arXiv subjects

Neil Sinclair

Publications and source records attributed to Neil Sinclair.

At least 19 recordsLinked to original sources

arXiv2026

Increased cyclicity of atomic transitions via coherent interference of decay paths

Optical readout is a fundamental tool in atomic state measurement, yet the fidelity of optical readout is frequently limited by imperfect photon collection. This can be mitigated when readout occurs on a cycling transition which continuously fluoresces under resonant excitation, thus increasing signal and enabling single-shot readout. We present a method to extend the cyclicity of atomic transitions via coherent destructive interference between spurious decay paths. We describe the characteristics of atomic systems in which this method can be implemented and model several examples in which the number of emitted photons is increased by multiple orders of magnitude.

quant-ph↗

arXiv2026

Heterogeneous Transfer of Thin Film BaTiO$_3$ onto Silicon for Device Fabrication

Thin film BaTiO$_3$ has one of the highest known Pockels coefficients (>1200 pm/V), making it an attractive material for use in electro-optic devices. It is advantageous to integrate BaTiO$_3$ on silicon to enable complementary metal-oxide-semiconductor (CMOS) compatible processing. However, synthesis of high-quality BaTiO$_3$ directly on silicon remains a challenge. Here, we synthesize BaTiO$_3$ using hybrid metal-organic molecular beam epitaxy (hMBE) and demonstrate its transfer onto silicon using thermocompression bonding and chemical lift-off. Hybrid metal-organic MBE enables self-regulated synthesis of highly stoichiometric thin films at high growth rates (>100nm/hr). Our transfer method results in millimeter-scale areas of atomically flat, crack-free BaTiO$_3$ making it a potentially scalable method. Finally, we demonstrate the applicability of our process to device fabrication through characterization of lithographically-patterned and etch-transferred sub-micron features.

cond-mat.mtrl-sci↗

arXiv2025

Spectral-temporal processing using integrated recursive electro-optic circuit

Advances in integrated photonics have enabled unprecedented level of control of light, powering a wide range of photonic technologies from communications and computing to precision metrology and quantum information. However, the conventional on-chip optical signal processing approaches based on optical waveguides and cavities suffer from their large physical footprint and narrow operating bandwidth, respectively. To address this, we propose and experimentally demonstrate, using the thin film lithium niobate (TFLN) photonics, a modular, recursive optical signal processing framework. In our approach, fast electro-optic (EO) switch is used to either keep an optical packet inside the loop, with the processing element embedded within, or to release it from the loop and direct it towards the output waveguide. By configuring the switch on a timescale shorter than a time the photon spends traversing the loop, this architecture can achieve different optical pathlengths in a compact footprint without sacrificing optical bandwidth. As an example, we embed a phase-modulator (PM) inside the loop and demonstrate a frequency shift of optical packets up to 420 GHz, using only a 3 GHz sinusoidal microwave signal. By replacing the PM with chirped Bragg gratings (CBG), we demonstrate recursive delay line featuring large group delays of 28 ps/nm over a 30 nm optical bandwidth. Finally, by introducing asymmetric Mach-Zehnder interferometer (AMZI) inside the loop, we demonstrate a reconfigurable differentiation of the optical packet in time, up to an unprecedented fifth-order. Our results establish a powerful and scalable platform for multifunctional photonic processing, setting the stage for next-generation integrated systems with ultrahigh reconfigurability and spectral-temporal versatility.

physics.optics↗

arXiv2025

Universal dynamics and microwave control of programmable cavity electro-optic frequency combs

