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Niccolò Bigagli

Publications and source records attributed to Niccolò Bigagli.

18 recordsLinked to original sources

High-rate Scalable Entanglement Swapping Between Remote Entanglement Sources on Deployed New York City Fibers

Entanglement swapping between photon pairs generated at physically separated nodes over telecommunication fiber infrastructure is an essential step towards the quantum internet, enabling applications such as quantum repeaters, blind quantum computing, distributed quantum computing, and distributed quantum sensing. However, successful networked entanglement swapping relies on generating indistinguishable pairs of photons and preserving them over deployed fibers. This has limited most previous demonstrations to laboratory settings or relied on sophisticated methods to maintain the necessary indistinguishability. Here, we demonstrate a scalable entanglement swapping experiment using naturally indistinguishable entanglement sources based on warm atomic vapor cells. Without sharing lasers or optical frequency references between nodes, nor the need for pulsing the sources, we achieve a swapping rate of nearly 500 pairs/s while maintaining the CHSH parameter above 2. Additionally, we demonstrate the scalability of our method by maintaining the quality of the entanglement swapping on 17.6-km of deployed fibers in NYC, relying on commercially available SPADs at the spoke nodes, SNSPDs at the hub and standard time-synchronization techniques. Our work paves the way for the practical deployment of large-scale hub-and-spoke quantum networks within cities and data centers.

quant-ph

Bichromatic Quantum Teleportation of Weak Coherent Polarization States on a Metropolitan Fiber

As quantum technologies mature, telecommunication operators have a clear opportunity to unlock and scale new services by providing the connectivity layer that links quantum computers, sensors, clocks, and other quantum devices. Realizing this opportunity requires demonstrating quantum networking protocols, including quantum teleportation, under real-world conditions on existing telecom infrastructure. In this work, we demonstrate quantum teleportation over Deutsche Telekom's metropolitan fiber testbed in Berlin using commercial components deployed at the telecom datacenter. A local Bell-state measurement between 795 nm photons from a weak coherent source and from a bichromatic warm-atom entangled photon source enables conditional state transfer onto an O-band photon, which is transmitted through a 30-km field-deployed fiber loop under real-world environmental conditions. The teleported state is reconstructed after propagation via state tomography, achieving an average teleportation fidelity of 90\% on the deployed link. System performance is evaluated in both the absence and the presence of co-propagating C-band classical traffic within the same fiber, demonstrating compatibility with wavelength-division multiplexed telecom infrastructure carrying live data channels.

quant-ph

Observation of Self-Bound Droplets of Ultracold Dipolar Molecules

Ultracold gases of dipolar molecules have long been envisioned as a platform for the realization of novel quantum phases. Recent advances in collisional shielding, protecting molecules from inelastic losses, have enabled the creation of degenerate Fermi gases and, more recently, Bose-Einstein condensation of dipolar molecules. However, the observation of quantum phases in ultracold molecular gases that are driven by dipole-dipole interactions has so far remained elusive. In this work, we report the formation of self-bound droplets and droplet arrays in an ultracold gas of strongly dipolar sodium-cesium molecules. Starting from a molecular Bose-Einstein condensate (BEC), microwave dressing fields are used to induce dipole-dipole interactions with controllable strength and anisotropy. By varying the speed at which interactions are induced, covering a dynamic range of four orders of magnitude, we prepare droplets under equilibrium and non-equilibrium conditions, observing a transition from robust one-dimensional (1D) arrays to fluctuating two-dimensional (2D) structures. The droplets exhibit densities up to 100 times higher than the initial BEC, reaching the strongly interacting regime, and suggesting the possibility of a quantum-liquid or crystalline state. This work establishes ultracold molecules as a system for the exploration of strongly dipolar quantum matter and opens the door to the realization of self-organized crystal phases and dipolar spin liquids in optical lattices.

cond-mat.quant-gas

High-Fidelity Quantum Entanglement Distribution in Metropolitan Fiber Networks with Co-propagating Classical Traffic

