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Nicholas Boechler

Publications and source records attributed to Nicholas Boechler.

At least 19 recordsLinked to original sources

Three phases of odd robotic active matter

Nonreciprocal interactions in active matter are known to generate exotic mechanical behaviors such as odd elasticity and odd viscosity. However, these phenomena have largely been studied in isolation, raising a fundamental question: Is there a single system that embodies these distinct regimes of odd matter and can transition between phases, establishing a unified phase diagram for nonreciprocal active matter? To address this, we introduce a tunable robotic active matter platform, the Magnetomechanically Augmented Spinning roBotic (MASBot) collective, in which particle-level control of chirality, activity, and pairwise interactions enables access to distinct phases of odd matter. By continuously increasing repulsive forces relative to attractive and transverse forces, we experimentally map a transition from an odd elastic crystal to an odd viscous liquid, and then to a chiral active gas. We find that this latter phase forms a non-space-filling, nonreciprocal active gas stabilized by long-range hydrodynamic attractive forces, whose statistical signatures are consistent with those of a two-dimensional self-gravitating point vortex gas. Within these phases, adjusting spinning frequency and introducing spatially patterned activity allows us to fine-tune odd mechanical responses and tailor power spectra. Further polar and rotational symmetry breaking at the particle scale leads to novel emergent states such as phase separation and collective translation. Together, our system provides a fundamental experimental testbed for nonequilibrium physics and establishes a blueprint for treating robotic swarms as programmable states of matter, enabling functions that range from resilient structures to adaptive swarm reconfiguration.

cond-mat.soft

Single-particle limit of a topological edge state in a locally resonant band gap

Topological metamaterials promise unprecedented wave control. Here, we theoretically and numerically investigate a one-dimensional Su-Schrieffer-Heeger (SSH)-inspired stiffness dimer modified with a local resonator, which imparts a frequency-dependent effective stiffness to the unit cell. The resonator introduces an attenuation singularity: at a frequency at which the effective stiffness vanishes, the spatial attenuation of waves diverges. By tuning a dimerization parameter, we migrate this singularity from one band gap to the other via an intermediate flat-band state, transferring the dominant local-resonance character between the gaps without closing either gap and while preserving the underlying band topology. Crucially, when the resulting topological edge state intersects the attenuation singularity, the edge state collapses onto a single boundary particle, forming a single-particle mode (SPM). This yields an inverse participation ratio of exactly unity, the theoretical limit for localization in a discrete system. Moreover, this extreme localization can be realized at low frequencies, below the first Bragg-type band gap. Further, we demonstrate that while random disorder detunes this mode, merely tuning the boundaries stabilizes the single-particle mode over a broad parameter range. Our findings provide a clear pathway to designing ultra-localized edge states in low-frequency regimes, where band topology guarantees the edge mode and local resonance drives its single-particle confinement.

physics.app-ph

Mechanochemical feedback drives complex inertial dynamics in active solids

Active solids combine internal active driving with elasticity to realize states with nonequilibrium mechanics and autonomous motion. They are often studied in overdamped settings, e.g., in soft materials, and the role of inertia is less explored. We construct a model of a chemically active solid that incorporates mechanochemical feedback and show that, when feedback overwhelms mechanical damping, autonomous inertial dynamics can spontaneously emerge through sustained consumption of chemical fuel. By combining numerical simulations, analysis and dynamical systems approaches, we show how active feedback drives complex nonlinear dynamics on multiple time-scales, including limit cycles and chaos. Our results suggest design principles for creating ultrafast actuators and autonomous machines from soft, chemically-powered solids.

cond-mat.soft

Computational inverse design of acoustoplasmonic metasurfaces

Optical and acoustic metasurfaces are two-dimensional arrays of subwavelength elements that locally modulate or phase shift incident waves. Acoustoplasmonic metasurfaces combine the physics of light and sound, producing acoustic wavefronts in response to optical stimuli. Herein, we present a computational inverse acoustoplasmonic metasurface design algorithm for desired optically-generated acoustic wave fields. We consider gold nanoparticles producing spherical acoustic waves in water, and the resulting acoustic wave propagation along the plane containing the nanoparticle array. We demonstrate how our algorithm can be used to design metasurfaces that can be used to achieve complex acoustic wave fields. This includes the design of a single metasurface that produces acoustic wave fields mimicking two different Morse code patterns upon stimulation with two orthogonal polarization states of light. This work provides a new tool for the design of complex optically generated acoustic wavefronts, enabling functionality beyond what would be achievable with off-optical-resonance optoacoustic excitation.

physics.app-ph

Electric-Field-Controlled Chemical Reaction via Piezo-Chemistry Creates Programmable Material Stiffness

