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Nuno A. M. Araújo

Publications and source records attributed to Nuno A. M. Araújo.

At least 19 recordsLinked to original sources

Spinning Living Crystals of Run-and-Tumble Particles with Environmental Feedback

Collective rotations are common in active matter, enhancing cohesion, transport, and mixing. They are typically attributed to chiral non-reciprocal dynamics due to intrinsic particle chirality, torque-generating interactions among units, or geometric confinement. Here, we uncover a different mechanism for rotational order in active matter where a dynamic environment coordinates the self-organization of non-chiral active particles into living crystals exhibiting sustained collective solid-like rotations. At intermediate densities, feedback from a fluctuating landscape of passive Brownian particles stabilizes large living crystals of obstacle-avoiding run-and-tumble agents. Strikingly, this environmental feedback also produces living crystals with qualitatively distinct dynamics: collective solid-like spinning emerges for particles with long persistence times approaching ballistic motion, rather than for particles moving by conventional enhanced diffusion. Beyond revealing a new route to collective rotational order in active matter, these findings highlight the integral role of a dynamic environment in self-organization and suggest environment-mediated design principles for active materials with unconventional dynamical responses.

cond-mat.soft↗

Porosity and Material Disorder Drive Distinct Channelization Transition

Flow through porous media can reshape the medium through erosion and deposition, producing preferential flow channels across a wide range of natural and industrial systems. Yet the mechanisms by which spatial disorder triggers channelization remain unclear. Here we derive a continuum description for the coupled evolution of flow and porosity by coarse-graining pore-scale dynamics and validating the resulting model with pore-scale simulations. Using this framework, we show that different sources of disorder lead to qualitatively distinct behaviors. Disorder in erosion resistance produces a discontinuous transition to localized flow, with permanent channels appearing only above a finite disorder strength. In contrast, even extremely weak fluctuations in the initial porosity destabilize homogeneous flow and trigger persistent channelization. These results reveal an unexpected sensitivity of evolving porous media to structural heterogeneity, suggesting that channelization can arise generically even in nearly uniform materials.

physics.flu-dyn↗

Persistence-Driven Void Formation in Dense Active-Passive Mixtures

It is well established that dilute active dopants can melt an arrested amorphous solid by enhancing cage breaking and accelerating structural relaxation. Yet it remains unclear whether increasing persistence simply amplifies this effective melting or instead reorganizes the fluidization mechanism itself. Here we show that, in a minimal active-passive mixture, increasing persistence drives a crossover from homogeneous fluidization to a localized mechanical instability, demonstrating that sustained active forcing restructures relaxation in space rather than merely strengthening it. Persistent dopants accumulate stress and nucleate voids as their mechanically perturbed regions overlap. In this regime, rearrangements localize at void boundaries, and active and passive particles exhibit comparable mobility, producing dynamics reminiscent of crowd mosh pits. Persistence therefore reorganizes fluidization through stress accumulation and confinement, revealing a distinct nonequilibrium localization mechanism in disordered solids.

cond-mat.soft↗

Janus Percolation in Anisotropic Limited-Degree Networks

Many real-world infrastructures, from sensor and road networks to power grids, are spatially embedded and anisotropic, with constraints on the maximum number of links each node can establish. Such systems can be represented as anisotropic limited-degree networks, in which each node forms at most q outgoing links preferentially oriented along a fixed direction. By increasing the node density sigma at fixed q, we uncover a reentrant percolation transition: a giant strongly connected component emerges, but unexpectedly disintegrates again at high densities. This counterintuitive behavior implies that adding nodes, normally expected to enhance robustness, can instead reduce mutual accessibility and weaken global connectivity. The critical behavior displays two coexisting "faces": random-percolation scaling along the preferred direction and directed-percolation scaling transversely, therefore we name this phenomenon Janus percolation, in analogy with the dual-faced Roman god. These findings demonstrate that anisotropy and degree limitation can jointly induce a novel reentrant connectivity with mixed universality that bridges the universality classes of random and directed percolation, providing fresh insight into how structural constraints shape connectivity and resilience in spatial networks.

