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Nicola Paradiso

Publications and source records attributed to Nicola Paradiso.

At least 19 recordsLinked to original sources

Origin of the superconductor-insulator transition in disordered two-dimensional films

Theory predicts the superconductor-to-insulator transition (SIT) to emerge from the competition between Anderson localization, which tends to localize single-particle wavefunctions, and superconductivity, which establishes long-range correlations in the superconducting order parameter. In two-dimensional (2D) superconducting films, the transition temperature $T_\text{c}$ at which resistance vanishes, $R_\Box(T_\text{BKT}){=}0$, is set by the Berezinskii-Kosterlitz-Thouless (BKT) mechanism and satisfies $T_\text{BKT}< T_{c0}$, where $T_{c0}$ is the mean-field transition temperature. In weakly disordered samples $T_\text{BKT}\lesssim T_{c0}$, whereas increasing disorder drives $T_\text{BKT}\ll T_{c0}$ near the SIT. Whether the finite-temperature transition retains its BKT character throughout this crossover remains an open question. Here, we investigate the evolution of both sheet resistance $R_\Box(T)$ and superfluid stiffness $J_s(T)$ over a wide range of disorder strength $W$. We establish that even near the SIT, the finite-temperature transition from the superconducting to the resistive state remains of BKT type. However, as disorder approaches the critical value, the zero temperature superfluid phase stiffness, $J_s(0)$, is found to vanish rapidly while $T_{c0}$ remains finite, which we attribute to quantum phase fluctuations as the drive for the zero-temperature transition. Three decades after its experimental discovery by Haviland, Liu, and Goldman, our measurements clarify the origin of the SIT in 2D films.

cond-mat.supr-con

Giant anomalous Josephson effect as a probe of spin texture in topological insulators

Surface states of topological insulators feature chiral spin-momentum locking. When such states are used as weak link between two superconductors, their spin texture gives rise to the anomalous Josephson effect, i.e., to a $φ_0$ shift in the current phase relation. In this work, we explore the anomalous Josephson effect in junctions where the weak link is a HgTe nanowire. We observe a giant anomalous $φ_0$-shift of the current-phase relation, which we attribute to the fact that HgTe surface states feature a single Fermi contour. Moreover, by varying the orientation of the in-plane magnetic field, we obtain information about the spin texture in momentum space. In particular, we found that the spin is not exactly perpendicular to the momentum, but shows a significant deviation of 19 degrees. Our results establish the anomalous Josephson effect as a sensitive tool to probe the spin texture of chiral 2D systems.

cond-mat.supr-con

Spontaneous supercurrents and vortex depinning in two-dimensional arrays of $φ_0$-junctions

Two-dimensional arrays of ballistic Josephson junctions are important as model systems for synthetic quantum materials. Here, we investigate arrays of multiterminal junctions which exhibit a phase difference $φ_0$ at zero current. When applying an in-plane magnetic field we observe nonreciprocal vortex depinning currents. We explain this effect in terms of a ratchet-like pinning potential, which is induced by spontaneous supercurrent loops. Supercurrent loops arise in multiterminal $φ_0$-junction arrays as a consequence of next-nearest neighbor Josephson coupling. Tuning the density of vortices to commensurate values of the frustration parameter results in an enhancement of the ratchet effect. In addition, we find a surprising sign reversal of the ratchet effect near frustration 1/3. Our work calls for the search for novel magnetic structures in artificial crystals in the absence of time-reversal symmetry.

cond-mat.supr-con

Link between supercurrent diode and anomalous Josephson effect revealed by gate-controlled interferometry

In Josephson diodes the asymmetry between positive and negative current branch of the current-phase relation leads to a polarity-dependent critical current and Josephson inductance. The supercurrent nonreciprocity can be described as a consequence of the anomalous Josephson effect -- a $φ_0$-shift of the current-phase relation -- in multichannel ballistic junctions with strong spin-orbit interaction. In this work, we simultaneously investigate $φ_0$-shift and supercurrent diode efficiency on the same Josephson junction by means of a superconducting quantum interferometer. By electrostatic gating, we reveal a direct link between $φ_0$-shift and diode effect. Our findings show that the supercurrent diode effect mainly results from magnetochiral anisotropy induced by spin-orbit interaction in combination with a Zeeman field.

