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Neill Lambert

Publications and source records attributed to Neill Lambert.

At least 37 records · Page 2Linked to original sources

Sudden change of the photon output field marks phase transitions in the quantum Rabi model

The experimental observation of quantum phase transitions predicted by the quantum Rabi model in quantum critical systems is usually challenging due to the lack of signature experimental observables associated with them. Here, we describe a method to identify the dynamical critical phenomenon in the quantum Rabi model consisting of a three-level atom and a cavity at the quantum phase transition. Such a critical phenomenon manifests itself as a sudden change of steady-state output photons in the system driven by two classical fields, when both the atom and the cavity are initially unexcited. The process occurs as the high-frequency pump field is converted into the low-frequency Stokes field and multiple cavity photons in the normal phase, while this conversion cannot occur in the superradiant phase. The sudden change of steady-state output photons is an experimentally accessible measure to probe quantum phase transitions, as it does not require preparing the equilibrium state.

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Modeling the unphysical pseudomode model with physical ensembles: simulation, mitigation, and restructuring of non-Markovian quantum noise

The influence of a Gaussian environment on a quantum system can be described by effectively replacing the continuum with a discrete set of ancillary quantum and classical degrees of freedom. This defines a pseudomode model which can be used to classically simulate the reduced system dynamics. Here, we consider an alternative point of view and analyze the potential benefits of an analog or digital quantum simulation of the pseudomode model itself. Superficially, such a direct experimental implementation is, in general, impossible due to the unphysical properties of the effective degrees of freedom involved. However, we show that the effects of the unphysical pseudomode model can still be reproduced using measurement results over an ensemble of physical systems involving ancillary harmonic modes and an optional stochastic driving field. This is done by introducing an extrapolation technique whose efficiency is limited by stability against imprecision in the measurement data. We examine how such a simulation would allow us to (i) perform accurate quantum simulation of the effects of complex non-perturbative and non-Markovian environments in regimes that are challenging for classical simulation, (ii) conversely, mitigate potential unwanted non-Markovian noise present in quantum devices, and (iii) restructure some of some of the properties of a given physical bath, such as its temperature.

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The Closed and Open Unbalanced Dicke Trimer Model: Critical Properties and Nonlinear Semiclassical Dynamics

We study a generalization of a recently introduced Dicke trimer model [Phys. Rev. Lett. 128, 163601, Phys. Rev. Research 5, L042016], which allows for cavity losses and unbalanced light-matter interactions (in which rotating and counter-rotating terms can be tuned independently). We find that in the extreme unbalanced limit, the $U(1)$ symmetry of the Tavis-Cummings model is restored, qualitatively altering the critical phenomena in the superradiant phase due to the presence of a zero-energy mode. To analyze this general regime, we develop a semiclassical theory based on a re-quantization technique. This theory also provides further physical insight on a recently reported anomalous finite critical fluctuations in the time-reversal broken regime. Moving to the open-Dicke case, by introducing local dissipation to the cavities, we observe the emergence of a rich range of nonequilibrium phases characterized by trivial and non-trivial dynamical signatures. In the former case, we identify, when time-reversal symmetry is present, a new stationary phase that features superradiant states in two of the three cavities and a normal state in the other cavity. In the latter case, we observe the emergence of dynamical phases in which the system exhibits superradiant oscillations, characterized by periodic or chaotic phase space patterns. The landscape of transitions associated with these dynamical phases features a wide range of qualitatively different behaviours such as Hopf bifurcations, anomalous Hopf bifurcations, collisions between basins of attraction, and exterior crises. We highlight how the two-critical-scalings feature of the closed model is robust under dissipation while the phenomenon of anomalous finite critical fluctuations becomes a mean-field scaling in the open model.

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Observation of a superradiant phase transition with emergent cat states

Superradiant phase transitions (SPTs) are important for understanding light-matter interactions at the quantum level, and play a central role in criticality-enhanced quantum sensing. So far, SPTs have been observed in driven-dissipative systems, but the emergent light fields did not show any nonclassical characteristic due to the presence of strong dissipation. Here we report an experimental demonstration of the SPT featuring the emergence of a highly nonclassical photonic field, realized with a resonator coupled to a superconducting qubit, implementing the quantum Rabi model. We fully characterize the light-matter state by Wigner matrix tomography. The measured matrix elements exhibit quantum interference intrinsic of a photonic mesoscopic superposition, and reveal light-matter entanglement

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Kondo QED: The Kondo effect and photon trapping in a two-impurity Anderson model ultra-strongly coupled to light

