arXiv subjects

Norman O. Birge

Publications and source records attributed to Norman O. Birge.

At least 37 records · Page 2Linked to original sources

arXiv2018

Phase Control in a Spin-Triplet SQUID

It is now well established that a Josephson junction made from conventional spin-singlet superconductors containing ferromagnetic layers can carry spin-triplet supercurrent under certain conditions. The first experimental signature of that fact is the propagation of such supercurrent over long distances through strong ferromagnetic materials. Surprisingly, one of the most salient predictions of the theory has yet to be verified experimentally -- namely that a Josephson junction containing three magnetic layers with coplanar magnetizations should exhibit a ground-state phase shift of either zero or pi depending on the relative orientations of those magnetizations. Here we demonstrate this property using Josephson junctions containing three different types of magnetic layers, chosen so that the magnetization of one layer can be switched by 180 degrees without disturbing the other two. Phase-sensitive detection is accomplished using a superconducting quantum interference device, or SQUID. Such a phase-controllable junction could be used as the memory element in a fully-superconducting computer.

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arXiv2018

Spin-valve Josephson junctions for cryogenic memory

Josephson junctions containing two ferromagnetic layers are being considered for use in cryogenic memory. Our group recently demonstrated that the ground-state phase difference across such a junction with carefully chosen layer thicknesses could be controllably toggled between zero and $π$ by switching the relative magnetization directions of the two layers between the antiparallel and parallel configurations. However, several technological issues must be addressed before those junctions can be used in a large-scale memory. Many of these issues can be more easily studied in single junctions, rather than in the Superconducting QUantum Interference Device (SQUID) used for the phase-sensitive measurements. In this work, we report a comprehensive study of spin-valve junctions containing a Ni layer with a fixed thickness of 2.0 nm, and a NiFe layer of thickness varying between 1.1 and 1.8 nm in steps of 0.1 nm. We extract the field shift of the Fraunhofer patterns and the critical currents of the junctions in the parallel and antiparallel magnetic states, as well as the switching fields of both magnetic layers. We also report a partial study of similar junctions containing a slightly thinner Ni layer of 1.6 nm and the same range of NiFe thicknesses. These results represent the first step toward mapping out a ``phase diagram" for phase-controllable spin-valve Josephson junctions as a function of the two magnetic layer thicknesses.

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arXiv2017

Spin-triplet supercurrent in Josephson junctions containing a synthetic antiferromagnet with perpendicular magnetic anisotropy

We present measurements of Josephson junctions containing three magnetic layers with noncolinear magnetizations. The junctions are of the form $S/F^{\prime}/N/F/N/F^{\prime \prime}/S$, where $S$ is superconducting Nb, $F^\prime$ is either a thin Ni or Permalloy layer with in-plane magnetization, $N$ is the normal metal Cu, $F$ is a synthetic antiferromagnet (SAF) with magnetization perpendicular to the plane, composed of Pd/Co multilayers on either side of a thin Ru spacer, and $F^{\prime \prime}$ is a thin Ni layer with in-plane magnetization. The supercurrent in these junctions decays more slowly as a function of the $F$-layer thickness than for similar spin-singlet junctions not containing the $F^\prime$ and $F^{\prime \prime}$ layers. The slower decay is the prime signature that the supercurrent in the central part of these junctions is carried by spin-triplet pairs. The junctions containing $F^{\prime}=$ Permalloy are suitable for future experiments where either the amplitude of the critical current or the ground-state phase difference across the junction is controlled by changing the relative orientations of the magnetizations of the $F^{\prime}$ and $F^{\prime \prime}$ layers.

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arXiv2017

Critical Current Oscillations of Elliptical Josephson Junctions with Single-Domain Ferromagnetic Layers

Josephson junctions containing ferromagnetic layers are of considerable interest for the development of practical cryogenic memory and superconducting qubits. Such junctions exhibit a phase shift of $π$ for certain ranges of ferromagnetic layer thickness. We present studies of Nb based micron-scale elliptically-shaped Josephson junctions containing ferromagnetic barriers of Ni$_{81}$Fe$_{19}$ or Ni$_{65}$Co$_{20}$Fe$_{15}$. By applying an external magnetic field, the critical current of the junctions are found to follow characteristic Fraunhofer patterns, and display sharp switching behavior suggestive of single-domain magnets. The high quality of the Fraunhofer patterns enables us to extract the maximum value of the critical current even when the peak is shifted significantly outside the range of the data due to the magnetic moment of the ferromagnetic layer. The maximum value of the critical current oscillates as a function of the ferromagnetic barrier thickness, indicating transitions in the phase difference across the junction between values of zero and $π$. We compare the data to previous work and to models of the 0-$π$ transitions based on existing theories.

