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Nicolas Rougemaille

Publications and source records attributed to Nicolas Rougemaille.

36 records · Page 2Linked to original sources

Extensive degeneracy, Coulomb phase and magnetic monopoles in an artificial realization of the square ice model

Artificial spin ice systems have been introduced as a possible mean to investigate frustration effects in a well-controlled manner by fabricating lithographically-patterned two-dimensional arrangements of interacting magnetic nanostructures. This approach offers the opportunity to visualize unconventional states of matter, directly in real space, and triggered a wealth of studies at the frontier between nanomagnetism, statistical thermodynamics and condensed matter physics. Despite the strong efforts made these last ten years to provide an artificial realization of the celebrated square ice model, no simple geometry based on arrays of nanomagnets succeeded to capture the macroscopically degenerate ground state manifold of the corresponding model. Instead, in all works reported so far, square lattices of nanomagnets are characterized by a magnetically ordered ground state consisting of local flux-closure configurations with alternating chirality. Here, we show experimentally and theoretically, that all the characteristics of the square ice model can be observed if the artificial square lattice is properly designed. The spin configurations we image after demagnetizing our arrays reveal unambiguous signatures of an algebraic spin liquid state characterized by the presence of pinch points in the associated magnetic structure factor. Local excitations, i.e. classical analogues of magnetic monopoles, are found to be free to evolve in a massively degenerated, divergence-free vacuum. We thus provide the first lab-on-chip platform allowing the investigation of collective phenomena, including Coulomb phases and ice-like physics.

cond-mat.mes-hall↗

Fragmentation of magnetism in artificial kagome dipolar spin ice

Geometrical frustration in magnetic materials often gives rise to exotic, low-temperature states of matter, like the ones observed in spin ices. Here we report the imaging of the magnetic states of a thermally-active artificial magnetic ice that reveal the fingerprints of a spin fragmentation process. This fragmentation corresponds to a splitting of the magnetic degree of freedom into two channels and is evidenced in both real and reciprocal space. Furthermore, the internal organization of both channels is interpreted within the framework of a hybrid spin-charge model that directly emerges from the parent spin model of the kagome dipolar spin ice. Our experimental and theoretical results provide insights into the physics of frustrated magnets and deepen our understanding of emergent fields through the use of tailor-made magnetism.

cond-mat.mes-hall↗

Magnetic domain walls in nanostrips of single-crystalline $\mathrm{Fe}_4\mathrm{N}(001)$ thin films with fourfold in-plane magnetic anisotropy

We investigated head-to-head domain walls in nanostrips of epitaxial $\mathrm{Fe}_4\mathrm{N}(001)$ thin films, displaying a fourfold magnetic anisotropy. Magnetic force microscopy and micromagnetic simulations show that the domain walls have specific properties, compared to soft magnetic materials. In particular, strips aligned along a hard axis of magnetization are wrapped by partial flux-closure concertina domains below a critical width, while progressively transforming to zigzag walls for wider strips. Transverse walls are favored upon initial application of a magnetic field transverse to the strip, while transformation to a vortex walls is favored upon motion under a longitudinal magnetic field. In all cases the magnetization texture of such fourfold anisotropy domain walls exhibits narrow micro-domain walls, which may give rise to peculiar spin-transfer features.

cond-mat.mtrl-sci↗

Anatomy and giant enhancement of the perpendicular magnetic anisotropy of cobalt-graphene heterostructures

We report strongly enhanced perpendicular magnetic anisotropy (PMA) of Co films by graphene coating from both first-principles and experiments. Our calculations show that graphene can dramatically boost the surface anisotropy of Co films up to twice the value of its pristine counterpart and can extend the out-of-plane effective anisotropy up to unprecedented thickness of 25~Å. These findings are supported by our experiments on graphene coating on Co films grown on Ir substrate. Furthermore, we report layer-resolved and orbital-hybridization-resolved anisotropy analysis which help understanding the physical mechanisms of PMA and more practically can help design structures with giant PMA. As an example, we propose super-exchange stabilized Co-graphene heterostructures with a robust out-of-plane constant effective PMA and linearly increasing interfacial anisotropy as a function of film thickness. These findings point towards possibilities to engineer graphene/ferromagnetic metal heterostructures with giant magnetic anisotropy more than 20 times larger compared to conventional multilayers, which constitutes a hallmark for future graphene and traditional spintronic technologies.

cond-mat.mtrl-sci↗

Head-to-head domain walls in one-dimensional nanostructures: an extended phase diagram ranging from strips to cylindrical wires