The Kondo effect is one of the most studied examples of strongly correlated quantum many-body physics. Another type of strongly correlated physics that has only recently been explored in detail (and become experimentally accessible) is that of ultrastrong coupling between light and matter. Here, we study a system which we denote as "Kondo QED") that combines both phenomena, consisting of a two-impurity Anderson model ultra-strongly coupled to a single-mode cavity. While presented as an abstract model, it is relevant for a range of future hybrid cavity-QED systems. Using the hierarchical equations of motion approach we show that the ultrastrong coupling of cavity photons to the electronic states (impurity) noticeably suppresses the electronic Kondo resonance due to the destruction of many-body correlations of the Kondo cloud. We observe this transfer of correlations from the Kondo cloud to the cavity by computing the entropy and mutual information of the impurity-cavity subsystems. In addition, in the weak lead-coupling limit and at zero-bias, the model exhibits a ground-state photon accumulation effect originating entirely from counter-rotating terms in the impurity-cavity interaction. Interestingly, in the strong lead-coupling limit, this accumulation is ``Kondo-enhanced'' by new transition paths opening when increasing the hybridization to the leads. This suggests a new mechanism for the generation of real photons from virtual states. We further show that the suppression of the Kondo effect is stable under broadening of the cavity resonance as a consequence of the interaction to an external bosonic continuum. Our findings pave the way for the simultaneous control of both the Kondo QED effect and a photon accumulation effect using the ultrastrong coupling of light and matter.

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A quantum-classical decomposition of Gaussian quantum environments: a stochastic pseudomode model

We show that the effect of a Gaussian Bosonic environment linearly coupled to a quantum system can be simulated by a stochastic Lindblad master equation characterized by a set of ancillary Bosonic modes initially at zero temperature and classical stochastic fields. We test the method for Ohmic environments with exponential and polynomial cut-offs against, respectively, the Hierarchical Equations of Motion and the deterministic pseudomode model with respect to which the number of ancillary quantum degrees of freedom is reduced. For a subset of rational spectral densities, all parameters are explicitly specified without the need of any fitting procedure, thereby simplifying the modeling strategy. Interestingly, the classical fields in this decomposition must sometimes be imaginary-valued, which can have counter-intuitive effects on the system properties which we demonstrate by showing that they can decrease the entropy of the system, in contrast to real-valued fields.

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A pseudo-fermion method for the exact description of fermionic environments: from single-molecule electronics to Kondo resonance

We develop a discrete fermion approach for modelling the strong interaction of an arbitrary system interacting with continuum electronic reservoirs. The approach is based on a pseudo-fermion decomposition of the continuum bath correlation functions, and is only limited by the accuracy of this decomposition. We show that to obtain this decomposition one can allow for imaginary pseudo-fermion parameters, and strong damping in individual pseudo-fermions, without introducing unwanted approximations. For a non-interacting single-resonant level, we benchmark our approach against an analytical solution and an exact hierachical-equations-of-motion approach. We also show that, for the interacting case, this simple method can capture the strongly correlated low-temperature physics of Kondo resonance.

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QuTiP-BoFiN: A bosonic and fermionic numerical hierarchical-equations-of-motion library with applications in light-harvesting, quantum control, and single-molecule electronics

The "hierarchical equations of motion" (HEOM) method is a powerful exact numerical approach to solve the dynamics and find the steady-state of a quantum system coupled to a non-Markovian and non-perturbative environment. Originally developed in the context of physical chemistry, it has also been extended and applied to problems in solid-state physics, optics, single-molecule electronics, and biological physics. Here we present a numerical library in Python, integrated with the powerful QuTiP platform, which implements the HEOM for both bosonic and fermionic environments. We demonstrate its utility with a series of examples. For the bosonic case, we include demonstrations of fitting arbitrary spectral densities, and an example of the dynamics of energy transfer in the Fenna-Matthews-Olson photosynthetic complex, showing how a suitable non-Markovian environment can protect against pure dephasing. We also demonstrate how the HEOM can be used to benchmark different strategies for dynamical decoupling of a spin from its environment, and show that the Uhrig pulse-spacing scheme is less optimal than equally spaced pulses when the environment's spectral density is very broad. For the fermionic case, we present an integrable single-impurity example, used as a benchmark of the code, and a more complex example of an impurity strongly coupled to a single vibronic mode, with applications to single-molecule electronics.

