arXiv subjects

Nikolai Kiesel

Publications and source records attributed to Nikolai Kiesel.

At least 19 recordsLinked to original sources

arXiv2026

Dark Optical Trapping of Resonant Transition-Metal Dichalcogenide Particles

Mitigating recoil events and minimizing optically induced heating are central challenges in the precise control and cooling of macroscopic particles. To overcome this, we propose trapping resonant dielectric particles for applications in ultra-high vacuum (UHV) levitodynamics. Contrary to other approaches, where suppressing the parasitic resonant scattering was achieved in a standing wave geometry, here we propose a single beam geometry in a dark trap regime. As a promising material platform, we focus on a class of transition-metal dichalcogenide (TMD) particles with high polarizability, characterized by refractive indices in the range $3.7$-$4.8$ and densities up to $9.3~\mathrm{g\,cm^{-3}}$. Using full Mie theory, we identify a range of TMD particle radii that support stable axial and radial magnetic quadrupole trapping in a bottle-beam configuration. We predict that for WS$_2$ particles with a mass of $0.5 \times 10^{12}\,\mathrm{amu}$, one can expect suppression of the scattering rate relative to the mechanical frequency down to $\Gamma/\Omega \simeq 0.02$. This corresponds to a coherence time extended by approximately three orders of magnitude compared with silica particles of the same mass trapped in conventional bright optical traps at UHV. Combined with significantly reduced internal heating, remaining well below the melting point of the material, dark trapping of resonant TMD macroscopic particles emerges as a promising platform for exploring quantum physics with large masses.

physics.optics↗

arXiv2025

Entropy production and non-Gaussianity of fast processes at weak damping

We present a method of estimating the rate of entropy production in underdamped dynamics by decomposing it into contributions originating in different non-equilibrium effects. Specifically, a non-zero average velocity, a non-thermal width of the velocity distribution, correlations between position and velocity and non-Gaussian velocity statistics represent different ways in which the system can be out of equilibrium and each give rise to a positive contribution to the overall entropy production rate. We demonstrate that each contribution can be separately estimated from experimental trajectory data of levitated nano-particles subject to non-linear forces. We find that the majority of the entropy production rate can be attributed to the first three contributions which can be estimated from the first and second moments of the position and velocity and therefore result in a useful \enquote{Gaussian} estimate for the entropy production rate.

cond-mat.stat-mech↗

arXiv2025

Free expansion of a charged nanoparticle via electrostatic compensation

Coherent wavepacket expansion is a key component of recent proposals aiming to create non-classical states of a levitated dielectric nanoparticle. Free evolution, i.e., releasing the particle from its harmonic trapping potential and allowing its position variance to grow, is a simple but effective expansion scheme, but requires accurate force compensation to avoid significant mean displacements of the wavepacket during the free evolution. Here, using an optical trap-release-recapture sequence, we demonstrate an electrostatic compensation technique that enables free evolution without significant mean displacement in 3D, successfully compensating both gravity and stray electric fields. To achieve 100 microsecond free evolution times with charged particles, we developed methods to map and correct for force cross-talk, as well as to control the environmental charge state. Combined with a low decoherence environment, our approach enables the preparation of largely delocalized states without the need for long freefall trajectories or a low-gravity environment.

quant-ph↗

arXiv2025

Feedback stabilization of a nanoparticle at the intensity minimum of an optical double-well potential

In this work, we develop and analyze adaptive feedback control strategies to stabilize and confine a nanoparticle at the unstable intensity minimum of an optical double-well potential. The resulting stochastic optimal control problem for a noise-driven mechanical particle in a nonlinear optical potential must account for unavoidable experimental imperfections such as measurement nonlinearities and slow drifts of the optical setup. To address these issues, we simplify the model in the vicinity of the unstable equilibrium and employ indirect adaptive control techniques to dynamically follow changes in the potential landscape. Our approach leads to a simple and efficient Linear Quadratic Gaussian (LQG) controller that can be implemented on fast and cost-effective FPGAs, ensuring accessibility and reproducibility. We demonstrate that this strategy successfully tracks the intensity minimum and significantly reduces the nanoparticle's residual state variance, effectively lowering its center-of-mass temperature. While conventional optical traps rely on confining optical forces in the light field at the intensity maxima, trapping at intensity minima mitigates absorption heating, which is crucial for advanced quantum experiments. Since LQG control naturally extends into the quantum regime, our results provide a promising pathway for future experiments on quantum state preparation beyond the current absorption heating limitation, like matter-wave interference and tests of the quantum-gravity interface.

