arXiv subjects

Niklas Luhmann

Publications and source records attributed to Niklas Luhmann.

9 recordsLinked to original sources

arXiv2025

Picogram-Level Nanoplastic Analysis with Nanoelectromechanical System Fourier Transform Infrared Spectroscopy: NEMS-FTIR

We present a photothermal infrared spectroscopy-based approach for the chemical characterization and quantification of nanoplastics. By combining the high sensitivity of nanoelectromechanical systems (NEMS) with the wide spectral range and ubiquity of commercially available Fourier transform infrared (FTIR) spectrometers, NEMS-FTIR offers a time-efficient and cryogen-free option for the rapid, routine analysis of nanoplastics in aqueous samples. Polypropylene, polystyrene, and polyvinyl chloride nanoplastics with nominal diameters ranging from 54 to 262 nm were analyzed by NEMS-FTIR with limits of detection ranging from 101 pg to 353 pg, one order of magnitude lower than values reported for pyrolysis-gas chromatography-mass spectrometry of nanoplastics. The absorptance measured by NEMS-FTIR could be further converted to absolute sample mass using the attenuation coefficient, as demonstrated for polystyrene. Thanks to the wide spectral range of NEMS-FTIR, nanoplastic particles from different polymers could be readily identified, even when present in a mixture. The potential of NEMS-FTIR for the analysis of real samples was demonstrated by identifying the presence of nanoplastics released in water during tea brewing. Polyamide leachates in the form of fragments and smaller oligomers could be identified in the brewing water without sample pre-concentration, even in the presence of an organic matrix. Accelerated aging of the nylon teabags under elevated temperature and UV radiation showed further release of polyamide over time.

physics.ins-det↗

arXiv2025

Uncooled Thermal Infrared Detection Near the Fundamental Limit Using a Nanomechanical Resonator with a Broadband Absorber

This paper introduces a thermal infrared detector utilizing a nano-optomechanical silicon nitride (SiN) resonator, equipped with a free-space impedance-matched (FSIM) absorber composed of a platinum (Pt) thin film, offering a broadband spectral absorptance on average of 47%. To reduce photothermal back-action caused by intensity fluctuations of the readout laser, the FSIM absorber incorporates a circular clearance for the laser. The study provides a comprehensive characterization of the thermal time constant, power responsivity, and frequency stability of the resonators, with experimental results compared to analytical models and finite element method (FEM) simulations. The fastest thermal response is observed for the smallest 1 mm resonators, with a thermal time constant tau_th = 14 ms. The noise equivalent power (NEP) of the resonators is assessed, showing that the smallest 1 mm resonators exhibit the best sensitivity, with NEP = 27 pW/sqrt(Hz) and a respective specific detectivity of D* = 3.8e9 cm sqrt(Hz)/W. This is less than three times below the theoretical maximum for an ideal IR detector with 50% absorptance. This places our resonators among the most sensitive room-temperature IR detectors reported to date offering an extended spectral range from the near-IR to far-IR. This work underscores the potential of nano-optomechanical resonators for high-performance IR sensing applications.

physics.ins-det↗

arXiv2024

Room temperature, cavity-free capacitive strong coupling to mechanical motion

The back-action damping of mechanical motion by electromagnetic radiation is typically overwhelmed by internal loss channels unless demanding experimental ingredients such as superconducting resonators, high-quality optical cavities, or large magnetic fields are employed. Here we demonstrate the first room temperature, cavity-free, all-electric device where back-action damping exceeds internal loss, enabled by a mechanically compliant parallel-plate capacitor with a nanoscale plate separation and an aspect ratio exceeding 1,000. The device has four orders of magnitude lower insertion loss than a comparable commercial quartz crystal and achieves a position imprecision rivaling optical interferometers. With the help of a back-action isolation scheme, we observe radiative cooling of mechanical motion by a remote cryogenic load. This work provides a technologically accessible route to high-precision sensing, transduction, and signal processing.

cond-mat.mes-hall↗

arXiv2023

Resonance frequency tracking schemes for micro- and nanomechanical resonators

Nanomechanical resonators can serve as high performance detectors and have potential to be widely used in the industry for a variety of applications. Most nanomechanical sensing applications rely on detecting changes of resonance frequency. In commonly used frequency tracking schemes, the resonator is driven at or close to its resonance frequency. Closed-loop systems can continually check whether the resonator is at resonance and accordingly adjust the frequency of the driving signal. In this work, we study three resonance frequency tracking schemes, a feedback-free (FF), a self-sustaining oscillator (SSO), and a phase-locked loop oscillator (PLLO) scheme. We improve and extend the theoretical models for the FF and the SSO tracking schemes, and test the models experimentally with a nanoelectromechanical system (NEMS) resonator. We employ a SSO architecture with a pulsed positive feedback topology and compare it to the commonly used PLLO and FF schemes. We show that all tracking schemes are theoretically equivalent and that they all are subject to the same speed versus accuracy trade-off characteristics. In order to verify the theoretical models, we present experimental steady-state measurements for all tracking schemes. Frequency stability is characterized by computing the Allan deviation. We obtain almost perfect correspondence between the theoretical models and the experimental measurements. These results show that the choice of the tracking scheme is dictated by cost, robustness and usability in practice as opposed to fundamental theoretical differences in performance.