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Quantifying Quantumness of Channels Without Entanglement

Quantum channels breaking entanglement, incompatibility, or nonlocality are defined as such because they are not useful for entanglement-based, one-sided device-independent, or device-independent quantum information processing, respectively. Here, we show that such breaking channels are related to complementary tests of macrorealism i.e., temporal separability, channel unsteerability, temporal unsteerability, and the temporal Bell inequality. To demonstrate this we first define a steerability-breaking channel, which is conceptually similar to entanglement and nonlocality-breaking channels and prove that it is identical to an incompatibility-breaking channel. A hierarchy of quantum non-breaking channels is derived, akin to the existing hierarchy relations for temporal and spatial quantum correlations. We then introduce the concept of channels that break temporal correlations, explain how they are related to the standard breaking channels, and prove the following results: (1) A robustness-based measure for non-entanglement-breaking channels can be probed by temporal nonseparability. (2) A non-steerability-breaking channel can be quantified by channel steering. (3) Temporal steerability and non-macrorealism can be used for, respectively, distinguishing unital steerability-breaking channels and nonlocality-breaking channels for a maximally entangled state. Finally, a two-dimensional depolarizing channel is experimentally implemented as a proof-of-principle example to demonstrate the hierarchy relation of non-breaking channels using temporal quantum correlations

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Space-time dual quantum Zeno effect: Interferometric engineering of open quantum system dynamics

Superposition of trajectories, which modify quantum evolutions by superposing paths through interferometry, has been utilized to enhance various quantum communication tasks. However, little is known about its impact from the viewpoint of open quantum systems. Thus, we examine this subject from the perspective of system-environment interactions. We show that the superposition of multiple trajectories can result in quantum state freezing, suggesting a space-time dual to the quantum Zeno effect. Moreover, non-trivial Dicke-like super(sub)radiance can be triggered without utilizing multi-atom correlations.

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Pulse-level noisy quantum circuits with QuTiP

The study of the impact of noise on quantum circuits is especially relevant to guide the progress of Noisy Intermediate-Scale Quantum (NISQ) computing. In this paper, we address the pulse-level simulation of noisy quantum circuits with the Quantum Toolbox in Python (QuTiP). We introduce new tools in qutip-qip, QuTiP's quantum information processing package. These tools simulate quantum circuits at the pulse level, leveraging QuTiP's quantum dynamics solvers and control optimization features. We show how quantum circuits can be compiled on simulated processors, with control pulses acting on a target Hamiltonian that describes the unitary evolution of the physical qubits. Various types of noise can be introduced based on the physical model, e.g., by simulating the Lindblad density-matrix dynamics or Monte Carlo quantum trajectories. In particular, the user can define environment-induced decoherence at the processor level and include noise simulation at the level of control pulses. We illustrate how the Deutsch-Jozsa algorithm is compiled and executed on a superconducting-qubit-based processor, on a spin-chain-based processor and using control optimization algorithms. We also show how to easily reproduce experimental results on cross-talk noise in an ion-based processor, and how a Ramsey experiment can be modeled with Lindblad dynamics. Finally, we illustrate how to integrate these features with other software frameworks.

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Hidden nonmacrorealism: reviving the Leggett-Garg inequality with stochastic operations

The Leggett-Garg inequality (LGI) distinguishes nonmacrorealistic channels from macrorealistic ones by constraining the experimental outcomes of the underlying system. In this work, we propose a class of channels which, initially, cannot violate the LGI (in the form of the temporal Bell inequality) but can violate it after the application of stochastic pre- and post- operations (SPPOs). As a proof-of-principle experiment, we demonstrate the stochastic pre- and post- operations in an amplitude-damping channel with photonic qubits. We denote the above phenomenon as hidden nonmacrorealistic channels. We also discuss the relationship between this hidden nonmacrorealistic channels (in terms of the temporal Clauser-Horne-Shimony-Holt (CHSH) inequality) and the strongly nonlocality-breaking channel, which breaks the hidden spatial CHSH nonlocality for arbitrary states. In general, if the channel satisfies hidden nonmacrorealism, it is not a strongly CHSH nonlocality-breaking channel.

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General bound on the performance of counter-diabatic driving acting on dissipative spin systems

Counter-diabatic driving (CD) is a technique in quantum control theory designed to counteract nonadiabatic excitations and guide the system to follow its instantaneous energy eigenstates, and hence has applications in state preparation, quantum annealing, and quantum thermodynamics. However, in many practical situations, the effect of the environment cannot be neglected, and the performance of the CD is expected to degrade. To arrive at general bounds on the resulting error of CD in this situation we consider a driven spin-boson model as a prototypical setup. The inequalities we obtain, in terms of either the Bures angle or the fidelity, allow us to estimate the maximum error solely characterized by the parameters of the system and the bath. By utilizing the analytical form of the upper bound, we demonstrate that the error can be systematically reduced through optimization of the external driving protocol of the system. We also show that if we allow a time-dependent system-bath coupling angle, the obtained bound can be saturated and realizes unit fidelity.