The spatial and temporal control of material properties at a distance has yielded many unique innovations including photo-patterning, 3D-printing, and architected material design. To date, most of these innovations have relied on light, heat, sound, or electric current as stimuli for controlling the material properties. Here, we demonstrate that an electric field can induce chemical reactions and subsequent polymerization in composites via piezoelectrically-mediated transduction. The response to an electric field rather than through direct contact with an electrode is mediated by a nanoparticle transducer, i.e., piezoelectric ZnO, which mediates reactions between thiol and alkene monomers, resulting in tunable moduli as a function of voltage, time, and the frequency of the applied AC power. The reactivity of the mixture and the modulus of a na\"ive material containing these elements can be programmed based on the distribution of the electric field strength. This programmability results in multi-stiffness gels. Additionally, the system can be adjusted for the formation of an electro-adhesive. This simple and generalizable design opens new avenues for facile application in adaptive damping and variable-rigidity materials, adhesive, soft robotics, and potentially tissue engineering.

physics.chem-ph

Observation of mechanical kink control and generation via phonons

Kinks (or domain walls) are localized transitions between distinct ground states associated with a topological invariant, and are central to many phenomena across physics, from condensed matter to cosmology. While phonon (i.e., small-amplitude vibration) wave packets have been theorized to deterministically interact with kinks and initiate their movement, this interaction has remained elusive in experiments, where only uncontrollable stochastic kink motion generated by thermal phonons or dislocation glide by low-frequency quasi-static loading have been observed. This is partly because all physical systems that support kinks are, at some level, discrete, making deterministic phonon control of kinks extremely challenging due to the existence of Peierls-Nabarro (PN) barrier. Here, we demonstrate, for the first time, experimental observation of phonon-mediated control and generation of mechanical kinks, which we enable using a topological metamaterial that constitutes an elastic realization of the Kane-Lubensky chain model. Our metamaterial overcomes the PN barrier by supporting a single, topologically protected kink that requires zero energy to form and move. Using simulations that show close agreement with our experimental observations, we also reveal unique dynamics of phonon interplay with highly discrete kinks, including long-duration motion and a continuous family of internal modes, features absent in other discrete nonlinear systems. This work introduces a new paradigm for topological kink control, with potential applications in material stiffness tuning, shape morphing, locomotion, and robust signal transmission.

nlin.PS

Minimizing finite viscosity enhances relative kinetic energy absorption in bistable mechanical metamaterials but only with sufficiently fine discretization: a nonlinear dynamical size effect

Bistable mechanical metamaterials have shown promise for mitigating the harmful consequences of impact by converting kinetic energy into stored strain energy, offering an alternative and potentially synergistic approach to conventional methods of attenuating energy transmission. In this work, we numerically study the dynamic response of a one-dimensional bistable metamaterial struck by a high speed impactor (where the impactor velocity is commensurate with the sound speed), using the peak kinetic energy experienced at midpoint of the metamaterial compared to that in an otherwise identical linear system as our performance metric. We make five key findings: 1) The bistable material can counter-intuitively perform better (to nearly 1000x better than the linear system) as the viscosity decreases (but remains finite), but only when sufficiently fine discretization has been reached (i.e. the system approaches sufficiently close to the continuum limit); 2) This discretization threshold is sharp, and depends on the viscosity present; 3) The bistable materials can also perform significantly worse than linear systems (for low discretization and viscosity or zero viscosity); 4) The dependence on discretization stems from the partition of energy into trains of solitary waves that have pulse lengths proportional to the unit cell size, where, with intersite viscosity, the solitary wave trains induce high velocity gradients and thus enhanced damping compared to linear, and low-unit-cell-number bistable, materials; and 5) When sufficiently fine discretization has been reached at low viscosities, the bistable system outperforms the linear one for a wide range of impactor conditions. The first point is particularly important, as it shows the existence of a nonlinear dynamical size effect, where, given a protective layer of some thickness...

nlin.PS

Customizable wave tailoring materials enabled by nonlinear bilevel inverse design

Passive transformation of waves via nonlinear systems is ubiquitous in settings ranging from acoustics to optics and electromagnetics. Passivity is of particular importance for responding rapidly to stimuli and nonlinearity enormously expands signal transformability compared to linear systems due to the breaking of superposition. It is well known that different types of nonlinearity yield vastly different effects on propagating signals, which raises the question of ``what precise nonlinearity is the best for a given wave tailoring application?'' Considering a one-dimensional spring-mass chain as a testbed, we couple the shape optimization of structures for tailored nonlinear constitutive responses with reduced-order nonlinear dynamical inverse design. Using minimization of peak kinetic energy transmission from impact as a case study, we identify ideal nonlinear constitutive responses and the geometries needed to achieve them. As part of this, we show the large sensitivity of this metric to small changes in nonlinearity, and thus the need for high precision, free-form nonlinearity tailoring. We validate our predictions using impact experiments in a chain of nonlinear springs and masses. This work sets the foundation for broader passive nonlinear mechanical wave tailoring material design, with applications to computing, signal processing, shock mitigation, and autonomous materials.