The Quantum Internet, a network of quantum-enabled infrastructure, represents the next frontier in telecommunications, promising capabilities that cannot be attained by classical counterparts. A crucial step in realizing such large-scale quantum networks is the integration of entanglement distribution within existing telecommunication infrastructure. Here, we demonstrate a real-world scalable quantum networking testbed deployed within Deutsche Telekom's metropolitan fibers in Berlin. Using commercially available quantum devices and standard add-drop multiplexing hardware, we distributed polarization-entangled photon pairs over dynamically selectable fiber paths ranging from 10~m to 60 km, and showed entanglement distribution over up to approximately 100~km. Quantum signals, transmitted at 1324~nm (O-band), coexist with conventional bidirectional C-band traffic without dedicated fibers or infrastructure changes. Active stabilization of the polarization enables robust long-term performance, achieving entanglement Bell-state fidelity bounds between 85-99% and Clauser-Horne-Shimony-Holt parameter $S$-values between 2.36-2.74 during continuous multiday operation. By achieving a high-fidelity entanglement distribution with less than 1.5% downtime, we confirm the feasibility of hybrid quantum-classical networks under real-world conditions at the metropolitan scale. These results establish deployment benchmarks and provide a practical roadmap for telecom operators to integrate quantum capabilities.

quant-ph

Double Microwave Shielding

We develop double microwave shielding, which has recently enabled evaporative cooling to the first Bose-Einstein condensate of polar molecules [Bigagli et al., Nature 631, 289 (2024)]. Two microwave fields of different frequency and polarization are employed to effectively shield polar molecules from inelastic collisions and three-body recombination. Here, we describe in detail the theory of double microwave shielding. We demonstrate that double microwave shielding effectively suppresses two- and three-body losses. Simultaneously, dipolar interactions and the scattering length can be flexibly tuned, enabling comprehensive control over interactions in ultracold gases of polar molecules. We show that this approach works universally for a wide range of molecules. This opens the door to studying many-body physics with strongly interacting dipolar quantum matter.

cond-mat.quant-gas

Extreme Loss Suppression and Wide Tunability of Dipolar Interactions in an Ultracold Molecular Gas

Ultracold dipolar molecules hold great promise for the creation of novel quantum states of matter, but the realization of long-lived molecular bulk samples with strong dipole-dipole interactions has remained elusive. Here, we realize a collisionally stable gas of ultracold ground state molecules with a lifetime of several seconds. Utilizing double microwave dressing, we achieve an extreme suppression of inelastic two- and three-body losses by factors of more than 10,000 and 1,000, respectively. We find that losses remain suppressed across a wide range of dipole-dipole interactions, allowing the continuous tuning of the dipolar length from 0 to 1 um $\sim$ 20,000 $a_0$. Combined with the recent realization of Bose-Einstein condensation of dipolar molecules, our findings open the door to the exploration of strongly dipolar quantum liquids.

cond-mat.quant-gas

Automated Graph-Based Detection of Quantum Control Schemes: Application to Molecular Laser Cooling

One of the demanding frontiers in ultracold quantum science is identifying laser cooling schemes for complex atoms and molecules out of their vast spectra of internal states. Motivated by the prospect of expanding the set of available ultracold molecules for applications in fundamental physics, chemistry, astrochemistry, and quantum simulation, we propose and demonstrate an automated graph-based search approach for viable laser cooling schemes. The method is time efficient, reproduces the results of previous manual searches, and reveals a plethora of new potential laser cooling schemes. We discover laser cooling schemes for YO, C$_2$, OH$^+$, CN, and CO$_2$, including surprising schemes that start from highly excited states or do not rely on a strong main transition. A central insight of this work is that the reinterpretation of quantum states and transitions between them as a graph can dramatically enhance the ability to identify new quantum control schemes for complex quantum systems. As such, this approach will also apply to complex atoms and, in fact, any complex many-body quantum system with a discrete spectrum of internal states.

quant-ph

Dressed-State Spectroscopy and Magic Trapping of Microwave-Shielded NaCs Molecules

We report on the optical polarizability of microwave-shielded ultracold NaCs molecules in an optical dipole trap. While dressing a pair of rotational states with a microwave field, we observe a marked dependence of the optical polarizability on the intensity and detuning of the dressing field. To precisely characterize differential energy shifts between dressed rotational states, we establish dressed-state spectroscopy. For strong dressing fields, we find that a magic rotational transition can be engineered and demonstrate its insensitivity to laser intensity fluctuations. The results of this work have direct relevance for evaporative cooling and the recent demonstration of molecular Bose-Einstein condensates [Bigagli, et al., Nature (2024)] and may open a door to precision microwave spectroscopy in interacting many-body systems of microwave-shielded molecules.