physics.ins-det↗

arXiv2021

Thermal IR detection with nanoelectromechanical silicon nitride trampoline resonators

Nanoelectromechanical (NEMS) resonators are promising uncooled thermal infrared (IR) detectors to overcome existing sensitivity limits. Here, we investigated nanoelectromechanical trampoline resonators made of silicon nitride (SiN) as thermal IR detectors. Trampolines have an enhanced responsivity of more than two orders of magnitude compared to state-of-the-art SiN drums. The characterized NEMS trampoline IR detectors yield a sensitivity in terms of noise equivalent power (NEP) of 7pW/$\sqrt{Hz}$ and a thermal response time as low as 4 ms. The detector area features an impedance-matched metal thin-film absorber with a spectrally flat absorption of 50% over the entire mid-IR spectral range from 1$\mu m$ to 25$\mu m$.

physics.app-ph↗

arXiv2020

Thermal transport and frequency response of localized modes on low-stress nanomechanical silicon nitride drums featuring a phononic bandgap structure

Development of broadband thermal sensors for the detection of, among others, radiation, single nanoparticles, or single molecules is of great interest. In recent years, photothermal spectroscopy based on the shift of the resonance frequency of stressed nanomechanical resonators has been successfully demonstrated. Here, we show the application of soft-clamped phononic crystal membranes made of silicon nitride as thermal sensors. It is experimentally demonstrated how a quasi-bandgap remains even at very low tensile stress, in agreement with finite element method simulations. An increase of the relative responsivity of the fundamental defect mode is found when compared to that of uniform square membranes of equal size, with enhancement factors as large as an order of magnitude. We then show phononic crystals engineered inside nanomechanical trampolines, which results in additional reduction of the tensile stress and increased thermal isolation, resulting in further enhancement of the responsivity. Finally, defect mode and bandgap tuning is shown by laser heating of the defect to the point where the fundamental defect mode completely leaves the bandgap.

physics.app-ph↗

arXiv2020

Thermal radiation dominated heat transfer in nanomechanical silicon nitride drum resonators

Nanomechanical silicon nitride (SiN) drum resonators are currently employed in various fields of applications that arise from their unprecedented frequency response to physical quantities. In the present study, we investigate the thermal transport in nanomechanical SiN drum resonators by analytical modelling, computational simulations, and experiments for a better understanding of the underlying heat transfer mechanism causing the thermal frequency response. Our analysis indicates that radiative heat loss is a non-negligible heat transfer mechanism in nanomechanical SiN resonators limiting their thermal responsivity and response time. This finding is important for optimal resonator designs for thermal sensing applications as well as cavity optomechanics.

physics.app-ph↗

arXiv2019

Ultrathin 2 nm gold as ideal impedance-matched absorber for infrared light

Thermal detectors are a cornerstone of infrared (IR) and terahertz (THz) technology due to their broad spectral range. These detectors call for suitable broad spectral absorbers with minimalthermal mass. Often this is realized by plasmonic absorbers, which ensure a high absorptivity butonly for a narrow spectral band. Alternativly, a common approach is based on impedance-matching the sheet resistance of a thin metallic film to half the free-space impedance. Thereby, it is possible to achieve a wavelength-independent absorptivity of up to 50 %, depending on the dielectric properties of the underlying substrate. However, existing absorber films typicallyrequire a thickness of the order of tens of nanometers, such as titanium nitride (14 nm), whichcan significantly deteriorate the response of a thermal transducers. Here, we present the application of ultrathin gold (2 nm) on top of a 1.2 nm copper oxide seed layer as an effective IR absorber. An almost wavelength-independent and long-time stable absorptivity of 47(3) %, ranging from 2 $\mu$m to 20 $\mu$m, could be obtained and is further discussed. The presented gold thin-film represents analmost ideal impedance-matched IR absorber that allows a significant improvement of state-of-the-art thermal detector technology.

physics.optics↗

arXiv2017

Effect of oxygen plasma on nanomechanical silicon nitride resonators

Precise control of tensile stress and intrinsic damping is crucial for the optimal design of nanomechanical systems for sensor applications and quantum optomechanics in particular. In this letter we study the in uence of oxygen plasma on the tensile stress and intrinsic damping of nanomechanical silicon nitride resonators. Oxygen plasma treatments are common steps in micro and nanofabrication. We show that oxygen plasma of only a few minutes oxidizes the silicon nitride surface, creating several nanometer thick silicon dioxide layers with a compressive stress of 1.30(16)GPa. Such oxide layers can cause a reduction of the e ective tensile stress of a 50 nm thick stoichiometric silicon nitride membrane by almost 50%. Additionally, intrinsic damping linearly increases with the silicon dioxide lm thickness. An oxide layer of 1.5nm grown in just 10s in a 50W oxygen plasma almost doubled the intrinsic damping. The oxide surface layer can be e ciently removed in bu ered HF.

cond-mat.mes-hall↗