Memory with Onsager-Casimir symmetry: Rotating particle in a viscoelastic fluid
We study the stochastic dynamics of a rotating Brownian particle in a non-Markovian fluid. Experimentally, we find that rotation enhances the long-time diffusivity of the particle and generates time-antisymmetric cross-correlations between orthogonal displacement components in the plane perpendicular to the rotation axis. To rationalize these observations, we introduce a minimal linear model in which a tracer is coupled to a slow bath degree of freedom and rotation enters through an advective coupling. Eliminating the bath variable yields a generalized Langevin equation with a non-reciprocal memory kernel. This kernel rotates in time, forming a logarithmic spiral, and it obeys Onsager-Casimir symmetry under reversal of the rotation vector, and the corresponding fluctuation-response relation. From the latter we obtain a geometric construction that links two-time cross-correlations to the transverse response of the particle in bulk. Unlike the ordinary Einstein relation, this relation involves the antisymmetric sector of the response. Our experiments and theory are in qualitative agreement, establishing rotating colloids in viscoelastic fluids as a minimal realization of Onsager-Casimir symmetry in time-nonlocal stochastic dynamics