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O. G. Polischuk

Publications and source records attributed to O. G. Polischuk.

62 records · Page 4Linked to original sources

CdWO4 crystal scintillators from enriched isotopes for double beta decay experiments

Cadmium tungstate crystal scintillators enriched in 106Cd and 116Cd were developed. The produced scintillators exhibit good optical and scintillation properties, and a low level of radioactive contamination. Experiments to search for double beta decay of 106Cd and 116Cd are in progress at the Gran Sasso National Laboratories of the INFN (Italy). Prospects to further improve the radiopurity of the detectors by recrystallization are discussed.

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First search for double-beta decay of 184Os and 192Os

A search for double-beta decay of osmium has been realized for the first time with the help of an ultra-low background HPGe gamma detector at the underground Gran Sasso National Laboratories of the INFN (Italy). After 2741 h of data taking with a 173 g ultra-pure osmium sample limits on double-beta processes in 184Os have been established at the level of T_{1/2} about 10^{14}-10^{17} yr. Possible resonant double-electron captures in 184Os were searched for with a sensitivity T_{1/2} about 10^{16} yr. A half-life limit T_{1/2} > 5.3 10^{19} yr was set for the double-beta decay of 192Os to the first excited level of 192Pt. The radiopurity of the osmium sample has been investigated and radionuclides 137Cs, 185Os and 207Bi were detected in the sample, while activities of 40K, 60Co, 226Ra and 232Th were limited at the mBq/kg level.

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Search for double beta decay processes in 106Cd with the help of 106CdWO4 crystal scintillator

A search for the double beta processes in 106Cd was carried out at the Gran Sasso National Laboratories of the INFN (Italy) with the help of a 106CdWO4 crystal scintillator (215 g) enriched in 106Cd up to 66%. After 6590 h of data taking, new improved half-life limits on the double beta processes in 106Cd were established at the level of 10^{19}-10^{21} yr; in particular, T_{1/2}(2νεβ^+) > 2.1 10^{20} yr, T_{1/2}(2ν2β^+) > 4.3 10^{20} yr, and T_{1/2}(0ν2ε) > 1.0 10^{21} yr. The resonant neutrinoless double electron captures to the 2718 keV, 2741 keV and 2748 keV excited states of 106Pd are restricted to T_{1/2}(0ν2K) > 4.3 10^{20} yr, T_{1/2}(0νKL1) > 9.5 10^{20} yr and T_{1/2}(0νKL3) > 4.3 10^{20} yr, respectively (all limits at 90% C.L.). A possible resonant enhancement of the 0ν2εprocesses is estimated in the framework of the QRPA approach. The radioactive contamination of the 106CdWO4 crystal scintillator is reported.

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Searches for neutrinoless resonant double electron captures at LNGS

Several experiments were performed during last years at underground (3600 m w.e.) Laboratori Nazionali del Gran Sasso (LNGS) of the INFN (Italy) to search for resonant 2$\varepsilon0ν$ captures in 96Ru, 106Cd, 136Ce, 156Dy, 158Dy, 180W, 184Os, 190Pt with the help of HP Ge semiconductor detectors, and ZnWO4 and 106CdWO4 crystal scintillators. No evidence for r-2$\varepsilon0ν$ decays was found, and only T_{1/2} limits were established in the range of 10^{14}-10^{21} yr.

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Low background detector with enriched 116CdWO4 crystal scintillators to search for double beta decay of 116Cd

A cadmium tungstate crystal boule enriched in $^{116}$Cd to 82% with mass of 1868 g was grown by the low-thermal-gradient Czochralski technique. The isotopic composition of cadmium and the trace contamination of the crystal were estimated by High Resolution Inductively Coupled Plasma Mass-Spectrometry. The crystal scintillators produced from the boule were subjected to characterization that included measurements of transmittance and energy resolution. A low background scintillation detector with two $^{116}$CdWO$_4$ crystal scintillators (586 g and 589 g) was developed. The detector was running over 1727 h deep underground at the Gran Sasso National Laboratories of the INFN (Italy), which allowed to estimate the radioactive contamination of the enriched crystal scintillators. The radiopurity of a third $^{116}$CdWO$_4$ sample (326 g) was tested with the help of ultra-low background high purity germanium $γ$ detector. Monte Carlo simulations of double $β$ processes in $^{116}$Cd were used to estimate the sensitivity of an experiment to search for double $β$ decay of $^{116}$Cd.

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First search for double beta decay of platinum by ultra-low background HP Ge gamma spectrometry

A search for double beta processes in 190Pt and 198Pt was realized with the help of ultra-low background HP Ge 468 cm^3 gamma spectrometer in the underground Gran Sasso National Laboratories of the INFN (Italy). After 1815 h of data taking with 42.5 g platinum sample, T_{1/2} limits on 2beta processes in 190Pt (εβ^+ and 2ε) have been established on the level of 10^{14}-10^{16} yr, 3 to 4 orders of magnitude higher than those known previously. In particular, a possible resonant double electron capture in 190Pt was restricted on the level of 2.9 \times 10^{16} yr at 90% C.L. In addition, T_{1/2} limit on 2 beta^- decay of 198Pt (2ν+0ν) to the 2^+_1 excited level of 198Hg has been set at the first time: T_{1/2}>3.5 \times 10^{18} yr. The radiopurity level of the used platinum sample is reported.

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First observation of alpha decay of 190-Pt to the first excited level (E_{exc}=137.2 keV) of 186-Os

The alpha decays of naturally occurring platinum isotopes, which are accompanied by the emission of gamma quanta, have been searched for deep underground (3600 m w.e.) in the Gran Sasso National Laboratories of the INFN (Italy). A sample of Pt with mass of 42.5 g and a natural isotopic composition has been measured with a low background HP Ge detector (468 cm^3) during 1815 h. The alpha decay of 190-Pt to the first excited level of 186-Os (J^π= 2^+, E_{exc}=137.2 keV) has been observed for the first time, with the half-life determined as: T_{1/2} = 2.6_{-0.3}^{+0.4} (stat.) \pm 0.6 (syst.) \times 10^{14} yr. The T_{1/2} limits for the alpha decays of other Pt isotopes have been determined at level of T_{1/2} \simeq 10^{16}-10^{20} yr. These limits have been set for the first time or they are better than those known from earlier experiments.

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Radioactive contamination of ZnWO4 crystal scintillators

The radioactive contamination of ZnWO4 crystal scintillators has been measured deep underground at the Gran Sasso National Laboratory (LNGS) of the INFN in Italy with a total exposure 3197 kg x h. Monte Carlo simulation, time-amplitude and pulse-shape analyses of the data have been applied to estimate the radioactive contamination of the ZnWO4 samples. One of the ZnWO4 crystals has also been tested by ultra-low background gamma spectrometry. The radioactive contaminations of the ZnWO4 samples do not exceed 0.002 -- 0.8 mBq/kg (depending on the radionuclide), the total alpha activity is in the range: 0.2 - 2 mBq/kg. Particular radioactivity, beta active 65Zn and alpha active 180W, has been detected. The effect of the re-crystallization on the radiopurity of the ZnWO4 crystal has been studied. The radioactive contamination of samples of the ceramic details of the set-ups used in the crystals growth has been checked by low background gamma spectrometry. A project scheme on further improvement of the radiopurity level of the ZnWO4 crystal scintillators is briefly addressed.

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