cond-mat.supr-con

Sharpness of the Berezinskii-Kosterlitz-Thouless transition in ultrathin NbN films

We present a comprehensive investigation of the Berezinskii-Kosterlitz-Thouless (BKT) transition in ultrathin strongly disordered NbN films. Measurements of resistance, current-voltage characteristics and kinetic inductance on the very same device reveal a consistent picture of a sharp unbinding transition of vortex-antivortex pairs that fit standard renormalization group theory without extra assumptions in terms of inhomogeneity. Our experiments demonstrate that the previously observed broadening of the transition is not an intrinsic feature of strongly disordered superconductors and provide a clean starting point for the study of dynamical effects at the BKT transition.

cond-mat.supr-con

Sign reversal of the AC and DC supercurrent diode effect and 0-$π$-like transitions in ballistic Josephson junctions

The recent discovery of intrinsic supercurrent diode effect, and its prompt observation in a rich variety of systems, has shown that nonreciprocal supercurrents naturally emerge when both space- and time-inversion symmetries are broken. In Josephson junctions, nonreciprocal supercurrent can be conveniently described in terms of spin-split Andreev states. Here, we demonstrate a sign reversal of the supercurrent diode effect, in both its AC and DC manifestations. In particular, the AC diode effect -- i.e., the asymmetry of the Josephson inductance as a function of the supercurrent -- allows us to probe the current-phase relation near equilibrium. Using a minimal theoretical model, we can then link the sign reversal of the AC diode effect to the so-called 0-$π$-like transition, a predicted, but still elusive feature of multi-channel junctions. Our results demonstrate the potential of inductance measurements as sensitive probes of the fundamental properties of unconventional Josephson junctions.

cond-mat.supr-con

Anisotropic vortex squeezing in synthetic Rashba superconductors: a manifestation of Lifshitz invariants

Most of 2D superconductors are of type II, i.e., they are penetrated by quantized vortices when exposed to out-of-plane magnetic fields. In presence of a supercurrent, a Lorentz-like force acts on the vortices, leading to drift and dissipation. The current-induced vortex motion is impeded by pinning at defects, enabling the use of superconductors to generate high magnetic fields without dissipation. Usually, the pinning strength decreases upon any type of pair-breaking. Here we show that in Rashba superconductors the application of an in-plane field leads, instead, to an unexpected enhancement of pinning. When rotating the in-plane component of the field with respect to the current direction, the vortex inductance turns out to be highly anisotropic. We explain this phenomenon as a manifestation of Lifshitz invariant terms in the Ginzburg-Landau free energy, which are enabled by inversion and time-reversal symmetry breaking and lead to an elliptic squeezing of vortex cores. Our experiment provides access to a fundamental property of Rashba superconductors and offers an entirely new approach to vortex manipulation.

cond-mat.supr-con

Supercurrent diode effect and magnetochiral anisotropy in few-layer NbSe$_2$

Nonreciprocal transport refers to charge transfer processes that are sensitive to the bias polarity. Until recently, nonreciprocal transport was studied only in dissipative systems, where the nonreciprocal quantity is the resistance. Recent experiments have, however, demonstrated nonreciprocal supercurrent leading to the observation of a supercurrent diode effect in Rashba superconductors, opening the vision of dissipationless electronics. Here we report on a supercurrent diode effect in NbSe$_2$ constrictions obtained by patterning NbSe$_2$ flakes with both even and odd layer number. The observed rectification is driven by valley-Zeeman spin-orbit interaction. We demonstrate a rectification efficiency as large as 60%, considerably larger than the efficiency of devices based on Rashba superconductors. In agreement with recent theory for superconducting transition metal dichalcogenides, we show that the effect is driven by an out-of-plane magnetic field component. Remarkably, we find that the effect becomes field-asymmetric in the presence of an additional in-plane field component transverse to the current direction. Supercurrent diodes offer a further degree of freedom in designing superconducting quantum electronics with the high degree of integrability offered by van der Waals materials.

cond-mat.supr-con

Effect of Rashba and Dresselhaus spin-orbit coupling on supercurrent rectification and magnetochiral anisotropy of ballistic Josephson junctions

