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Nicolas Bonod

Publications and source records attributed to Nicolas Bonod.

29 records · Page 2Linked to original sources

Transverse multipolar light-matter couplings in evanescent waves

We present an approach to study the interaction between matter and evanescent fields. The approach is based on the decomposition of evanescent plane waves into multipoles of well-defined angular momentum transverse to both decay and propagation directions. We use the approach to identify the origin of the recently observed directional coupling of emitters into guided modes, and of the opposite Zeeman state excitation of atoms near a fiber. We explain how to rigorously quantify both effects, and show that the directionality and the difference in excitation rates grow exponentially with the multipolar order of the light-matter interaction. We also use the approach to study and maximize the transverse torque exerted by an evanescent plane wave onto a given spherical absorbing particle. The maximum occurs at the quadrupolar order of the particle, and for a particular polarization of the plane wave. All the obtained physical insights can be traced back to the two main features of the decomposition of evanescent plane waves into transverse multipolar modes: A polarization independent exponential dominance of modes with large transverse angular momentum, and a polarization controlled parity selection rule.

physics.optics↗

Optimal interactions of light with magnetic and electric resonant particles

This work studies the limits of far and near-field electromagnetic response of sub-wavelength scatterers, like the unitary limit and of lossless scatterers, and the ideal absorption limit of lossy particles. These limit behaviors are described in terms of analytic formulas that approximate finite size effects while rigorously including radiative corrections. This analysis predicts the electric and/or magnetic limit responses of both metallic and dielectric nanoparticles while quantitatively describing near-field enhancements.

physics.optics↗

Equalizing the near and far electromagnetic fields around particles made of different materials

We demonstrate that the electromagnetic fields scattered by particles made of different materials can be equalized. Emphasize is placed first in metallic nanoparticles that host localized surface plasmons and it is shown that their electromagnetic fields can be identically reproduced with dielectric particles. We derive the explicit formulas relating the different constitutive parameters that yield identical electromagnetic responses. This method provides the dielectric permittivities of spherical particles that reproduce the strong near electric field intensities observed around metallic particles featuring localized surface plasmon resonances in optics or near infrared frequencies. We also demonstrate the ability of homogenous dielectric particles to host the magnetic resonances predicted for exotic materials with negative permeability.

physics.optics↗

Purcell factor of Mie resonators featuring electric and magnetic modes

We present a modal approach to compute the Purcell factor in Mie resonators exhibiting both electric and magnetic resonances. The analytic expressions of the normal modes are used to calculate the effective volumes. We show that important features of the effective volume can be predicted thanks to the translation-addition coefficients of a displaced dipole. Using our formalism, it is easy to see that, in general, the Purcell factor of Mie resonators is not dominated by a single mode, but rather by a large superposition. Finally we consider a silicon resonator homogeneously doped with electric dipolar emitters, and we show that the average electric Purcell factor dominates over the magnetic one.

physics.optics↗

Optimizing Nanoparticle Designs to Reach Ideal Light Absorption

Ideal absorption describes a particular means of optimizing light-matter interactions with a host of potential applications. This work presents new analytic formulas and describes semi-analytical methods for the design of electric or magnetic ideal absorption in nanoparticles. These formulas indicate that ideal absorption is attainable in homogeneous spheres with known materials at specific sizes and frequencies. They also provide a means of designing core-shell particles to produce ideal absorption at virtually any frequency in the visible and near infrared range.

physics.optics↗

Controllable emission of a dipolar source coupled with a magneto-dielectric resonant subwavelength scatterer

We demonstrate experimentally and theoretically that a local excitation of a single scatterer of relative dielectric permittivity ε = 6 permits to excite broad dipolar and quadrupolar electric and magnetic resonances that shape the emission pattern in an un- precedented way. By suitably positioning the feed with respect to the sphere at a ?=3 distance, this compact antenna is able to spectrally sort the electromagnetic emission ei- ther in the forward or in the backward direction, together with a high gain in directivity. Materials with ε = 6 can be found in the whole spectrum of frequencies promising Mie antennas to become an enabling technology in numbers of applications, ranging from quantum single photon sources to telecommunications.

physics.optics↗

Enhancing magnetic near-field intensities with dielectric resonators

We measure strong magnetic field intensities in a subwavelength gap separating two dielectric resonators. This dimer magnetic antenna is characterized in the GHz spectral regime when considering three conditions of illumination. We detail the different magneto-electric couplings involved in the enhancement of the near magnetic field and derive the analytical expression of the magnetic field intensities. The results reported here in the GHz domain can be extended to other spectral domains since they are obtained with a dielectric permittivity 16 that can be observed in a very broad spectrum ranging from optics to radio-frequencies.

physics.optics↗

Photonic engineering of hybrid metal-organic chromophores

We experimentally demonstrate control of the absorption and emission properties of individual emitters by photonic antennas in suspension. The method results in a new class of water-soluble chromophores with unprecedented photophysical properties, such as short lifetime, low quantum yield but high brightness.

physics.optics↗

Mode-balancing far field control of light localization in nanoantennas

Light localization is controlled at a scale of lambda/10 in the harmonic regime from the far field domain in a plasmonic nanoantenna. The nanoantenna under study consists of 3 aligned spheres 50 nm in diameter separated by a distance of 5 nm. By simply tuning the orientation of an incident plane wave, symmetric and antisymmetric mode-balancing induces a strong enhancement of the near field intensity in one cavity while nullifying the light intensity in the other cavity. Furthermore, it is demonstrated that the dipolar moment of a plasmonic particle can be fully extinguished when strongly coupled with a dimer of identical nanoparticles. Consequently, optical transparency can be achieved in an ultra-compact symmetric metallic structure.

physics.optics↗

Compact metallo-dielectric optical antenna for ultra directional and enhanced radiative emission

We report the design of highly efficient optical antennas employing a judicious synthesis of metallic and dielectric materials. In the proposed scheme, a pair of metallic coupled nanoparticles permits large enhancements in both excitation strength and radiative decay rates, while a high refractive index dielectric microsphere is employed to efficiently collect light without spoiling the emitter quantum efficiency. Our simulations indicate potential fluorescence rate enhancements of 3 orders of magnitude over the entire optical frequency range.

physics.optics↗

Radiative and non-radiative photokinetics alteration inside a single metallic nanometric aperture

We resolve the photokinetic rates enhancement of Rhodamine 6G molecules diffusing in a water-glycerol mixture within a single nanometric aperture milled in an opaque aluminium film. Combining fluorescence correlation spectroscopy and lifetime measurements, we report the relative influence of excitation, radiative and non-radiative decay in the fluorescence process, giving a detailed description of the physics behind the overall 15 fold enhancement of the average fluorescence rate per molecule. This procedure is broadly adaptable to a wide range of nanostructures.

quant-ph↗