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O. Dorvaux

Publications and source records attributed to O. Dorvaux.

At least 19 recordsLinked to original sources

The electromagnetic decay of $^{250m}$No and the stability of neutron deficient Rf isotopes

The electromagnetic decay of the $\approx$40 $\mu$s isomer of $^{250}$No has been investigated using the \textsc{Geant4} toolkit for the simulations of the interaction of particles through matter. It is concluded that the decay does not follow the pattern established in the lighter isotones, where the isomer decays directly to members of the ground state rotational band. An alternative scenario is proposed. The implications on the location of the isotopic border for neutron deficient Rf isotopes are discussed.

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Structure studies of 257Db through combined α, γ and internal-conversion-electron spectroscopy

This work reports on the study of the decay properties along the $^{257}$Db decay chain using the GABRIELA setup. The first observation of a high-K isomer in $^{257}$Db is presented. In addition, an unreported $α$-decay branch in $^{249}$Md has been evidenced, allowing to constrain the differences in energy of the $α$-decaying levels in $^{249}$Md, $^{253}$Lr and $^{257}$Db. Finally, the combination of the observed fine structure $α$-decay from the high-spin state in $^{257}$Db with the first observation the internal decay in $^{253}$Lr requires a revision of level and decay scheme. In particular, a change of parity for the high-spin state from 9/2$^{+}$ to 9/2$^{-}$ in the $^{257}$Db is suggested, and the implications of such a change are also discussed.

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Towards the Discovery of New Elements: Production of Livermorium (Z=116) with 50Ti

The $^{244}$Pu($^{50}$Ti,$xn$)$^{294-x}$Lv reaction was investigated at Lawrence Berkeley National Laboratory's 88-Inch Cyclotron facility. The experiment was aimed at the production of a superheavy element with $Z\ge 114$ by irradiating an actinide target with a beam heavier than $^{48}$Ca. Produced Lv ions were separated from the unwanted beam and nuclear reaction products using the Berkeley Gas-filled Separator and implanted into a newly commissioned focal plane detector system. Two decay chains were observed and assigned to the decay of $^{290}$Lv. The production cross section was measured to be $σ_{\rm prod}=0.44(^{+58}_{-28})$~pb at a center-of-target center-of-mass energy of 220(3)~MeV. This represents the first published measurement of the production of a superheavy element near the `Island-of-Stability', with a beam of $^{50}$Ti and is an essential precursor in the pursuit of searching for new elements beyond $Z=118$.

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$^{178}$Hg and asymmetric fission of neutron-deficient pre-actinides

Fission at low excitation energy is an ideal playground to probe the impact of nuclear structure on nuclear dynamics. While the importance of structural effects in the nascent fragments is well-established in the (trans-)actinide region, the observation of asymmetric fission in several neutron-deficient pre-actinides can be explained by various mechanisms. To deepen our insight into that puzzle, an innovative approach based on inverse kinematics and an enhanced version of the VAMOS++ heavy-ion spectrometer was implemented at the GANIL facility, Caen. Fission of $^{178}$Hg was induced by fusion of $^{124}$Xe and $^{54}$Fe. The two fragments were detected in coincidence using VAMOS++ supplemented with a new SEcond Detection arm. For the first time in the pre-actinide region, access to the pre-neutron mass and total kinetic energy distributions, and the simultaneous isotopic identification of one the fission fragment, was achieved. The present work describes the experimental approach, and discusses the pre-neutron observables in the context of an extended asymmetric-fission island located south-west of $^{208}Pb. A comparison with different models is performed, demonstrating the importance of this "new" asymmetric-fission island for elaborating on driving effects in fission.