cond-mat.stat-mech↗

Mapping the discrete folding landscape

Folding is emerging as a promising manufacturing process to transform flat materials into functional structures, offering efficiency by reducing the need for welding, gluing, and molding, while minimizing waste and enabling automation. Designing target shapes requires not only to determine cuts and folds, but also folding pathways. Simple combinatorics is impractical as the possibilities grow factorially with the number of folds. To address this, we present a graph-based algorithm for polyhedral shapes. By representing the target shape as a graph, where nodes correspond to faces and edges represent adjacency, the algorithm identifies all possible fold sequences and maps the configuration space into a discrete set of intermediate configurations. This systematic mapping is critical for the design of optimized processes, the simplifying of folding operations, the reduction of failures, and the improvement of manufacturing reliability.

cond-mat.soft↗

Shape transitions of sedimenting confined droplets and capsules: from oblate to bullet-like geometries

The transport and deformation of confined droplets and flexible capsules are central to diverse phenomena and applications, from biological flows in microcapillaries to industrial processes in porous media. Inspired by experiments, we perform numerical simulations to investigate their shape dynamics under varying levels of confinement and particle flexibility. A transition from an oblate to a bullet-like shape is observed at a confinement threshold, independent of flexibility, which agrees with our analytical calculations. A fluid-structure interaction analysis reveals two regimes: a pressure-dominated and a viscous-dominated regime. For highly flexible particles, the pressure-dominated regime prevails and the deformation is enhanced. These findings offer new insights into the transport of flexible particles in confined environments, with implications for biomedical applications, filtration technologies, and multiphase fluid mechanics.

cond-mat.soft↗

Ranked percolation model for the caking time of amorphous molecular powders

When amorphous molecular powders are exposed to high humidity levels or temperatures, the particle viscosity increases due to plasticization, promoting the formation of sinter bridges between pairs of particles in contact. Over time, these bridges facilitate particle agglomeration, eventually leading to the formation of a macroscopic cake that alters the mechanical properties and affects product quality. In this work, we model the caking process of amorphous powders subjected to a temperature shock as a bond percolation problem and investigate how particle bed heterogeneities influence the percolation threshold and, consequently, the expected caking times. Our findings indicate that a slight dispersion in particle size lowers the percolation threshold compared to a monodisperse bed or random percolation in polydisperse systems. Furthermore, we show that the expected caking time exhibits a non-monotonic behavior with the size dispersion, initially decreasing for low dispersion values and increasing for higher values. These results provide insights into the role of the particle size distribution on the caking dynamics of amorphous molecular powders

cond-mat.soft↗

Inverse design of self-folding 3D shells

Self-folding is an emerging paradigm for the inverse design of three-dimensional structures. While most efforts have concentrated on the shape of the net, our approach introduces a new design dimension-bond specificity between the edges. We transform this design process into a Boolean Satisfiability problem to derive solutions for various target structures. This method significantly enhances the yield of the folding process. Furthermore, by linearly combining independent solutions, we achieve designs for shape-shifting nets wherein the dominant structure evolves with varying external conditions. This approach is demonstrated through coarse-grained simulations on two examples of triangular and square nets capable of folding into multiple target shapes.

cond-mat.soft↗

Roadmap for Animate Matter

Humanity has long sought inspiration from nature to innovate materials and devices. As science advances, nature-inspired materials are becoming part of our lives. Animate materials, characterized by their activity, adaptability, and autonomy, emulate properties of living systems. While only biological materials fully embody these principles, artificial versions are advancing rapidly, promising transformative impacts across various sectors. This roadmap presents authoritative perspectives on animate materials across different disciplines and scales, highlighting their interdisciplinary nature and potential applications in diverse fields including nanotechnology, robotics and the built environment. It underscores the need for concerted efforts to address shared challenges such as complexity management, scalability, evolvability, interdisciplinary collaboration, and ethical and environmental considerations. The framework defined by classifying materials based on their level of animacy can guide this emerging field encouraging cooperation and responsible development. By unravelling the mysteries of living matter and leveraging its principles, we can design materials and systems that will transform our world in a more sustainable manner.

