arXiv subjects

Norberto Daniel Lanzillotti-Kimura

Publications and source records attributed to Norberto Daniel Lanzillotti-Kimura.

15 recordsLinked to original sources

arXiv2026

High-Performance Nanophononic Resonators in Self-Suspended WSe$_2$ Domes and Drums

Van der Waals materials are ideally suited for the implementation of high-frequency nanophononic resonators with atomically flat interfaces. Here, we present two versatile van der Waals-based nanophononic architectures: First, we introduce self-supporting nano-domes of WSe$_2$ as a scalable platform for the simultaneous generation of hundreds of high-quality nanoacoustic resonators with resonance frequencies in the 100 GHz range. Second, we engineer self-supporting nano-drums that reach record-high working frequencies for 2D-semiconductor transducers beyond 1 THz. Through optical pump-probe spectroscopy experiments and photoelastic linear chain model calculations, we gain a detailed understanding of the intricate interplay between phononic mode hybridization across heterostructures, the differences between modes close to the center and edge of the acoustic Brillouin zone, and the temporal structure of the photoelastic response. Both architectures have potential applications in low-cost nanoacoustic probing and the ultrafast modulation of quantum emitters in two-dimensional semiconductors. While nano-drums surpass the THz frequency barrier, nano-domes appear as an accessible, low-cost alternative for developing scalable nanophononic technologies.

cond-mat.mes-hall↗

arXiv2026

Boundary-dominated optomechanics in silicon metamaterial membranes

Stimulated Brillouin scattering in integrated photonic waveguides enables coherent coupling between optical photons and gigahertz acoustic phonons, providing a powerful mechanism for on-chip microwave photonics and opto-acoustic signal processing. Despite theoretical predictions of ultra-strong Brillouin interactions arising from enhanced light-sound coupling at device boundaries, most state-of-the-art integrated demonstrations remain governed by bulk photoelastic effects. This limitation stems from trade-offs between optical loss, interaction with waveguide boundaries and accessible phonon frequencies associated with the use of transverse-electric optical modes coupled to horizontally breathing mechanical modes. Here we demonstrate a new approach based on transverse-magnetic optical modes coupled to vertically breathing mechanical modes in suspended silicon membranes engineered with subwavelength metamaterial claddings. In this geometry, the interaction is dominated by the moving-boundary effect occurring at smooth top and bottom interfaces, while the phonon frequency is set primarily by the membrane thickness rather than its width. We observe forward Brillouin interactions at a record frequency of 12 GHz with a gain of 7200 W$^{-1}$ m$^{-1}$ and a mechanical quality factor of 620, yielding the highest Brillouin gain-to-quality-factor ratio reported in silicon waveguides. The devices exhibit net Brillouin amplification in millimeter-scale waveguides with pump powers below 15 mW, establishing a scalable platform for high-frequency integrated opto-acoustic signal processing.

physics.optics↗

arXiv2025

Towards Environmentally Responsive Hypersound Materials

The engineering of acoustic phonons in the gigahertz (GHz) range holds significant potential for technological breakthroughs in areas such as data processing, sensing and quantum communication. Novel approaches for nanophononic resonators responsive to external stimuli provide additional control and functionality for these devices. Mesoporous thin films (MTFs) for example, featuring nanoscale ordered pores, support GHz-range acoustic resonances. These materials are sensitive to environmental changes, such as liquid and vapor infiltration, modifying their effective optical and elastic properties. Here, a SiO$_{2}$ MTF-based open-cavity nanoacoustic resonator is presented, in which the MTF forms the topmost layer and is exposed to the environment. Using a transient reflectivity setup, acoustic responses under varying humidity conditions are investigated. A pronounced shift in acoustic resonance frequency with changes in relative humidity is observed for the first time, demonstrating a simple way to tune hypersound confinement. In addition, resonators with varying pore sizes and thicknesses are compared, revealing that resonance frequencies are primarily influenced by material properties and film thickness, rather than pore size. The proposed open-cavity resonator design provides a versatile platform for future studies on the mechanical response of MTFs to liquid and vapor infiltration, opening the gate to environment-responsive hypersound devices.

