SearcharxivSearch

arXiv subjects

Nils Torge Mecker

Publications and source records attributed to Nils Torge Mecker.

3 recordsLinked to original sources

Revisiting N$_2$-N$_2$ collisional linewidth models for S-branch rotational Raman scattering

This paper presents an evaluation of two commonly accepted Raman linewidth models typically used to fit CARS model parameters to data; the Modified Exponential Gap (MEG) and the Energy Corrected Sudden (ECS) models. The adjustable parameters in each model have been fit to published experimental linewidths, and comparisons are made to the various publications that have already provided similar adjustable constants. The approaches presented in the literature are discussed as are differences with the findings presented here.

physics.data-an

Optimising hybrid rotational femtosecond/picosecond coherent anti-Stokes Raman spectroscopy (HR-CARS) in nitrogen at high pressures and temperatures

We demonstrate the use of hybrid rotational femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman spectroscopy (HR-CARS) as a technique for temperature measurements in nitrogen gas at high pressures and temperatures. A broadband pulse shaper-adjusted 42 fs pulse interacts with a narrow-bandwidth, frequency-upconverted 5.5 ps pulse in a cell containing nitrogen at pressures of 1-70 atm and temperatures of 300-1000 K. A computational code is used to model spectra and fit experimental results to obtain best-fit temperatures. We demonstrate good qualitative fits as well as good accuracy and precision between thermocouple measured and best-fit temperatures over the explored pressure and temperature regimes. The overall average percentage temperature difference between thermocouple measurements and best-fit temperatures is -0.3% with a standard deviation of 7.1%, showing the suitability of HR-CARS for characterising high pressure and temperature environments.

physics.optics

Dual-probe 1-d hybrid fs/ps rotational CARS for simultaneous single-shot temperature, pressure, and O2/N2 measurements

We employ dual-probe 1-d fs/ps hybrid rotational coherent anti-Stokes Raman spectroscopy to investigate simultaneous temperature, pressure, and O2/N2 measurements for gas-phase diagnostics. The dual-probe HRCARS technique allows for simultaneous measurements from the time and frequency-domain. A novel approach for measuring pressure, which offers high accuracy (<1%) and precision (0.42%) is presented. The technique is first demonstrated in a chamber for a range of pressures (1-1.5 bar). This technique shows an impressive capability of resolving 1-d pressure gradients arising from a N2 jet impinging on a surface, both in laminar and turbulent conditions. The technique is shown to be capable of resolving single-shot pressure gradients (0.04 bar/mm) originating from kinetic energy conversion to pressure, and resolves characteristic O2/N2 structures from laminar and turbulent mixing.

physics.optics