arXiv subjects

Nicholas Dale

Publications and source records attributed to Nicholas Dale.

6 recordsLinked to original sources

arXiv2026

Ferromagnetic interlayer exchange coupling in a few layers of CrSBr on a gold thin film

The two-dimensional character of van der Waals magnets allows for efficient control of their properties via proximity effects and electrical stimuli, making them promising candidates for application in spin-electronics. We use spin-polarized low energy electron microscopy to directly image the magnetic texture of thin CrSBr on top of a Au film, uncovering a ferromagnetic ground state for CrSBr thicknesses smaller than 11 nm. We argue that the stabilization of the ferromagnetic ordering - as compared to the conventional antiferromagnetic one - is obtained via electron transfer from the Au film to the CrSBr flakes, in agreement with ab-initio density functional theory calculations. Reflected-electron spectroscopy shows clear differences in the unoccupied density of states between a few layers of CrSBr on Au and bulk CrSBr, pointing towards electronic band structure modification in thin CrSBr. This work sheds light on the possibility to tune magnetic properties of two-dimensional magnets via substrate engineering.

cond-mat.mtrl-sci↗

arXiv2024

Relativistic and nonrelativistic spin splitting above and below the Fermi level in a $g$-wave altermagnet

Nonrelativistic spin splitting (NRSS) challenges conventional wisdom about antiferromagnets by allowing spin-split electronic bands even in collinear orders with zero net magnetization. This sub-class of antiferromagnets, recently dubbed "altermagnets," enforces distinctive spin textures via spin-group symmetries in the crystal. However, direct experimental evidence for such symmetry-driven magnetism remains scarce, and distinguishing it from relativistic spin splitting presents additional challenges. Here, we combine first-principles calculations, symmetry analysis, and two spin-resolved spectroscopies--angle-resolved photoemission (spin-ARPES) and our newly developed spin- and angle-resolved electron reflection spectroscopy (spin-ARRES)--to achieve the first complete momentum-resolved mapping of relativistic (RSS) and nonrelastivistic (NRSS) spin splitting in CoNb$_4$Se$_8$. By probing both the occupied (spin-ARPES) and unoccupied (spin-ARRES) electronic states in a single experiment, we uncover a series of momentum-dependent spin splitting phenomena each of which switch sign under sixfold rotations and persists far above and below the Fermi level. Crucially, distinct nodal planes in momentum space distinguish NRSS from RSS features. Additionally, the observed collapse of NRSS and the persistence of RSS above the N\'eel temperature, distinguishes a genuine magnetic phase transition from inversion symmetry breaking. Our work demonstrates, for the first time, the combined power of spin-ARPES and spin-ARRES in capturing the full spin texture across an extended energy range, positioning CoNb$_4$Se$_8$ as a prototype for exploring spin-group-based phenomena. These findings open new routes for engineering spin-based functionalities ranging from neuromorphic computing to unconventional superconductivity in layered antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2022

Revealing the order parameter dynamics of 1T-TiSe$_2$ following optical excitation

The formation of a charge density wave state is characterized by an order parameter. The way it is established provides unique information on both the role that correlation plays in driving the charge density wave formation and the mechanism behind its formation. Here we use time and angle resolved photoelectron spectroscopy to optically perturb the charge-density phase in 1T-TiSe$_2$ and follow the recovery of its order parameter as a function of energy, momentum and excitation density. Our results reveal that two distinct orders contribute to the gap formation, a CDW order and pseudogap-like order, manifested by an overall robustness to optical excitation. A detailed analysis of the magnitude of the the gap as a function of excitation density and delay time reveals the excitonic long-range nature of the CDW gap and the short-range Jahn-Teller character of the pseudogap order. In contrast to the gap, the intensity of the folded Se$_{4p}$* band can only give access to the excitonic order. These results provide new information into the the long standing debate on the origin of the gap in TiSe$_2$ and place it in the same context of other quantum materials where a pseudogap phase appears to be a precursor of long-range order.

cond-mat.str-el↗

arXiv2022

Polarization dependent photoemission as a probe of the magnetic ground state in the layered ferromagnet VI3

Layered ferromagnets are thrilling materials from both a fundamental and technological point of view. VI3 is an interesting example, with a complex magnetism that differentiates it from the first reported Cr based layered ferromagnets. Here, we show in an indirect way through Angle Resolved Photoemission Spectroscopy (ARPES) experiments, the importance of spin-orbit coupling setting the electronic properties of this material. Our light polarized photoemission measurements point to a ground state with a half-filled e'_+- doublet, where a gap opening is triggered by spin-orbit coupling enhanced by electronic correlations.

cond-mat.mes-hall↗

arXiv2022

Mapping the dispersion of the occupied and unoccupied band structure in photoexcited 1T-TiSe$_2$

Charge density waves (CDW) are states of broken symmetry with a periodic modulation of charge and lattice typically leading to the opening of a gap in the band structure. In the model CDW system 1T-TiSe$_2$ such a gap opens up between its Se$_{4p}$ valence and Ti$_{3d}$ conduction band, accompanied by a change of dispersion. These changes are crucial in understanding the CDW phase, as they provide a measure of the Se$_{4p}$-Ti$_{3d}$ hybridization strength and characteristic mechanistic features. Using time- and angle-resolved photoelectron spectroscopy (trARPES), the unoccupied band structure is populated with near-infrared (NIR) pump pulses which allows to to directly visualize the parabolically-shaped Ti$_{3d}$ conduction band. Furthermore, we observe a transient change of effective mass in the Se$_{4p}$ valence band following photoexcitation. This occurs alongside an overall reduction due to weakening of the CDW phase and is accompanied by an oscillating component with the frequency of the characteristic A$_{1g}$ phonon. These observations, enabled by trAPRES, highlight the importance of the lattice contributions in establishing the CDW order in 1T-TiSe$_2$.

cond-mat.str-el↗

arXiv2021

Correlation-Driven Electron-Hole Asymmetry in Graphene Field Effect Devices

Electron-hole asymmetry is a fundamental property in solids that can determine the nature of quantum phase transitions and the regime of operation for devices. The observation of electron-hole asymmetry in graphene and recently in the phase diagram of bilayer graphene has spurred interest into whether it stems from disorder or from fundamental interactions such as correlations. Here, we report an effective new way to access electron-hole asymmetry in 2D materials by directly measuring the quasiparticle self-energy in graphene/Boron Nitride field effect devices. As the chemical potential moves from the hole to the electron doped side, we see an increased strength of electronic correlations manifested by an increase in the band velocity and inverse quasiparticle lifetime. These results suggest that electronic correlations play an intrinsic role in driving electron hole asymmetry in graphene and provide a new insight for asymmetries in more strongly correlated materials.

cond-mat.mes-hall↗