cond-mat.mes-hall↗

arXiv2025

Stimulated Forward Brillouin Scattering in Subwavelength Silicon Membranes

Brillouin scattering enables efficient and coherent conversion between optical photons and gigahertz-frequency phonons. Integrated circuits that harness this nonlinear interaction have immense potential for signal processing, quantum transduction, and sensing applications. However, achieving strong overlap and tight confinement of optical and mechanical modes in silicon nanophotonic waveguides remains a significant challenge. Here, we propose and demonstrate a novel strategy that enables independent control of optical and mechanical modes in periodically segmented silicon waveguides. Our approach combines two distinct periodic lattices: one with a period shorter than half of the optical wavelength, providing light guiding by metamaterial-induced index contrast, and another that creates a complete phononic bandgap confining acoustic modes. This dual-lattice strategy opens new degrees of freedom to optimize optomechanical confinement and coupling simultaneously. Based on this approach, we experimentally demonstrate remarkably high Brillouin gain of $G_\mathrm{B}=2673$ W$^{-1}$m$^{-1}$, resulting in a Stokes gain of 3 dB and an anti-Stokes loss of 4 dB with 6.4 MHz mechanical linewidth. These results illustrate the potential of subwavelength silicon metamaterials for engineering on-chip optomechanical interactions.

physics.optics↗

arXiv2024

Polarization-controlled Brillouin scattering in elliptical optophononic resonators

The fast-growing development of optomechanical applications has motivated advancements in Brillouin scattering research. In particular, the study of high frequency acoustic phonons at the nanoscale is interesting due to large range of interactions with other excitations in matter. However, standard Brillouin spectroscopy schemes rely on fixed wavelength filtering, which limits the usefulness for the study of tunable optophononic resonators. It has been recently demonstrated that elliptical optophononic micropillar resonators induce different energy-dependent polarization states for the Brillouin and the elastic Rayleigh scattering, and that a polarization filtering setup could be implemented to increase the contrast between the inelastic and elastic scattering of the light. An optimal filtering configuration can be reached when the polarization states of the laser and the Brillouin signal are orthogonal from each other. In this work, we theoretically investigate the parameters of such polarization-based filtering technique to enhance the efficiency of Brillouin scattering detection. For the filtering optimization, we explore the initial wavelength and polarization state of the incident laser, as well as in the ellipticity of the micropillars, and reach an almost optimal configuration for nearly background-free Brillouin detection. Our findings are one step forward on the efficient detection of Brillouin scattering in nanostructures for potential applications in fields such as optomechanics and quantum communication.

physics.optics↗

arXiv2024

Photonic and phononic modes in acoustoplasmonic toroidal nanopropellers

Non-conventional resonances, both acoustic and photonic, are found in metallic particles with a toroidal nanopropeller geometry that is generated by sweeping a three-lobed 2D-shape along a spiral with twisting angle, $α$. For both optical and acoustic cases, spectral location of resonances experiences a red-shift as a function of $α$. We demonstrate that the optical case can be understood as a natural evolution of resonances as the spiral length of the toroidal nanopropeller increases with $α$, implying a huge helicity dependent absorption cross section. In the case of acoustic response, two red-shifting breathing modes are identified. Additionally, even small $α$ allows the appearance of new low-frequency resonances, whose spectral dispersion depends on a competition between length of the generative spiral and the pitch of the toroidal nanopropeller.

physics.optics↗

arXiv2023

Elliptical micropillars for efficient generation and detection of coherent acoustic phonons

Coherent acoustic phonon generation and detection assisted by optical resonances are at the core of efficient optophononic transduction processes. However, when dealing with a single optical resonance, the optimum generation and detection conditions take place at different laser wavelengths, i.e. different detunings from the cavity mode. In this work, we theoretically propose and experimentally demonstrate the use of elliptical micropillars to reach these conditions simultaneously at a single wavelength. Elliptical micropillar optophononic resonators present two optical modes with orthogonal polarizations at different wavelengths. By employing a cross-polarized scheme pump-probe experiment, we exploit the mode splitting and couple the pump beam to one mode while the probe is detuned from the other one. In this way, at a particular micropillar ellipticity, both phonon generation and detection processes are enhanced. We report an enhancement of a factor of ~3.1 when comparing the signals from elliptical and circular micropillars. Our findings constitute a step forward in tailoring the light-matter interaction for more efficient ultrahigh-frequency optophononic devices.

physics.optics↗

arXiv2023

Effects of surface roughness and top layer thickness on the performance of Fabry-Perot cavities and responsive open resonators based on distributed Bragg reflectors