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arXiv2016

Critical Current Oscillations of Josephson Junctions Containing PdFe Nanomagnets

Josephson junctions with ferromagnetic layers are vital elements in a new class of cryogenic memory devices. One style of memory device contains a spin valve with one "hard" magnetic layer and one "soft" layer. To achieve low switching fields, it is advantageous for the soft layer to have low magnetization and low magnetocrystalline anisotropy. A candidate class of materials that fulfills these criteria is the Pd$_{1-x}$Fe$_{x}$ alloy system with low Fe concentrations. We present studies of micron-scale elliptically-shaped Josephson junctions containing Pd$_{97}$Fe$_{3}$ layers of varying thickness. By applying an external magnetic field, the critical current of the junctions are found to follow characteristic Fraunhofer patterns. The maximum value of the critical current, extracted from the Fraunhofer patterns, oscillates as a function of the ferromagnetic barrier thickness, indicating transitions in the phase difference across the junction between values of zero and $π$.

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arXiv2015

Amplitude control of spin-triplet supercurrent in S/F/S Josephson junctions

Josephson junctions made with conventional s-wave superconductors and containing multiple layers of ferromagnetic materials can carry spin-triplet supercurrent in the presence of certain types of magnetic inhomogeneity. In junctions containing three ferromagnetic layers, the triplet supercurrent is predicted to be maximal when the magnetizations of adjacent layers are orthogonal, and zero when the magnetizations of any two adjacent layers are parallel. Here we demonstrate on-off control of the spin-triplet supercurrent in such junctions, achieved by rotating the magnetization direction of one of the three layers by 90$^{\circ}$. We obtain "on-off" ratios of 5, 7, and 19 for the supercurrent in the three samples studied so far. These observations directly confirm one of the most salient predictions of the theory, and pave the way for applications of spin-triplet Josephson junctions in the nascent area of "superconducting spintronics."

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arXiv2015

Controllable 0-pi Josephson junctions containing a ferromagnetic spin valve

Superconductivity and ferromagnetism are antagonistic forms of order, and rarely coexist. Many interesting new phenomena occur, however, in hybrid superconducting/ferromagnetic systems. For example, a Josephson junction containing a ferromagnetic material can exhibit an intrinsic phase shift of pi in its ground state for certain thicknesses of the material. Such "pi-junctions" were first realized experimentally in 2001, and have been proposed as circuit elements for both high-speed classical superconducting computing and for quantum computing. Here we demonstrate experimentally that the phase state of a Josephson junction containing two ferromagnetic layers can be toggled between 0 and pi by changing the relative orientation of the two magnetizations. These controllable 0-pi junctions have immediate applications in cryogenic memory where they serve as a necessary component to an ultra-low power superconducting computer. Such a fully superconducting computer is estimated to be orders of magnitude more energy-efficient than current semiconductor-based supercomputers. Phase controllable junctions also open up new possibilities for superconducting circuit elements such as superconducting "programmable logic," where they could function in superconducting analogs to field-programmable gate arrays.

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arXiv2012

Area-dependence of spin-triplet supercurrent in ferromagnetic Josephson junctions

Josephson junctions containing multiple ferromagnetic layers can carry spin-triplet supercurrent under certain conditions. Large-area junctions containing multiple domains are expected to have a random distribution of 0 or pi coupling across the junction surface, whereas magnetized samples should have uniquely pi coupling everywhere. We have measured the area dependence of the critical current in such junctions, and confirm that the critical current scales linearly with area in magnetized junctions. For as-grown (multi-domain) samples, the results are mixed. Samples grown on a thick Nb base exhibit critical currents that scale sub-linearly with area, while samples grown on a smoother Nb/Al multilayer base exhibit critical currents that scale linearly with area. The latter results are consistent with a theoretical picture due to Zyuzin and Spivak that predicts that the as-grown samples should have global pi/2 coupling.

