arXiv subjects

Niklas Scheuler

Publications and source records attributed to Niklas Scheuler.

3 recordsLinked to original sources

arXiv2025

Impact of the valence band on Rydberg excitons in cuprous oxide quantum wells

The complex valence band structure of bulk cuprous oxide necessitates going beyond the parabolic approximation to precisely estimate exciton binding energies. The same is true for excitons in cuprous oxide quantum wells, for which many effects have been obtained so far only qualitatively within a hydrogenlike two-band model. Here, we derive the complete Hamiltonian for excitons in cuprous oxide quantum wells based on the Luttinger-Kohn model, taking into account the full complex valence band structure. Symmetry properties of the system are discussed. Numerical results based on the diagonalization of the Hamiltonian using B-spline functions reveal the energy shifts and the lifting of degeneracies due to the nondiagonal coupling terms of the complex valence band. The relative oscillator strengths of the excitonic transitions induced by circularly polarized light are also calculated.

cond-mat.mes-hall↗

arXiv2024

Resonance energies and linewidths of Rydberg excitons in Cu$_2$O quantum wells

Rydberg excitons are the solid-state analog of Rydberg atoms and can, e.g., for cuprous oxide, easily reach a large size in the region of $\mu$m for principal quantum numbers up to $n=25$. The fabrication of quantum well-like structures in the crystal leads to quantum confinement effects and opens the possibility to study a crossover from three-dimensional to two-dimensional excitons. For small widths of the quantum well (QW) there are several well separated Rydberg series between various scattering thresholds leading to the occurrence of electron-hole resonances with finite lifetimes above the lowest threshold. By application of the stabilization method to the parametric dependencies of the real-valued eigenvalues of the original three-dimensional Schr\"{o}dinger equation we calculate the resonance energies and linewidths for Rydberg excitons in QWs in regimes where a perturbative treatment is impossible. The positions and finite linewidths of resonances at energies above the third threshold are compared with the complex resonance energies obtained within the framework of the complex-coordinate-rotation technique. The excellent agreement between the results demonstrates the validity of both methods for intermediate sizes of the QW-like structures, and thus for arbitrary widths.

cond-mat.mes-hall↗

arXiv2023

Energy states of Rydberg excitons in finite crystals: From weak to strong confinement

Due to quantum confinement, excitons in finite-sized crystals behave rather differently than in bulk materials. We investigate the dependence of energies of Rydberg excitons on the strengths of parabolic as well as rectangular confinement potentials in finite-sized crystals. The evolution of the energy levels of hydrogen-like excitons in the crossover region from weak to strong parabolic confinement is analyzed for different quantum numbers by numerical solution of the two-dimensional Schr\"{o}dinger equation. The energy spectrum of hydrogen-like excitons in Cu$_{2}$O-based rectangular quantum wells is, in turn, obtained numerically from the solution of the three-dimensional Schr\"{o}dinger equation as a function of the quantum well width. Various crossings and avoided crossings of Rydberg energy levels are observed and categorized based on the symmetry properties of the exciton wave function. Particular attention is paid to the two limiting cases of narrow and wide quantum wells attributed to strong and weak confinement, respectively. The energies obtained with the pure Coulomb interaction are compared with the results originating from the Rytova-Keldysh potential, i.e., by taking into account the dielectric contrast in the quantum well and in the barrier.

cond-mat.mes-hall↗