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Study of the production and decay properties of neutron-deficient nobelium isotopes

The new neutron-deficient isotope $^{249}$No was synthesized for the first time in the fusion-evaporation reaction $^{204}$Pb($^{48}$Ca,3n)$^{249}$No. After separation, using the kinematic separator SHELS, the new isotope was identified with the GABRIELA detection system through genetic correlations with the known daughter and granddaughter nuclei $^{245}$Fm and $^{241}$Cf. The alpha-decay activity of $^{249}$No has an energy of 9129(22)$~$keV and half-life 38.3(2.8) ms. An upper limit of 0.2\% was measured for the fission branch of $^{249}$No. Based on the present data and recent information on the decay properties of $^{253}$Rf and aided by Geant4 simulations, the ground state of $^{249}$No is assigned the 5/2$^+$[622] neutron configuration and a partial decay scheme from $^{253}$Rf to $^{245}$Fm could be established. The production cross-section was found to be $σ$(3n)=0.47(4) nb at a mid-target beam energy of 225.4 MeV, which corresponds to the maximum of the calculated excitation function. Correlations of the $^{249}$No alpha activity with subsequent alpha decays of energy 7728(20) keV and half-life $1.2_{-0.4}^{+1.0}$ min provided a firm measurement of the electron-capture or $β^{+}$ branch of $^{245}$Fm to $^{245}$Es. The excitation function for the 1n, 2n and 3n evaporation channels was measured. In the case of the 2n-evaporation channel $^{250}$No, a strong variation of the ground state and isomeric state populations as a function of bombarding energy could be evidenced.

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Spontaneous fission of 246Fm

An experiment on the study of the $^{246}$Fm spontaneous fission was conducted using the SHELS separator. The isotope was synthesized in the complete fusion reaction of $^{40}$Ar beam ions and $^{208}$Pb target nuclei. The neutron yields of $^{246}$Fm spontaneous fission ($\overlineν = 3.79\pm0.30$, $σ^{2}_ν = 2.1$) were obtained using the SFiNx detector system. The multiplicity distribution of emitted prompt neutrons was restored using the Tikhonov method of statistical regularisation ($\overlineν_{r} = 3.79\pm0.20$, $σ^{2}_{νr} = 2.8$). The spontaneous fission branching ratio ($b_{SF} = 0.061\pm0.005$) and the half-life ($T_{1/2} = 1.50^{+0.08}_{-0.07}$ s) of the isotope were determined. The experimental data were compared with scission point model predictions. Excellent convergence was observed in the average number of neutrons per spontaneous fission process. However, the forms of the experimental and model prompt neutron multiplicity distributions differ significantly.

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Fission properties of $^{253}$Rf and the stability of neutron-deficient Rf isotopes

An analysis of recent experimental data [J. Khuyagbaatar et al., Phys. Rev. C 104, L031303 (2021)] has established the existence of two fissioning states in $^{253}$Rf: the ground state and a low-lying isomeric state, most likely involving the same neutron single-particle configurations as in the lighter isotone $^{251}$No. The ratio of fission half-lives measured in $^{253}$Rf was used to predict the fission properties of the 1/2$^{+}$ isomeric state in $^{251}$No and draw conclusions as to the stability against fission of even lighter Rf systems. This paper focusses again on the fission properties of $^{253}$Rf and their impact on the stability of other neutron deficient isotopes, using new and improved data collected from two experiments performed at the Flerov Laboratory of Nuclear Reactions in Dubna, Russia. Two fission activities with half-lives of 52.8(4.4)$~μ$s and 9.9(1.2) ms were measured in the case of $^{253}$Rf, confirming the results of J. Kkuyagbaatar et al. A third state, at much higher excitation energy, was also observed through the detection of its electromagnetic decay to the 52.8$~μ$s state. This observation leads to the opposite quantum-configuration assignments for the fissioning states as compared to the ones established by J. Khuyagbaatar et al., namely that the higher-spin state has the shortest fission half-life. This inversion of the ratio of fission hindrances between the low and high-spin states is corroborated in the isotone $^{251}$No by the non observation of any substantial fission branch from the low-spin isomer.

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Alpha-decay spectroscopy of $^{257}$Rf

The decay properties of the ground state and excited states of $^{257}$Rf have been investigated with the detector array GABRIELA at the FLNR, Dubna. The electromagnetic decay of a new excited state in $^{253}$No has been observed. The state lies 750 keV above the ground state and is favourably populated in the alpha decay of the low-lying spin isomer of $^{257}$Rf. It decays to the 9/2$^-$ ground state by an M1 transition and is assigned the 11/2$^-$[725] Nilsson configuration. The presence of this state suggests a possible reinterpretation of the decay of the high-K isomer in $^{253}$No.