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Unveiling and veiling a Schrödinger cat state from the vacuum

Deep in the ultrastrong light-matter coupling regime, it has been predicted that the ground state of a two-level atom interacting with a cavity mode takes the form of a "virtual" Schrödinger cat entangled state between light and matter. We propose a method to convert this Schrödinger cat state from virtual to real, and back again, by driving the atom with optimally chosen pulses. Our system consists of a four-level atom, with two of these levels ultrastrongly coupled to a cavity mode. We show that the Schrödinger cat state can be converted between virtual and real by making use of either an ideal ultrafast pulse or a multi-tone π-pulse. In addition to allowing us to observe these unusual virtual states this method could also be used to generate entangled cat states on demand for quantum information processing.

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The Fermionic influence superoperator: a canonical derivation for the development of methods to simulate the influence of a Fermionic environment on a quantum system with arbitrary parity symmetry

We present a canonical derivation of an influence superoperator which generates the reduced dynamics of a Fermionic quantum system linearly coupled to a Fermionic environment initially at thermal equilibrium. We use this formalism to derive a generalized-Lindblad master equation (in the Markovian limit) and a generalized version of the hierarchical equations of motion valid in arbitrary parity-symmetry conditions, important for the correct evaluation of system correlation functions and spectra.

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Quantum steering as a witness of quantum scrambling

Quantum information scrambling describes the delocalization of local information to global information in the form of entanglement throughout all possible degrees of freedom. A natural measure of scrambling is the tripartite mutual information (TMI), which quantifies the amount of delocalized information for a given quantum channel with its state representation, i.e., the Choi state. In this work, we show that quantum information scrambling can also be witnessed by temporal quantum steering for qubit systems. We can do so because there is a fundamental equivalence between the Choi state and the pseudo-density matrix formalism used in temporal quantum correlations. In particular, we propose a quantity as a scrambling witness, based on a measure of temporal steering called temporal steerable weight. We justify the scrambling witness for unitary qubit channels by proving that the quantity vanishes whenever the channel is non-scrambling.

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Nonequilibrium heat transport and work with a single artificial atom coupled to a waveguide: emission without external driving

We observe the continuous emission of photons into a waveguide from a superconducting qubit without the application of an external drive. To explain this observation, we build a two-bath model where the qubit couples simultaneously to a cold bath (the waveguide) and a hot bath (a secondary environment). Our results show that the thermal-photon occupation of the hot bath is up to 0.14 photons, 35 times larger than the cold waveguide, leading to nonequilibrium heat transport with a power of up to 132 zW, as estimated from the qubit emission spectrum. By adding more isolation between the sample output and the first cold amplifier in the output line, the heat transport is strongly suppressed. Our interpretation is that the hot bath may arise from active two-level systems being excited by noise from the output line. We also apply a coherent drive, and use the waveguide to measure thermodynamic work and heat, suggesting waveguide spectroscopy is a useful means to study quantum heat engines and refrigerators. Finally, based on the theoretical model, we propose how a similar setup can be used as a noise spectrometer which provides a new solution for calibrating the background noise of hybrid quantum systems.

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Experimental test of non-macrorealistic cat-states in the cloud

The Leggett-Garg inequality attempts to classify experimental outcomes as arising from one of two possible classes of physical theories: those described by macrorealism (which obey our intuition about how the macroscopic classical world behaves), and those that are not (e.g., quantum theory). The development of cloud-based quantum computing devices enables us to explore the limits of macrorealism in new regimes. In particular, here we take advantage of the properties of the programmable nature of the IBM quantum experience to observe the violation of the Leggett-Garg inequality (in the form of a ``quantum witness") as a function of the number of constituent systems (qubits), while simultaneously maximizing the `disconnectivity', a potential measure of macroscopicity, between constituents. Our results show that two-qubit and four-qubit ``cat states" (which have large disconnectivity) are seen to violate the inequality, and hence can be classified as nonmacrorealistic. In contrast, a six-qubit cat state does not violate the ``quantum-witness" beyond a so-called clumsy invasive-measurement bound, and thus is compatible with ``clumsy macrorealism". As a comparison, we also consider un-entangled product states with n = 2, 3, 4, and 6 qubits, in which the disconnectivity is low.

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