Simultaneous breaking of inversion- and time-reversal symmetry in Josephson junction leads to a possible violation of the $I(φ)=-I(-φ)$ equality for the current-phase relation. This is known as anomalous Josephson effect and it produces a phase shift $φ_0$ in sinusoidal current-phase relations. In ballistic Josephson junctions with non-sinusoidal current phase relation the observed phenomenology is much richer, including the supercurrent diode effect and the magnetochiral anisotropy of Josephson inductance. In this work, we present measurements of both effects on arrays of Josephson junctions defined on epitaxial Al/InAs heterostructures. We show that the orientation of the current with respect to the lattice affects the magnetochiral anisotropy, possibly as the result of a finite Dresselhaus component. In addition, we show that the two-fold symmetry of the Josephson inductance reflects in the activation energy for phase slips.

cond-mat.supr-con

Supercurrent and phase slips in a ballistic carbon nanotube embedded into a van der Waals heterostructure

We demonstrate long-range superconducting correlations in a several micrometer-long carbon nanotube encapsulated in a van der Waals stack between hBN and NbSe$_2$. We show that a substantial supercurrent flows through the nanotube section beneath the NbSe$_2$ crystal as well as through the 2 $μ$m-long section not in contact with it. As expected for superconductors of nanoscopic cross section, the current-induced breakdown of superconductivity is characterized by resistance steps due to the nucleation of phase slip centers. All elements of our hybrid device are active building blocks of several recently proposed setups for realization of Majorana fermions in carbon nanotubes.

cond-mat.supr-con

A Josephson junction supercurrent diode

Transport is called nonreciprocal when not only the sign, but also the absolute value of the current, depends on the polarity of the applied voltage. It requires simultaneously broken inversion and time-reversal symmetries, e.g., by the interplay of spin-orbit coupling and magnetic field. So far, observation of nonreciprocity was always tied to resistivity, and dissipationless nonreciprocal circuit elements were elusive. Here, we engineer fully superconducting nonreciprocal devices based on highly-transparent Josephson junctions fabricated on InAs quantum wells. We demonstrate supercurrent rectification far below the transition temperature. By measuring Josephson inductance, we can link nonreciprocal supercurrent to the asymmetry of the current-phase relation, and directly derive the supercurrent magnetochiral anisotropy coefficient for the first time. A semi-quantitative model well explains the main features of our experimental data. Nonreciprocal Josephson junctions have the potential to become for superconducting circuits what $pn$-junctions are for traditional electronics, opening the way to novel nondissipative circuit elements.

cond-mat.supr-con

Josephson inductance as a probe for highly ballistic semiconductor-superconductor weak links

We present simultaneous measurements of Josephson inductance and DC transport characteristics of ballistic Josephson junctions based upon an epitaxial Al-InAs heterostructure. The Josephson inductance at finite current bias directly reveals the current-phase relation. The proximity-induced gap, the critical current and the average value of the transparency $\barτ$ are extracted without need for phase bias, demonstrating, e.g.,~a near-unity value of $\barτ=0.94$. Our method allows us to probe the devices deeply in the non-dissipative regime, where ordinary transport measurements are featureless. In perpendicular magnetic field the junctions show a nearly perfect Fraunhofer pattern of the critical current, which is insensitive to the value of $\barτ$. In contrast, the signature of supercurrent interference in the inductance turns out to be extremely sensitive to $\barτ$.

cond-mat.supr-con

Bright excitons with negative-mass electrons

Bound electron-hole excitonic states are generally not expected to form with charges of negative effective mass. We identify such excitons in a single layer of the semiconductor WSe2, where they give rise to narrow-band upconverted photoluminescence in the UV, at an energy of 1.66 eV above the first band-edge excitonic transition. Negative band curvature and strong electron-phonon coupling result in a cascaded phonon progression with equidistant peaks in the photoluminescence spectrum, resolvable to ninth order. Ab initio GW-BSE calculations with full electron-hole correlations unmask and explain the admixture of upper conduction-band states to this complex many-body excitation: an optically bright, bound exciton in resonance with the semiconductor continuum. This exciton is responsible for atomic-like quantum-interference phenomena such as electromagnetically induced transparency. Since band curvature can be tuned by pressure or strain, synthesis of exotic quasiparticles such as flat-band excitons with infinite reduced mass becomes feasible.