Electro-optic (EO) frequency combs are foundational for metrology and spectroscopy. Specifically, microresonator-based cavity EO combs are distinguished by efficient sideband generation, precisely controlled by microwave signals, enabling high-performance integrated frequency references and pulse sources. However, the apparent simplicity of these devices, often described by the EO modulation-induced coupling of nearest-neighbor cavity modes, has limited investigations of their fundamental physics, thereby restricting their full potential. Here, we uncover the universal dynamics and complete frequency lattice connectivity underpinning cavity EO microcombs, as well as characterize the full space of nonlinear optical states, controlled by modulation depth and optical detuning, using the thin-film lithium niobate photonic platform. Leveraging this understanding, we design complex long-range couplings between cavity modes to realize programmable spectro-temporal shaping of the generated combs and pulses. We achieve three technological advances, including repetition-rate flexibility, substantial comb bandwidth extension beyond traditional scaling laws, and resonantly-enhanced flat-top spectrum. Our results provide physical insights for synchronously driven cavity-based EO systems, broadly defined, paving the way for electrically controlled and electrically enhanced comb generators for next-generation photonic applications.

physics.optics↗

arXiv2025

Photonic quantum information with time-bins: Principles and applications

Long-range quantum communication, distributed quantum computing, and sensing applications require robust and reliable ways to encode transmitted quantum information. In this context, time-bin encoding has emerged as a promising candidate due to its resilience to mechanical and thermal perturbations, depolarization from refractive index changes, and birefringence in fiber optic media. Time-bin quantum bits (qubits) can be produced in various ways, and each implementation calls for different considerations regarding design parameters, component compatibility (optical, electrical, electro-optical), and measurement procedures. Here, we provide a comprehensive overview of experimental methods for preparing and characterizing time-bin qubits (TBQs) for quantum communication protocols, with an assessment of their advantages and limitations. We discuss challenges in transmitting TBQs over optical fibers and free-space channels, and methods to overcome them. We also analyze the selection of key time-bin parameters and component requirements across experiments. This leads us to explore the preparation and characterization of time-bin entanglement and examine requirements for interference of time-bins from separate sources. Further, we cover preparation and characterization techniques for high-dimensional time-bin states, namely qudits, and the generation of time-bin entangled qudit pairs. We review time-energy entanglement and key experimental realizations. Finally, we present notable applications of time-bin encoded quantum states, from quantum communication protocols to photonic quantum computation. This work serves as an accessible introduction and a comprehensive review of recent developments.

quant-ph↗

arXiv2025

Ultracoherent self-assembled diamond nanomechanics reveals superfluid dynamics

From gravitational-wave detection, protein force microscopy, to exploration of quantum-classical boundaries, many anticipated discoveries in fundamental science require improving measurement sensitivity limits. Through the fluctuation-dissipation theorem, mechanical dissipation sets the acoustic noise for this limit. Yet, even in high-purity crystals, the microscopic mechanisms responsible for the acoustic loss remain poorly understood. Tension-induced dissipation dilution offers a route to ultralow acoustic loss, but is challenging to implement in crystalline materials including single-crystal diamond. Here we realize a strain-engineered diamond nanomechanical platform using a liquid-assisted van der Waals self-assembly process that harnesses intrinsic surface forces to apply tensile stress exceeding 1 GPa. At cryogenic temperatures these resonators achieve quality factors beyond 10 billion (intrinsic material quality factors beyond 100 million). This exceptional coherence turns them into a sensitive probe for residual dissipation, elucidating three distinct two-level-system channels and one topological dissipation channel from a surface superfluid helium film. Our work shows how advancing mechanical coherence opens access to new regimes of physics in hybrid quantum systems, precision metrology, and condensed-matter physics.

cond-mat.mes-hall↗

arXiv2025

Satellites promise global-scale quantum networks

Academia, governments, and industry around the world are on a quest to build long-distance quantum communication networks for a future quantum internet. Using air and fiber channels, quantum communication quickly faced the daunting challenge of exponential photon loss with distance. Quantum repeaters were invented to solve the loss problem by probabilistically establishing entanglement over short distances and using quantum memories to synchronize the teleportation of such entanglement to long distances. However, due to imperfections and complexities of quantum memories, ground-based proof-of-concept repeater demonstrations have been restricted to metropolitan-scale distances. In contrast, direct photon transmission from satellites through empty space faces almost no exponential absorption loss and only quadratic beam divergence loss. A single satellite successfully distributed entanglement over more than 1,200 km. It is becoming increasingly clear that quantum communication over large intercontinental distances (e.g. 4,000-20,000 km) will likely employ a satellite-based architecture. This could involve quantum memories and repeater protocols in satellites, or memory-less satellite-chains through which photons are simply reflected, or some combination thereof. Rapid advancements in the space launch and classical satellite communications industry provide a strong tailwind for satellite quantum communication, promising economical and easier deployment of quantum communication satellites.

