arXiv subjects

Niladri Banerjee

Publications and source records attributed to Niladri Banerjee.

13 recordsLinked to original sources

arXiv2026

Dynamical Josephson Effect Between a Singlet and a Triplet Superconductor

Phase-sensitive Josephson effect has long been central to identifying unconventional pairing symmetries in superconductors. Although the selection rules governing Josephson junctions (JJs) are generally determined by the symmetries of the constituent superconductors, we demonstrate that this paradigm is modified in the dynamic regime. By modeling a JJ where spin-singlet and spin-triplet superconductors are separated by a two-dimensional electron gas, we show that a time-dependent gate voltage qualitatively changes the underlying selection rules. This modification arises as a consequence of the gate-controlled spin-orbit coupling. A harmonic modulation of the gate voltage generates an oscillatory $\cos \phi$ Josephson component which vanishes in the static limit. The resulting charge current contains both dissipationless and dissipative components, with the latter strongly suppressed at low temperatures. This dynamical Josephson effect could transform the use of JJs in qubits, as sources of spin-triplet currents, and as platforms for proximity effects.

cond-mat.supr-con↗

arXiv2025

Weak-anti-localization-to-spin-dependent scattering at a proximity-magnetized heavy metal interface

A change in a materials electrical resistance with magnetic field (magnetoresistance) results from quantum interference effects and, or spin-dependent transport, depending on materials properties and dimensionality. In disordered conductors, electron interference leads to weak localization or anti-localization; in contrast, ferromagnetic conductors support spin-dependent scattering, leading to giant magnetoresistance (GMR). By varying the thickness of Au between 4 and 28 nm in a EuS/Au/EuS spin-switches, we observe a crossover from weak anti-localization to interfacial GMR. The crossover is related to a magnetic proximity effect in Au due to electron scattering at the insulating EuS interface. The proximity-induced exchange field in Au suppresses weak anti-localization, consistent with Maekawa-Fukuyama theory. With increasing Au thickness, GMR emerges along with spin Hall magnetoresistance. These findings demonstrate spin transport governed by interfacial exchange fields, building a framework for spintronic functionality without metallic magnetism.

cond-mat.mtrl-sci↗

arXiv2024

Colloquium: Spin-orbit effects in superconducting hybrid structures

Spin-orbit coupling (SOC) relates to the interaction between an electron's motion and its spin, and is ubiquitous in solid-state systems. Although the effect of SOC in normal-state phenomena has been extensively studied, its role in superconducting hybrid structures and devices opens many unexplored questions. In conjunction with broken symmetries and material inhomogeneities within superconducting hybrid structures, SOC may have additional contributions, beyond its effects in homogenous materials. Remarkably, even with well-established magnetic or nonmagnetic materials and conventional s-wave spin-singlet superconductors, SOC leads to emergent phenomena including equal-spin triplet pairing and topological superconductivity (hosting Majorana states), a modified current-phase relationship in Josephson junctions, and nonreciprocal transport. SOC is also responsible for transforming quasiparticles in superconducting structures which enhances the spin Hall effect and changes spin dynamics. Taken together, SOC in superconducting hybrid structures and the potential for electric tuning of the SOC strength, creates fascinating possibilities to advance superconducting spintronic devices for energy-efficient computing, and enable topological fault-tolerant quantum computing. By providing a description of experimental techniques and theoretical methods to study SOC, this Colloquium describes the current understanding of resulting phenomena in superconducting structures and offers a framework to select and design a growing class of materials systems where SOC plays an important role.

cond-mat.supr-con↗

arXiv2024

Realisation of de Gennes$'$ Absolute Superconducting Switch with a Heavy Metal Interface