Optical and acoustic resonators based on distributed Bragg reflectors (DBRs) hold significant potential across various domains, from lasers to quantum technologies. In ideal conditions with perfectly smooth interfaces and surfaces, the DBR resonator quality factor primarily depends on the number of DBR pairs and can be arbitrarily increased by adding more pairs. Here, we present a comprehensive analysis of the impact of top layer thickness variation and surface roughness on the performance of both Fabry-Perot and open-cavity resonators based on DBRs. Our findings illustrate that even a small, nanometer-scale surface roughness can appreciably reduce the quality factor of a given cavity. Moreover, it imposes a limitation on the maximum achievable quality factor, regardless of the number of DBR pairs. These effects hold direct relevance for practical applications, which we explore further through two case studies. In these instances, open nanoacoustic resonators serve as sensors for changes occurring in dielectric materials positioned on top of them. Our investigation underscores the importance of accounting for surface roughness in the design of both acoustic and optical DBR-based cavities, while also quantifying the critical significance of minimizing roughness during material growth and device fabrication processes.

physics.optics↗

arXiv2023

Design of Cost-Effective Nanoacoustic Devices based on Mesoporous Thin Films

Gigahertz acoustic resonators have the potential to advance data processing and quantum communication. However, they are expensive and lack responsiveness to external stimuli, limiting their use in sensing applications. In contrast, low-cost nanoscale mesoporous materials, known for their high surface-to-volume ratio, have shown promise in various applications. We recently demonstrated that mesoporous silicon dioxide (SiO2) and titanium dioxide (TiO2) thin layers can support coherent acoustic modes in the 5 to 100 GHz range. In this study, we propose a new method for designing tunable acoustic resonators using mesoporous thin films on acoustic distributed Bragg reflectors. By infiltrating the pores with different chemicals, the material's properties could be altered and achieve tunability in the acoustic resonances. We present four device designs and use simulations to predict resonators with Q-factors up to 1000. We also observe that the resonant frequency and intensity show a linear response to relative humidity, with a tunability of up to 60 %. Our platform offers a unique opportunity to design cost-effective nanoacoustic sensing and reconfigurable optoacoustic nanodevices.

cond-mat.mes-hall↗

arXiv2023

Topological Nanophononic Interface States Using High-Order Bandgaps in the One-Dimensional Su-Schrieffer-Heeger Model

Topological interface states in periodic lattices have emerged as valuable assets in the fields of electronics, photonics, and phononics, owing to their inherent robustness against disorder. Unlike electronics and photonics, the linear dispersion relation of hypersound offers an ideal framework for investigating higher-order bandgaps. In this work, we propose a design strategy for the generation and manipulation of topological nanophononic interface states within high-order bandgaps of GaAs/AlAs multilayered structures. These states arise from the band inversion of two concatenated superlattices that exhibit inverted spatial mode symmetries around the bandgap. By adjusting the thickness ratio of the unit cells in these superlattices, we are able to engineer interface states in different bandgaps, enabling the development of versatile topological devices spanning a wide frequency range. Moreover, we demonstrate that such interface states can also be generated in hybrid structures that combine two superlattices with bandgaps of different orders centered around the same frequency. These structures open up new avenues for exploring topological confinement in high-order bandgaps, providing a unique platform for unveiling and better understanding complex topological systems.

cond-mat.mes-hall↗

arXiv2023

Genetic optimization of Brillouin scattering gain in subwavelength-structured silicon membrane waveguides

On-chip Brillouin optomechanics has great potential for applications in communications, sensing, and quantum technologies. Tight confinement of near-infrared photons and gigahertz phonons in integrated waveguides remains a key challenge to achieving strong on-chip Brillouin gain. Here, we propose a new strategy to harness Brillouin gain in silicon waveguides, based on the combination of genetic algorithm optimization and periodic subwavelength structuration to engineer photonic and phononic modes simultaneously. The proposed geometry is composed of a waveguide core and a lattice of anchoring arms with a subwavelength period requiring a single etch step. The waveguide geometry is optimized to maximize the Brillouin gain using a multi-physics genetic algorithm. Our simulation results predict a remarkable Brillouin gain exceeding 3300 1/(W m), for a mechanical frequency near 15 GHz.

physics.optics↗

arXiv2022

Brillouin Scattering Selection Rules in Polarization-Sensitive Photonic Resonators