So far magnetic domain walls in one-dimensional structures have been described theoretically only in the cases of flat strips, or cylindrical structures with a compact cross-section, either square or disk. Here we describe an extended phase diagram unifying the two pictures, extensively covering the (width,thickness) space. It is derived on the basis of symmetry and phase-transition arguments, and micromagnetic simulations. A simple classification of all domain walls in two varieties is proposed on the basis of their topology: either with a combined transverse/vortex character, or of the Bloch-point type. The exact arrangement of magnetization within each variety results mostly from the need to decrease dipolar energy, giving rise to asymmetric and curling structures. Numerical evaluators are introduced to quantify curling, and scaling laws are derived analytically for some of the iso-energy lines of the phase diagram.

cond-mat.mes-hall↗

Manipulating domain wall chirality by current pulses in Permalloy/Ir nanostrips

Using magnetic force microscopy and micromagnetic simulations, we studied the effect of Oersted magnetic fields on the chirality of transverse magnetic domain walls in Fe$_{20}$Ni$_{80}$/Ir bilayer nanostrips. Applying nanosecond current pulses with a current density of around $2\times10^{12}$ A/m$^2$, the chirality of a transverse domain wall could be switched reversibly and reproducibly. These current densities are similar to the ones used for current-induced domain wall motion, indicating that the Oersted field may stabilize the transverse wall chirality during current pulses and prevent domain wall transformations.

cond-mat.mtrl-sci↗

Observation of Bloch-point domain walls in cylindrical magnetic nanowires

Topological protection is an elegant way of warranting the integrity of quantum and nanosized systems. In magnetism one example is the Bloch-point, a peculiar object implying the local vanishing of magnetization within a ferromagnet. Its existence had been postulated and described theoretically since several decades, however it has never been observed. We con rm experimentally the existence of Bloch points, imaged within domain walls in cylindrical magnetic nanowires, combining surface and transmission XMCD-PEEM magnetic microscopy. This opens the way to the experimental search for peculiar phenomena predicted during the motion of Bloch-point-based domain walls.

cond-mat.mtrl-sci↗

Direct Observation of Massless Domain Wall Dynamics in Nanostripes with Perpendicular Magnetic Anisotropy

Domain wall motion induced by nanosecond current pulses in nanostripes with perpendicular magnetic anisotropy (Pt/Co/AlO$_x$) is shown to exhibit negligible inertia. Time-resolved magnetic microscopy during current pulses reveals that the domain walls start moving, with a constant speed, as soon as the current reaches a constant amplitude, and no or little motion takes place after the end of the pulse. The very low 'mass' of these domain walls is attributed to the combination of their narrow width and high damping parameter $α$. Such a small inertia should allow accurate control of domain wall motion, by tuning the duration and amplitude of the current pulses.

cond-mat.mtrl-sci↗

Phase diagram of magnetic domain walls in spin valve nano-stripes

We investigate numerically the transverse versus vortex phase diagram of head-to-head domain walls in Co/Cu/Py spin valve nano-stripes (Py: Permalloy), in which the Co layer is mostly single domain while the Py layer hosts the domain wall. The range of stability of the transverse wall is shifted towards larger thickness compared to single Py layers, due to a magnetostatic screening effect between the two layers. An approached analytical scaling law is derived, which reproduces faithfully the phase diagram.

cond-mat.mtrl-sci↗

Direct observation of Oersted-field-induced magnetization dynamics in magnetic nanostripes

We have used time-resolved x-ray photoemission electron microscopy to investigate the magnetization dynamics induced by nanosecond current pulses in NiFe/Cu/Co nanostripes. A large tilt of the NiFe magnetization in the direction transverse to the stripe is observed during the pulses. We show that this effect cannot be quantitatively understood from the amplitude of the Oersted field and the shape anisotropy. High frequency oscillations observed at the onset of the pulses are attributed to precessional motion of the NiFe magnetization about the effective field. We discuss the possible origins of the large magnetization tilt and the potential implications of the static and dynamic effects of the Oersted field on current-induced domain wall motion in such stripes.

cond-mat.mtrl-sci↗

Asymmetric hysteresis of Néel caps in flux-closure magnetic dots

We investigated with XMCD-PEEM magnetic imaging the magnetization reversal processes of Néel caps inside Bloch walls in self-assembled, micron-sized Fe(110) dots with flux-closure magnetic state. In most cases the magnetic-dependent processes are symmetric in field, as expected. However, some dots show pronounced asymmetric behaviors. Micromagnetic simulations suggest that the geometrical features (and their asymmetry) of the dots strongly affect the switching mechanism of the Néel caps.

cond-mat.mtrl-sci↗

How many bits may fit in a single magnetic dot? XMCD-PEEM evidences the switching of Néel caps inside Bloch domain walls