In 1966, Pierre-Gilles de Gennes proposed a non-volatile mechanism for switching superconductivity on and off in a magnetic device. This involved a superconductor (S) sandwiched between ferromagnetic (F) insulators in which the net magnetic exchange field could be controlled through the magnetisation-orientation of the F layers. Because superconducting switches are attractive for a range of applications, extensive studies have been carried out on $F/S/F$ structures. Although these have demonstrated a sensitivity of the superconducting critical temperature ($T_{c}$) to parallel (P) and antiparallel (AP) magnetisation-orientations of the F layers, corresponding shifts in $T_c$ (i.e., ${\Delta}T_c = T_{c,AP} - T_{c,P}$) are lower than predicted with ${\Delta}T_c$ only a small fraction of $T_{c,AP}$, precluding the development of applications. Here, we report $EuS/Au/Nb/EuS$ structures where EuS is an insulating ferromagnet, Nb is a superconductor and Au is a heavy metal. For P magnetisations, the superconducting state in this structure is quenched down to the lowest measured temperature of 20 mK meaning that ${\Delta}T_c/T_{c,AP}$ is practically 1. The key to this so-called absolute switching effect is a sizable spin-mixing conductance at the $EuS/Au$ interface which ensures a robust magnetic proximity effect, unlocking the potential of $F/S/F$ switches for low power electronics.

cond-mat.supr-con↗

arXiv2024

Enhanced controllable triplet proximity effect in superconducting spin-orbit coupled spin valves with modified superconductor/ferromagnet interfaces

In a superconductor/ferromagnet hybrid, a magnetically controlled singlet-to-triplet Cooper pair conversion can modulate the superconducting critical temperature. In these triplet superconducting spin valves, such control usually requires inhomogeneous magnetism. However, in the presence of spin-orbit coupling from an interfacial heavy-metal layer, the singlet/triplet conversion rate and thus the critical temperature, can be controlled via the magnetization direction of a single homogeneous ferromagnet. Here, we report significantly enhanced controllable pair conversion to a triplet state in a Nb/Pt/Co/Pt superconducting spin valve in which Pt/Co/Pt is homogeneously magnetized and proximity-coupled to a superconducting layer of Nb. The Co/Pt interface furthest away from Nb is modified by a sub-nanometer-thick layer of Cu or Au. We argue that the enhancement is most likely associated from an improvement of the Co/Pt interface due to the insertion of Cu and Au layers. Additionally, the higher normalized orbital moments in Au measured using X-ray magnetic circular dichroism shows that increasing spin-orbit coupling enhances the triplet proximity effect - an observation supported by our theoretical calculations. Our results provide a pathway to enhancing triplet pair creation by interface engineering for device development in superspintronics.

cond-mat.supr-con↗

arXiv2023

Memristive behavior of functionalized graphene quantum dot and polyaniline nanocomposites

Zero-dimensional graphene quantum dots (GQD) dispersed in conducting polymer matrix display a striking range of optical, mechanical, and thermoelectric properties which can be utilized to design next-generation sensors and low-cost thermoelectric. This exotic electrical property in GQDs is achieved by exploiting the concentration of the GQDs and by tailoring the functionalization of the GQDs. However, despite extensive investigation, the nonlinear resistivity behavior leading to memristive like characteristic has not been explored much. Here, we report electrical characterisation of nitrogen functionalized GQD (NGQD) embedded in a polyaniline (PANI) matrix. We observe a strong dependence of the resistance on current and voltage history, the magnitude of which depends on the NGQD concentration and temperature. We explain this memristive property using a phenomenological model of the alignment of PANI rods with a corresponding charge accumulation arising from the NGQD on its surface. The NGQD-PANI system is unique in its ability to matrix offers a unique pathway to design neuromorphic logic and synaptic architectures with crucial advantages over existing systems.

cond-mat.mes-hall↗

arXiv2022

The interplay between structural, magnetic and electronic states in the pyrochlore iridate Eu2Ir2O7

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory (DFT) based calculations. The temperature dependent powder x-ray diffraction clearly rules out any change in the lattice symmetry below the MIT, nevertheless a clear anomaly in the Ir-O-Ir bond angle and Ir-O bond length is evident at the onset of MIT. From the x-ray absorption near edge structure (XANES) spectroscopic study of Ir-L3 and L2 edges, the effective spin-orbit coupling is found to be intermediate, at least quite far from the strong atomic spin-orbit coupling limit. Powder neutron diffraction measurement is in line with an all-in-all-out magnetic structure of the Ir-tetrahedra in this compound, which is quite common among rare-earth pyrochlore iridates. The sharp change in the Ir-O-Ir bond angle around the MIT possibly arises from the exchange striction mechanism, which favors an enhanced electron correlation via weakening of Ir-Ir orbital overlap and an insulating phase below TMI . The theoretical calculations indicate an insulating state for shorter bond angle validating the experimental observation. Our DFT calculations show a possibility of intriguing topological phase below a critical value of the Ir-O distance, which is shorter than the experimentally observed bond length. Therefore, a topological state may be realized in bulk Eu2Ir2O7 sample if the Ir-O bond length can be reduced by the application of sufficient external pressure.