eess.SY↗

arXiv2025

Roadmap on Quantum Thermodynamics

The last two decades has seen quantum thermodynamics become a well established field of research in its own right. In that time, it has demonstrated a remarkably broad applicability, ranging from providing foundational advances in the understanding of how thermodynamic principles apply at the nano-scale and in the presence of quantum coherence, to providing a guiding framework for the development of efficient quantum devices. Exquisite levels of control have allowed state-of-the-art experimental platforms to explore energetics and thermodynamics at the smallest scales which has in turn helped to drive theoretical advances. This Roadmap provides an overview of the recent developments across many of the field's sub-disciplines, assessing the key challenges and future prospects, providing a guide for its near term progress.

quant-ph↗

arXiv2024

Stabilizing nanoparticles in the intensity minimum: feedback levitation on an inverted potential

We demonstrate the stable trapping of a levitated nanoparticle on top of an inverted potential using a combination of optical readout and electrostatic control. The feedback levitation on an inverted potential (FLIP) method stabilizes the particle at an intensity minimum. By using a Kalman-filter-based linear-quadratic-Gaussian (LQG) control method, we confine a particle to within $\sigma_x = (9.0 \pm 0.5) nm$ of the potential maximum at an effective temperature of $(16 \pm 1) K$ in a room-temperature environment. Despite drifts in the absolute position of the potential maximum, we can keep the nanoparticle at the apex by estimating the drift from the particle dynamics using the Kalman filter. Our approach may enable new levitation-based sensing schemes with enhanced bandwidth. It also paves the way for optical levitation at zero intensity of an optical potential, which alleviates decoherence effects due to material-dependent absorption and is hence relevant for macroscopic quantum experiments.

physics.optics↗

arXiv2023

Hollow-core fiber loading of nanoparticles into ultra-high vacuum

Many experiments in the field of optical levitation with nanoparticles today are limited by the available technologies for particle loading. Here we introduce a new particle loading method that solves the main challenges, namely deterministic positioning of the particles and clean delivery at ultra-high vacuum levels as required for quantum experiments. We demonstrate the efficient loading, positioning, and repositioning of nanoparticles in the range of $100-755\,\mathrm{nm}$ diameter into different lattice sites of a standing wave optical trap, as well as direct loading of nanoparticles at an unprecedented pressure below $10^{-9}\,\mathrm{mbar}$. Our method relies on the transport of nanoparticles within a hollow-core photonic crystal fiber using an optical conveyor belt, which can be precisely positioned with respect to the target trap. Our work opens the path for increasing nanoparticle numbers in the study of multiparticle dynamics and high turn-around times for exploiting the quantum regime of levitated solids in ultra-high vacuum.

physics.optics↗

arXiv2023

Convergence to the asymptotic large deviation limit

Large deviation theory offers a powerful and general statistical framework to study the asymptotic dynamical properties of rare events. The application of the formalism to concrete experimental situations is, however, often restricted by finite statistics. Data might not suffice to reach the asymptotic regime or judge whether large deviation estimators converge at all. We here experimentally investigate the large deviation properties of the stochastic work and heat of a levitated nanoparticle subjected to nonequilibrium feedback control. This setting allows us to determine for each quantity the convergence domain of the large deviation estimators using a criterion that does not require the knowledge of the probability distribution. By extracting both the asymptotic exponential decay and the subexponential prefactors, we demonstrate that singular prefactors significantly restrict the convergence characteristics. Our results provide unique insight into the approach to the asymptotic large deviation limit and underscore the pivotal role of singular prefactors.

