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Nimrod Moiseyev

Publications and source records attributed to Nimrod Moiseyev.

At least 37 records · Page 2Linked to original sources

Optical absorption in atoms and molecules near laser-induced exceptional points

We present a non-Hermitian theory of atomic and molecular absorption, which enables computing the absorption spectrum of multi-electron atoms and molecules without using any fitting parameters. We propose a method for optically inducing exceptional points in atomic systems, and show that slight changes in the laser parameters may lead to dramatic changes in the absorption lineshape. We demonstrate these predictions for helium using exact ab-initio electronic-structure data. Finally, we derive a simple formula for the Fano asymmetry factor and evaluate it for a model xenon atom.

physics.chem-ph↗

Resonance poles and threshold energies for hadron physical problems by a model-independent universal algorithm

We show how complex resonance poles and threshold energies for systems in hadron physics can be accurately obtained by using a method based on the Padé-approximant which was recently developed for the calculation of resonance poles for atomic and molecular auto-ionization systems. The main advantage of this method is the ability to calculate the resonance poles and threshold energies from \emph{real} spectral data. In order to demonstrate the capabilities of this method we apply it here to an analytical model as well as to experimental data for the squared modulus of the vector pion form factor, the S0 partial wave amplitude for $ππ$ scattering and the cross section ratio $R(s)$ for $e^+e^-$ collisions. The extracted values for the resonance poles of the $ρ(770)$ and the $f_0(500)$ or $σ$ meson are in very good agreement with the literature. When the data are noisy the prediction of decay thresholds proves to be less accurate but feasible.

hep-ph↗

The effect of polarization on the propagation distance of leaky guided modes

We show that transverse-magnetic (TM) leaky modes can propagate further than transverse electric (TE) modes in real-index dielectric waveguides. We compute the density of states and find that while the TE spectrum contains only overlapping resonances, the TM spectrum typically contains several isolated peaks. By transforming the TM equation into a Schrödinger-type equation, we show that these isolated peaks arise due to $δ$-function barriers at the core-cladding interface. Our theory is useful for a range of applications, including filtering TM modes from initially unpolarized light and transferring information between distant waveguides.

physics.optics↗

Light stops at exceptional points

Almost twenty years ago the light was slowed down to less than $10^{-7}$ of its vacuum speed in a cloud of ultracold atoms of sodium. Upon a sudden turn-off of the coupling laser, a slow light pulse can be imprinted on cold atoms such that it can be read out and converted into photon again. In this process, the light is stopped by absorbing it and storing its shape within the atomic ensemble. Alternatively, the light can be stopped at the band edge in photonic-crystal waveguides, where the group speed vanishes. Here we extend the phenomenon of stopped light to the new field of parity-time (PT) symmetric systems. We show that zero group speed in PT symmetric optical waveguides can be achieved if the system is prepared at an exceptional point, where two optical modes coalesce. This effect can be tuned for optical pulses in a wide range of frequencies and bandwidths, as we demonstrate in a system of coupled waveguides with gain and loss.

physics.optics↗

Excited State Quantum Phase Transitions Studied from a Non-Hermitian Perspective

A main distinguishing feature of non-Hermitian quantum mechanics is the presence of exceptional points (EPs). They correspond to the coalescence of two energy levels and their respective eigenvectors. Here, we use the Lipkin-Meshkov-Glick (LMG) model as a testbed to explore the strong connection between EPs and the onset of excited state quantum phase transitions (ESQPTs). We show that for finite systems, the exact degeneracies (EPs) obtained with the non-Hermitian LMG Hamiltonian continued into the complex plane are directly linked with the avoided crossings that characterize the ESQPTs for the real (physical) LMG Hamiltonian. The values of the complex control parameter $α$ that lead to the EPs approach the real axis as the system size $N\rightarrow \infty$. This happens for both, the EPs that are close to the separatrix that marks the ESQPT and also for those that are far away, although in the latter case, the rate the imaginary part of $α$ reduces to zero as $N$ increases is smaller. With the method of Padé approximants, we can extract the critical value of $α$.

cond-mat.stat-mech↗

Quantum correlation effects on two successive measurements that are presented by non-commuting operators

