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Nick O. Jaensson

Publications and source records attributed to Nick O. Jaensson.

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Bayesian inference in active microrheology with wall and particle-particle interactions

Active microrheology infers rheological properties from the motion of a force-driven probe. In small samples, however, the probe is often close to walls or other probes, and the resulting hydrodynamic interactions bias the inferred parameters. We present a Bayesian framework in which these interactions are built into simplified analytical models for Newtonian and linear viscoelastic fluids and test it on noisy synthetic data from finite-element simulations of Newtonian and Oldroyd-B fluids. Accounting for the interactions substantially improves the accuracy of the inferred parameters. Near a wall, oblique forcing allows the material parameters and the wall distance to be identified jointly from a single experiment. In the nonlinear viscoelastic regime, posterior predictive checks over multiple force levels reveal the inadequacy of the linear model. Finally, when the probe size is comparable to the heterogeneity length scale, the framework distinguishes spatial variations in the modulus from measurement noise.

cond-mat.soft

Bayesian Model Selection for Complex Flows of Yield Stress Fluids

Modeling yield stress fluids in complex flow scenarios presents significant challenges, particularly because conventional rheological characterization methods often yield material parameters that are not fully representative of the intricate constitutive behavior observed in complex conditions. We propose a Bayesian uncertainty quantification framework for the calibration and selection of constitutive models for yield stress fluids, explicitly accounting for uncertainties in both modeling accuracy and experimental observations. The framework addresses the challenge of complex flow modeling by making discrepancies that emanate from rheological measurements explicit and quantifiable. We apply the Bayesian framework to rheological measurements and squeeze flow experiments on Carbopol 980. Our analysis demonstrates that Bayesian model selection yields robust probabilistic predictions and provides an objective assessment of model suitability through evaluated plausibilities. The framework naturally penalizes unnecessary complexity and shows that the optimal model choice depends on the incorporated physics, the prior information, and the availability of data. In rheological settings, the Herschel-Bulkley and biviscous power law models perform well. However, when these rheological outcomes are used as prior information for a rheo-informed squeeze flow analysis, a significant mismatch with the experimental data is observed. This is due to the yield stress inferred from rheological measurements not being representative of the complex squeeze flow case. In contrast, an expert-informed squeeze flow analysis, based on broader priors, yields accurate predictions. These findings highlight the limitations of translating rheological measurements to complex flows and underscore the value of Bayesian approaches in quantifying model bias and guiding model selection under uncertainty.

physics.flu-dyn

Uncertainty quantification for the squeeze flow of generalized Newtonian fluids

The calibration of rheological parameters in the modeling of complex flows of non-Newtonian fluids can be a daunting task. In this paper we demonstrate how the framework of Uncertainty Quantification (UQ) can be used to improve the predictive capabilities of rheological models in such flow scenarios. For this demonstration, we consider the squeeze flow of generalized Newtonian fluids. To systematically study uncertainties, we have developed a tailored squeeze flow setup, which we have used to perform experiments with glycerol and PVP solution. To mimic these experiments, we have developed a three-region truncated power law model, which can be evaluated semi-analytically. This fast-to-evaluate model enables us to consider uncertainty propagation and Bayesian inference using (Markov chain) Monte Carlo techniques. We demonstrate that with prior information obtained from dedicated experiments - most importantly rheological measurements - the truncated power law model can adequately predict the experimental results. We observe that when the squeeze flow experiments are incorporated in the analysis in the case of Bayesian inference, this leads to an update of the prior information on the rheological parameters, giving evidence of the need for recalibration in the considered complex flow scenario. In the process of Bayesian inference we also obtain information on quantities of interest that are not directly observable in the experimental data, such as the spatial distribution of the three flow regimes. In this way, besides improving the predictive capabilities of the model, the uncertainty quantification framework enhances the insight into complex flow scenarios.

physics.flu-dyn