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Complete set of bound negative-parity states in the neutron-rich 18N nucleus

High-resolution gamma-ray spectroscopy of 18N is performed with the Advanced GAmma Tracking Array AGATA, following deep-inelastic processes induced by an 18O beam on a 181Ta target. Six states are newly identified, which together with the three known excitations exhaust all negative-parity excited states expected in 18N below the neutron threshold. Spin and parities are proposed for all located states on the basis of decay branchings and comparison with large-scale shell-model calculations performed in the p-sd space, with the YSOX interaction. Of particular interest is the location of the 0^-_1 and 1^-_2 excitations, which provide strong constrains for cross-shell p-sd matrix elements based on realistic interactions, and help to simultaneously reproduce the ground and first-excited states in 16N and 18N, for the first time. Understanding the 18N structure may also have significant impact on neutron-capture cross-section calculations in r-process modeling including light neutron-rich nuclei.

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Accessing tens-to-hundreds femtoseconds nuclear state lifetimes with low-energy binary heavy-ion reactions

A novel Monte Carlo technique has been developed to determine lifetimes of excited states in the tens-to-hundreds femtoseconds range. The method is applied to low-energy heavy-ion binary reactions populating nuclei with complex velocity distributions. Its relevance is demonstrated in connection with the $^{18}$O(7.0 MeV/u) + $^{181}$Ta experiment, performed at GANIL with the AGATA+VAMOS+PARIS setup, to study neutron-rich O, C, N, ... nuclei. Excited states in $^{17}$O and $^{19}$O, with known lifetimes, are used to validate the method over the $\sim$20-400 fs lifetime-sensitivity range. Emphasis is given to the unprecedented position resolution provided by $γ$-tracking arrays, which turns out to be essential for reaching the required accuracy in Doppler-shift correction, at the basis of the detailed analysis of $γ$-ray lineshape and resulting state lifetime determination. The technique is anticipated to be an important tool for lifetime investigations in exotic neutron-rich nuclei, produced with intense ISOL-type beams.

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Testing ab initio nuclear structure in neutron-rich nuclei: lifetime measurements of second 2+ states in 16C and 20O

To test the predictive power of ab initio nuclear structure theory, the lifetime of the second 2+ state in neutron-rich 20O, tau(2+_2 ) = 150(+80-30) fs, and an estimate for the lifetime of the second 2+ state in 16C have been obtained, for the first time. The results were achieved via a novel Monte Carlo technique that allowed us to measure nuclear state lifetimes in the tens-to-hundreds femtoseconds range, by analyzing the Doppler-shifted gamma-transition line shapes of products of low-energy transfer and deep-inelastic processes in the reaction 18O (7.0 MeV/u) + 181Ta. The requested sensitivity could only be reached owing to the excellent performances of the AGATA gamma-tracking array, coupled to the PARIS scintillator array and to the VAMOS++ magnetic spectrometer. The experimental lifetimes agree with predictions of ab initio calculations using two- and three-nucleon interactions, obtained with the valence-space in-medium similarity renormalization group for 20O, and with the no-core shell model for 16C. The present measurement shows the power of electromagnetic observables, determined with high-precision gamma spectroscopy, to assess the quality of first-principles nuclear structure calculations, complementing common benchmarks based on nuclear energies. The proposed experimental approach will be essential for short lifetimes measurements in unexplored regions of the nuclear chart, including r-process nuclei, when intense ISOL-type beams become available.

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New front and back-end electronics for the upgraded GABRIELA detection system

The GABRIELA [1] set-up is used at the FLNR to perform detailed nuclear structure studies of transfermium nuclei. Following the modernization of the VASSILISSA separator (SHELS) [2] the GABRIELA detection system has also been upgraded. The characteristics of the upgraded detection system will be presented along with results from some recent electronics tests.

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High-spin structures of 124-131Te: Competition of proton and neutron pair breakings

The 124-131Te nuclei have been produced as fission fragments in two fusion reactions induced by heavy-ions (12C + 238U at 90 MeV bombarding energy and 18O + 208Pb at 85 MeV) and studied with the Euroball array. Their high-spin level schemes have been extended to higher excitation energy from the triple gamma-ray coincidence data. The gamma-gamma angular correlations have been analyzed in order to assign spin and parity values to many observed states. Moreover the half-lives of isomeric states have been measured from the delayed coincidences between the fission-fragment detector SAPhIR and Euroball, as well as from the timing information of the Ge detectors. The behaviors of the yrast structures identified in the present work are first discussed in comparison with the general features known in the mass region, particularly the breakings of neutron pairs occupying the nuh11/2 orbit identified in the neighboring Sn nuclei. The experimental level schemes are then compared to shell-model calculations performed in this work. The analysis of the wave functions shows the effects of the proton-pair breaking along the yrast lines of the heavy Te isotopes.