Two measurements of $A$ and $B$ are carried out one after the other. The measurements of $A$ are controlled by the parameter $λ_A$ in the Kraus operator, where the measurements of $B$ are controlled by the parameter $λ_B$. Strong measurements imply that the parameters in the Kraus operators approach infinite large values while weak measurements are carried out when the parameters approach zero. Here we prove that by repeating on the two successive measurements of $A$ and $B$ then: (1) Average over all measurements of $A$ is invariant of the measurement strength parameters $λ_A$ and $λ_B$. It implies that all surprising results obtained in weak measurements of $A$ are washed out when the average is taken. (2) If the operators $\hat A$ and $\hat B$ commute then the mean value of $B$ as obtained by taking the average of the results for $B$ over all measurements is invariant of $λ_A$ and $λ_B$. Moreover it is exactly equal to the expectation value of $\hat B$ as expected for strong measurements of $B$. (3) If $\hat A$ and $\hat B$ do not commute \textit{and} another condition given in this paper is satisfied then the mean value of the results obtained for $B$ depends on the value of $λ_A$ and not on the value of $λ_B$. An illustrative possible experiment to show the effect of the strength of the measurements of A on the results obtained for the measurements of B is given.

quant-ph↗

Direct probe of anisotropy in atom-molecule collisions via quantum scattering resonances

Anisotropy is a fundamental property of particle interactions. It occupies a central role in cold and ultra-cold molecular processes, where long range forces have been found to significantly depend on orientation in ultra-cold polar molecule collisions. Recent experiments have demonstrated the emergence of quantum phenomena such as scattering resonances in the cold collisions regime due to quantization of the intermolecular degrees of freedom. Although these states have been shown to be sensitive to interaction details, the effect of anisotropy on quantum resonances has eluded experimental observation so far. Here, we directly measure the anisotropy in atom-molecule interactions via quantum resonances by changing the quantum state of the internal molecular rotor. We observe that a quantum scattering resonance at a collision energy of $k_B$ x 270 mK appears in the Penning ionization of molecular hydrogen with metastable helium only if the molecule is rotationally excited. We use state of the art ab initio and multichannel quantum molecular dynamics calculations to show that the anisotropy contributes to the effective interaction only for $H_2$ molecules in the first excited rotational state, whereas rotationally ground state $H_2$ interacts purely isotropically with metastable helium. Control over the quantum state of the internal molecular rotation allows us to switch the anisotropy on or off and thus disentangle the isotropic and anisotropic parts of the interaction. These quantum phenomena provide a challenging benchmark for even the most advanced theoretical descriptions, highlighting the advantage of using cold collisions to advance the microscopic understanding of particle interactions.

physics.chem-ph↗

Parameter estimation in atomic spectroscopy using exceptional points

The dynamics of spontaneous emission of an atomic system is studied in the framework of an open quantum system. The resulting quantum master equation for the atomic system is non hermitian. The generator $\mathcal{L}$ can possess non-hermitian degeneracies, i.e. exceptional points ($EP$), for specific values of the external laser driving amplitude and detuning from the atomic lines. We suggest to employ the special properties of these $EP$s for accurate parameter estimation. The method is demonstrated for the atomic spectrum of $S \rightarrow P$ transitions of $~^{85}$Rb and $~^{40}$Ca$~^+$.

quant-ph↗

Dynamically encircling exceptional points in a waveguide: asymmetric mode switching from the breakdown of adiabaticity

Physical systems with loss or gain feature resonant modes that are decaying or growing exponentially with time. Whenever two such modes coalesce both in their resonant frequency and their rate of decay or growth, a so-called "exceptional point" occurs, around which many fascinating phenomena have recently been reported to arise. Particularly intriguing behavior is predicted to appear when encircling an exceptional point sufficiently slowly, like a state-flip or the accumulation of a geometric phase. Experiments dedicated to this issue could already successfully explore the topological structure of exceptional points, but a full dynamical encircling and the breakdown of adiabaticity inevitably associated with it remained out of reach of any measurement so far. Here we demonstrate that a dynamical encircling of an exceptional point can be mapped onto the problem of scattering through a two-mode waveguide, which allows us for the first time to access the elusive effects occurring in this context. Specifically, we present experimental results from a waveguide structure that steers incoming waves around an exceptional point during the transmission process. In this way mode transitions are induced that make this device perfectly suited as a robust and asymmetric switch between different waveguide modes. Our work opens up new and exciting avenues to explore exceptional point physics at the crossroads between fundamental research and practical applications.