cond-mat.str-el↗

arXiv2021

Superconductivity assisted change of the perpendicular magnetic anisotropy in V/MgO/Fe junctions

Controlling the perpendicular magnetic anisotropy (PMA) in thin films has received considerable attention in recent years due to its technological importance. PMA based devices usually involve heavy-metal (oxide)/ferromagnetic-metal bilayers, where, thanks to interfacial spin-orbit coupling (SOC), the in-plane (IP) stability of the magnetization is broken. Here we show that in V/MgO/Fe(001) epitaxial junctions with competing in-plane and out-of-plane (OOP) magnetic anisotropies, the SOC mediated interaction between a ferromagnet (FM) and a superconductor (SC) enhances the effective PMA below the superconducting transition. This produces a partial magnetization reorientation without any applied field for all but the largest junctions, where the IP anisotropy is more robust; for the smallest junctions there is a reduction of the field required to induce a complete OOP transition ($H_\text{OOP}$) due to the stronger competition between the IP and OOP anisotropies. Our results suggest that the degree of effective PMA could be controlled by the junction lateral size in the presence of superconductivity and an applied electric field. We also discuss how the $H_\text{OOP}$ field could be affected by the interaction between magnetic stray fields and superconducting vortices. Our experimental findings, supported by numerical modelling of the ferromagnet-superconductor interaction, open pathways to active control of magnetic anisotropy in the emerging dissipation-free superconducting spin electronics.

cond-mat.supr-con↗

arXiv2021

Structural and transport properties of 4f electron doped Y1-x(Dy)xPdBi topological semi-metallic thin films

We report the effect of 4f electron doping on structural, electrical and magneto-transport properties of Dy doped half Heusler Y1-x(Dy)xPdBi (x =0, 0.2, 0.5, 1) thin films grown by pulsed laser deposition. The Dy doping leads to lattice contraction which increases from 0% for the parent x =0 sample to approx 1.3% for x=1 sample with increase in Dy doping. The electrical transport measurements show a typical semi-metallic behaviour in the temperature range 3K to 300K and a sharp drop in resistivity at low temperatures (less than 3K) for all the samples. Magnetotransport measurements and Shubnikov de-Hass oscillations at high magnetic fields demonstrate that for these topologically non-trivial samples, Dy doping induced lattice contraction plays an active role in modifying the Fermi surface, carrier concentration and the effective electron mass. There is an uniform suppression of the onset of superconductivity with increased Dy doping which is possibly related to the increasing local exchange field arising from the 4f electrons in Dy. Our results indicate that we can tune various band structure parameters of YPdBi by f electron doping and strained thin films of Y1-x(Dy)xPdBi show surface dominated relativistic carrier transport at low temperatures.

cond-mat.mtrl-sci↗

arXiv2021

Strain driven emergence of topological non-triviality in YPdBi thin films

Half-Heusler compounds exhibit a remarkable variety of emergent properties such as heavy-fermion behaviour, unconventional superconductivity and magnetism. Several of these compounds have been predicted to host topologically non-trivial electronic structures. Remarkably, recent theoretical studies have indicated the possibility to induce non-trivial topological surface states in an otherwise trivial half-Heusler system by strain engineering. Here, using magneto-transport measurements and first principles DFT-based simulations, we demonstrate topological surface states on strained [110] oriented thin films of YPdBi grown on (100) MgO. These topological surface states arise in an otherwise trivial semi-metal purely driven by strain. Furthermore, we observe the onset of superconductivity in these strained films highlighting the possibility of engineering a topological superconducting state. Our results demonstrate the critical role played by strain in engineering novel topological states in thin film systems for developing next-generation spintronic devices.