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High-spin structures of 88Kr and 89Rb: Evolution from collective to single-particle behaviors

The high-spin states of the two neutron-rich nuclei, 88Kr and 89R have been studied from the 18O + 208Pb fusion-fission reaction. Their level schemes were built from triple gamma-ray coincidence data and gamma-gamma angular correlations were analyzed in order to assign spin and parity values to most of the observed states. The two levels schemes evolve from collective structures to single-particle excitations as a function of the excitation energy. Comparison with results of shell-model calculations gives the specific proton and neutron configurations which are involved to generate the angular momentum along the yrast lines.

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High-spin structures of 136Cs

Odd-odd 136Cs nuclei have been produced in the 18O + 208Pb and 12C + 238U fusion-fission reactions and their gamma rays studied with the Euroball array. The high-spin level scheme has been built up to ~ 4.7 MeV excitation energy and spin I ~ 16 hbar from the triple gamma-ray coincidence data. The configurations of the three structures observed above ~ 2 MeV excitation energy are first discussed by analogy with the proton excitations identified in the semi-magic 137Cs nucleus, which involve the three high-j orbits lying above the Z=50 gap, pi g_{7/2}, pi d_{5/2} and pi h_{11/2}. This is confirmed by the results of shell-model calculations performed in this work.

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High-spin structures of five N=82 isotones: 136Xe, 137Cs, 138Ba, 139La, and 140Ce

Five N=82 isotones have been produced in two fusion-fission reactions and their gamma-rays studied with the Euroball array. The high-spin states of 139La have been identified for the first time, while the high-spin yrast and near-to-yrast structures of the four others have been greatly extended. From angular correlation analysis,spin values have been assigned to some states of 136Xe and 137Cs. Several cascades involving gamma-rays of 139La have been found to be delayed, they deexcite an isomeric state with T1/2= 315(35) ns located at 1800-keV excitation energy. The excited states of these five N=82 isotones are expected to be due to various proton excitations involving the three high-j subshells located above the Z=50 shell closure. This is confirmed by the results of shell-model calculations performed in this work. In addition, high-spin states corresponding to the excitation of the neutron core have been unambiguously identified in 136Xe, 137Cs, and 138Ba.

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High-spin states with seniority v=4,4,6 in 119-126Sn

The 119-126Sn nuclei have been produced as fission fragments in two reactions induced by heavy ions: 12C+238U at 90 MeV bombarding energy, 18O+208Pb at 85 MeV. Their level schemes have been built from gamma rays detected using the Euroball array. High-spin states located above the long-lived isomeric states of the even- and odd-A 120-126Sn nuclei have been identified. Moreover isomeric states lying around 4.5 MeV have been established in 120,122,124,126Sn from the delayed coincidences between the fission fragment detector SAPhIR and the Euroball array. The states located above 3-MeV excitation energy are ascribed to several broken pairs of neutrons occupying the nu h11/2 orbit. The maximum value of angular momentum available in such a high-j shell, i.e. for mid-occupation and the breaking of the three neutron pairs, has been identified. This process is observed for the first time in spherical nuclei.

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Clusters in Light Nuclei

A great deal of research work has been undertaken in the alpha-clustering study since the pioneering discovery, half a century ago, of 12C+12C molecular resonances. Our knowledge of the field of the physics of nuclear molecules has increased considerably and nuclear clustering remains one of the most fruitful domains of nuclear physics, facing some of the greatest challenges and opportunities in the years ahead. In this work, the occurence of "exotic" shapes in light N=Z alpha-like nuclei is investigated. Various approaches of superdeformed and hyperdeformed bands associated with quasimolecular resonant structures are presented. Results on clustering aspects are also discussed for light neutron-rich Oxygen isotopes.

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