physics.optics↗

Exceptional points for parameter estimation in open quantum systems: Analysis of the Bloch equations

We suggest to employ the dissipative nature of open quantum systems for the purpose of parameter estimation: The dynamics of open quantum systems is typically described by a quantum dynamical semigroup generator ${\cal L}$. The eigenvalues of ${\cal L}$ are complex, reflecting unitary as well as dissipative dynamics. For certain values of parameters defining ${\cal L}$, non-hermitian degeneracies emerge, i.e. exceptional points ($EP$). The dynamical signature of these $EP$s corresponds to a unique time evolution. This unique feature can be employed experimentally to locate the $EP$s and thereby to determine the intrinsic system parameters with a high accuracy. This way we turn the disadvantage of the dissipation into an advantage. We demonstrate this method in the open system dynamics of a two-level system described by the Bloch equation, which has become the paradigm of diverse fields in physics, from NMR to quantum information and elementary particles.

quant-ph↗

Atomic and molecular complex resonances from real eigenvalues using standard (hermitian) electronic structure calculations

Complex eigenvalues, resonances, play an important role in large variety of fields in physics and chemistry. For example, in cold molecular collision experiments and electron scattering experiments, autoionizing and pre-dissociative metastable resonances are generated. However, the computation of complex resonance eigenvalues is difficult, since it requires severe modifications of standard electronic structure codes and methods. Here we show how resonance eigenvalues, positions and widths, can be calculated using the standard, widely used, electronic-structure packages. Our method enables the calculations of the complex resonance eigenvalues by using analytical continuation procedures (such as Padé). The key point in our approach is the existence of narrow analytical passages from the real axis to the complex energy plane. In fact, the existence of these analytical passages relies on using finite basis sets. These passages become narrower as the basis set becomes more complete, whereas in the exact limit, these passages to the complex plane are closed. As illustrative numerical examples we calculated the autoionization resonances of helium, hydrogen anion and hydrogen molecule. We show that our results are in an excellent agreement with the results obtained by other theoretical methods and with available experimental results.

quant-ph↗

Interatomic Coulombic Decay in two coupled Quantum Wells

Interatomic coulombic decay (ICD) is a relaxation process induced by electronic correlation. In this work we study the ICD process in a two coupled Quantum wells (QWs) nano-structure. We study a simple one-dimensional effective potential using experimental parameters of the semiconductor QW layers i.e. using the single band effective-mass approximation . In our calculations we consider the discontinuity of the effective mass of the electron in each of the QW layers. We control the ICD lifetime by changing the distance between the two wells. The expected overall trend is a decrease of ICD lifetime with a decrease in the distance between the wells. We show that the distance can be tuned such that the emitted ICD electron is trapped in a meta-stable state in the continuum i.e. a one electron resonance state. This causes the life time of the ICD to be an order of magnitude smaller even in very long distances, and improves the efficiency of the ICD. For the ICD to be dominant decay mechanism it must prevail over all other possible competitive decay processes. We have found that the lifetime of the ICD is on the timescale of picoseconds. Therefore, based on our results we can design an experiment that will observe the ICD phenomenon in QWs nano-structure for the first time. This work can lead to designing a wavelength sensitive detector which is efficient even in low intensities.

cond-mat.mes-hall↗

Perturbation theory for quasienergy (Floquet) solutions in the low-frequency regime of the oscillating electric field

For a simple illustrative model Hamiltonian for Xenon in low frequency linearly polarized laser field we obtain a remarkable agreement between the zero-order energy as well as amplitude and phase of the zero-order Floquet states and the exact eigenvalues and eigenfunctions of the Floquet operator. Here we use as a zero-order Hamiltonian the adiabatic Hamiltonian where time is used as an instantaneous parameter. Moreover, for a variety of low laser frequencies, $ω$, the deviation of the zero-order solutions from the exact quasi-energy (QE) Floquet solutions approaches zero at the time the oscillating laser field is maximal. This remarkable result gives a further justification to the validity of the first step in the simple man model. It should be stressed that the numerical calculations of the exact QE (Floquet) solutions become extremely difficult when $ω$ approaches zero and many Floquet channels are nested together and are coupled by the laser field. This is the main motivation for the development of perturbation theory for QE (Floquet) solutions when the laser frequency is small, to avoid the need to represent the Floquet operator by a matrix when the Fourier functions are used as a basis set. A way to calculate the radius of convergence of the perturbational expansion of the Floquet solutions in $ω$ is given.