cond-mat.stat-mech↗

arXiv2022

Fast Quantum Interference of a Nanoparticle via Optical Potential Control

We introduce and theoretically analyze a scheme to prepare and detect non-Gaussian quantum states of an optically levitated particle via the interaction with a light pulse that generates cubic and inverted potentials. We show that this allows operating on short time- and lengthscales, which significantly reduces the demands on decoherence rates in such experiments. Specifically, our scheme predicts the observation of interference of nanoparticles with a mass above $10^8$ atomic mass units delocalised over several nanometers, on timescales of milliseconds, when operated at vacuum levels around $10^{-10}$~mbar and at room temperature. We discuss the prospect of using this approach for coherently splitting the wavepacket of massive dielectric objects using neither projective measurements nor an internal level structure.

quant-ph↗

arXiv2022

Observation of strong and tunable light-induced dipole-dipole interactions between optically levitated nanoparticles

Arrays of optically trapped nanoparticles have emerged as a promising platform for the study of complex non-equilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the interactions between particles. However, the optical interactions studied thus far only provide conservative optical binding forces of limited tunability. Here we demonstrate a coupling mechanism that is orders of magnitude stronger and has new qualitative features. These effects arise from the previously unexplored phase coherence between the optical fields that drive the light-induced dipole-dipole interaction. In addition, polarization control allows us to observe electrostatic coupling between charged particles in the array. Our results pave the way for a fully programmable many-body system of interacting nanoparticles with tunable dissipative and nonreciprocal interactions, which are instrumental for exploring entanglement and topological phases in arrays of levitated nanoparticles.

physics.optics↗

arXiv2022

MAQRO -- BPS 2023 Research Campaign Whitepaper

The objective of the proposed MAQRO mission is to harness space for achieving long free-fall times, extreme vacuum, nano-gravity, and cryogenic temperatures to test the foundations of physics in macroscopic quantum experiments. This will result in the development of novel quantum sensors and a means to probe the foundations of quantum physics at the interface with gravity. Earlier studies showed that the proposal is feasible but that several critical challenges remain, and key technologies need to be developed. These new technologies will open up the potential for achieving additional science objectives. The proposed research campaign aims to advance the state of the art and to perform the first macroscopic quantum experiments in space. Experiments on the ground, in micro-gravity, and in space will drive the proposed research campaign during the current decade to enable the implementation of MAQRO within the subsequent decade.

quant-ph↗

arXiv2022

Non-Markovian feedback control and acausality: an experimental study

Causality is an important assumption underlying nonequilibrium generalizations of the second law of thermodynamics known as fluctuation relations. We here experimentally study the nonequilibrium statistical properties of the work and of the entropy production for an optically trapped, underdamped nanoparticle continuously subjected to a time-delayed feedback control. Whereas the non-Markovian feedback depends on the past position of the particle for a forward trajectory, it depends on its future position for a time-reversed path, and is therefore acausal. In the steady-state regime, we show that the corresponding fluctuation relations in the long-time limit exhibit a clear signature of this acausality, even though the time-reversed dynamics is not physically realizable.

cond-mat.stat-mech↗

arXiv2021

Non-equilibrium quantum thermodynamics of a particle trapped in a controllable time-varying potential

Many advanced quantum techniques feature non-Gaussian dynamics, and the ability to manipulate the system in that domain is the next-stage in many experiments. One example of meaningful non-Gaussian dynamics is that of a double-well potential. Here we study the dynamics of a levitated nanoparticle undergoing the transition from an harmonic potential to a double-well in a realistic setting, subjecting to both thermalisation and localisation. We characterise the dynamics of the nanoparticle from a thermodynamic point-of-view, investigating the dynamics with the Wehrl entropy production and its rates. Furthermore, we investigate coupling regimes where the the quantum effect and thermal effect are of the same magnitude, and look at suitable squeezing of the initial state that provides the maximum coherence. The effects and the competitions of the unitary and the dissipative parts onto the system are demonstrated. We quantify the requirements to relate our results to a bonafide experiment with the presence of the environment, and discuss the experimental interpretations of our results in the end.