cond-mat.mtrl-sci

Backscattering-free edge states below all bands in two-dimensional auxetic media

Unidirectional and backscattering-free propagation of sound waves is of fundamental interest in physics, and highly sought-after in engineering. Current strategies utilize topologically protected chiral edge modes in bandgaps, or complex mechanisms involving active constituents or nonlinearity. Here we propose a new class of passive, linear, one-way edge states based on spin-momentum locking of Rayleigh waves in two-dimensional media in the limit of vanishing bulk modulus, which provides $100\%$ unidirectional and backscattering-free edge propagation at a broad range of frequencies instead of residing in gaps between bulk bands. We further show that such modes are characterized by a new topological winding number that is analogous to discrete angular momentum eigenvalues in quantum mechanics. These passive and backscattering-free edge waves have the potential to enable a new class of phononic devices in the form of lattices or continua that work in previously inaccessible frequency ranges.

cond-mat.soft

Tailoring high precision polynomial architected material constitutive responses via inverse design

The design of specified nonlinear mechanical responses into a structure or material is a highly sought after capability, which would have a significant impact in areas such as wave tailoring in metamaterials, impact mitigation, soft robotics, and biomedicine. Here, we present a topology optimization approach to design structures for desired polynomial nonlinear behavior, wherein we formulate the problem in such a way as to decouple the nonlinear response from the stiffness. We show results across qualitatively different polynomial behaviors while achieving a high degree of precision, creating a path toward analytically tractable nonlinear dynamical systems. The approach enables access to previously difficult to design for, or hitherto unachieved, nonlinear behavior via optimized structures, which can furthermore be incorporated as unit cells of designer materials with tailored nonlinear properties.

cond-mat.mtrl-sci

Dependence of the kinetic energy absorption capacity of bistable mechanical metamaterials on impactor mass and velocity

Using an alternative mechanism to dissipation or scattering, bistable structures and mechanical metamaterials have shown promise for mitigating the detrimental effects of impact by reversibly locking energy into strained material. Herein, we extend prior works on impact absorption via bistable metamaterials to computationally explore the dependence of kinetic energy transmission on the velocity and mass of the impactor, with strain rates exceeding $10^2$ s$^{-1}$. We observe a large dependence on both impactor parameters, ranging from significantly better to worse performance than a comparative linear material. We then correlate the variability in performance to solitary wave formation in the system and give analytical estimates of idealized energy absorption capacity under dynamic loading. In addition, we find a significant dependence on damping accompanied by a qualitative difference in solitary wave propagation within the system. The complex dynamics revealed in this study offer potential future guidance for the application of bistable metamaterials to applications including human and engineered system shock and impact protection devices.

physics.app-ph

Synthetically Non-Hermitian Nonlinear Wave-like Behavior in a Topological Mechanical Metamaterial

Topological mechanical metamaterials have enabled new ways to control stress and deformation propagation. Exemplified by Maxwell lattices, they have been studied extensively using a linearized formalism. Herein, we study a two-dimensional topological Maxwell lattice by exploring its large deformation quasi-static response using geometric numerical simulations and experiments. We observe spatial nonlinear wave-like phenomena such as harmonic generation, localized domain switching, amplification-enhanced frequency conversion, and solitary waves. We further map our linearized, homogenized system to a non-Hermitian, non-reciprocal, one-dimensional wave equation, revealing an equivalence between the deformation fields of two-dimensional topological Maxwell lattices and nonlinear dynamical phenomena in one-dimensional active systems. Our study opens a new regime for topological mechanical metamaterials and expands their application potential in areas including adaptive and smart materials, and mechanical logic, wherein concepts from nonlinear dynamics may be used to create intricate, tailored spatial deformation and stress fields greatly exceeding conventional elasticity.

cond-mat.soft

Duality of Topological Edge States in a Mechanical Kitaev Chain

We theoretically investigate and experimentally demonstrate the existence of topological edge states in a mechanical analog of the Kitaev chain with a non-zero chemical potential. Our system is a one-dimensional monomer system involving two coupled degrees of freedom, i.e., transverse displacement and rotation of elastic elements. Due to the particle-hole symmetry, a topologically nontrivial bulk leads to the emergence of edge states in a finite chain with fixed boundaries. In contrast, a topologically trivial bulk also leads to the emergence of edge states in a finite chain, but with free boundaries. We unravel a duality in our system that predicts the existence of the latter edge states. This duality involves the iso-spectrality of a subspace for finite chains, and as a consequence, a free chain with topologically trivial bulk maps to a fixed chain with a nontrivial bulk. Lastly, we provide the conditions under which the system can exhibit perfectly degenerate in-gap modes, akin to Majorana zero modes. These findings suggest that mechanical systems with fine-tuned degrees of freedom can be fertile testbeds for exploring the intricacies of Majorana physics.