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arXiv2011

Proximity-induced density-of-states oscillations in a superconductor/strong-ferromagnet system

We have measured the evolution of the tunneling density of states (DOS) in superconductor/ferromagnet (S/F) bilayers with increasing F-layer thickness, where F in our experiment is the strong ferromagnet Ni. As a function of increasing Ni thickness, we detect multiple oscillations in the DOS at the Fermi energy from differential conductance measurements. The features in the DOS associated with the proximity effect change from normal to inverted twice as the Ni thickness increases from 1 to 5 nm.

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arXiv2011

Optimization of spin-triplet supercurrent in ferromagnetic Josephson junctions

In the past year, several groups have observed evidence for long-range spin-triplet supercurrent in Josephson junctions containing ferromagnetic (F) materials. In our work, the spin-triplet pair correlations are created by non-collinear magnetizations between a central Co/Ru/Co "synthetic antiferromagnet" (SAF) and two outer thin F layers. Here we present data showing that the spin-triplet supercurrent is enhanced up to 20 times after our samples are subject to a large in-plane magnetizing field. This surprising result can be explained if the Co/Ru/Co SAF undergoes a "spin-flop" transition, whereby the two Co layer magnetizations end up perpendicular to the magnetizations of the two thin F layers. Direct experimental evidence for the spin-flop transition comes from scanning electron microscopy with polarization analysis and from spin-polarized neutron reflectometry.

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arXiv2011

Spin-memory loss at Co/Ru interfaces

We have determined the spin-memory-loss parameter, $δ_{Co/Ru}$, by measuring the transmission of spin-triplet and spin-singlet Cooper pairs across Co/Ru interfaces in Josephson junctions and by Current-Perpendicular-to-Plane Giant Magnetoresistance (CPP-GMR) techniques. The probability of spin-memory loss at the Co/Ru interface is $(1-exp(-δ_{Co/Ru}))$. From the CPP-MR, we obtain $δ_{Co/Ru} = 0.34^{+0.04}_{-0.02}$ that is in good agreement with $δ_{Co/Ru} = 0.35 \pm 0.08$ obtained from spin-triplet transmission. For spin-singlet transmission, we have $δ_{Co/Ru} = 0.64 \pm 0.05$ that is different from that obtained from CPP-GMR and spin-triplet transmission. The source of this difference is not understood.

cond-mat.mes-hall↗

arXiv2009

Observation of spin-triplet superconductivity in Co-based Josephson Junctions

We have measured a long-range supercurrent in Josephson junctions containing Co (a strong ferromagnetic material) when we insert thin layers of either PdNi or CuNi weakly-ferromagnetic alloys between the Co and the two superconducting Nb electrodes. The critical current in such junctions hardly decays for Co thicknesses in the range of 12-28 nm, whereas it decays very steeply in similar junctions without the alloy layers. The long-range supercurrent is controllable by the thickness of the alloy layer, reaching a maximum for a thickness of a few nm. These experimental observations provide strong evidence for induced spin-triplet pair correlations, which have been predicted to occur in superconducting/ferromagnetic hybrid systems in the presence of certain types of magnetic inhomogeneity.

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arXiv2009

Superconducting Tunneling Spectroscopy of a Carbon Nanotube Quantum Dot

We report results on superconducting tunneling spectroscopy of a carbon nanotube quantum dot. Using a three-probe technique that includes a superconducting tunnel probe, we map out changes in conductance due to band structure, excited states, and end-to-end bias. The superconducting probe allows us to observe enhanced spectroscopic features, such as robust signals of both elastic and inelastic co-tunneling. We also see evidence of inelastic scattering processes inside the quantum dot.

cond-mat.str-el↗

arXiv2009

Measurement of spin memory lengths in PdNi and PdFe ferromagnetic alloys

Weakly ferromagnetic alloys are being used by several groups in the study of superconducting/ferromagnetic hybrid systems. Because spin-flip and spin-orbit scattering in such alloys disrupt the penetration of pair correlations into the ferromagnetic material, it is desirable to have a direct measurement of the spin memory length in such alloys. We have measured the spin memory length at 4.2 K in sputtered Pd0.88Ni0.12 and Pd0.987Fe0.013 alloys using methods based on current-perpendicular-to-plane giant magnetoresistance. The alloys are incorporated into hybrid spin valves of various types, and the spin memory length is determined by fits of the Valet-Fert spin-transport equations to data of magnetoresistance vs. alloy thickness. For the case of PdNi alloy, the resulting values of the spin memory length are lsf(PdNi) = 2.8 +/- 0.5 nm and 5.4 +/- 0.6 nm, depending on whether or not the PdNi is exchange biased by an adjacent Permalloy layer. For PdFe, the spin memory length is somewhat longer, lsf(PdFe) = 9.6 +/- 2 nm, consistent with earlier measurements indicating lower spin-orbit scattering in that material. Unfortunately, even the longer spin memory length in PdFe may not be long enough to facilitate observation of spin-triplet superconducting correlations predicted to occur in superconducting/ferromagnetic hybrid systems in the presence of magnetic inhomogeneity.

