual-comb spectrometers require implicit compromises between optical bandwidth, experimental simplicity, and acquisition speed. In this work, we introduce a simple and efficient dual-comb spectrometer that converts robust Er:fiber frequency combs from the near-infrared to the ultraviolet and visible with thin-film lithium niobate (TFLN) nanophotonic waveguides. Using real-time signal processing, we retrieve coherently averaged dual-comb spectra over nearly 120 THz of simultaneous bandwidth in the visible with 100 MHz spectral resolution. With these capabilities, we measure the broadband absorption spectrum of molecular iodine (I2), demonstrating the broadest visible spectral coverage of a dual-comb spectrometer to date. Additional measurements of NO2, atomic rubidium, and atomic sodium further illustrate the achievable combination of spectroscopic bandwidth, resolution, and intrinsic frequency accuracy. Our results demonstrate the powerful integration of low-power frequency combs, nonlinear nanophotonics, and digital signal processing to enable a compact, efficient and versatile approach to high-resolution mapping of complex absorption spectra across 500 THz in the UV-visible and near-infrared spectral regions for multiple applications beyond the research lab

physics.optics↗

Sub-femtosecond stabilization of multicore fiber for high-fidelity quantum networking at 100% duty cycle

Originally envisioned as a solution for the capacity crunch in telecommunications networks, multicore fibers (MCF) are contributing to scientific fields beyond telecom, such as sensing and metrology. Confined within the same cladding, the cores of MCF have a high degree of noise correlation which can be harnessed for a variety of applications. Here, we investigate MCF as a solution to the challenging problem of quantum and classical light co-existence in quantum networks by operating the quantum and stabilization light in separate but highly correlated cores of a 7-core MCF. Over 40 km of spooled fiber, we achieved 100 attosecond integrated jitter on one core by using phase information derived from another core. This allows for 100% duty cycle on a quantum channel while maintaining a low spurious photon rate from crosstalk between stabilization and quantum channels. With cycle-slip-free stabilization over 6 hours, frequency detuning between designated stabilization and quantum channels, and an additional 40 dB rejection of noise photons provided by the low optical crosstalk between cores, we achieved a Raman scattering-induced spurious photon rate of only 0.01 photons/s in 100 GHz bandwidth. Our results with MCF are a promising approach to ultra-stable quantum networks with 100% duty cycle on the quantum channel.

physics.optics↗

Dual-comb correlation spectroscopy of thermal light

The detection of light of thermal origin is the principal means by which humanity has learned about our world and the cosmos. In optical astronomy, in particular, direct detection of thermal photons and the resolution of their spectra have enabled discoveries of the broadest scope and impact. Such measurements, however, do not capture the phase of the thermal fields--a parameter that has proven crucial to transformative techniques in radio astronomy such as synthetic aperture imaging. Over the last 25 years, tremendous progress has occurred in laser science, notably in the phase-sensitive, broad bandwidth, high resolution, and traceable spectroscopy enabled by the optical frequency comb. In this work, we directly connect the fields of frequency comb laser spectroscopy and passive optical sensing as applied to astronomy, remote sensing, and atmospheric science. We provide fundamental sensitivity analysis of dual-comb correlation spectroscopy (DCCS), whereby broadband thermal light is measured via interferometry with two optical frequency combs. We define and experimentally verify the sensitivity scaling of DCCS at black body temperatures relevant for astrophysical observations. Moreover, we provide comparison with direct detection techniques and more conventional laser heterodyne radiometry. Our work provides the foundation for future exploration of comb-based broadband synthetic aperture hyperspectral imaging across the infrared and optical spectrum.

physics.optics↗

From ultra-noisy to ultra-stable: optimization of the optoelectronic laser lock

We demonstrate thermal-noise-limited direct locking of a semiconductor distributed feedback (DFB) laser to a sub-1 mL volume, ultrastable optical cavity, enabling extremely compact and simple ultrastable laser systems. Using the optoelectronic laser locking method, we realize over 140 dB suppression of the DFB free-running laser noise at 10 Hz offset, a level we estimate to be ~ 70 dB greater than Pound-Drever-Hall locking can provide, and reach a phase noise level of -120 dBc/Hz at 200 kHz offset. We also demonstrate a new feedforward noise correction method that improves the quality of the heterodyne beat with an optical frequency comb by providing another 60 dB of laser noise rejection - a level that is 15 dB greater than predicted by current models. With feedforward, we transfer the cavity thermal noise limit across the comb spectrum despite the fact that the cavity-locked laser itself is noisy. These results establish a simple, low noise, compact approach to ultrastable laser locking that is compatible with integrated photonics, with applications in low phase noise microwave generation, sensing, and satellite ranging.

