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Nico S. Bassler

Publications and source records attributed to Nico S. Bassler.

9 recordsLinked to original sources

Symbolic Quantum-Trajectory Method for Multichannel Dicke Superradiance

We solve Dicke superradiance with two or more competing collective decay channels of tunable rates using a symbolic quantum-trajectory construction. The method yields closed time-domain populations and observables as finite combinations of exponential terms for arbitrary numbers of emitters and arbitrary decay rates. For two channels, the behavior of the stationary ground-state distribution resembles a first-order phase transition at the point where the channel-rate ratio is equal to unity. For balanced $d$-channel decay, we obtain scaling laws for the superradiant peak time and intensity. These results unify and extend single-channel Dicke dynamics to multilevel emitters and provide a compact tool for cavity and waveguide experiments, where permutation-symmetric reservoirs engineer multiple collective decay paths.

quant-ph↗

Scaling theory of decoherence in Dicke superradiance

The survival of many-body coherence depends on the competition between correlation buildup and decoherence. In Dicke superradiance, collective emission builds up correlations, producing a peak intensity scaling as $N^2$ for $N$ emitters. We develop a scaling theory including local dephasing and spontaneous emission and obtain fully collective, partially collective, and independent-emitter scaling regimes. The boundary of the fully collective regime defines a continuous phase transition in a transient observable. Local decoherence can prevent $N^2$ scaling despite increasing $N$.

quant-ph↗

Dicke superradiance in degenerate quantum matter: interplay of exchange statistics and spatial confinement

Collective radiance effects in quantum degenerate systems, such as superradiance and subradiance of a partially inverted ensemble, are shaped by the interplay of spatial confinement and exchange statistics. We investigate this interplay using a purely dissipative field theoretic quartic Lindblad master equation, which captures the nonlinear dynamics of the combined motional and electronic manifolds. This approach captures the interplay between the permutational symmetry of the Lindbladian and the exchange symmetry of the particles, quantifying how bosonic enhancement and Pauli blocking dictate superradiant and subradiant scaling. We identify two distinct routes to distinguishable dynamics: thermal dilution of the initial state at high temperatures and the dynamical breakdown of collective order via recoil induced transport in soft traps. This analysis provides a benchmark for collective emission in quantum-degenerate atomic systems with coupled motional and internal dynamics, such as optical lattice clocks and spinor gases, when dissipation is engineered to control recoil and motional heating.

cond-mat.quant-gas↗

Absence of Entanglement Growth in Dicke Superradiance

Dicke superradiance describes an ensemble of $N$ permutationally invariant two-level systems collectively emitting radiation with a peak radiated intensity scaling as $N^2$. Although individual Dicke states are typically entangled, the density matrix during superradiant decay is a mixture of such states, raising the subtle question of whether the total state is entangled or separable. We resolve this by showing analytically that for all $N$, starting from the fully excited state, the collective decay preserves separability for all times. This answers a longstanding question on the role of entanglement in Dicke superradiance and underscores that, despite collective dissipation, separable states remain separable under these dynamics.

quant-ph↗

Solving Dicke superradiance analytically: A compendium of methods

We present several analytical approaches to the Dicke superradiance problem, which involves determining the time evolution of the density operator for an initially inverted ensemble of $N$ identical two-level systems undergoing collective spontaneous emission. This serves as one of the simplest cases of open quantum system dynamics that allows for a fully analytical solution. We explore multiple methods to tackle this problem, yielding a solution valid for any time and any number of spins. These approaches range from solving coupled rate equations and identifying exceptional points in non-Hermitian evolution to employing combinatorial and probabilistic techniques, as well as utilizing a quantum jump unraveling of the master equation. The analytical solution is expressed as a residue sum obtained from a contour integral in the complex plane, suggesting the possibility of fully analytical solutions for a broader class of open quantum system dynamics problems.

quant-ph↗

Purcell modified Doppler cooling of quantum emitters inside optical cavities

Standard cavity cooling of atoms or dielectric particles is based on the action of dispersive optical forces in high-finesse cavities. We investigate here a complementary regime characterized by large cavity losses, resembling the standard Doppler cooling technique. For a single two-level emitter a modification of the cooling rate is obtained from the Purcell enhancement of spontaneous emission in the large cooperativity limit. This mechanism is aimed at cooling of quantum emitters without closed transitions, which is the case for molecular systems, where the Purcell effect can mitigate the loss of population from the cooling cycle. We extend our analytical formulation to the many particle case governed by weak individual coupling but exhibiting collective strong Purcell enhancement to a cavity mode.

quant-ph↗

Scaling law for Kasha's rule in photoexcited molecular aggregates

We study the photophysics of molecular aggregates from a quantum optics perspective, with emphasis on deriving scaling laws for the fast non-radiative relaxation of collective electronic excitations, referred to as Kasha's rule. Aggregates exhibit an energetically broad manifold of collective states with delocalized electronic excitations originating from near field dipole-dipole exchanges between neighboring monomers. Photo-excitation at optical wavelengths, much larger than the monomer-monomer average separation, addresses almost exclusively symmetric collective states, which for an arrangement known as H-aggregate, show an upward hypsochromic shift. The extremely fast subsequent non-radiative relaxation via intramolecular vibrational modes populates lower energy, subradiant states, resulting in an effective inhibition of fluorescence. Our analytical treatment allows for the derivation of an approximate scaling law of this relaxation process, linear in the number of available low energy vibrational modes and directly proportional to the dipole-dipole interaction strength between neighbouring monomers.

quant-ph↗

Metasurface-based hybrid optical cavities for chiral sensing

Quantum metasurfaces, i.e., two-dimensional subwavelength arrays of quantum emitters, can be employed as mirrors towards the design of hybrid cavities, where the optical response is given by the interplay of a cavity-confined field and the surface modes supported by the arrays. We show that, under external magnetic field control, stacked layers of quantum metasurfaces can serve as helicity-preserving cavities. These structures exhibit ultranarrow resonances and can enhance the intensity of the incoming field by orders of magnitude, while simultaneously preserving the handedness of the field circulating inside the resonator, as opposed to conventional cavities. The rapid phase shift in the cavity transmission around the resonance can be exploited for the sensitive detection of chiral scatterers passing through the cavity. We discuss possible applications of these resonators as sensors for the discrimination of chiral molecules.

quant-ph↗

Linear optical elements based on cooperative subwavelength emitter arrays

We describe applications of two-dimensional subwavelength quantum emitter arrays as efficient optical elements in the linear regime. For normally incident light, the cooperative optical response, stemming from emitter-emitter dipole exchanges, allows the control of the array's transmission, its resonance frequency, and bandwidth. Operations on fully polarized incident light, such as generic linear and circular polarizers as well as phase retarders can be engineered and described in terms of Jones matrices. Our analytical approach and accompanying numerical simulations identify optimal regimes for such operations and reveal the importance of adjusting the array geometry and of the careful tuning of the external magnetic fields amplitude and direction.

quant-ph↗