SearcharxivSearch

arXiv subjects

Noriaki Kida

Publications and source records attributed to Noriaki Kida.

6 recordsLinked to original sources

Discovery of transient topological crystalline order in optically driven SnSe

Ultrafast optical excitation provides a powerful route for accessing emergent quantum phases far from equilibrium, enabling transient light-induced phenomena such as magnetism, ferroelectricity, and superconductivity. However, extending this approach to induce topological phases, especially in conventional semiconductors, remains challenging. Here, we report the observation of a thermally inaccessible, transient topological crystalline order in the layered semiconductor SnSe, a trivial insulator with a sizable (~ 0.8 eV) band gap, induced by femtosecond above-gap excitation. Time- and angle-resolved photoemission spectroscopy directly reveals the sub-picosecond emergence of Dirac-like linear dispersions within the band gap. Their features, including a high Fermi velocity (~ 2.5x10^5 m/s), multiple Dirac points away from high-symmetry momenta, and independence from probe photon energy, are consistent with mirror-symmetry-protected surface states of a topological crystalline insulator. The observed spectral dynamics, combined with density functional theory calculations, indicate that the femtosecond excitation transiently increases lattice symmetry, enabling topological crystalline order to emerge. Our discovery opens new avenues for ultrafast optical control of topological quantum phases in semiconductors, with potential applications in quantum and spintronic devices.

cond-mat.mtrl-sci

Strong terahertz radiation via rapid polarization reduction in photoinduced ionic-to-neutral transition of tetrathiafulvalene-p-chloranil

Terahertz lights are usually generated through the optical rectification process within a femtosecond laser pulse in non-centrosymmetric materials. Here, we report a new generation mechanism of terahertz lights based upon a photoinduced phase transition (PIPT), in which an electronic structure is rapidly changed by a photoirradiation. When a ferroelectric organic molecular compound, tetrathiafulvalene-p-chloranil, is excited by a femtosecond laser pulse, the ionic-to-neutral transition is driven and simultaneously a strong terahertz radiation is produced. By analyzing the terahertz electric-field waveforms and their dependence on the polarization direction of the incident laser pulse, we demonstrate that the terahertz radiation originates from the ultrafast decrease of the spontaneous polarization in the photoinduced ionic-to-neutral transition. The efficiency of the observed terahertz radiation via the PIPT mechanism is found to be much higher than that via the optical rectification in the same material and in a typical terahertz emitter, ZnTe.

cond-mat.mtrl-sci

Terahertz radiation by subpicosecond spin-polarized photocurrent originating from Dirac electrons in a Rashba-type polar semiconductor

The spin-splitting energy bands induced by the relativistic spin-orbit interaction in solids provide a new opportunity to manipulate the spin-polarized electrons on the sub-picosecond time scale. Here, we report one such example in a bulk Rashba-type polar semiconductor BiTeBr. Strong terahertz electromagnetic waves are emitted after the resonant excitation of the interband transition between the Rashba-type spin-splitting energy bands with a femtosecond laser pulse circularly polarized. The phase of the emitted terahertz waves is reversed by switching the circular polarization. This suggests that the observed terahertz radiation originates from the subpicosecond spin-polarized photocurrents, which are generated by the asymmetric depopulation of the Dirac state. Our result provides a new way for the current-induced terahertz radiation and its phase control by the circular polarization of incident light without external electric fields.

cond-mat.str-el

Chirality of Matter Shows Up via Spin Excitations

Right- and left-handed circularly polarized light interact differently with electronic charges in chiral materials. This asymmetry generates the natural circular dichroism and gyrotropy, also known as the optical activity. Here we demonstrate that optical activity is not a privilege of the electronic charge excitations but it can also emerge for the spin excitations in magnetic matter. The square-lattice antiferromagnet Ba$_2$CoGe$_2$O$_7$ offers an ideal arena to test this idea, since it can be transformed to a chiral form by application of external magnetic fields. As a direct proof of the field-induced chiral state, we observed large optical activity when the light is in resonance with spin excitations at sub-terahertz frequencies. In addition, we found that the magnetochiral effect, the absorption difference for the light beams propagating parallel and anti-parallel to the applied magnetic field, has an exceptionally large amplitude close to 100%. All these features are ascribed to the magnetoelectric nature of spin excitations as they interact both with the electric and magnetic components of light.

cond-mat.str-el

Terahertz radiation by ultrafast spontaneous polarization modulation in multiferroic BiFeO$_3$ thin films

Terahertz (THz) radiation has been observed from multiferroic BiFeO$_3$ thin films via ultrafast modulation of spontaneous polarization upon carrier excitation with illumination of femtosecond laser pulses. The radiated THz pulses from BiFeO$_3$ thin films were clarified to directly reflect the spontaneous polarization state, giving rise to a memory effect in a unique style and enabling THz radiation even at zero-bias electric field. On the basis of our findings, we demonstrate potential approaches to ferroelectric nonvolatile random access memory with nondestructive readability and ferroelectric domain imaging microscopy using THz radiation as a sensitive probe.

cond-mat.str-el

Spectroscopic evidence for a charge-density-wave condensate in a charge-ordered manganite: Observation of collective excitation mode in Pr$_{\text{0.7}}$Ca$_{\text{0.3}}$MnO$_{\text{3}}$ by using THz time-domain spectroscopy

THz time-domain spectroscopy was used to directly probe the low-energy (0.5--5 meV) electrodynamics of the charge-ordered manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$. We revealed the existence of a finite peak structure around 2--3 meV well below the charge gap $\sim300$ meV. In analogy to the low-energy optical properties of the well-studied low-dimensional materials, we attributed this observed structure to the collective excitation mode arising from the charge-density-wave condensate. This finding provides the importance role of the quasi-one dimensional nature of the charge and orbital ordering in Pr$_{0.7}$Ca$_{0.3}$MnO$_3$.

cond-mat.str-el