quant-ph↗

arXiv2025

Efficient and high-fidelity entanglement in cavity QED without high cooperativity

The so-called state-carving protocol generates high-fidelity entangled states at an atom-cavity interface without requiring high cavity cooperativity. However, this protocol is limited to 50\% efficiency, which restricts its applicability. We propose a simple modification to the state-carving protocol to achieve efficient entanglement generation, with unit probability in principle. Unlike previous two-photon schemes, ours employs only one photon which interacts with the atoms twice - avoiding separate photon detections which causes irrecoverable probability loss. We present a detailed description and performance evaluation of our protocol under non-ideal conditions. High fidelity of 0.999 can be achieved with cavity cooperativity of only 34. Efficient state-carving paves the way for large-scale entanglement generation at cavity-interfaces for modular quantum computing, quantum repeaters and creating arbitrary shaped atomic graph states, essential for one-way quantum computing.

quant-ph↗

arXiv2025

A sub-volt near-IR lithium tantalate electro-optic modulator

We demonstrate a low-loss integrated electro-optic Mach-Zehnder modulator in thin-film lithium tantalate at 737 nm, featuring a low half-wave voltage-length product of 0.65 V$\cdot$cm, an extinction ratio of 30 dB, low optical loss of 5.3 dB, and a detector-limited bandwidth of 20 GHz. A small $<2$ dB DC bias drift relative to quadrature bias is measured over 16 minutes using 4.3 dBm of on-chip power in ambient conditions, which outperforms the 8 dB measured using a counterpart thin-film lithium niobate modulator. Finally, an optical loss coefficient of 0.5 dB/cm for a thin-film lithium tantalate waveguide is estimated at 638 nm using a fabricated ring resonator.

physics.optics↗

arXiv2025

Robust Poling and Frequency Conversion on Thin-Film Periodically Poled Lithium Tantalate

We explore a robust fabrication process for periodically-poled thin-film lithium tantalate (PP-TFLT) by systematically varying fabrication parameters and confirming the quality of inverted domains with second-harmonic microscopy (SHM). We find a periodic poling recipe that can be applied to both acoustic-grade and optical-grade film, electrode material, and presence of an oxide interlayer. By using a single high-voltage electrical pulse with peak voltage time of 10 ms or less and a ramp-down time of 90 s, rectangular poling domains are established and stabilized in the PP-TFLT. We employ our robust periodic poling process in a controllable pole-after-etch approach to produce PP-TFLT ridge waveguides with normalized second harmonic generation (SHG) conversion efficiencies of 208 %W-1cm-2 from 1550 nm to 775 nm in line with the theoretical value of 244 %W-1cm-2. This work establishes a high-performance poling process and demonstrates telecommunications band SHG for thin-film lithium tantalate, expanding the capabilities of the platform for frequency mixing applications in quantum photonics, sensing, and spectroscopy.

physics.optics↗

arXiv2025

Analytical Modeling of Real-World Photonic Quantum Teleportation

We develop analytical models for realistic photonic quantum teleportation experiments with time-bin qubits, utilizing phase space methods from quantum optics. These models yield analytical expressions for Hong-Ou-Mandel interference visibilities and qubit fidelities, accounting for imperfections such as loss, photon distinguishability, and unwanted multi-photon events in single and entangled photon sources. Our expressions agree with the Hong-Ou-Mandel interference visibilities and teleportation fidelities reported by Valivarthi et al. (PRX Quantum 1, 020317, 2020). We use these models to predict and analyze the outcomes of future teleportation experiments under varying degrees of imperfections.