physics.optics↗

Enabling a multifunctional telecommunications fiber optic network: Ultrastable optical frequency transfer and attosecond timing in deployed multicore fiber

The telecommunications industry's deployment of billions of kilometers of optical fiber has created a vast global network that can be exploited for additional applications such as environmental sensing, quantum networking and international clock comparisons. However, for reasons such as the unidirectionality of long-haul fiber links, telecom fiber networks cannot always be adapted for important applications beyond data transmission. Fortunately, new multicore optical fibers create the opportunity for application coexistence with data traffic, creating expansive multifunctional networks. Towards that end, we propose and demonstrate the faithful transfer of ultrastable optical signals through multicore fiber in a way that is compatible with the unidirectionality of long-haul fiber optic systems, demonstrating a fractional frequency instability of 3x10-19 at 10,000 seconds. This opens the door towards intercontinental optical clock comparisons, with applications in fundamental physics and the redefinition of the second.

physics.optics↗

Dual-Comb Photothermal Microscopy

We introduce a new parallelized approach to photothermal microscopy that utilizes mid-infrared dual-comb lasers, enabling simultaneous measurements at hundreds of wavelengths. This technology allows for high-speed, label-free chemical identification with super-resolution infrared imaging, overcoming the limitations of slow, single-wavelength-laser methods.

physics.optics↗

Mid-Infrared Hyperspectral Microscopy with Broadband 1-GHz Dual Frequency Combs

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of broadband sources can provide a third dimension of chemical specificity. However, to enable widespread deployment, mid-infrared microscopy platforms need to be compact and robust while offering high speed, broad bandwidth and high signal-to-noise ratio (SNR). In this study, we experimentally showcase the integration of a broadband, high-repetition-rate dual-comb spectrometer (DCS) in the mid-infrared range with a scanning microscope. We employ a set of 1-GHz mid-infrared frequency combs, demonstrating their capability for high-speed and broadband hyperspectral imaging of polymers and ovarian tissue. The system covers 1000 $\mathrm{cm^{-1}}$ at $\mathrm{ν_c=2941 \; cm^{-1}}$ with 12.86 kHz spectra acquisition rate and 5 $\mathrm{μm}$ spatial resolution. Taken together, our experiments and analysis elucidate the trade-off between bandwidth and speed in DCS as it relates to microscopy. This provides a roadmap for the future advancement and application of high-repetition-rate DCS hyperspectral imaging.

physics.optics↗

Ultrastable vacuum-gap Fabry-Pérot cavities operated in air

We demonstrate a vacuum-gap ultrastable optical reference cavity that does not require a vacuum enclosure. Our simple method of optical contact bonding in a vacuum environment allows for cavity operation in air while maintaining vacuum between the cavity mirrors. Vacuum is maintained long term, with no observed degradation in cavity stability for over 1 year after bonding. For a 1550 nm laser stabilized to a 9.7 mL in-vacuum bonded cavity, the measured Allan deviation is $2.4\times 10^{-14}$ at 1 s and its phase noise is thermal-noise-limited from 0.1 Hz to 10 kHz, reaching about -105 dBc/Hz at 10 kHz offset frequency. This represents the highest stability of any oscillator operated without a vacuum enclosure. Furthermore, we demonstrate a 0.5 mL in-vacuum bonded cavity created using microfabricated mirrors and cavity dicing, with phase noise reaching -95 dBc/Hz at 10 kHz offset frequency. By relieving the need for high-vacuum enclosures, we greatly enhance the portability and utility of low noise, compact cavity-stabilized lasers, with applications ranging from environmental sensing to mobile optical clocks to ultralow noise microwave generation.

physics.optics↗

Temperature, Pressure, Velocity, and Water Vapor Mole Fraction Profiles in a Ramjet Combustor using Dual Frequency Comb Spectroscopy and a High Temperature Absorption Database

Accurate diagnostics of the combustor region of ramjet engines can improve engine design and create benchmarks for computational fluid dynamics models. Previous works demonstrate that dual frequency comb spectroscopy can provide low uncertainty diagnostics of multiple flow parameters in the non-combusting regions of ramjets. However, the high temperatures present in the combustor present a challenge for broadband spectroscopic absorption models that are used to interpret measurements in these regions. Here, we utilize a new water vapor absorption database created for high temperature water-air mixtures to fit spectra measured in a ground-test ramjet engine with a broadband near-infrared dual comb absorption spectrometer. We extract 2D profiles of pressure, temperature, water mole fraction, and velocity using this new database. We demonstrate that the new database provides the lowest fit residuals compared to other water vapor absorption databases. We compare computational fluid dynamics simulations of the combustor with the measured data to demonstrate that the simulations overpredict heat release and water vapor production.

