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Nitish Mathur

Publications and source records attributed to Nitish Mathur.

4 recordsLinked to original sources

Tunable magnetotransport through kinetically hindered first-order phase transitions in an antiferromagnetic metal

Controllable multilevel resistance states are of interest for memory technologies like neuromorphic computing, but robust materials platforms toward such behavior remain limited. Here, we show that the non-centrosymmetric antiferromagnetic metal CeCoGe$_3$ suggests one such route through a kinetically hindered first-order magnetic transition. Cooling through the kinetically hindered first-order transition in an applied magnetic field produces a magnetic glass state in which high- and low-temperature magnetic phases coexist. The relative fraction of these phases can be controlled by the applied field in which the sample is cooled, and the electrical resistance is directly sensitive to that fraction. As a result, it is demonstrated that CeCoGe$_3$ supports stable multilevel resistive states. These results identify kinetically hindered first-order phase transitions as a promising route towards controllable multilevel magnetoresistive states.

cond-mat.str-el

Directionally Locked Heteroepitaxy with a Structurally Modulated van der Waals Material

Precise orientation of symmetry-mismatched epilayers on van der Waals (vdW) substrates via heteroepitaxy has commonly been achieved through surface treatment processes to accommodate weak interlayer registry and bonding strength, thereby limiting the range of material combinations for heterostructure design. In this study, we investigate the influence of lattice instabilities in a structurally modulated vdW TaCo2Te2 substrate on the growth and alignment of a symmetry-mismatched bulk CoxTey epilayer using in situ heating in a transmission electron microscope (TEM). We show that a Peierls-like lattice instability occurs in TaCo2Te2 at a transition temperature of ~523 K, which was corroborated by phonon calculations. Post-heat-treated samples reveal a thermally induced surface diffusion process and the dominant lateral growth of the CoxTey epilayer on the TaCo2Te2 vdW layers, as observed in cross-sectional TEM images. Temperature-dependent selected area electron diffraction (SAED) patterns reveal that the quasi-vdW CoxTey/TaCo2Te2 heterointerface acquires directional locking by aligning larger interlayer lattice mismatch along the lattice instability axis of TaCo2Te2, while preserving a strong lattice matching along the orthogonal direction. This heterostructure exhibits precise interlayer registry with one-dimensional lattice incommensuration along the lattice instability axis, resulting from structural distortion to accommodate lattice-mismatch strain. Moreover, the interfacial reconstruction of TaCo2Te2 back to the distorted phase stabilizes the lattice-locking of the quasi-vdW heterointerface at elevated temperatures. These findings encourage the expansion of material diversity for designing and predicting novel multi-dimensional heterostructures by leveraging lattice instabilities to guide epitaxy.

cond-mat.mtrl-sci

Atomically Sharp Internal Interface in a Chiral Weyl Semimetal Nanowire

Internal interfaces in Weyl semimetals (WSMs) are predicted to host distinct topological features that are different from the commonly studied external interfaces (crystal-to-vacuum boundaries). However, the lack of atomically sharp and crystallographically oriented internal interfaces in WSMs makes it difficult to experimentally investigate hidden topological states buried inside the material. Here, we study a unique internal interface known as merohedral twin boundary in chemically synthesized single-crystal nanowires (NWs) of CoSi, a chiral WSM of space group P213 (No. 198). High resolution scanning transmission electron microscopy reveals that this internal interface is (001) twin plane and connects two enantiomeric counterparts at an atomically sharp interface with inversion twinning. Ab-initio calculations show localized internal Fermi arcs at the (001) twin boundary that can be clearly distinguished from both external Fermi arcs and bulk states. These merohedrally twinned CoSi NWs provide an ideal material system to probe unexplored topological properties associated with internal interfaces in WSMs.

cond-mat.mtrl-sci

Transport signatures of Fermi arcs at twin boundaries in Weyl materials

One of the most striking signatures of Weyl fermions is their surface Fermi arcs. Less known is that Fermi arcs can also be localized at internal twin boundaries where two Weyl materials of opposite chirality meet. In this work, we derive constraints on the topology and connectivity of these "internal Fermi arcs." We show that internal Fermi arcs can exhibit transport signatures and propose two probes: quantum oscillations and a quantized chiral magnetic current. We propose merohedrally twinned B20 materials as candidates to host internal Fermi arcs, verified through both model and ab initio calculations. Our theoretical investigation sheds lights on the topological features and motivates experimental studies into the intriguing physics of internal Fermi arcs.

cond-mat.mes-hall