quant-ph↗

arXiv2025

Entanglement swapping systems toward a quantum internet

We demonstrate conditional entanglement swapping, i.e. teleportation of entanglement, between time-bin qubits at the telecommunication wavelength of 1536.4 nm with high fidelity of 87\%. Our system is deployable, utilizing modular, off-the-shelf, fiber-coupled, and electrically controlled components such as electro-optic modulators. It leverages the precise timing resolution of superconducting nanowire detectors, which are controlled and read out via a custom developed graphical user interface. The swapping process is described, interpreted, and guided using characteristic function-based analytical modeling that accounts for realistic imperfections. Our system supports quantum networking protocols, including source-independent quantum key distribution, with an estimated secret key rate of approximately 0.5 bits per sifted bit.

quant-ph↗

arXiv2025

Purcell-enhanced emissions from diamond color centers in slow light photonic crystal waveguides

Quantum memories based on emitters with optically addressable spins rely on efficient photonic interfaces, often implemented as nanophotonic cavities with ideally narrow spectral linewidths and small mode volumes. However, these approaches require nearly perfect spectral and spatial overlap between the cavity mode and quantum emitter, which can be challenging. This is especially true in the case of solid-state quantum emitters that are often randomly positioned and can suffer from significant inhomogeneous broadening. An alternative approach to mitigate these challenges is to use slow-light waveguides that can enhance light-matter interaction across large optical bandwidths and large areas. Here, we demonstrate diamond slow light photonic crystal (PhC) waveguides that enable broadband optical coupling to embedded silicon-vacancy (SiV) color centers. We take advantage of the recently demonstrated thin-film diamond photonic platform to fabricate fully suspended two-dimensional PhC waveguides. Using this approach, we demonstrate waveguide modes with high group indices up to 70 and observe Purcell-enhanced emissions of the SiVs coupled to the waveguide mode. Our approach represents a practical diamond platform for robust spin-photon interfaces with color centers.

quant-ph↗

arXiv2024

Integrated electro-optic digital-to-analog link for efficient computing and arbitrary waveform generation

The rapid growth in artificial intelligence and modern communication systems demands innovative solutions for increased computational power and advanced signaling capabilities. Integrated photonics, leveraging the analog nature of electromagnetic waves at the chip scale, offers a promising complement to approaches based on digital electronics. To fully unlock their potential as analog processors, establishing a common technological base between conventional digital electronic systems and analog photonics is imperative to building next-generation computing and communications hardware. However, the absence of an efficient interface has critically challenged comprehensive demonstrations of analog advantage thus far, with the scalability, speed, and energy consumption as primary bottlenecks. Here, we address this challenge and demonstrate a general electro-optic digital-to-analog link (EO-DiAL) enabled by foundry-based lithium niobate nanophotonics. Using purely digital inputs, we achieve on-demand generation of (i) optical and (ii) electronic waveforms at information rates up to 186 Gbit/s. The former addresses the digital-to-analog electro-optic conversion challenge in photonic computing, showcasing high-fidelity MNIST encoding while consuming 0.058 pJ/bit. The latter enables a pulse-shaping-free microwave arbitrary waveform generation method with ultrabroadband tunable delay and gain. Our results pave the way for efficient and compact digital-to-analog conversion paradigms enabled by integrated photonics and underscore the transformative impact analog photonic hardware may have on various applications, such as computing, optical interconnects, and high-speed ranging.

physics.optics↗

arXiv2024

Integrated lithium niobate photonic computing circuit based on efficient and high-speed electro-optic conversion