cond-mat.quant-gas

Observation of Bose-Einstein Condensation of Dipolar Molecules

Ensembles of particles governed by quantum mechanical laws exhibit fascinating emergent behavior. Atomic quantum gases, liquid helium, and electrons in quantum materials all show distinct properties due to their composition and interactions. Quantum degenerate samples of bosonic dipolar molecules promise the realization of novel phases of matter with tunable dipolar interactions and new avenues for quantum simulation and quantum computation. However, rapid losses, even when reduced through collisional shielding techniques, have so far prevented cooling to a Bose-Einstein condensate (BEC). In this work, we report on the realization of a BEC of dipolar molecules. By strongly suppressing two- and three-body losses via enhanced collisional shielding, we evaporatively cool sodium-cesium (NaCs) molecules to quantum degeneracy. The BEC reveals itself via a bimodal distribution and a phase-space-density exceeding one. BECs with a condensate fraction of 60(10) % and a temperature of 6(2) nK are created and found to be stable with a lifetime close to 2 seconds. This work opens the door to the exploration of dipolar quantum matter in regimes that have been inaccessible so far, promising the creation of exotic dipolar droplets, self-organized crystal phases, and dipolar spin liquids in optical lattices.

cond-mat.quant-gas

Collisionally Stable Gas of Bosonic Dipolar Ground State Molecules

Stable ultracold ensembles of dipolar molecules hold great promise for many-body quantum physics, but high inelastic loss rates have been a long-standing challenge. Recently, it was shown that gases of fermionic molecules can be effectively stabilized through external fields. However, many quantum applications will benefit from molecular ensembles with bosonic statistics. Here, we stabilize a bosonic gas of strongly dipolar NaCs molecules against inelastic losses via microwave shielding, decreasing losses by more than a factor of 200 and reaching lifetimes on the scale of 1 second. We also measure high elastic scattering rates, a result of strong dipolar interactions, and observe the anisotropic nature of dipolar collisions. Finally, we demonstrate evaporative cooling of a bosonic molecular gas to a temperature of 36(5) nK, increasing its phase-space density by a factor of 20. This work is a critical step towards the creation of a Bose-Einstein condensate of dipolar molecules.

cond-mat.quant-gas

Laser Scheme for Doppler Cooling of the Hydroxyl Cation (OH$^+$)

We report on a cycling scheme for Doppler cooling of trapped OH$^+$ ions using transitions between the electronic ground state $X^3Σ^-$ and the first excited triplet state $A^3Π$. We have identified relevant transitions for photon cycling and repumping, have found that coupling into other electronic states is strongly suppressed, and have calculated the number of photon scatterings required to cool OH$^+$ to a temperature where Raman sideband cooling can take over. In contrast to the standard approach, where molecular ions are sympathetically cooled, our scheme does not require co-trapping of another species and opens the door to the creation of pure samples of cold molecular ions with potential applications in quantum information, quantum chemistry, and astrochemistry. The laser cooling scheme identified for OH$^+$ is efficient despite the absence of near-diagonal Franck-Condon factors, suggesting that broader classes of molecules and molecular ions are amenable to laser cooling than commonly assumed.

physics.atom-ph

A planar cloverleaf antenna for the creation of circularly polarized microwave fields

We report on the design and characterization of a compact microwave antenna for atomic and molecular physics experiments. The antenna is comprised of four loop antennas arranged in cloverleaf shape, allowing for precise adjustment of polarization by tuning the relative phase of the loops. We optimize the antenna for left-circularly polarized microwaves at 3.5 GHz and characterize its performance using ultracold NaCs molecules as a precise quantum sensor. Observing an unusually high Rabi frequency of $2π\times 46$ MHz, we extract an electric field amplitude of 33(2) V/cm at 22 mm distance from the antenna. The polarization ellipticity is 2.3(4) degrees, corresponding to a 24 dB suppression of right-circular polarization. The cloverleaf antenna is planar and provides large optical access, making it highly suitable for quantum control of atoms and molecules, and potentially other quantum systems that operate in the microwave regime.

physics.atom-ph

Efficient Pathway to NaCs Ground State Molecules

We present a study of two-photon pathways for the transfer of NaCs molecules to their rovibrational ground state. Starting from NaCs Feshbach molecules, we perform bound-bound excited state spectroscopy in the wavelength range from 900~nm to 940~nm, covering more than 30 vibrational states of the $c \, ^3Σ^+$, $b \, ^3Π$, and $B \, ^1Π$ electronic states. Analyzing the rotational substructure, we identify the highly mixed $c \, ^3Σ^+_1 \, |v=22 \rangle \sim b \, ^3Π_1 \, | v=54\rangle$ state as an efficient bridge for stimulated Raman adiabatic passage (STIRAP). We demonstrate transfer into the NaCs ground state with an efficiency of up to 88(4)\%. Highly efficient transfer is critical for the realization of many-body quantum phases of strongly dipolar NaCs molecules and high fidelity detection of single molecules, for example, in spin physics experiments in optical lattices and quantum information experiments in optical tweezer arrays.