physics.flu-dyn↗

Complete reactants-to-products observation of a gas-phase chemical reaction with broad, fast mid-infrared frequency combs

Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing diagnostic approaches provide incomplete information. For example, mass spectrometry is optimized to gather snapshots of the presence of many chemical species, while conventional laser spectroscopy can quantify a single chemical species through time. Here we optimize for multiple objectives by introducing a high-speed and broadband, mid-infrared dual frequency comb absorption spectrometer. The optical bandwidth of >1000 cm-1 covers absorption fingerprints of many species with spectral resolution <0.03 cm-1 to accurately discern their absolute quantities. Key to this advance are 1 GHz pulse repetition rate frequency combs covering the 3-5 um region that enable microsecond tracking of fast chemical process dynamics. We demonstrate this system to quantify the abundances and temperatures of each species in the complete reactants-to-products breakdown of 1,3,5-trioxane, which exhibits a formaldehyde decomposition pathway that is critical to modern low temperature combustion systems. By maximizing the number of observed species and improving the accuracy of temperature and concentration measurements, this spectrometer advances understanding of chemical reaction pathways and rates and opens the door for novel developments such as combining high-speed chemistry with machine learning.

physics.chem-ph↗

Spatially resolved mass flux measurements with dual comb spectroscopy

Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate that laser absorption spectroscopy with mode-locked frequency combs can simultaneously measure all of the components of mass flux (velocity, temperature, pressure, and species mole fraction) with low uncertainty, spatial resolution corresponding to the laser line of sight, and no supplemental sensor readings. The low uncertainty is provided by the broad spectral bandwidth, high resolution, and extremely well-known and controlled frequency axis of stabilized, mode-locked frequency combs. We demonstrate these capabilities using dual frequency comb spectroscopy (DCS) in the isolator of a ground-test supersonic propulsion engine at Wright-Patterson Air Force Base. The mass flux measurements are consistent within 3.6% of the facility-level engine air supply values. A vertical scan of the laser beams in the isolator measures the spatially resolved mass flux, which is compared with computational fluid dynamics simulations. A rigorous uncertainty analysis demonstrates a instrument uncertainty of ~0.4%, and total uncertainty (including non-instrument sources) of ~7% for mass flux measurements. These measurements demonstrate DCS with mode-locked frequency combs as a low-uncertainty mass flux sensor for a variety of applications.

physics.app-ph↗

Supersonic Combustion Diagnostics with Dual Comb Spectroscopy

Supersonic engine development requires accurate and detailed measurements of fluidic and thermodynamic parameters to optimize engine designs and benchmark computational fluid dynamic (CFD) simulations. Here, we demonstrate that dual frequency comb spectroscopy (DCS) with mode-locked frequency combs can provide simultaneous absolute measurements of several flow parameters with low uncertainty across a range of conditions owing to the broadband and ultrastable optical frequency output of the lasers. We perform DCS measurements across a 6800-7200 cm-1 bandwidth covering hundreds of H2O absorption features resolved with a spectral point spacing of 0.0067 cm-1 and point spacing precision of 1.68 x 10-10 cm-1. We demonstrate 2D profiles of velocity, temperature, pressure, water mole fraction, and air mass flux in a ground-test dual-mode ramjet at Wright-Patterson Air Force Base. The narrow angles of the measurement beams offer sufficient spatial resolution to resolve properties across an oblique shock train in the isolator and the thermal throat of the combustor. We determine that the total measurement uncertainties for the various parameters range from 1% for temperature to 9% for water vapor mole fraction, with the absorption database/model that is used to interpret the data typically contributing the most uncertainty (leaving the door open for even lower uncertainty in the future). CFD at the various measurement locations show good agreement, largely falling within the DCS measurement uncertainty for most profiles and parameters.

physics.app-ph↗

1-GHz mid-infrared frequency comb spanning 3 to 13 μm

Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously combine the high-speed, high spectral resolution, and broad optical bandwidth needed to accurately study complex, transient events in chemistry, combustion, and microscopy. However, such a spectrometer has not yet been demonstrated due to the lack of GHz MIR frequency combs with broad and full spectral coverage. Here, we introduce the first broadband MIR frequency comb laser platform at 1 GHz repetition rate that achieves spectral coverage from 3 to 13 μm. This frequency comb is based on a commercially available 1.56 μm mode-locked laser, robust all-fiber Er amplifiers and intra-pulse difference frequency generation (IP-DFG) of few-cycle pulses in \c{hi}(2) nonlinear crystals. When used in a dual comb spectroscopy (DCS) configuration, this source will simultaneously enable measurements with μs time resolution, 1 GHz (0.03 cm-1) spectral point spacing and a full bandwidth of >5 THz (>166 cm-1) anywhere within the MIR atmospheric windows. This represents a unique spectroscopic resource for characterizing fast and non-repetitive events that are currently inaccessible with other sources.