cond-mat.mtrl-sci↗

Lattice Boltzmann simulation of deformable fluid-filled bodies: progress and perspectives

With the rapid development of studies involving droplet microfluidics, drug delivery, cell detection, and microparticle synthesis, among others, many scientists have invested significant efforts to model the flow of these fluid-filled bodies. Motivated by the intricate coupling between hydrodynamics and the interactions of fluid-filled bodies, several methods have been developed. The objective of this review is to present a compact foundation of the methods used in the literature in the context of lattice Boltzmann methods. For hydrodynamics, we focus on the lattice-Boltzmann method due to its specific ability to treat time and spatial-dependent boundary conditions and to incorporate new physical models in a computationally efficient way. We split the existing methods into two groups with regard to the interfacial boundary: fluid-structure and fluid-fluid methods. The fluid-structure methods are characterised by the coupling between fluid dynamics and mechanics of the flowing body, often used in applications involving membranes and similar flexible solid boundaries. We further divide fluid-structure-based methods into two subcategories, those which treat the fluid-structure boundary as a continuum medium and those that treat it as a discrete collection of individual springs and particles. Next, we discuss the fluid-fluid methods, particularly useful for the simulations of fluid-fluid interfaces. We focus on models for immiscible droplets and their interaction in a suspending fluid and describe benchmark tests to validate the models for fluid-filled bodies.

cond-mat.soft↗

3D model for surface accumulation of chiral and non-chiral microswimmers

Persistent motion of microswimmers near boundaries is known to result in surface accumulation. Recently it was shown experimentally that surface accumulation of microswimmers is impacted primarily by steric forces and short-ranged hydrodynamics. A way to control surface accumulation is by reducing the contact surface area between swimmers and surface by modifying its topography, typically through the application of microscale structure. In this work, we introduce a three-dimensional(3D) model of a microswimmer navigating a volume bounded by a top and bottom surface. We describe the swimmer-surface interaction with an effective short-ranged hydrodynamic alignment force, and study numerically the effect of surface textures, modelled by convex obstacles, on the surface accumulation of chiral and non-chiral microswimmers. We find that, depending on the angular velocity of the swimmer, and the alignment force, convex obstacles can either hinder or enhance surface accumulation. We discuss potential applications to sorting of microswimmers by their angular velocity.

cond-mat.soft↗

Continuum model for extraction and retention in porous media

Several natural and industrial processes involve the extraction or retention of a solute by a fluid invading a network of channels. Examples include aquifer contamination, chemical filtration, and coffee extraction. We propose a continuum equation to model these processes, parametrized by the Péclet number and the rate of mass transfer between the solid and the fluid. We study the time dependence of the extracted mass for different values of the parameter space. The continuum description is validated by combining extraction experiments with coffee and computational fluid dynamics. An analytical solution is derived for the limit of slow mass transfer, which is corroborated by numerical simulations.

physics.flu-dyn↗

Optimal face-to-face coupling for fast self-folding kirigami

Kirigami-inspired designs can enable self-folding three-dimensional materials from flat, two-dimensional sheets. Hierarchical designs of connected levels increase the diversity of possible target structures, yet they can lead to longer folding times in the presence of fluctuations. Here, we study the effect of rotational coupling between levels on the self-folding of two-level kirigami designs driven by thermal noise in a fluid. Naturally present due to hydrodynamic resistance, we find that optimization of this coupling as control parameter can significantly improve a structure's self-folding rate and yield.