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arXiv2009

Josephson Junctions with a synthetic antiferromagnetic interlayer

We report measurements of the critical current vs. Co thickness in Nb/Cu/Co/Ru/Co/Cu/Nb Josephson junctions, where the inner Co/Ru/Co trilayer is a "synthetic antiferromagnet" with the magnetizations of the two Co layers coupled antiparallel to each other via the 0.6 nm-thick Ru layer. Due to the antiparallel magnetization alignment, the net intrinsic magnetic flux in the junction is nearly zero, and such junctions exhibit excellent Fraunhofer patterns in the critical current vs. applied magnetic field, even with total Co thicknesses as large as 23 nm. There are no apparent oscillations in the critical current vs. Co thickness, consistent with theoretical expectations for this situation. The critical current of the junctions decays over 4 orders of magnitude as the total Co thickness increases from 3 to 23 nm. These junctions may serve as useful templates for future explorations of spin-triplet superconducting correlations, which are predicted to occur in supercon- ducting/ferromagnetic hybrid systems in the presence of certain types of magnetic inhomogeneity.

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arXiv2009

Asymmetric noise probed with a Josephson junction

Fluctuations of the current through a tunnel junction are measured using a Josephson junction. The current noise adds to the bias current of the Josephson junction and affects its switching out of the supercurrent branch. The experiment is carried out in a regime where switching is determined by thermal activation. The variance of the noise results in an elevated effective temperature, whereas the third cumulant, related to its asymmetric character, leads to a difference in the switching rates observed for opposite signs of the current through the tunnel junction. Measurements are compared quantitatively with recent theoretical predictions.

cond-mat.mes-hall↗

arXiv2009

Critical Current Behavior in Josephson Junctions with the Weak Ferromagnet PdNi

We have studied the variation of critical current in Superconductor/Ferromagnet/Superconductor (S/F/S) Josephson Junctions as a function of ferromagnet thickness using a weakly-ferromagnetic alloy Pd82Ni12. Measurements were performed for the thickness range 32 to 100 nm, over which the critical current density decreases by five orders of magnitude. The critical current density oscillates with a period of 12.9 +/- 0.3 nm, and decays over a characteristic length of 8.0 +/- 0.5 nm. There is no evidence of a crossover to a slower decay, which might indicate the presence of long-range spin-triplet pair correlations. We discuss possible reasons for their absence, including the possibility of strong spin flip scattering in PdNi.

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arXiv2008

Nonequilibrium transport in mesoscopic multi-terminal SNS Josephson junctions

We report the results of several nonequilibrium experiments performed on superconducting/normal/superconducting (S/N/S) Josephson junctions containing either one or two extra terminals that connect to normal reservoirs. Currents injected into the junctions from the normal reservoirs induce changes in the electron energy distribution function, which can change the properties of the junction. A simple experiment performed on a 3-terminal sample demonstrates that quasiparticle current and supercurrent can coexist in the normal region of the S/N/S junction. When larger voltages are applied to the normal reservoir, the sign of the current-phase relation of the junction can be reversed, creating a "$π$-junction." We compare quantitatively the maximum critical currents obtained in 4-terminal $π$-junctions when the voltages on the normal reservoirs have the same or opposite sign with respect to the superconductors. We discuss the challenges involved in creating a "Zeeman" $π$-junction with a parallel applied magnetic field and show in detail how the orbital effect suppresses the critical current. Finally, when normal current and supercurrent are simultaneously present in the junction, the distribution function develops a spatially inhomogeneous component that can be interpreted as an effective temperature gradient across the junction, with a sign that is controllable by the supercurrent. Taken as a whole, these experiments illustrate the richness and complexity of S/N/S Josephson junctions in nonequilibrium situations.

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