cond-mat.mtrl-sci↗

arXiv2020

Superconductivity-induced change in magnetic anisotropy in epitaxial ferromagnet-superconductor hybrids with spin-orbit interaction

The interaction between superconductivity and ferromagnetism in thin film superconductor/ferromagnet heterostructures is usually reflected by a change in superconductivity of the S layer set by the magnetic state of the F layers. Here we report the converse effect: transformation of the magnetocrystalline anisotropy of a single Fe(001) layer, and thus its preferred magnetization orientation, driven by the superconductivity of an underlying V layer through a spin-orbit coupled MgO interface. We attribute this to an additional contribution to the free energy of the ferromagnet arising from the controlled generation of triplet Cooper pairs, which depends on the relative angle between the exchange field of the ferromagnet and the spin-orbit field. This is fundamentally different from the commonly observed magnetic domain modification by Meissner screening or domain wall-vortex interaction and offers the ability to fundamentally tune magnetic anisotropies using superconductivity - a key step in designing future cryogenic magnetic memories.

cond-mat.supr-con↗

arXiv2019

Long-ranged triplet supercurrent in a single in-plane ferromagnet with spin-orbit coupled contacts to superconductors

By converting conventional spin-singlet Cooper pairs to polarized spin-triplet pairs, it is possible to sustain long-ranged spin-polarized supercurrents flowing through strongly polarized ferromagnets. Obtaining such a conversion via spin-orbit interactions, rather than magnetic inhomogeneities, has recently been explored in the literature. A challenging aspect with regard to experimental detection has been that in order for Rashba spin-orbit interactions, present e.g. at interfaces due to inversion symmetry breaking, to generate such long-ranged supercurrents, an out-of-plane component of the magnetization is required. This limits the choice of materials and can induce vortices in the superconducting region complicating the interpretation of measurements. Therefore, it would be desirable to identify a way in which Rashba spin-orbit interactions can induce long-ranged supercurrents for purely in-plane rotations of the magnetization. Here, we show that this is possible in a lateral Josephson junction where two superconducting electrodes are placed in contact with a ferromagnetic film via two thin, heavy normal metals. The magnitude of the supercurrent in such a setup becomes tunable by the in-plane magnetization angle when using only a single magnetic layer. These results could provide a new and simpler way to generate controllable spin-polarized supercurrents than previous experiments which utilized complicated magnetically textured Josephson junctions.

cond-mat.supr-con↗

arXiv2019

Magnetization reorientation due to the superconducting transition in heavy-metal heterostructures

Recent theoretical and experimental work has demonstrated how the superconducting critical temperature ($T_c$) can be modified by rotating the magnetization of a single homogeneous ferromagnet proximity-coupled to the superconducting layer. This occurs when the superconductor and ferromagnet are separated by a thin heavy normal metal that provides an enhanced interfacial Rashba spin-orbit interaction. We consider the reciprocal effect: magnetization reorientation driven by the superconducting phase transition. We solve the tight-binding Bogoliubov-de Gennes equations on a lattice self-consistently and find that the relative angle between the spin-orbit field and the magnetization gives rise to a contribution in the free energy even in the normal state due to band-structure effects. For temperatures below $T_c$, superconductivity gives rise to a competing contribution. By lowering the temperature, in addition to reorientation of the favored magnetization direction from in-plane to out-of-plane, a $π/4$ in-plane rotation for thicker ferromagnetic layers is possible. Furthermore, computation of $T_c$ of the structure in the ballistic limit shows a dependence on the in-plane orientation of the magnetization, in contrast to our previous result on the diffusive limit. This finding is relevant with respect to thin-film heterostructures since these are likely to be in the ballistic regime of transport. Finally, we discuss the experimental feasibility of observing the magnetic anisotropy induced by the superconducting transition when other magnetic anisotropies, such as the shape anisotropy for a ferromagnetic film, are taken into account. Our work suggests that the superconducting condensation energy in principle can trigger a reorientation of the magnetization of a thin-film ferromagnet upon lowering the temperature below $T_c$, in particular for ferromagnets with weak magnetic anisotropies.

cond-mat.supr-con↗