physics.optics↗

Single-cycle all-fiber frequency comb

Single-cycle pulses with deterministic carrier-envelope phase enable the study and control of light-matter interactions at the sub-cycle timescale, as well as the efficient generation of low-noise multi-octave frequency combs. However, current single-cycle light sources are difficult to implement and operate, hindering their application and accessibility in a wider range of research. In this paper, we present a single-cycle 100 MHz frequency comb in a compact, turn-key, and reliable all-silica-fiber format. This is achieved by amplifying 2 $μ$m seed pulses in heavily-doped Tm:fiber, followed by cascaded self-compression to yield 6.8 fs pulses with 215 kW peak power and 374 mW average power. The corresponding spectrum covers more than two octaves, from below 700 nm up to 3500 nm. Driven by this single-cycle pump, supercontinuum with 180 mW of integrated power and a smooth spectral amplitude between 2100 and 2700 nm is generated directly in silica fibers. To broaden applications,few-cycle pulses extending from 6 $μ$m to beyond 22 $μ$m with long-term stable carrier-envelope phase are created using intra-pulse difference frequency, and electro-optic sampling yields comb-tooth-resolved spectra. Our work demonstrates the first all-fiber configuration that generates single-cycle pulses, and provides a practical source to study nonlinear optics on the same timescale.

physics.optics↗

Demonstration of a uniform, high-pressure, high-temperature gas cell with a dual frequency comb absorption spectrometer

Accurate absorption models for gases at high pressure and temperature support advanced optical combustion diagnostics and aid in the study of harsh planetary atmospheres. Developing and validating absorption models for these applications requires recreating the extreme temperature and pressure conditions of these environments in static, uniform, well-known conditions in the laboratory. Here, we present the design of a new gas cell to enable reference-quality absorption spectroscopy at high pressure and temperature. The design centers on a carefully controlled quartz sample cell housed at the core of a pressurized ceramic furnace. The half-meter sample cell is relatively long compared to past high- pressure and temperature absorption cells, and is surrounded by a molybdenum heat spreader that enables high temperature uniformity over the full length of the absorbing gas. We measure the temperature distribution of the sample gas using in situ thermocouples, and fully characterize the temperature uniformity across a full matrix of conditions up to 1000 K and 50 bar. The results demonstrate that the new design enables highly uniform and precisely known conditions across the full absorbing path length. Uniquely, we test the new gas cell with a broadband, high-resolution dual frequency comb spectrometer that enables highly resolved absorption spectroscopy across a wide range of temperature and pressure conditions. With this system, we measure the spectrum of CO$_2$ between 6800 and 7000 cm$^{-1}$ at pressures between 0.2 and 20 bar, and temperatures up to 1000 K. The measurements reveal discrepancies from spectra predicted by the HITRAN2016 database with a Voigt line shape at both low- and high-pressure conditions. These results motivate future work to expand absorption models and databases to accurately model high-pressure and -temperature spectra in combustion and planetary science research.

physics.ins-det↗

Fully phase-stabilized 1 GHz turnkey frequency comb at 1.56 $μ$m

Low noise and high repetition rate optical frequency combs are desirable for many applications from timekeeping to precision spectroscopy. For example, gigahertz repetition rate sources greatly increase the acquisition speed of spectra in a dual-comb modality when compared to lower repetition rate sources, while still maintaining sufficient instantaneous resolution to resolve ro-vibrational signatures from molecules in a variety of conditions. In this paper, we present the stabilization and characterization of a turnkey commercial 1~GHz mode-locked laser that operates at telecom wavelengths (1.56 $μ$m). Fiber amplification and spectral broadening result in the high signal-to-noise ratio detection and stabilization of $\textit{f}_{\textit{ceo}}$ with 438 mrad of residual phase noise (integrated from 10$^2$ to 10$^7$ Hz). Simultaneously, we stabilize the beatnote between the nearest comb mode and a cavity stabilized continuous-wave laser at 1.55 $μ$m with 41 mrad of residual phase noise (integrated from 10$^2$ to 10$^7$ Hz). This robust, self-referenced comb system is built with off-the-shelf polarization-maintaining fiber components and will be useful for a wide range of low noise frequency comb applications that benefit from the increased repetition rate.

physics.optics↗