Here we show a photonic computing accelerator utilizing a system-level thin-film lithium niobate circuit which overcomes this limitation. Leveraging the strong electro-optic (Pockels) effect and the scalability of this platform, we demonstrate photonic computation at speeds up to 1.36 TOPS while consuming 0.057 pJ/OP. Our system features more than 100 thin-film lithium niobate high-performance components working synergistically, surpassing state-of-the-art systems on this platform. We further demonstrate binary-classification, handwritten-digit classification, and image classification with remarkable accuracy, showcasing our system's capability of executing real algorithms. Finally, we investigate the opportunities offered by combining our system with a hybrid-integrated distributed feedback laser source and a heterogeneous-integrated modified uni-traveling carrier photodiode. Our results illustrate the promise of thin-film lithium niobate as a computational platform, addressing current bottlenecks in both electronic and photonic computation. Its unique properties of high-performance electro-optic weight encoding and conversion, wafer-scale scalability, and compatibility with integrated lasers and detectors, position thin-film lithium niobate photonics as a valuable complement to silicon photonics, with extensions to applications in ultrafast and power-efficient signal processing and ranging.

physics.optics↗

arXiv2024

Free-space quantum information platform on a chip

Emerging technologies that employ quantum physics offer fundamental enhancements in information processing tasks, including sensing, communications, and computing. Here, we introduce the quantum phased array, which generalizes the operating principles of phased arrays and wavefront engineering to quantum fields, and report the first quantum phased array technology demonstration. An integrated photonic-electronic system is used to manipulate free-space quantum information to establish reconfigurable wireless quantum links in a standalone, compact form factor. Such a robust, scalable, and integrated quantum platform can enable broad deployment of quantum technologies with high connectivity, potentially expanding their use cases to real-world applications. We report the first, to our knowledge, free-space-to-chip interface for quantum links, enabled by 32 metamaterial antennas with more than 500,000 sub-wavelength engineered nanophotonic elements over a 550 x 550 $\mathrm{\mu m}^2$ physical aperture. We implement a 32-channel array of quantum coherent receivers with 30.3 dB shot noise clearance and 90.2 dB common-mode rejection ratio that downconverts the quantum optical information via homodyne detection and processes it coherently in the radio-frequency domain. With our platform, we demonstrate 32-pixel imaging of squeezed light for quantum sensing, reconfigurable free-space links for quantum communications, and proof-of-concept entanglement generation for measurement-based quantum computing. This approach offers targeted, real-time, dynamically-adjustable free-space capabilities to integrated quantum systems that can enable wireless quantum technologies.

quant-ph↗

arXiv2024

Optical Investigations of Coherence and Relaxation Dynamics of a Thulium-doped Yttrium Gallium Garnet Crystal at sub-Kelvin Temperatures for Optical Quantum Memory

Rare-earth ion-doped crystals are of great interest for quantum memories, a central component in future quantum repeaters. To assess the promise of 1$\%$ Tm$^{3+}$-doped yttrium gallium garnet (Tm:YGG), we report measurements of optical coherence and energy-level lifetimes of its $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$ transition at a temperature of around 500 mK and various magnetic fields. Using spectral hole burning, we find hyperfine ground-level (Zeeman level) lifetimes of several minutes at magnetic fields of less than 1000 G. We also measure coherence time exceeding one millisecond using two-pulse photon echoes. Three-pulse photon echo and spectral hole burning measurements reveal that due to spectral diffusion, the effective coherence time reduces to a few $\mu$s over a timescale of around two hundred seconds. Finally, temporal and frequency-multiplexed storage of optical pulses using the atomic frequency comb protocol is demonstrated. Our results suggest Tm:YGG to be promising for multiplexed photonic quantum memory for quantum repeaters.

quant-ph↗

arXiv2024

Stable electro-optic modulators using thin-film lithium tantalate

We demonstrate electro-optic modulators realized in low-loss thin-film lithium tantalate with superior DC-stability (<1 dB power fluctuation from quadrature with 12.1 dBm input) compared to equivalent thin-film lithium niobate modulators (5 dB fluctuation) over 46 hours.

physics.optics↗