Data storage relies on the handling of two states, called bits. The market of mass storage is currently still dominated by magnetic technology, hard disk drives for the broad public and tapes for massive archiving. In these devices each bit is stored in the form of the direction of magnetization of nanosized magnetic domains, i.e. areas of ferromagnetic materials displaying a uniform magnetization. While miniaturization is the conventional way to fuel the continuous increase of device density, disruptive solutions are also sought. To these pertain in recent years many fundamental studies no longer considering the magnetic domains themselves, but the manipulation of the domain walls (DWs) that separate such domains. Concepts of storage and logic based on the propagation of DWs along lithographically-patterned stripes have been patented, while many fundamental aspects of DW propagation deeply related to condensed matter physics are still hotly debated. If one now considers magnetic dots of submicrometer dimensions, the magnetization has a tendency to curl along the outer edges of the nanostructure to close its magnetic flux and thereby reduce its magnetostatic energy. Then both domains and DWs of well-defined geometries arise, whose combined manipulation has been proposed as a multilevel magnetic storage scheme...

cond-mat.mtrl-sci↗

Controlled switching of Néel caps in flux-closure magnetic dots

While magnetic hysteresis usually considers magnetic domains, the switching of the core of magnetic vortices has recently become an active topic. We considered Bloch domain walls, which are known to display at the surface of thin films flux-closure features called Néel caps. We demonstrated the controlled switching of these caps under a magnetic field, occurring via the propagation of a surface vortex. For this we considered flux-closure states in elongated micron-sized dots, so that only the central domain wall can be addressed, while domains remain unaffected.

cond-mat.other↗

High domain wall velocity at zero magnetic field induced by low current densities in spin-valve nanostripes

Current-induced magnetic domain wall motion at zero magnetic field is observed in the permalloy layer of a spin-valve-based nanostripe using photoemission electron microscopy. The domain wall movement is hampered by pinning sites, but in between them high domain wall velocities (exceeding 150 m/s) are obtained for current densities well below $10^{12} \unit{A/m^2}$, suggesting that these trilayer systems are promising for applications in domain wall devices in case of well controlled pinning positions. Vertical spin currents in these structures provide a potential explanation for the increase in domain wall velocity at low current densities.

cond-mat.mtrl-sci↗

X-ray photoelectron emission microscopy in combination with x-ray magnetic circular dichroism investigation of size effects on field-induced Néel-cap reversal

X-ray photoelectron emission microscopy in combination with x-ray magnetic circular dichroism is used to investigate the influence of an applied magnetic field on Néel caps (i.e., surface terminations of asymmetric Bloch walls). Self-assembled micron-sized Fe(110) dots displaying a moderate distribution of size and aspect ratios serve as model objects. Investigations of remanent states after application of an applied field along the direction of Néel-cap magnetization give clear evidence for the magnetization reversal of the Néel caps around 120 mT, with a $\pm$20 mT dispersion. No clear correlation could be found between the value of the reversal field and geometrical features of the dots.

cond-mat.mtrl-sci↗

Magnetostructure of MnAs on GaAs revisited

The ferromagnetic to nonferromagnetic (α-β) phase transition in epitaxial MnAs layers on GaAs(100) is studied by x-ray magnetic circular dichroism and x-ray magnetic linear dichroism photoemission electron microscopy in order to elucidate the nature of the controversial nonferromagnetic state of β-MnAs. In the coexistence region of the two phases the β phase shows a clear XMLD signal characteristic of antiferromagnetism. The nature and the possible causes of the elusiveness of this magnetic state are discussed.

cond-mat.mtrl-sci↗

Self-organization and magnetic domain microstructure of Fe nanowire arrays

Starting from essentially flat nanometer-thick Fe films, epitaxially grown at room temperature on W(110) surfaces, we used carefully tuned annealing schedules to produce periodic arrays of nanoscale ferromagnetic wires. The structural transition from continuous films to nanowire arrays is accompanied with an in-plane 90 degree rotation of the spontaneous magnetization. Using spin-polarized low-energy electron microscopy to map the local magnetization directions while annealing, we studied the role of the dewetting mechanism on the self-organization and magnetization reorientation processes.

cond-mat.mtrl-sci↗

Labyrinthine Island Growth during Pd/Ru(0001) Heteroepitaxy

Using low energy electron microscopy we observe that Pd deposited on Ru only attaches to small sections of the atomic step edges surrounding Pd islands. This causes a novel epitaxial growth mode in which islands advance in a snakelike motion, giving rise to labyrinthine patterns. Based on density functional theory together with scanning tunneling microscopy and low energy electron microscopy we propose that this growth mode is caused by a surface alloy forming around growing islands. This alloy gradually reduces step attachment rates, resulting in an instability that favors adatom attachment at fast advancing step sections.

cond-mat.mtrl-sci↗