The selection rules governing spontaneous Brillouin scattering in crystalline solids are usually taken as intrinsic material properties, locking the relative polarization of excitation and signal in bulk. In this work, we independently manipulate these polarization states by means of optical resonances in elliptical micropillars and demonstrate a polarization-based filtering scheme for Brillouin spectroscopy in the 20-100 GHz range, important for telecom applications. This strong modification of selection rules using elliptical micropillars can be extended to any optical system with localized, polarization-sensitive modes, such as plasmonic resonators, photonic crystals, birefringent micro-, and nanostructures. Our polarization control protocol will thus find applications in the engineering of light-matter interactions in optomechanical, optoelectronic and quantum optics devices.

physics.optics↗

arXiv2021

Generating 10-GHz phonons in nanostructured silicon membrane optomechanical cavity

Flexible control of photons and phonons in silicon nanophotonic waveguides is a key feature for emerging applications in communications, sensing and quantum technologies. Strong phonon leakage towards the silica under-cladding hampers optomechanical interactions in silicon-on-insulator. This limitation has been circumvented by totally or partially removing the silica under-cladding to form pedestal or silicon membrane waveguides. Remarkable optomechanical interactions have been demonstrated in silicon using pedestal strips, membrane ribs, and photonic/phononic crystal membrane waveguides. Still, the mechanical frequencies are limited to the 1-5 GHz range. Here, we exploit the periodic nanostructuration in Si membrane gratings to shape GHz phononic modes and near-infrared photonic modes, achieving ultrahigh mechanical frequency (10 GHz) and strong photon-phonon overlap (61.5%) simultaneously. Based on this concept, we experimentally demonstrate a one-dimension optomechanical micro-resonator with a high mechanical frequency of 10 GHz and a quality factor of 1000. These results were obtained at room temperature and ambient conditions with an intracavity optical power below 1 mW, illustrating the efficient optical driving of the mechanical mode enabled by the proposed approach.

physics.optics↗

arXiv2021

Silicon-on-insulator optomechanical microresonator with tight photon and phonon confinement

The implementation of optomechanical devices in silicon-on-insulator (SOI), the canonical silicon photonics technology is seriously hampered by the strong phonon leakage into the silica under-cladding. This limitation has been partially circumvented by total or partial removal of the silica under-cladding to form Si membranes or pedestal waveguides. However, this approach complicates integration with standard silicon optoelectronics circuitry, limiting the versatility and application of the strategy. Here, we propose and demonstrate a new strategy to confine photons and phonons in SOI without removing the silica under-cladding. Inspired by end-fire antenna arrays, we implement a periodic nanostructuration of silicon that simultaneously enables cancelling phonon leakage by destructive interference and guiding of photons by metamaterial index confinement. Based on this concept, we implement SOI optomechanical micro-resonators yielding remarkable optomechanical coupling (go=49 kHz) between 0.66 GHz mechanical modes and near-infrared optical modes. The mechanical mode exhibits a measured quality factor of Qm = 730, the largest reported for SOI optomechanical resonators, without silica removal. This value compares favorably with state-of-the-art Si membrane waveguides recently used to demonstrate remarkable Brillouin interactions in silicon (Qm ~ 700). These results open a new path for developing optomechanics in SOI without the need for silica removal, allowing seamless co-integration with current Si optoelectronics circuits, with a great potential for applications in communications, sensing, metrology, and quantum technologies.

physics.optics↗

arXiv2018

Topological nanophononic states by band inversion

Nanophononics is essential for the engineering of thermal transport in nanostructured electronic devices, it greatly facilitates the manipulation of mechanical resonators in the quantum regime, and could unveil a new route in quantum communications using phonons as carriers of information. Acoustic phonons also constitute a versatile platform for the study of fundamental wave dynamics, including Bloch oscillations, Wannier Stark ladders and other localization phenomena. Many of the phenomena studied in nanophononics were indeed inspired by their counterparts in optics and electronics. In these fields, the consideration of topological invariants to control wave dynamics has already had a great impact for the generation of robust confined states. Interestingly, the use of topological phases to engineer nanophononic devices remains an unexplored and promising field. Conversely, the use of acoustic phonons could constitute a rich platform to study topological states. Here, we introduce the concept of topological invariants to nanophononics and experimentally implement a nanophononic system supporting a robust topological interface state at 350 GHz. The state is constructed through band inversion, i.e. by concatenating two semiconductor superlattices with inverted spatial mode symmetries. The existence of this state is purely determined by the Zak phases of the constituent superlattices, i.e. that one-dimensional Berry phase. We experimentally evidenced the mode through Raman spectroscopy. The reported robust topological interface states could become part of nanophononic devices requiring resonant structures such as sensors or phonon lasers.

cond-mat.mes-hall↗