quant-ph↗

arXiv2021

Nonequilibrium control of thermal and mechanical changes in a levitated system

Fluctuation theorems are fundamental extensions of the second law of thermodynamics for small nonequilibrium systems. While work and heat are equally important forms of energy exchange, fluctuation relations have not been experimentally assessed for the generic situation of simultaneous mechanical and thermal changes. Thermal driving is indeed generally slow and more difficult to realize than mechanical driving. Here, we use feedback cooling techniques to implement fast and controlled temperature variations of an underdamped levitated microparticle that are one order of magnitude faster than the equilibration time. Combining mechanical and thermal control, we verify the validity of a fluctuation theorem that accounts for both contributions, well beyond the range of linear response theory. Our results allow the investigation of general far-from-equilibrium processes in microscopic systems that involve fast mechanical and thermal changes at the same time.

cond-mat.stat-mech↗

arXiv2021

Experimental nonequilibrium memory erasure beyond Landauer's bound

The clean world of digital information is based on noisy physical devices. Landauer's principle provides a deep connection between information processing and the underlying thermodynamics by setting a lower limit on the energy consumption and heat production of logically irreversible transformations. While Landauer's original formulation assumes equilibrium, real devices often do operate far from equilibrium. We show experimentally that the nonequilibrium character of a memory state enables full erasure with reduced power consumption as well as negative heat production. We implement the optimized erasure protocols in an optomechanical two-state memory. To this end, we introduce dynamical shaping of nonlinear potential landscapes as a powerful tool for levitodynamics as well as the investigation of far-from-equilibrium processes.

cond-mat.stat-mech↗

arXiv2021

Real-time optimal quantum control of mechanical motion at room temperature

The ability to accurately control the dynamics of physical systems by measurement and feedback is a pillar of modern engineering. Today, the increasing demand for applied quantum technologies requires to adapt this level of control to individual quantum systems. Achieving this in an optimal way is a challenging task that relies on both quantum-limited measurements and specifically tailored algorithms for state estimation and feedback. Successful implementations thus far include experiments on the level of optical and atomic systems. Here we demonstrate real-time optimal control of the quantum trajectory of an optically trapped nanoparticle. We combine confocal position sensing close to the Heisenberg limit with optimal state estimation via Kalman filtering to track the particle motion in phase space in real time with a position uncertainty of 1.3 times the zero point fluctuation. Optimal feedback allows us to stabilize the quantum harmonic oscillator to a mean occupation of $n=0.56\pm0.02$ quanta, realizing quantum ground state cooling from room temperature. Our work establishes quantum Kalman filtering as a method to achieve quantum control of mechanical motion, with potential implications for sensing on all scales. In combination with levitation, this paves the way to full-scale control over the wavepacket dynamics of solid-state macroscopic quantum objects in linear and nonlinear systems.

quant-ph↗

arXiv2020

Detecting nonclassical correlations in levitated cavity optomechanics

Nonclassical optomechanical correlations enable optical control of mechanical motion beyond the limitations of classical driving. Here we investigate the feasibility of using pulsed cavity-optomechanics to create and verify nonclassical phase-sensitive correlations between light and the motion of a levitated nanoparticle in a realistic scenario. We show that optomechanical two-mode squeezing can persist even at the elevated temperatures of state-of-the-art experimental setups. We introduce a detection scheme based on optical homodyning that allows revealing nonclassical correlations without full optomechanical state tomography. We provide an analytical treatment using the rotating wave approximation (RWA) in the resolved-sideband regime and prove its validity with a full numerical solution of the Lyapunov equation beyond the RWA. We build on parameters of current experiments for our analysis and conclude that the observation of nonclassical correlations is possible today.

quant-ph↗

arXiv2020

Thermodynamics of continuous non-Markovian feedback control

Feedback control mechanisms are ubiquitous in science and technology, and play an essential role in regulating physical, biological and engineering systems. The standard second law of thermodynamics does not hold in the presence of measurement and feedback. Most studies so far have extended the second law for discrete, Markovian feedback protocols; however, non-Markovian feedback is omnipresent in processes where the control signal is applied with a non-negligible delay. Here, we experimentally investigate the thermodynamics of continuous, time-delayed feedback control using the motion of an optically levitated, underdamped microparticle. We test the validity of a generalized second law which bounds the energy extracted from the system and study the breakdown of feedback cooling for very large time delays.

quant-ph↗