physics.atom-ph↗

Entanglement and spin squeezing in non-Hermitian phase transitions

We show that non-Hermitian dynamics generate substantial entanglement in many-body systems. We consider the non-Hermitian Lipkin-Meshkov-Glick model and show that its phase transition occurs with maximum multiparticle entanglement: there is full N-particle entanglement at the transition, in contrast to the Hermitian case. The non-Hermitian model also exhibits more spin squeezing than the Hermitian model, showing that non-Hermitian dynamics are useful for quantum metrology. Experimental implementations with trapped ions and cavity QED are discussed.

cond-mat.quant-gas↗

Breakdown of adiabatic transfer of light in waveguides in the presence of absorption

In atomic physics, adiabatic evolution is often used to achieve a robust and efficient population transfer. Many adiabatic schemes have also been implemented in optical waveguide structures. Recently there has been increasing interests in the influence of decay and absorption, and their engineering applications. Here it is shown that even a small decay can significantly influence the dynamical behaviour of a system, above and beyond a mere change of the overall norm. In particular, a small decay can lead to a breakdown of adiabatic transfer schemes, even when both the spectrum and the eigenfunctions are only sightly modified. This is demonstrated for the generalization of a STIRAP scheme that has recently been implemented in optical waveguide structures. Here the question how an additional absorption in either the initial or the target waveguide influences the transfer property of the scheme is addressed. It is found that the scheme breaks down for small values of the absorption at a relatively sharp threshold, which can be estimated by simple analytical arguments.

quant-ph↗

Nuclear wave packet quantum interference in the intense laser dissociation of the $\mathrm{D}_{2}^{+}$ molecule

Recently it has been recognized that electronic conical intersections in molecular systems can be induced by laser light even in diatomics. As is known a direct consequence of these accidental degeneracies is the appearence of nonadiabatic effects which has a strong impact on the nuclear quantum dynamics. Studying the photodissociation process of the $\mathrm{D}_{2}^{+}$ molecule, we report here some novel and observable quantum interference phenomena that arise from the topological singularity induced by a strong laser field.

physics.atm-clus↗

The time-asymmetric quantum state exchange mechanism

We show here that due to non-adiabatic couplings in decaying systems applying the same time-dependent protocol in the forward and reverse direction to the same mixed initial state leads to different final pure states. In particular, in laser driven molecular systems applying a specifically chosen positively chirped laser pulse or an equivalent negatively chirped laser pulse yields entirely different final vibrational states. This phenomenon occurs when the laser frequency and intensity are slowly varied around an exceptional point (EP) in the laser intensity and frequency parameter space where the non-hermitian spectrum of the problem is degenerate. The protocol implies that a positively chirped laser pulse traces a counter-clockwise loop in time in the laser parameters' space whereas a negatively chirped pulse follows the same loop in the clockwise direction. According to this protocol one can choose the final pure state from any initial state. The obtained results imply the intrinsic non-adiabaticity of quantum transport around an EP, and offer a way to observe the EP experimentally in time-dependent quantum systems.

quant-ph↗

A third-order exceptional point effect on the dynamics of a single particle in a time-dependent harmonic trap

The time evolution of a single particle in a harmonic trap with time dependent frequency omega(t) is well studied. Nevertheless here we show that, when the harmonic trap is opened (or closed) as function of time while keeping the adiabatic parameter mu = [d omega(t)/dt]/omega(t)^2 fixed, a sharp transition from an oscillatory to a monotonic exponential dynamics occurs at mu = 2. At this transition point the time evolution has a third-order exceptional point (EP) at all instants. This situation, where an EP of a time-dependent Hermitian Hamiltonian is obtained at any given time, is very different from other known cases. Our finding is relevant to the dynamics of a single ion in a magnetic, optical, or rf trap, and of diluted gases of ultracold atoms in optical traps.

quant-ph↗