cond-mat.soft↗

Environmental Memory Boosts Group Formation of Clueless Individuals

The formation of groups of interacting individuals improves performance and fitness in many decentralised systems, from micro-organisms to social insects, from robotic swarms to artificial intelligence algorithms. Often, group formation and high-level coordination in these systems emerge from individuals with limited information-processing capabilities implementing low-level rules of communication to signal to each other. Here, we show that, even in a community of clueless individuals incapable of processing information and communicating, a dynamic environment can coordinate group formation by transiently storing memory of the earlier passage of individuals. Our results identify a new mechanism of indirect coordination via shared memory that is primarily promoted and reinforced by dynamic environmental factors, thus overshadowing the need for any form of explicit signalling between individuals. We expect this pathway to group formation to be relevant for understanding and controlling self-organisation and collective decision making in both living and artificial active matter in real-life environments.

cond-mat.soft↗

Collective transport of droplets through porous media

The flow of deformable particles, such as droplets, dragged by a fluid, through a network of narrow pores inside rocks or other porous media is key in a range of applications, from enhanced oil recovery and water filtration to lab on a chip sorting of cells. The collective dynamics and its impact on the flow are poorly understood. Here, using droplets as a prototype, we show that collective transport can occur for conditions under which a single particle would get trapped at a pore channel. When a series of droplets gets trapped, the fluids flow is affected significantly, leading to an increase of the pressure difference across the pore channels, which in turn squeezes the particles through the channels. We analyze the conditions for a single droplet to flow through one pore and derive the corresponding Bond number. We also obtain a rule for the collective flow of droplets in porous media.

physics.flu-dyn↗

Dispersion of activity at an active-passive nematic interface

Efficient nutrient mixing is crucial for the survival of bacterial colonies and other living systems. This raises the question of whether the optimization of mixing through the emergence of active turbulent motion in bacterial swarms played a role in the evolution of bacterial shapes. Here, to address this question, we solve the hydrodynamic equation for active nematics coupled with an advection-diffusion equation for the nutrients. The latter models a conserved activity field and mimics the conservation of nutrients in bacterial swarms. At the interface between active and passive nematic phases, in addition to diffusion, the activity is transported by interfacial flows and in turn modifies them through active stresses. We find that the interfacial dispersion of the conserved activity is subdiffusive due to the emergence of a barrier of negative defects at the active-passive interface, which hinders the propagation of the motile positive defects. Furthermore, we observe a non-monotonic dependence of the generalized diffusion coefficient on the aligning parameter, which is related to the shape of the particles. Our simulations suggest that there is an optimal shape that maximizes the dispersion of conserved activity at the active-passive nematic interface.

cond-mat.soft↗

Cell response in free-packed granular systems

The study of the interactions of living adherent cells with mechanically stable (visco)elastic materials enables understanding and exploiting physiological phenomena mediated by cell-extracellular communication. However, insight on the interaction of cells and surrounding objects with different stability patterns upon cell contact might unveil cell responses that may be engineered for innovative applications. Here, it is hypothesized that the efficiency of cell attachment, spreading and movement across a free-packed granular bed of microparticles depend on microparticle diameter, raising the possibility of a necessary minimum traction force for the reinforcement of cell-particle bonds, and long-term cell adhesion. The results suggest that microparticles with 14-20 μm are prone to cell-mediated mobility, holding the potential of inducing early cell detachment, while objects with diameters from 38-85 μm enable long-lasting cell adhesion and proliferation. An in-silico hybrid particle-based model that addresses time-dependent biological mechanisms of cell adhesion is proposed, providing inspiration for engineering platforms to address healthcare-related challenges.

physics.bio-ph↗

The role of disorder in the motion of chiral swimmers in the presence of obstacles

The presence of obstacles is intuitively expected to hinder the diffusive transport of micro-swimmers. However, for chiral micro-swimmers, a low density of obstacles near a surface can enhance their diffusive behavior, due to the rectification of the chiral motion by the obstacles. Here, we study numerically the role that disorder plays in determining the transport dynamics of chiral micro-swimmers on surfaces with obstacles. We consider different densities of regularly spaced obstacles and distinct types of disorder: noise in the dynamics of the micro-swimmer, quenched noise in the positions of the obstacles as well as obstacle size polydispersity. We show that, depending on the type and strength of the disorder, the presence of obstacles can either enhance or hinder transport, and discuss implications for the control of active transport in disordered media.

cond-mat.soft↗