physics.atom-ph

Ultracold Gas of Dipolar NaCs Ground State Molecules

We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a peak density of $1.0(4) \times 10^{12}$ cm$^{-3}$. We demonstrate comprehensive quantum state control by preparing the molecules in a specific electronic, vibrational, rotational, and hyperfine state. Employing the tunability and strength of the permanent electric dipole moment of NaCs, we induce dipole moments of up to 2.6 D. Dipolar systems of NaCs molecules are uniquely suited to explore strongly interacting phases in dipolar quantum matter.

cond-mat.quant-gas

A High Phase-Space Density Gas of NaCs Feshbach Molecules

We report on the creation of ultracold gases of bosonic Feshbach molecules of NaCs. The molecules are associated from overlapping gases of Na and Cs using a Feshbach resonance at 864.12(5) G. We characterize the Feshbach resonance using bound state spectroscopy, in conjunction with a coupled-channel calculation. By varying the temperature and atom numbers of the initial atomic mixtures, we demonstrate the association of NaCs gases over a wide dynamic range of molecule numbers and temperatures, reaching 70 nK for our coldest systems and a phase-space density near 0.1. This is an important stepping-stone for the creation of degenerate gases of strongly dipolar NaCs molecules in their absolute ground state.

cond-mat.quant-gas

Overlapping Bose-Einstein Condensates of $^{23}$Na and $^{133}$Cs

We report on the creation of dual-species Bose-Einstein condensates (BECs) of $^{23}$Na atoms and $^{133}$Cs atoms. We demonstrate sympathetic cooling of Cs with Na in a magnetic quadrupole trap and a crossed optical dipole trap, leading to Na BECs with $8 \times 10^5$ atoms and Cs BECs with $3.5 \times 10^4$ atoms. Investigating cross-thermalization and lifetimes of the mixture, we find that the Na and Cs BECs are miscible and overlapping, interacting with a moderate interspecies scattering length of $18(4)\,a_0$ at $23\,$G and $29(4)\,a_0$ at $894\,$G and coexisting for tens of seconds. Overlapping condensates of Na and Cs offer new possibilities for many-body physics with ultracold bosonic mixtures and constitute an ideal starting point for the creation of ultracold ensembles of NaCs ground state molecules.

cond-mat.quant-gas

Laser Cooling Scheme for the Carbon Dimer ($^{12}$C$_2$)

We report on a scheme for laser cooling of $^{12}$C$_2$. We have calculated the branching ratios for cycling and repumping transitions and calculated the number of photon scatterings required to achieve deflection and laser cooling of a beam of $C_2$ molecules under realistic experimental conditions. Our results demonstrate that C$_2$ cooling using the Swan ($d^3Π_\text{g} \leftrightarrow a^3Π_\text{u}$) and Duck ($d^3Π_\text{g} \leftrightarrow c^3Σ_\text{u}^+$) bands is achievable via techniques similar to state-of-the-art molecular cooling experiments. The Phillips ($A^1Π_\text{u} \leftrightarrow X^1Σ_\text{g}^+$) and Ballik-Ramsay ($b^3Σ_\text{g}^- \leftrightarrow a^3Π_\text{u}$) bands offer the potential for narrow-line cooling. This work opens up a path to cooling of molecules with carbon-carbon bonds and may pave the way toward quantum control of organic molecules.

physics.atom-ph

Compact Two-Dimensional Magneto-Optical Trap for Ultracold Atom Setups

We report on the design, implementation, and performance of a compact two-dimensional magneto-optical trap (2D MOT) for cesium. In a small-volume vacuum chamber, the setup uses cesium dispensers in close proximity to the trapping region of the 2D MOT and operates at low vapor pressures in the $10^{-9}$ torr range. We achieve a cold atom flux of $4 \times 10^8$ atoms/s that is comparable to the performance of more complex atomic sources. The setup is simple to construct and can be adapted to a broad range of atomic species.

physics.atom-ph