cond-mat.mes-hall

Air tightness of hBN encapsulation and its impact on Raman spectroscopy of van der Waals materials

Raman spectroscopy is a precious tool for the characterization of van der Waals materials, e.g. for the determination of the layer number in thin exfoliated flakes. For sensitive materials, however, this method can be dramatically invasive. In particular, the light intensity required to obtain a significant Raman signal is sufficient to immediately photo-oxidize few-layer thick metallic van der Waals materials. In this work we investigated the impact of the environment on Raman characterization of thin NbSe$_2$ crystals. We show that in ambient conditions the flake is locally oxidized even for very low illumination intensity. On the other hand, we observe no degradation if the Raman measurements are performed either in vacuum or on fully hBN-encapsulated samples. Interestingly, we find that covering samples deposited on the usual SiO$_2$ surface only from the top is not sufficient to prevent diffusion of oxygen underneath the layers.

cond-mat.mtrl-sci

Phase slip lines in superconducting few-layer NbSe$_2$ crystals

We show the results of two-terminal and four-terminal transport measurements on few-layer NbSe$_2$ devices at large current bias. In all the samples measured, transport characteristics at high bias are dominated by a series of resistance jumps due to nucleation of phase slip lines, the two dimensional analogue of phase slip centers. In point contact devices the relatively simple and homogeneous geometry enables a quantitative comparison with the model of Skocpol, Beasley and Tinkham. In extended crystals the nucleation of a single phase slip line can be induced by mechanical stress of a region whose width is comparable to the charge imbalance equilibration length.

cond-mat.supr-con

Exciton diffusion and halo effects in monolayer semiconductors

We directly monitor exciton propagation in freestanding and SiO2-supported WS2 monolayers through spatially- and time-resolved micro-photoluminescence under ambient conditions. We find highly nonlinear behavior with characteristic, qualitative changes in the spatial profiles of the exciton emission and an effective diffusion coefficient increasing from 0.3 to more than 30 cm2/s, depending on the injected exciton density. Solving the diffusion equation while accounting for Auger recombination allows us to identify and quantitatively understand the main origin of the increase in the observed diffusion coefficient. At elevated excitation densities, the initial Gaussian distribution of the excitons evolves into long-lived halo shapes with micrometer-scale diameter, indicating additional memory effects in the exciton dynamics.

cond-mat.mes-hall

Dark states in a carbon nanotube quantum dot

Illumination of atoms by resonant lasers can pump electrons into a coherent superposition of hyperfine levels which can no longer absorb the light. Such superposition is known as dark state, because fluorescent light emission is then suppressed. Here we report an all-electric analogue of this destructive interference effect in a carbon nanotube quantum dot. The dark states are a coherent superposition of valley (angular momentum) states which are decoupled from either the drain or the source leads. Their emergence is visible in asymmetric current-voltage characteristics, with missing current steps and current suppression which depend on the polarity of the applied source-drain bias. Our results demonstrate for the first time coherent-population trapping by all-electric means in an artificial atom.

cond-mat.mes-hall

Momentum-space indirect interlayer excitons in transition metal dichalcogenide van der Waals heterostructures

Monolayers of transition metal dichalcogenides (TMDCs) feature exceptional optical properties that are dominated by excitons, tightly bound electron-hole pairs. Forming van der Waals heterostructures by deterministically stacking individual monolayers allows to tune various properties via choice of materials and relative orientation of the layers. In these structures, a new type of exciton emerges, where electron and hole are spatially separated. These interlayer excitons allow exploration of many-body quantum phenomena and are ideally suited for valleytronic applications. Mostly, a basic model of fully spatially-separated electron and hole stemming from the $K$ valleys of the monolayer Brillouin zones is applied to describe such excitons. Here, we combine photoluminescence spectroscopy and first principle calculations to expand the concept of interlayer excitons. We identify a partially charge-separated electron-hole pair in MoS$_2$/WSe$_2$ heterostructures residing at the $Γ$ and $K$ valleys. We control the emission energy of this new type of momentum-space indirect, yet strongly-bound exciton by variation of the relative orientation of the layers. These findings represent a crucial step towards the understanding and control of excitonic effects in TMDC heterostructures and devices.

cond-mat.mes-hall