cond-mat.mes-hall

Topology optimization of nonlinear periodically microstructured materials for tailored homogenized constitutive properties

A topology optimization method is presented for the design of periodic microstructured materials with prescribed homogenized nonlinear constitutive properties over finite strain ranges. The mechanical model assumes linear elastic isotropic materials, geometric nonlinearity at finite strain, and a quasi-static response. The optimization problem is solved by a nonlinear programming method and the sensitivities computed via the adjoint method. Two-dimensional structures identified using this optimization method are additively manufactured and their uniaxial tensile strain response compared with the numerically predicted behavior. The optimization approach herein enables the design and development of lattice-like materials with prescribed nonlinear effective properties, for use in myriad potential applications, ranging from stress wave and vibration mitigation to soft robotics.

cs.CE

Growing Phenotype-controlled Phononic Materials from Plant Cells Scaffolds

Biological composites offer self-healing properties, biocompatibility, high responsivity to external stimuli, and multifunctionality, due, in part, to their complex, hierarchical microstructure. Such materials can be inexpensively grown, and self-assembled from the bottom up, enabling democratized, sustainable manufacturing routes for micro- and nano-devices. While biological composites have been shown to incorporate rich photonic structures, their phononic properties have hitherto remained unexplored. In this study, we demonstrate that biological composites in the form of micron-thick decellularized onion cell scaffolds behave as an organic phononic material, with the presence of band gaps forbidding the propagation of elastic waves in select frequency ranges. We show that the onion cells' phononic properties can be phenotypically tuned, and anticipate these findings will yield new biologically-derived, "green", and genetically tailorable phononic materials.

physics.app-ph

Wrinkles Riding Waves in Soft Layered Materials

The formation of periodic wrinkles in soft layered materials due to mechanical instabilities is prevalent in nature and has been proposed for use in multiple applications. However, such phenomena have been explored predominantly in quasi-static settings. In this work, we measure the dynamics of soft elastomeric blocks with stiff surface films subjected to high-speed impact, and observe wrinkles forming along with, and riding upon, waves propagating through the system. We analyze our measurements with large-deformation, nonlinear visco-hyperelastic Finite Element simulations coupled to an analytical wrinkling model. The comparison between the measured and simulated dynamics shows good agreement, and suggests that inertia and viscoelasticity play an important role. This work encourages future studies of the dynamics of surface instabilities in soft materials, including large-deformation, highly nonlinear morphologies, and may have applications to areas including impact mitigation, soft electronics, and the dynamics of soft sandwich composites.

cond-mat.soft

Longitudinal Eigenvibration of Multilayer Colloidal Crystals and the Effect of Nanoscale Contact Bridges

Longitudinal contact-based vibrations of colloidal crystals with a controlled layer thickness are studied. These crystals consist of 390 nm diameter polystyrene spheres arranged into close packed, ordered lattices with a thickness of one to twelve layers. Using laser ultrasonics, eigenmodes of the crystals that have out-of-plane motion are excited. The particle-substrate and effective interlayer contact stiffnesses in the colloidal crystals are extracted using a discrete, coupled oscillator model. Extracted stiffnesses are correlated with scanning electron microscope images of the contacts and atomic force microscope characterization of the substrate surface topography after removal of the spheres. Solid bridges of nanometric thickness are found to drastically alter the stiffness of the contacts, and their presence is found to be dependent on the self-assembly process. Measurements of the eigenmode quality factors suggest that energy leakage into the substrate plays a role for low frequency modes but is overcome by disorder- or material-induced losses at higher frequencies. These findings help further the understanding of the contact mechanics, and the effects of disorder in three-dimensional micro- and nano-particulate systems, and open new avenues to engineer new types of micro- and nanostructured materials with wave tailoring functionalities via control of the adhesive contact properties.

cond-mat.mes-hall

Laser-Induced Spallation of Microsphere Monolayers

The detachment of a semi-ordered monolayer of polystyrene microspheres adhered to an aluminum-coated glass substrate is studied using a laser-induced spallation technique. The microsphere-substrate adhesion force is estimated from substrate surface displacement measurements obtained using optical interferometry, and a rigid-body model that accounts for the inertia of the microspheres. The estimated adhesion force is compared with estimates obtained from interferometric measurement of the out-of-plane microsphere contact resonance. Reasonable agreement is found between the two experiments. Scanning electron microscope images of detached monolayer regions reveal a unique morphology, namely, partially detached monolayer flakes composed of single hexagonal close packed crystalline domains. This work contributes to an improved understanding of microsphere adhesion and demonstrates a unique monolayer delamination morphology.

cond-mat.mes-hall